Synthesis and Growth Mechanism of Ultralong ZnO Nanocombs and Nanobelts on Cu Substrate

In the two-dimensional electron systems with strong coupling in MgZnO/ZnO heterostructures, the thermal behavior of Ising quantum Hall ferromagnets at the filling factor ν = 2 has been studied. The spin polarization of Hall ferromagnets has been detected by measuring the signal related to the inelastic light scattering by intrasubband spin excitons. A stepwise change in the spin polarization at the phase transition at the filling factors ν = 2,3, and 4 in the heterostructures with different electron densities has been observed. The thermal stability of the Hall ferromagnetic phases at ν = 2 has been studied and the Curie temperature has been estimated. It has been shown that the Curie temperature is determined by the formation energy for domain walls in the Ising quantum Hall ferromagnets.     

Verification of a new quantum simulation approach through its application to two-dimensional Ising lattices

A new quantum simulation approach has been applied in the present work to the two-dimensional (2D) ferromagnetic and antiferromagnetic Ising lattices to calculate their magnetic structures, magnetizations, free energies and specific heats in the absence of an external magnetic field. Surprisingly, no size effects could be observed in our simulations performed for the Ising lattices of different sizes. Most importantly, our calculated spontaneous thermally averaged spins for the two kinds of systems are exactly same as those evaluated with quantum mean field theory, and the magnetic structures simulated at all chosen temperatures are perfectly ferromagnetic or antiferromagnetic, verifying the correctness and applicability of our quantum model and computational algorithm. On the other hand, if the classical Monte Carlo (CMC) method is applied to the ferromagnetic 2D Ising lattice with S=1, it is able to generate correct magnetization well consistent with Onsager's theory; but in the case of S=1/2, the computational results of CMC are incomparable to those predicted with the quantum mean field theory, giving rise to very much reduced magnetization and considerably underestimated Curie temperature. The difficulty met by the CMC method is mainly caused by its improperly calculated exchange energy of the randomly selected spin in every simulation step, especially immediately below the transition temperature, where the thermal averages of spins are much less than 1/2, however they are assigned to ±1/2 by CMC to evaluate the exchange energies of the spins, such improper manipulation is obviously impossible to lead the code to converge to the right equilibrium states of the spin systems.     

The behaviour of physical quantities in thin films near the Curie point

The Valenta model of a thin ferromagnetic film in the critical region above the Curie point has been considered. Spatial and temperature dependence for spin correlation time and magnetic susceptibility has been obtained and discussed. The results have been generalized and expressions describing the behaviour of any physical quantity in more complicated models of a thin ferromagnetic film near the Curie temperature have been given.     

Magnetic Properties of XXZ Heisenberg Antiferromagnetic and Ferrimagnetic Nanotubes

The spin-1/2 antiferromagnetic and spin-(1/2, 1) ferrimagnetic single-walled nanotubes are described by XXZ Heisenberg model. The sublattice magnetization and the critical temperature of the system are calculated by using the double-time spin Green's function method. At zero temperature, with the increase of the exchange interaction in the circumferential direction, a maximum value appears in the sublattice magnetization curves of antiferromagnetic and ferrimagnetic systems. As the diameter of the tube increases, the spin quantum fluctuations and thermal fluctuations are suppressed. In addition, the spin quantum fluctuation of the spin-1/2 antiferromagnetic system is greater than that of the spin-(1/2, 1) ferrimagnetic system. The critical temperature of the system increases firstly and then tends to a constant with the increase of the diameter of tube, and it decreases to zero as the exchange anisotropy of the system disappears.     

High-temperature dynamics of surface magnetism in iron thin films

Finite-temperature magnetic properties of iron thin films are investigated by computer simulation over a broad range of temperatures up to the point of the ferromagnetic–paramagnetic phase transition. The coupled dynamics of atoms and magnetic moments is treated using the large-scale spin–lattice dynamics (SLD) algorithm. We investigate surface and bulk magnetic properties of iron, and how these properties vary as a function of temperature, film thickness and surface crystallography. We find that magnetization at surfaces is enhanced at low temperatures and suppressed at higher temperatures, in agreement with experimental observations. The effective Curie temperature of a film decreases as a function of thickness. Short-range magnetic order and non-vanishing spin–spin spatial correlations are found above the Curie temperature. The spin autocorrelation functions exhibit slower oscillations with longer decoherence times near the surface. We also find that the directional spin disorder has a significant effect on the surface strain.     

