Der Zerfall Co58m →Co58g

Co^58m , Co^58g and Co⁵⁵ were obtained by radiating nickel-foiles with deuterons of energies 11,5 MeV and 2,07 MeV. The γ-radiation was measured with NaJ scintillation spectrometers. For the isomeric transition of Co^58m was determinedT _1/2=(9.15±0.1)h,T _γ=(25±1)keV,α _K=2200±300 and α_L+M=1100±300. From these values it follows, that the radiation is ofM3-type. Twoγ-energies of 95 keV and 1322 keV were found belonging to Co⁵⁵.     

Der Zerfall des Tb158m

Tb^158m was produced from Tb¹⁵⁹ by (n, 2n) reaction and investigated using scintillation spectrometers. The following results were obtained: half-life\(T_{\tfrac{1}{2}} = (10.5 \pm 0.2)\) sec; energy of the isomeric transitionE _γ =(109.9±1.4) keV; conversion coefficients α _K =56±3; α _L +α _M +?=50±8; α_total=106±10;K/L-ratioK/L=1.3±0.3, yielding the multipole order of the isomeric transition to beM3. Upper limits for the direct beta transitions from the isomeric state to the ground states of the neighbouring even-even nuclei Gd¹⁵⁸ and Dy¹⁵⁸ are 10^?4 and 6·10^?3, respectively.     

Die Konversion des Hg199m

Hg^199m was produced from natural HgO by fastn irradiation. The cascade decay was investigated with scintillation spectrometers by application of the summing technique. The following results were obtained: half-lifeT _1/2=(43±0,5) min; energy of the isomeric transitionE _γ1=(375±3)keV; conversion coefficients α _K375=3,05±0,25; α_total=5,45±0,25; yielding the multipole order of the isomeric transition to beM4+(25±15)%E5; energy of the second transitionE _γ2=(159±2)keV; conversion coefficients α _K159=0,30±0,03; α_total=0,9±0,1, confirming the multipolarityE2 of this transition.     

Radioactive decay of Os191 and Os191m

Beta and gamma spectra of Os¹⁹¹ were studied using a magnetic double-focusing beta-spectrometer and a scintillation spectrometer. The isomeric state Os^191m decays through the 74·4 ± 0·1 keV (E3/M4=50) transition with a half-lifeT _1/2=13·0 ± 0·5 hours. A continuous beta spectrum withE _max=147 ± 3 keV and the gamma transitions 41·83 ± 0·05 keV (E3), 82·5 ± 0·3 keV and 129·4 ± 0·1 keV (70%M1 + 30%E2) were observed in the decay of the ground state of Os¹⁹¹. The conversion coefficient of the last transition was determined as 1·94 ±± — 0·10. Gamma transitions with energies of 47 keV and 185·8 keV were not observed.     

Determination of absoluteK-internal conversion coefficients of some transitions in Ce140 by the internal-external conversion method

The internalK-conversion coefficients of the 331, 431, 815 and 933 keV transitions following the decay of La¹⁴⁰ have been determined absolutely by the method of comparing internal and external conversion lines measured in a double — focusing beta — ray spectrometers. TheK-internal conversion coefficients of the 4+→2+ 487 keV transition in Ce¹⁴⁰ was used to normalize relativeK-electron and gamma-ray intensities for these transitions. The results obtained are:α _K (331)=0.04432±0.00471,α _K (431)=0.28110±0.02913,α _K (815)=0.00396±0.00043,α _K (933)=0.00282±0.00031. Multipolarity assignments based on these values are suggested. The 815 keV transition is found to be pure magnetic dipole character in good agreement with the theoretical values calculated bySliv andBand. The 331 and 933 keV transitions are proved to have magnetic dipole character withE2/M1 equal 0.2852±0.0143 and 0.1750±0.0088 respectively. The 431 keV transition was found to have magnetic octupole character. The results obtained are most consistent with the assignment 2+, 4+, 2+, 3+ and 1+ for the 1597, 2084, 2184, 2410 and 2515 keV levels respectively.     

Kern-Isomerie bei In116

The short lived indium isomer produced by thermal neutron capture is confirmed to be In¹¹⁶. A new determination of half-live andγ energy yieldsT _1/2=(2.17α0.07) sec andE _γ=(164±1) keV. From measurement of theK shell conversion coefficient follows that the multipolarity of the transition isE 3, leading to a spin and parity assignment of 8^? for the isomeric level.     

Die Konversion des79m Br

⁷⁹ mBr was produced by irradiation of natural Br with fast neutrons. The half-lifeT _1/2=(4.87±0.15) sec and the energyE _γ=(208±1) keV were remeasured. For the first time the conversion coefficients were determined to beα _K=0.25±0.02 and α_total=0.28±0.05, yielding the multipolarityE3 for the isomeric transition.     

