共查询到20条相似文献,搜索用时 31 毫秒
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Surface second-harmonic generation (SHG) of Si(1 1 1)-7×7 shows an increase in intensity for the surface-state transition (56%) and the strain-induced E0′ interband transition (32%) in response to the phase transition to “1×1” taking place around 1100 K. The SHG surface-state transition in “1×1” is assigned as the redshifted S3→U1 transition in 7×7 from the observation of no discernible changes in the resonant characteristics. From the symmetry and atomic geometry of the electronic states responsible for SHG, the intensity jump is related to the dissolution of the stacking fault in the “1×1” phase. 相似文献
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Scanning tunneling microscope-light emission (STM-LE) from the Si(1 1 1)-(7×7) surface has been measured using silver tips. For silver tips photon emission was enhanced by more than 100 times as compared with that for tungsten or platinum–iridium alloy tips. A broad spectrum with a single peak at ∼2.25 eV was observed. The spectrum obtained can be reproduced by a theory based on the macroscopic dielectric response of the tip-sample system, indicating that the observed emission arises from the localized plasmons on the silver tip excited by tunneling electrons. Spatial variations in the emission intensity at the atomic scale was observed even under low bias voltage (2 V) and low tunneling current (1 nA) conditions. 相似文献
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We have measured the coverage dependence of vibrational excitation spectra of C70 molecules adsorbed on a Si(1 1 1)-(7×7) surface using high-resolution electron-energy-loss spectroscopy. At the monolayer coverage, the intensity of the 57 meV peak increases, and those of the 83 and 178 meV peaks decrease. Taking into account the dipole selection rule, the change in intensity of the 57 meV peak indicates that the average angle between the long axes of C70 molecules and surface normal is about 40°. The decreases in intensities of the 83 and 178 meV peaks suggest that the rotational motion of molecules is quenched upon adsorption. We will discuss the Coriolis interaction between the accidentally degenerate A2″ and E1′ modes. 相似文献
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The adsorption of coronene (C24H12) on the Si(1 1 1)-(7 × 7) surface is studied using scanning tunneling microscopy (STM). Upon room temperature submonolayer deposition, we find that the coronene molecules preferentially adsorb on the unfaulted half of the 7 × 7 unit cell. Molecules adsorbed on different sites can be induced to move to the preferential sites by the action of the tip in repeated image scans. Imaging of the molecules is strongly bias dependent, and also critically depends on the adsorption site. We analyze the results in terms of differential bonding strength for the different adsorption sites and we identify those substrate atoms which participate in the bonding with the molecule. 相似文献
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中红外光纤合束器可将多个低功率的中红外激光器进行合束,从而实现较高的功率输出。本工作研制了一种7×1硫系玻璃光纤合束器(未熔接输出光纤),评估了其中红外传输特性。该光纤合束器由As40S60/As38S62光纤组束熔融拉锥而成,初始光纤的纤芯直径和包层直径分别为200μm和250μm,数值孔径为0.38~0.35(@2~6μm),拉锥比例R为3和4,锥形过渡区长度为2 cm。测试结果表明:当R=3时,制备的光纤合束器在3μm和4.6μm波长的端口传输效率分别为>90%和>87%;当R=4时,制备的光纤合束器在3μm和4.6μm波长的端口传输效率分别为>88%和>85%;光纤合束器输出端的光纤单丝之间未发生明显串扰。 相似文献
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《中国光学快报(英文版)》2015,(6)
All-fiber signal combiner is a key component for augmenting the fiber laser power. Presently the reported 7 × 1signal combiners are all have output fibers with core diameters larger than 100 μm. In order to improve the beam quality of the combiner, a fiber with smaller core of 50 μm diameter is chose to be the output fiber. An all-fiber7 × 1 signal combiner is fabricated with measured power transmission efficiency around 99% for each port. The beam quality is improved and the measured M2 are around 6 which are matched well with the theoretically calculated results. 相似文献
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We investigate the adsorption of organic molecular semiconductor perylene on(7 × 7) reconstructed Si(111)surface by ultraviolet photoemission spectroscopy.It is observed that seven features that derive from the organic material are located at 0.71,2.24,4.0,5.9,7.46,8.65 and 9.95 eV in binding energy.The theoretical calculation results reveal the most stable adsorption geometry of organic molecule perylene on Si(111)(7 × 7) substrates is at the beginning of deposition. 相似文献
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本文基于有相互作用的结构件的概念,对Si(111)7×7结构模型的稳定性进行研究。利用紧束缚法,计算了各种结构件的形成能及其相互作用能。由这些结构件可灵活地构成各种大单胞的表面结构并对其进行总能计算,而避免了大工作量的计算。对Si(111)5×5和7×7DAS模型,我们得到其表面能分别为-0.467eV和-0.477eV,与Qian和Chadi的结果很接近。并指出,Harrison提出的7×7吸附原子模型和Binnig等人提出的7×7吸附原子-空位模型都是不稳定的。 相似文献
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《Surface science》1988,197(3):L269-L272
A two-dimensional Hubbard Hamiltonian is introduced in order to analyse the many-body effects associated with a dangling bond Si(111) 7×7 surface state located at the Fermi energy. Our results indicate that many-body effects can offer an explanation of recently reported experimental data. 相似文献
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Using Scanning Tunneling Microscope (STM), we show that the surface undergoes phase transformation from disordered “1 × 1” to (7 × 7) reconstruction which is mediated by the formation of Si magic clusters. Mono-disperse Si magic clusters of size ~ 13.5 ± 0.5 Å can be formed by heating the Si(111) surface to 1200 °C and quenching it to room temperature at cooling rates of at least 100 °C/min. The structure consists of 3 tetra-clusters of size ~ 4.5 ? similar to the Si magic clusters that were formed from Si adatoms deposited by Si solid source on Si(111)-(7 × 7) [1]. Using real time STM scanning to probe the surface at ~ 400 °C, we show that Si magic clusters pop up from the (1 × 1) surface and form spontaneously during the phase transformation. This is attributed to the difference in atomic density between “disordered 1 × 1” and (7 × 7) surface structures which lead to the release of excess Si atoms onto the surface as magic clusters. 相似文献