具有三自旋相互作用XX模型纠缠特性研究

利用Concurrence判据,研究了具有三自旋相互作用的XX模型的纠缠特性;分别在铁磁和反铁磁模型中研究了三自旋相互作用J_2和温度T对两自旋纠缠度的影响.结果表明,三自旋相互作用J_2提高系统的两体纠缠度,但是提高程度会因最近邻自旋间发生铁磁、反铁磁相互作用而有所差异;并且J_2影响两自旋系统纠缠消失的临界温度T_C,T_C会随J_2的增大而减小.系统温度T影响两体纠缠度,随着温度的降低,纠缠度会得到提高.此外,分别在系统本征态和基态中研究了两自旋的纠缠度,求出了系统发生量子相变的量子临界点.     

Dynamical mean-field theory of a simplified double-exchange model

Simplified double-exchange model including transfer of the itinerant electrons with spin parallel to the localized spin in the same site and the indirect interaction J of kinetic type between localized spins is comprihensively investigated. The model is exactly solved in infinite dimensions. The exact equations describing the main ordered phases (ferromagnetic and antiferromagnetic) are obtained for the Bethe lattice with (z is the coordination number) in analytical form. The exact expression for the generalized paramagnetic susceptibility of the localized-spin subsystem is also obtained in analytical form. It is shown that temperature dependence of the uniform and the staggered susceptibilities has deviation from Curie-Weiss law. Dependence of Curie and Néel temperatures on itinerant-electron concentration is discussed to study instability conditions of the paramagnetic phase. Anomalous temperature behaviour of the chemical potential, the thermopower and the specific heat is investigated near the Curie point. It is found for J=0 that the system is unstable towards temperature phase separation between ferromagnetic and paramagnetic states. A phase separation connected with antiferromagnetic and the paramagnetic phases can occur only at . Zero-temperature phase diagram including the phase separation between ferromagnetic and antiferromagnetic states is given. Received 28 May 1999 and Received in final form 14 July 1999     

Ferromagnetic effect of a Mn delta layer in the GaAs barrier on the spin polarization of carriers in an InGaAs/GaAs quantum well

The polarization properties of the luminescence of an undoped InGaAs quantum well in InGaAs/GaAs het-erojunctions with a Mn delta layer in the GaAs barrier have been studied in a wide range of temperatures and magnetic fields. It has been found that the s, p-d exchange interaction of carriers in the quantum well with Mn ions in the δ layer leads to the ferromagnetic behavior of both the Zeeman splitting and spin polarization of the carriers with a Curie temperature typical of the Mn delta layer in the GaAs barrier. The saturation of the spin polarization of holes associated with their Fermi degeneracy has been observed at low temperatures (T < 20 K).     

Study of the ferromagnetic transition in a positionally frozen Heisenberg spin system

Using extensive Monte Carlo simulations with both particle and cluster orientational moves, in conjunction with finite size scaling and histogram reweighting techniques, we have determined the Curie temperature for two models of positionally frozen Heisenberg spin systems: a system with spatial correlations corresponding to a hard sphere fluid and a spatially random system. We find that the results for the positionally frozen hard sphere Heisenberg system are fairly similar to those previously obtained for the Heisenberg spin fluid and quantitatively agree with the mean field theory estimates. The random system undergoes the ferromagnetic transition at a higher temperature since the lack of core repulsion increases the spin correlations. In this case however the mean field theory overestimates by far the critical temperature.     

Coupled charge-spin dynamics of the magnetoresistive pyrochlore TI2Mn2O7 probed using ultrafast midinfrared spectroscopy

Optical-pump midinfrared probe spectroscopy is used to investigate coupled charge-spin dynamics in the magnetoresistive pyrochlore TI(2)Mn(2)O(7). We find that the temporal persistence of the photoexcited carrier density is strongly influenced by spin disorder above and below the ferromagnetic Curie temperature. Our results are consistent with a picture whereby spin disorder leads to spatial segregation of the initially excited Tl 6s-O 2p electron-hole pairs, effectively reducing the probability for recombination. This further implies that colossal magnetoresistance in these materials may be driven primarily by Mn t(2g) spin disorder.     

