Widely tunable ultraviolet sub-30-fs pulses from supercontinuum for transient spectroscopy

Focusing 800-nm pulses of 10–20 fs and ≤0.4 mJ into atmospheric-pressure argon gives rise to a supercontinuum extending down to 250 nm. We show that spectral cuts from this radiation can be shortened by a simple prism compressor down to 30 fs even near the UV cut-off. The resulting pulses have enough energy (several hundred nanojoules) to serve as a simple and rugged broadly tunable pump source in ultra-fast transient spectroscopy. Such an application is demonstrated for the first time, using pulses tuned over 280–320 nm to excite Cr(CO)₆; probing it by intense-field ionization at 800 nm, we determine the lifetime of initially populated states to be as short as 14 fs.PACS 42.65.Jx; 42.65.Ky; 42.65.Re; 42.72.Bj; 82.20.-w; 82.53.-k     

Widely tunable compact erbium-doped fiber ring laser for fiber-optic sensing applications

A compact erbium-doped ring-shaped fiber laser suitable for fiber-optic sensing applications has been developed. The fiber laser utilized a tunable fiber Fabry–Perot filter as the tuning element and had a moderate milli-Watt level power output over almost the whole tuning range from 1530 to 1595 nm with a power fluctuation of 0.15 dB. High repetition rate scanning of laser operation over the whole tuning range was achieved at rates of up to 200 Hz. Moreover, the performance of the ring-shaped fiber laser configured with a high-concentration erbium-doped fiber was investigated for its larger wavelength tunability of over 100 nm. Output power characteristics of this ring-shaped fiber laser were also investigated when it worked in a scanning mode. A distorted power wavelength dependence, as well as some pulsing phenomenon were observed in scanning mode.     

Generation of broadly tunable sub-30-fs infrared pulses by four-wave optical parametric amplification

We report on the generation of sub-30-fs near-IR light pulses by means of broadband four-wave parametric amplification in fused silica. This is achieved by frequency downconversion of visible broadband pulses provided by a commercial blue-pumped beta-barium borate crystal-based noncollinear optical parametric amplifier. The proposed method produces the IR idler pulses with energy up to ～20 μJ and tunable in wavelength from 1 to 1.5 μm. The shortest pulse duration is 17.6 fs, measured at 1.2 μm.     

Multimilliwatt ultrashort pulses continuously tunable in the visible from a compact fiber source

We report on a single-pass device that efficiently converts the broadband near-infrared output from a femtosecond fiber laser into a narrow spectrum in the visible. With fan-out poled MgO:LiNbO3 we obtain sub-picosecond, continuously tunable pulses in the 520-700 nm range. Conversion efficiencies as high as 30% are observed at typical pump power levels of 30 mW, corresponding to average output powers up to 9.5 mW. The specifications of our device are ideal for applications in confocal microscopy and frequency metrology.     

Generation of 47-fs pulses directly from an erbium-doped fiber laser

We show both numerically and experimentally that through appropriately selecting the output coupling position and strength in a mode-locked fiber laser, one can effectively manage the nonlinearity of the cavity. By implementing the technique together with cavity dispersion management in an erbium-doped fiber laser, we have achieved stable mode-locked pulses with a single-pulse energy of 2.08 nJ and pulse width of 46.2 fs directly from the laser.     

Widely ultra-narrow linewidth 104 nm tunable all-fiber compact erbium-doped ring laser

A widely tunable narrow linewidth compact erbium-doped all-fiber ring laser with 104 nm tuning range was reported. An all-fiber Fabry-Perot filter (FFP-TF) was used to realize the laser tuning output, and the wavelength at constant voltage had high time stability. With the 8 m length erbium-doped fiber as gain medium, we realized widely tunable laser from 1513 to 1617 nm with the linewidth less than 40 pm at any wavelength. Pumped by the 976 nm laser diode, the fiber laser worked with slope efficiency of above 10% and threshold of less than 21 mW.     

