Raman scattering in CdTe1-xSex and CdS1-xSex nanocrystals embedded in glass

Raman scattering on a series of glass composite samples containing CdTe_1-xSe_x and CdS_1-xSe_x nanocrystals with radii in the range [2nm, 12.5nm] is reported. By properly considering the size dependence of strain and confinement effects, the chemical composition and the lattice contraction is assessed. The polarization analysis of the scattering indicates that the Fröhlich electron-phonon interaction increases at decreasing the nanocrystal size.     

Picosecond time-resolved luminescence of localized excitons in CdS1-xSex

We present time-resolved luminescence results on CdS_0.36Se_0.64 which give a new insight on the kinetics of excitons localized by alloy potential fluctuations. By exciting in the localized exciton band with detection close to the exciting wavelength we obtain the lifetime across the band. Below the exciting laser energy two processes contribute to luminescence: transfer of localized excitons by tunnel effect assisted by acoustical phonons, and luminescence (assisted by acoustical phonons) of all the states excited at time t = 0 either directly or through their acoustical absorption wing. The time behavior of luminescence with respect to the detuning from the exciting energy helps to discriminate between those two contributions. Furthermore it shows that intermediate long-living states are involved in the exciton relaxation process.     

飞秒激光脉冲宽度和脉冲波形测试技术

飞秒激光在激光核聚变、卫星精密测距、激光微加工等领域具有重要的应用前景,同时也是产生太赫兹波的主要泵浦源。介绍了国内外飞秒激光脉冲宽度和脉冲波形的测试方法,比较了自相关法、频率分辨光学快门法、光谱相位相干直接电场重构法的优缺点。自相关法具有脉宽测量范围广、结构简单等特点,但不具备脉冲波形测试能力。光谱相位相干直接电场重构法对待测激光光束质量要求较高, 不适合大量程范围激光脉宽快速测量。为满足10 fs~5 ps大量程范围超短激光脉冲宽度和脉冲波形的测试需求,采用自相关法及二次谐波频率分辨光学开关法研制飞秒激光脉冲宽度和脉冲波形测试仪,时间分辨率优于2 fs。     

Influence of laser pulse width on absolute EUV-yield from Xe-clusters

Using 50 fs ( ∼ 2×10¹⁸ W/cm²) and 2 ps ( ∼ 5×10¹⁶ W/cm²) pulses from a Ti:Sa multi-TW laser at 800 nm wavelength large Xe-clusters ( 10⁵...10⁶ atoms per cluster) have been excited. Absolute yield measurements of EUV-emission in a wavelength range between 10 nm and 15 nm in combination with cluster target variation were carried out. The ps-laser pulse has resulted in about 30% enhanced and spatially more uniform EUV-emission compared to fs-laser excitation. Circularly polarized laser light instead of linear polarization results in enhanced emission which is probably caused by electrons gaining higher energies by the polarization dependent optical field ionization process. An absolute emission efficiency at 13.4 nm of up to 0.8% in 2π sr and 2.2% bandwidth has been obtained. Received 11 January 2001 and Received in final form 27 March 2001     

可调脉冲宽度的调Q掺铥双包层光纤激光器

在激光器输出平均功率一定的情况下,峰值功率主要取决于调制频率和脉冲宽度。这使得脉冲宽度的调节具有一定的实际应用价值。对调Q掺铥双包层光纤激光器进行研究,首先确定了激光器的最佳输出透过率,在65%最佳透过率时,得到2 m激光的输出功率3.9 W,斜率效率为31%。外接一个信号发生器,信号门宽从12 s变化到18 s,并测量了调制频率分别在30 kHz、40 kHz和50 kHz时输出脉冲宽度的变化情况,得到了555.6 W的最高峰值功率,实现了脉冲宽度从163.4 ns到207.9 ns的变化。实验情况证实了用外接信号发生器能有效控制激光器的输出脉冲宽度。     

Dispersion and compensation of temporal pulse width for femtosecond pulse laser ranging

We built an atmosphere dispersion model of femtosecond laser pulses that can calculate temporal pulse width travelling in air. The initial pulse duration of 100 fs can be broadened to 60 ps when propagating 200 km in the atmosphere. An experimental system has been established to compensate the large dispersion propagating 200 km in the atmosphere. The single model fiber (SMF) and the prism pairs were, respectively, used for coarse and fine compensation in the system. The pulse duration was consistently regulated 150 fs by moving the distance of prism pairs. This method can reach submicron resolution for a long distance by means of time of flight measurement.     

Dependence of the pressure pulse generated in an opticoacoustical receiver on the intensity of the exciting laser pulse

Calculations of the time form and amplitude of the acoustic signal generated in an absorbing gas that fills the cuvette of an opticoacoustical receiver in the case of a nonlinear nonsteady interaction with a single laser pulse are performed. Expressions relating the parameters of the acoustic signal with the characteristics of the laser pulse are derived, and an expression is proposed for the parameter characterizing the nonlinearity of the absorption of the given gas.     