Temperature dependence of the circular polarization of electroluminescence from spin-polarized light-emitting diodes based on InGaAs/GaAs heterostructures

The temperature dependence of the circular polarization degree of the electroluminescence from light-emitting diodes based on InGaAs/GaAs-quantum-well (QW) heterostructures with a closely located ferromagnetic Mn δ layer is investigated. It is found that the Mn δ layer ferromagnetically affects holes in the QW. This effect is characterized by spin polarization of the holes and the appearance of circularly polarized emission components under electroluminescence conditions. It is demonstrated that the ferromagnetic properties of a δ layer can be studied by analyzing the QW luminescence. The Curie temperatures of the ferromagnetic system are determined using the results of investigations.     

Comments on “magnetovolume effect and invar phenomena in ferromagnetic metals”, by T. Moriya and K. Usami

The thermal expansion data of a number of ferromagnetic alloys are reconsidered in the light of the statements of Moriya and Usami [1] that they support the spin fluctuation model of itinerant electron magnetism [2]. As a result of this reconsideration it is concluded that, though spin fluctuation effects may contribute significantly, single particle or Stoner excitations are of at least equal significance. The pressure dependence of the Curie temperature is also considered in the same way, although this phenomenon was not discussed in [1].     

Curie point singularity in the temperature derivative of resistivity in (Ga,Mn)As

We observe a singularity in the temperature derivative drho/dT of resistivity at the Curie point of high-quality (Ga,Mn)As ferromagnetic semiconductors with Tc's ranging from approximately 80 to 185 K. The character of the anomaly is sharply distinct from the critical contribution to transport in conventional dense-moment magnetic semiconductors and is reminiscent of the drho/dT singularity in transition metal ferromagnets. Within the critical region accessible in our experiments, the temperature dependence on the ferromagnetic side can be explained by dominant scattering from uncorrelated spin fluctuations. The singular behavior of drho/dT on the paramagnetic side points to the important role of short-range correlated spin fluctuations.     

Investigation of Mn incorporation in fifteen-period InGaAs/GaAs quantum well system

A ferromagnetic ordering with a Curie temperature of 50 K of fifteen layer of InGaMnAs/GaAs multi quantum wells (MQWs) structure grown on high resistivity (100) p-type GaAs substrates by molecular beam epitaxy (MBE) was found. It is likely that the ferromagnetic exchange coupling of sample with Curie temperature of 50 K is hole-mediated resulting in Mn substituting In or Ga sites. Temperature and excitation power dependent PL emission spectra of InGaMnAs MQWs sample grown at temperature of 170 °C show that an activation energy of Mn ion on the first quantum confinement level in InGaAs quantum well is 36 meV and impurity Mn is partly ionized. It is found that the activation energy of 36 meV of Mn ion in the QW is lower than the activation energy of 110 meV for a substitutional Mn impurity in GaAs. These measurements provide strong evidence that an impurity band existing in the bandgap due to substitutional Mn ions and it is the location of the Fermi level within the impurity band that determines Curie temperature.     

Generating and reversing spin accumulation by temperature gradient in a quantum dot attached to ferromagnetic leads

We propose to generate and reverse the spin accumulation in a quantum dot (QD) by using the temperature difference between the two ferromagnetic leads connected to the dot. The electrons are driven purely by the temperature gradient in the absence of an electric bias and a magnetic field. In the Coulomb blockade regime, we find two ways to reverse the spin accumulation. One is by adjusting the QD energy level with a fixed temperature gradient, and the other is by reversing the temperature gradient direction for a fixed value of the dot level. The spin accumulation in the QD can be enhanced by the magnitudes of both the leads’ spin polarization and the asymmetry of the dot-lead coupling strengths. The present device is quite simple, and the obtained results may have practical usage in spintronics or quantum information processing.     