Die isomeren Atomkerne: Yb169m,Yb175m,Yb177m

Short lived isomers of Yb were produced by neutron irradiation of enriched isotopes and have been investigated with the aid of scintillation spectrometers. Yb^169m decays with a half-life ofT _1/2=(46±2) sec emitting only L-radiation. This decay is assumed to be the same as the E 3-transition of 24 keV following the electron capture of Lu¹⁶⁹. Yb^175m [T _1/2=(0,072±0,005) sec] emitsγ-rays of (495±15) keV. The measured K-conversion coefficientα _{K 495}=0,24±0,04 and the total conversion coefficientα _{4 5}=0,6±0,3 indicate the transition to be M3. Yb^177m [T _1/2=(6,4±0,1) sec] decays by a cascade of twoγ-rays. The isomeric (228±3) keV-transition is followed by a (104±1,5) keV-radiation. The measured conversion coefficients areα _{K 228}=4,1±0,4 andα _{K 228}=6,5±0,5 for the first transition andα _{K 104}=0,39±0,05 andα ₁₀₄=0,51±0,05 for the second, indicating a M3-E1-cascade. For the M 3-transition the measured coefficients agree well with those calculated for a nucleus of finite size, but they differ by a factor of 1,5 for the E1-transition.     

Der Zerfall des Co60m und Zr90m

Co^60m was produced by the reaction Co⁵⁹ (n,γ) Co^60m ; its decay has been investigated by scintillation spectrometers. The half-period has been remeasured yielding a value ofT _1/2=(10·35 ±0·20) min. The isomeric decay mainly leads to the Co⁶⁰ ground state by a (58·6±0·6) keV transition. TheK-conversion coefficientα _K= 41±3 and the total conversion coefficientα=47±3 indicate the transition to beM3 and the spin of Co^60m to be 2⁺. Further Co^60m decays by beta transitions to Ni⁶⁰. The beta component (8·6±1·2)·10^?3%, log ft=7·32 leading to a (2·16±0·02) MeV level has been measured for the first time. A second component (0·24±0·03)%, log ft=7·23 leads to the 1·33 MeV level. The 2·16 MeV level decays to the Ni⁶⁰ ground state mainly by a 0·83–1·33 MeV cascade, in a few cases by a direct transition. The spin of the 2·16 MeV level is 2⁺. Zr^90m was produced by the reaction Zr⁹⁰ (n,n′) Zr^90m . The half-period was measured yielding a value ofT _1/2=(0·83±0·03) sec. Zr^90m decays in the following way: (77±5) % by a direct (2·31±0·02) MeV —E 5 transition to the Zr ground state and (23±5)% by a (132·5±1·5) keV-(2·18±0·03) MeV cascade detected for the first time in the isomeric decay. TheK-conversion coefficient of the 132·5 keV transition isα _k=(2·2±0·3) indicating this transition to beE3 and the spin of the 2·18 MeV level to be 2⁺. The Zr^90m -decay sheme is in accordance with the level sequence of Zr⁹⁰ as measured in the Nb⁹⁰ decay.     

Study of Er171 decay by means of an electron-gamma coincidence technique

The decay scheme of Er¹⁷¹ (7.8 h) has been reinvestigated by means of an electron-gamma coincidence spectrometer and a scintillation spectrometer with a transistorized RIDL-400 channel analyser. A careful unfolding of the high energy region of the gamma-ray spectrum revealed the presence of photopeaks at energies of approximately 371, 404, 543, 572, 618, 675, 738, 796, 869, 910 and 962 keV. The existence of 32 transitions in Tm¹⁷¹ was confirmed. Also, it is proved that the 277, 362 keV transitions are in coincidence with the 210 keV and that the 175 keV transition is in coincidence with the 86 keV transition. We revealed the doubt for the existence of the 166, 210, 236, 277 and 419 keV transitions. From coincidence and single counting rates the followingK-conversion coefficients of the 111, 116, 124, 296 and 308 keV transitions were determined to be: α _K (111)=1.561±0.062, α _K (116)=0.699±0.035, α _K (124)=0.608±0.024, α _K (296)=0.0197±0.0010, α _K (308)=0.0183±0.0009, which give the 116, 124 keV transitions an electric quadrupole character; the 111 keV transition a magnetic dipole character withE2/M1 equal 0.4528; and the 296, 308 keV transitions an electric dipole character withM2/E1 equal 0.0058 and 0.0071 respectively.     

Dasβ-Spektrum des Cs137

Theβ-ray spectrum of Cs¹³⁷ has been measured with an iron-free spectrometer. The energy of the soft component was found to beE ₀=514±2 keV. The parameterk of the hard-component shape factorC _2VA ⁽²⁾ (W)=q ²+kp ² was determined to bek=0.015±0.004. Theβ intensities amount to 6.5% (hard component) and 93.5% (soft component). TheK conversion coefficient of the isomeric transition was measured to beα _K=0.093±0.003, in excellent agreement withSliv's theoretical value.     