Spectral analysis of high-order harmonics generated by 30-fs and sub-10-fs laser pulses

The spectral properties of harmonic radiation generated in neon by laser pulses with duration from 30 fs down to 5 fs have been investigated. In the 30-fs temporal regime we have achieved continuously tunable sub-20-nm radiation by changing the gas jet position relative to the laser beam waist. We show that the results of a one-dimensional propagation code partially including three-dimensional focusing effects are in good agreement with the experimental results. Finally, we have performed a spectral characterization of harmonic radiation in the sub-10-fs temporal regime.     

Mid-infrared difference-frequency generation of ultrashort pulses tunable between 3.2 and 4.8 microm from a compact fiber source

We report single-pass difference-frequency generation of mid-infrared femtosecond pulses tunable in the 3.2-4.8 microm range from a two-branch mode-locked erbium-doped fiber source. Average power levels of up to 1.1 mW at a repetition rate of 82 MHz are obtained in the mid infrared. This is achieved via nonlinear mixing of 170 mW, 65 fs pump pulses at a fixed wavelength of 1.58 microm, with 11.5 mW, 40 fs pulses tunable in the near-infrared range between 1.05 and 1.18 microm. These values indicate that the tunable near-infrared input component is downconverted with a quantum efficiency that exceeds 30%.     

Ex vivo characterization of sub-10-fs pulses

An all-mirror dispersion-compensation setup is used to correct for quadratic and cubic phase distortions induced within a custom nonlinear optical microscope. Mouse tail tendon is used to characterize sub-10-fs pulses by interferometric autocorrelation. This is an ideal method for characterizing dispersion from the optical system, immersion medium, and wet biological sample. The generation of very short autocorrelations demonstrates the ability to compensate for phase distortions within the imaging system and efficient second-harmonic upconversion of the ultrashort pulse spectrum within collagen. Compensated autocorrelation traces are presented for biologically relevant objective lenses.     

Pulse characteristics of an optical parametric oscillator pumped by sub-30-fs light pulses

We obtained nearly transform-limited light pulses of 34 fs near 1.2 microm by pumping an optical parametric oscillator with a 2-mm-long KTP crystal by 26-fs pulses from a Ti:sapphire laser. The average power of the pulses that were obtained was greater than 50 mW, at an 80-MHz repetition rate. Attempts to downscale the pulse duration by decreasing the pump-pulse duration revealed remarkable limitations of the attainable pulse length for sub-30-fs pump pulses, in accordance with a recent theoretical study [J. Opt. Soc. Am. B 17, 741 (2000)].     

Semiconductor saturable absorber mirrors supporting sub-10-fs pulses

Received: 18 March 1997/Revised version: 12 May 1997     

A compact graphene Q-switched erbium-doped fiber laser using optical circulator and tunable fiber Bragg grating

We demonstrate a passively Q-switched tunable erbium-doped fiber laser(EDFL)based on graphene as a saturable absorber(SA).A three-port optical circulator(OC)and a strain-induced tunable fiber Bragg grating(TFBG)are used as the two end mirrors in an all-fiber linear cavity.The Q-switched EDFL has a low pump threshold of 23.8 mW.The pulse repetition rate of the fiber laser can be widely changed from 9.3 kHz to 69.7 kHz by increasing the pump power from23.8 mW to 219.9 mW.The minimum pulse duration is 1.7μs and the highest pulse energy is 25.4 nJ.The emission wavelength of the laser can be tuned from 1560.43 nm to 1566.27 nm by changing the central wavelength of the straininduced TFBG.     

Sum frequency generation of continuously tunable blue pulses from a two-branch femtosecond fiber source

We report on the generation of femtosecond blue pulses from a two-branch mode-locked erbium-doped fiber source. This is achieved by sum-frequency mixing in β-barium borate between the frequency doubled laser radiation at 770 nm and a tunable near-infrared component generated inside a highly nonlinear fiber. Small angle tuning of the nonlinear crystal leads to a continuously variable output wavelength in the visible band between 460 nm and 500 nm. Average power levels exceeding 1.5 mW were collected throughout the entire tuning range of our device, which delivered sub-300-fs pulses at a repetition rate of 98 MHz. These values indicate that the input near-infrared radiation is up-converted with a photon efficiency of 20%.     