The effect of laser peak power and pulse width on the hole geometry repeatability in laser percussion drilling

In this work, the two main factors that influence the repeatability of the laser percussion drilling process are identified. Experimental parametric analysis was carried out to correlate the laser parameters with the repeatability of a laser percussion drilling process. The experiment was conducted using a flash lamp pumped Nd:YAG laser to drill 2 mm thick mild steel sheets. The relationship between the percentage standard deviation (PSD) of entrance hole diameter, hole circularity and the operating parameters is established. Thirty-five holes were drilled and analysed for each set of identical laser parameters. The PSD of entrance hole diameter ranges between 1.47% and 4.78% for an operating window of 3.5–7 kW peak power, and 1–3 ms pulse width. The circularity of the entrance hole (defined as the ratio between the minimum and maximum diameters of the hole) ranges from 0.94 to 0.87, and is found to correlate with repeatability. The work shows that higher peak power, and shorter pulse width gives better hole geometry repeatability. The effect of melt ejection on hole geometry repeatability is also investigated. Melt ejection and spatter formation have been found to contribute to the poor repeatability of the process.     

脉宽对中红外激光带内损伤HgCdTe材料的影响

研究了脉宽对于中红外脉冲激光带内损伤碲镉汞（HgCdTe）材料阈值的影响,使用一维自洽模型对激光辐照HgCdTe材料程中的载流子数密度,载流子对数目流,载流子对能流,载流子温度和材料晶格温度等相关参数进行仿真计算。仿真结果表明,波长2.85 μm,脉宽30 ps～10 ns单脉冲激光带内辐照HgCdTe材料的损伤阈值为200～500 mJ/cm2。其中,300 ps～3 ns脉冲激光的损伤阈值相近,均为200 mJ/cm2且低于其他脉宽激光的损伤阈值。搭建实验光路并进行相关实验验证仿真模型的正确性。实验发现,波长2.85 μm、脉宽300 ps的单脉冲激光带内辐照HgCdTe材料的损伤阈值在200 mJ/cm2左右。相同条件下,10 ns单脉冲激光带内辐照HgCdTe材料的损伤阈值约474 mJ/cm2。百皮秒脉冲激光对HgCdTe材料的损伤过程结合了热击穿和光学击穿效应,其独特的毁伤机理加剧了材料的损伤。     

不同序列拉曼光脉冲对原子重力仪灵敏度的影响

研究了不同序列拉曼光脉冲对原子重力仪灵敏度的影响.结果表明,通过调节脉冲间隔可以改善原子干涉重力仪的灵敏度.在标准配置下,只考虑重力及一阶重力梯度时,三脉冲序列（π/2-π-π/2）的原子干涉重力仪具有较大的灵敏度,四脉冲序列（π/2-π-π-π/2）的原子干涉重力仪对重力不敏感,可用来测量重力梯度,五脉冲作用会降低原子干涉重力仪的灵敏度. 关键词： 原子重力仪 拉曼激光脉冲序列 灵敏度     

A holographic measurement of the pulse width of a Q-switched ruby laser

The pulse width of the output from a Q-switched ruby laser is measured on the basis of holography of a moving object. It is shown that, when the object is rotating, the relative brightness of the reconstructed image decreases gaussianly with increase of the velocity of the object. Furthermore, we propose how to measure the frequency sweep in the duration of the pulse and also to relax traditional restrictions on holography of a moving object.     

Dependence of peak power and pulse width for UV N2 superradiant pulses on operating conditions in a coaxial laser device

A coaxial integrated pulse-generator-gas-laser was operated with molecular nitrogen at 337 nm. At a repetition rate of 5 Hz peak power and half width of the light pulses have been studied as functions of tube length, pressure and applied voltage. Outputs of 30 kW with 3 nsec fwhm were reached. The shortest pulses observed had half widths of about 1 nsec.     

飞秒激光脉宽对三态阶跃型分子波包运动的影响研究

用含时波包法研究了三态阶跃型K2分子在强飞秒泵浦-探测激光场中脉宽对波包动力学过程的影响.研究表明激光场强较弱或者脉宽较短都可能不出现Autler-Townes分裂.波包的振荡周期随脉宽增长而增大,而振荡幅度随脉宽增长而减小. 脉宽影响Rabi振荡,而Rabi振荡的变化又导致了基态和激发态布居数周期性变化．首次量化了脉宽对激发态布居数的影响,表明变化频率随着泵浦场强的增强而增大．研究表明调节激光脉宽可实现对态布居数的选择性分布,可以为实验上实现分子的光控制提供重要参考．     

Theoretical investigation of laser pulse width dependence in a thermal confinement regime

Previous molecular dynamics (MD) simulations of ultraviolet (UV) laser ablation demonstrate the distinct dependence of material ejection on laser fluence and laser pulse duration. In this paper, we examine the pulse width dependence when the laser pulse widths are appropriate for the thermal confinement regime. We perform MD simulations of laser ablation with a laser pulse duration of 1 ns and compare with a pulse width of 150 ps as in previous simulations. The simulations confirm that the pulse width in thermal confinement regime does not dramatically influence the molecular ejection mechanism. The simulations reveal differentiations, however, in plume composition and the ablation threshold value. PACS 02.70.Ns; 61.80.Az; 79.20.Ap