Die Lebensdauer des 23/2-Dreiteilchenniveaus des Hafnium 177 und sein Zerfall durchK-verbotene Gamma-Übergänge

An isomeric state of Hf¹⁷⁷ withT _1/2=(1,12±0,10)s was found by a fast chemical separation of the hafnium daughter from the 155d Lu^177m activity. We measured the same half-life by observing the delayedβ-γ-coincidences. A systematic investigation of the whole region 5s≧T _1/2≧10^?7s by the technique of delayed coincidences gave no further isomerism. We assign the observed half-life to the 23/2 three particle state of Hf¹⁷⁷ at 1315 keV and assume that the second hypothetical three particle state at 1337 keV does not exist. The 21/2 rotational state of theK=9/2 band is populated by a strongly converted 14,16 keVγ-transition from the isomeric state at 1315 keV. The 14,16 keVM _I andN _I conversion lines were observed by use of a double focusing magneticβ-spectrometer. The isomerism is caused by theK-selection rule. The retardation of the following threeγ-transitions by different degrees ofK-forbiddeness is discussed. The pulse height spectrum, measured by means of a Li-drifted Ge-detector, does not show the 36,52 keV-γ-transition which was previously assumed to populate the 1301keV-state. In addition to the knownγ-transitions we found a 40,9 keV-line. This is probably the transition between the 1301,1 keV and the 1260,3 keV-states.     

Der Zerfall von Nb94 m

Using scintillation spectrometers and coincidence techniques the decay of Nb^{94 m} has been investigated. TheK-shell conversion coefficient of the 41.5 keV isomeric transition was found to be 570±100 indicating aM 3 transition. The maximum energy of theβ-decay to the 0.87 MeV level of Mo⁹⁴ is (1.15±0.03) MeV occurring (4·5±0·7)×10^?3 per disintegration, anotherβ-decay to the 1.57 MeV level was found to be (4·0±1·3)×10^?5. From this the parities and spins of the levels involved in the decay of Nb^{94 m} are determined.     

Die Faktoren der inneren Umwandlung beim35Br80m (4,4 Std)

The intensities of the 37keV- and 49keV-γ-rays of Br^80m have been measured with the aid of Na J-scintillation spectrometers and compared with the intensity of the conversion electrons registered by an anthracene split crystal spectrometer. It was possible to separate the 49 keV-γ-radiation from the intense 37 keV-line by selctive absorption with balanced Sm- and Gd-filters. The internal conversion coefficientsα(49 keV)=298±30 andα (37 keV)=1,59±0,10 are in good agreement with the calculated values for M₃- and E₁-transitions. The half life was measured yielding a value ofT _1/2=(4,40±0,05) h.     

Winkelkorrelationsmessungen an >30y Holmium 166 und Bestimmung desg R -Faktors des 4+-Rotationsniveaus von Erbium 166

The spins of several excited states of Er¹⁶⁶ have been investigated byγγ-angular correlation measurements. The spin sequence 0+, 2+, 4+, 6+ for the ground state rotational band was presumed to be correct. Unique assignments were derived for the states of 1076 keV, 1377 keV and 1785 keV asI=5, 7 and 6 respectively. These results are in agreement with the spins proposed byGallagher jr. andSoloviev. The multipolarities of theγ-transitions of 408 keV, 709 keV, 811 keV and 831 keV were derived as 95%E1+(5±1)%M2, 99·6%E1+(0·4±0·5)%M2, 99·1%E2+(0·9±0·3)%M1, and 96·1%E2+(3·9±1)%M1 respectively. The unusual mixing ratios of the transitions of 811 keV and 831 keV can be understood as a consequence of theK-selection rule. Eachγ-transition from the 1785 keV state should be stronglyK-forbidden and one expects a half-life ofT _1/2≈3·10^?9s. A measurement of the time spectrum of the coincidences between theβ-radiation and the high energyγ-lines gave however:T _1/2(1785 keV state)≦3·10^?10s. The rotation of the angular correlation between the 184 keV line and theγ-group at 820 keV has been measured in an external magnetic field of 53000 gauss as:ω·τ(4+)=0·083±0·006. This value contains small corrections for an additional rotation of the angular correlation of the 831 keV–184 keV triple cascade in the 6+state and for a small attenuation by internal fields. WithT _1/2(4+state)=1·23·10^?10s, andβ=7·08 one gets for theg-factorg _R=+0·266±0·024 in good agreement with recent results for the 2+ state.     