Influence of Magnetization on the Spin Pumping Efficiency in a Ferromagnet–Normal Metal Bilayer Structure

The problem of spin current generation and transformation into electric signals in thin-film ferromagnet/nonmagnetic metal bilayer structures is investigated. This direction is of considerable scientific interest and promising for applications in spintronics. An LSMO/Pt structure consisting of an epitaxial film of ferromagnetic manganite La2/3Sr1/3O3 grown on a single-crystal NdGaO3 substrate and coated with a platinum film has been studied experimentally. The spin current was generated by the spin pumping method upon the excitation of a ferromagnetic resonance in the ferromagnetic layer and was detected by the electric voltage USP arising in the nonmagnetic metal layer due to the inverse spin Hall effect. Owing to its relatively low Curie temperature (~350 K), using LSMO allowed the influence of ferromagnetic-layer magnetization on the spin current generation to be studied in detail in the temperature range 100–350 K. In this case, the influence of the shape of the ferromagnetic resonance line, which is the convolution of homogeneous (Lorentzian) spin packets and inhomogeneous Gaussian broadening (Voigt model), was consistently taken into account. As a result of our analysis of all the parameters defining USP, we have obtained the temperature dependence of the mixed spin conductance, which has turned out to be approximately proportional to the ferromagnet magnetization squared. This result is compared with existing theoretical models.     

Finite block spin phenomenology of spin glass

We herein explain the phase of spin glass by reference to finite block spin theory, in which the phase of the spin glass may be considered as being a ferromagnetic ordering between block spins comprised of random spins that have a majority of individual spins in a given sense. By making use of the Curie law of block spins, we obtained the magnetization, susceptibility, and specific heat for the lower and higher temperature approximations of the Brillouin function. Both the susceptibility and the specific heat thus obtained are in good agreement with existing experimental data, although in the latter case the agreement is less convincing near absolute zero temperature.     

Quantum Hall ferrimagnetism in lateral quantum dot molecules

We demonstrate the existence of ferrimagnetic and ferromagnetic phases in a spin phase diagram of coupled lateral quantum dot molecules in the quantum Hall regime. The spin phase diagram is determined from the Hartree-Fock configuration interaction method as a function of electron number N and magnetic field B. The quantum Hall ferrimagnetic phase corresponds to spatially imbalanced spin droplets resulting from strong interdot coupling of identical dots. The quantum Hall ferromagnetic phases correspond to ferromagnetic coupling of spin polarization at filling factors between nu=2 and nu=1.     

旁耦合于介观环与铁磁电极量子点系统中的自旋极化输运

借助单杂质Anderson模型哈密顿量,及利用格林函数和运动方程等理论,研究旁耦合于介观环和铁磁电极的量子点系统中的极化输运特性.结果表明,通过调节点-环耦合强度、铁磁电极中的极化强度、磁矩相对取向及温度等,均能实现控制体系中自旋极化电流的目的,达到自旋阀效应.为此系统作为一种新的自旋电子材料提供理论依据.     

Theory and simulation of positionally frozen Heisenberg spin systems

The structure, thermodynamics and the ferromagnetic phase transition of a positionally frozen disordered Heisenberg spin system are studied by means of extensive Monte Carlo calculations in combination with finite size scaling techniques, as well as resorting to the Replica Ornstein-Zernike formalism. The system is formed by a collection of Heisenberg spins whose spatial distribution corresponds to a soft sphere fluid with its particle positions frozen at a certain quench temperature. The spin orientations are allowed to equilibrate at a given equilibrium temperature. If the quench and equilibrium temperatures are similar the properties of the positionally frozen system are practically indistinguishable from those of the fully equilibrated Heisenberg spin fluid. On the other hand, one observes that as the quenching temperature of the spatial degrees of freedom increases, so does the Curie temperature of the Heisenberg spins. The theory fails to reproduce the location of the ferromagnetic transition, despite its relative accuracy in the determination of the orientational structure in the supercritical region.Received: 25 July 2003, Published online: 9 September 2003PACS: 75.50.Lk Spin glasses and other random magnets - 64.60.Fr Equilibrium properties near critical points