Production of dense plasmas with sub-10-fs laser pulses

Close to solid state density plasmas with peak electron temperatures of about 190 eV have been generated with sub-10-fs laser pulses incident on solid targets. Extreme ultraviolet (XUV) spectroscopy is used to investigate the K shell emission from the plasma. In the spectra, a series limit for the H- and He-like resonance lines becomes evident which is explained by pressure ionization in the dense plasma. The spectra are consistent with computer simulations calculating the XUV emission and the expansion of the plasma.     

Hollow fiber for flexible sub-20-fs pulse delivery

Delivery of sub-20-fs pulses through 80 cm of a chirped photonic crystal fiber with chirped-mirror precompensation is experimentally demonstrated. The pulses out of the fiber are within 15% of the bandwidth limit and exhibit a pulse energy of 1 nJ. Peak powers amount to 50 kW directly out of the fiber. Measurements indicate a good pulse contrast with little satellite content. The combination of a specially designed hollow fiber with chirped mirrors sets a new record for the pulse durations directly delivered through a fiber.     

Phase-dependent loss due to nonadiabatic ionization by sub-10-fs pulses

For the first time to the author's knowledge, the effect of phase-dependent loss that can be used to stabilize the phase of a sub-10-fs laser pulse with respect to the envelope is shown. This loss is caused by the nonadiabatic response of an atom illuminated by a short pulse, which leads to the dependence of the tunneling ionization on the absolute phase of the pulse. The phase selectivity can be employed as a phase-dependent filter within the laser cavity with important applications in nonlinear optics in the single-cycle regime.     

Tunable sub-10-fs ultraviolet pulses generated by achromatic frequency doubling

Tunable UV pulses shorter than 10 fs are generated by achromatic frequency doubling of a noncollinear optical parametric amplifier. With a suitable two-prism sequence we achieve first- and second-order achromatic phase matching and increase the natural bandwidth of the nonlinear crystal by a factor of 80. Extremely broad UV spectra with a Fourier limit of 2.9 fs are generated in a 360-microm-thick beta-barium borate crystal at a conversion efficiency of 20%. We compensate for the angular dispersion and the first-order chirp of the highly stable UV pulses with a second prism sequence and fully characterize the temporal pulse shape with zero-additional-phase spectral phase interferometry for direct electric-field reconstruction (ZAP-SPIDER). Pulses as short as 7 fs are generated by controlling the higher-order chirp with a deformable mirror.     

158-microJ pulses from a single-transverse-mode, large-mode-area erbium-doped fiber amplifier

We report the amplification of 10-100-pJ semiconductor diode pulses to an energy of 158 microJ and peak powers >100 kW in a multistage fiber amplifier chain based on a single-mode, large-mode-area erbium-doped amplifier design. To our knowledge these results represent the highest single-mode pulse energy extracted from any doped-fiber system.     

Sub-20-fs pulses tunable across the visible from a blue-pumped single-pass noncollinear parametric converter

Femtosecond pulses with center wavelengths between 470 and 750 nm are generated in a single-stage type I BBO optical parametric amplifier pumped by a frequency-doubled 1-kHz Ti:sapphire amplifier. A high-quality white-light continuum is used as the seed. Pulse durations as short as 16 fs and pulse energies of as much as 11 microJ are observed. The quantum efficiency is ~25% for both 7- and 40-microJ pump pulses. This unique combination of ultrashort pulse duration and high conversion is made possible by noncollinear phase matching that permits a sufficiently large amplification bandwidth. Simultaneously the group velocities of the signal and the idler are effectively matched. As a result widely tunable sub-20-fs pulses can be generated in a nonlinear crystal as thick as 2 mm.     

Mirror-dispersion-controlled OPA: a compact tool for sub-10-fs spectroscopy in the visible

We report on a sub-10-fs optical parametric amplifier in the visible, using noncollinear phase matching in #-barium borate, with a pulse compressor made exclusively of chirped dielectric mirrors. We employ mirrors of novel design, providing negative group delay dispersion for bandwidths of over 200 THz, up to the blue-green spectral region. The resulting setup, compact, easy to operate and reliable, is an ideal tool for ultrafast spectroscopy with extremely high time resolution. We use these pulses to observe in the time domain coherent oscillations in organic molecules with period as short as 16 fs.