Der Zerfall des 1,5 min-Isomers Co54m

Co^54m (T _1/2=1.43 min) was produced in iron-foils by irradiation with_dE=19 MeV deuterons. The gamma ray spectrum was investigated using a NaJ(Tl) scintillation spectrometer, a coincidence circuit and a Ge(Li)-counter. There were observed three gamma rays having the following energies and intensities per Co_54m decay: 411 keV (0.97±0.07), 1130keV (0.98±0.05), 1407 keV (1.00±0.05). The directional correlation between the pairs of gamma rays were determined. These results correspond to spin and parityJ _π=2⁺ for the 1407 keV,J _π=4⁺ for the 2537 keV, andJ _π=6⁺ for the 2948 keV energy level of Fe⁵⁴. The last-mentioned level was not excited in previous scattering experiments. Our results are compatible withE=210keV andJ _π=6⁺ or 7⁺ of the isomeric state of Co^54m .     

Der Faraday-Effekt an amorphen Selenschichten

Cl^38m was produced by neutron activation of chlorine containing samples in a pneumatic irradiation facility. The decay of the Cl³⁸-isomer was investigated by various scintillation spectrometer technics. The half-life and the internal conversion coefficient α of the 0.66 MeV isomeric transition was found to beT _1/2=0.74±0.03 sec and α=(5.0±1.2)×10^?4. These data suggest aM-3 transition between an isomeric state with the spinI=5^? and the ground-state of Cl-38 (I=2^?).     

Astrophysical <Emphasis Type="Italic">S</Emphasis>-factor of T(<Superscript>4</Superscript>He, γ)<Superscript>7</Superscript>Li reaction at <Emphasis Type="Italic">E</Emphasis><Subscript>cm</Subscript> = 15.7 keV

The astrophysical S-factor of the reaction T(⁴He, γ)⁷Li is measured for the first time at the center of mass energy E _cm = 15.7 keV, lower than the energy range of the Standard Big Bang Nucleosynthesis (SBBN) model. The experiment is performed on a Hall pulsed accelerator (TPU, Tomsk). An acceleration pulse length of 10 μs allows one to suppress the background of cosmic radiation and the ambient medium by five orders of magnitude. A beam intensity of ~ 5 × 10^{14 4}He⁺ ions per pulse allows one to measure an extremely low reaction yield. The yield of γ-quanta with the energies E _γ ⁰ = 2483.7 keV and E _γ ¹ = 2006.1 keV is registered by NaI(Tl) detectors with the efficiency ε = 0.331 ± 0.026. A method for direct measurement of the background from the chain of reactions T(⁴He, ⁴He)T→T(T, 2n)X→(n, γ) and/or (n, n′γ) which ends by neutron activation of materials surrounding the target is proposed and implemented in this study. The value of the astrophysical S-factor of the reaction T(⁴He, γ)⁷Li S _αt (E _cm = 15.7 keV) = 0.091 ± 0.032 keV b provides the choice from the set of experimental data for the astrophysical S _αt -factor in favor of experimental data [4] with S _αt (E _cm = 0) = 0.1067 ± 0.0064 keV b.     

Aufbau eines automatisch arbeitenden π√2-Spektrometers und Untersuchung des Konversionslinienspektrums von In114m und ThB mit Folgeprodukten

An automatically operatedπ√2 spectrometer is described. The regulated current supply is transistorized. With this spectrometer the electron spectra of In^114m and of ThB with daughter products have been investigated. TheK/L ratio of the 191 keV isomeric transition in In^114m was found to be 1·25±0·03, in excellent agreement with the theoretical value ofSliv andBand. In the electron spectrum of ThB and daughter products 46 lines were found betweenB?=1750Г cm andB?=10000Г cm. Some of them are new. Most important is a new weak line atB?=7030Г cm which fixes a new level atE=1·807 MeV in ThC′ (Po²¹²). Simultaneously the earlier reported discrepancy between electron andγ-ray intensities for 1·8 MeV transition energy is resolved. There is anE0 transition of 1·800 MeV while the new line is theK conversion line of a new radiative transition (most probablyM2). A spin ofI=2+ is assigned to the 1·680 MeV level of ThC′. The 0·953 MeV transition from this level isM1, withE0 admixture.     

TheK-conversion coefficient of the 321 keVE1 transition in Hf177

TheK-conversion coefficient of the 321 keVE1 transition in Hf¹⁷⁷ has been measured by means of an iron free double focusing beta-ray spectrometer, using the internalexternal conversion method. The result obtained for α _K (321)=0.162±0.016 is in disagreement with the theoretical values for pureE1 transition (α _K =0.0154) calculated bySliv andBand. The large anomaly observed in theK-conversion process of the inhibitedE1 transition is compatible with a largeM2 admixture or, more probable with the presence of penetration matrix elements.