Auger electron and characteristic energy loss spectra of plutonium

The Auger electron and characteristic loss spectra of plutonium have been obtained for the first time using a four grid retarding potential analyzer. The surface of this reactive metal was prepared by scribing in situ in good vacuum with a titanium carbide blade. Oxygen and carbon impurities were still present after scribing. The origin of the Auger electron and loss peaks is suggested, and a correlation is made with the peaks observed for uranium dioxide by Ellis and Campbell.     

Surface and bulk plasmon coupling observed in reflection electron energy loss spectra

Reflection electron energy loss spectra have been measured for a semiconductor and some metals (Si, Cu, Ag and Au). A novel procedure is presented to rigorously decompose the spectra into contributions corresponding to surface and volume excitations. The resulting distributions of energy losses in an individual surface loss are in good agreement with theory. In particular, the begrenzungs effect occurring at the boundary of a solid state plasma, i.e. the reduction of the intensity of bulk modes due to the coupling with surface modes, can be clearly observed in the retrieved energy loss distribution.     

Integrated absorption of a spectral line with the Voigt profile

A simple approximation has been found for the integrated absorpton of a spectral line with Voigt profile. It is expressed in terms of the integrated absorption of the Doppler and Lorentz profiles. The maximum error is 8%.     

关于介质吸收与色散的振子特性参数

根据共振模型，讨论影响介质的吸收与色散的振子特性参数，得到关于振子阻尼系数的振子数的解析式。据此，利用介质的吸收谱曲线可以定量计算振子的阻尼系数和振子数，这对研究和改善介质的吸收和色散特性有重要意义。我们已用此方法研究气液浓度的光电特性。     

Specification of spectral line shape and multiplex dispersion by self-imaging and moiré technique

Due to finite width of a spectral line, the visibility of the moiré fringes formed by a grating and the self-image of another similar grating reduces by the increase of the self-image order. This effect is exploited to specify the spectral line shape by evaluating the Fourier transform of a function related to the visibility. Even, by using in-expensive optics, the technique can provide the spectral line shapes of rather broad widths—of the order of nanometer and more—by precisions that are comparable by those obtained by expensive Fourier transform spectrometers.Besides, it is shown that by comparing the line shapes obtained with and without a dispersive medium between the gratings, one can specify the dispersion function of the medium in the wavelength range covered by the spectrum.     

Free electron laser spectral dynamics with a modulation of electron beam energy

Recent experimental and theoretical works on free electron laser spectral dynamics have pointed out the difficulty to obtain a narrow and stable spectrum operation. This goal can only be achieved by avoiding the sideband generation leading to a broadband and unstable spectrum. Tapered wiggler and two-frequency wiggler are well suited for combining sharp spectrum and high efficiency but are not really compatible with a wide tunability of laser light. Filtering sidebands is a good way for lower power experiments but it seems to be difficult to conceive wideband filters, specially in the far-infrared region. Modulation of electron energy is a new potential soft way for controlling the spectral dynamics of longpulse free electron laser. Spectral dynamics under the modulation is investigated in the linear and non-linear regimes in the far-infrared region. Simulations show that a pulsed and sharp spectrum behavior can be obtained by optimizing the modulation parameters. The interest of such a method for the far-infrared experiments is discussed.     

Reverse-saturated absorption and narrow line in the absorption spectrum of a V-type three-level medium

We study the absorption spectrum of a V-type three-level atom when the laser beam interacts only with one of its two transitions. With the presence of vacuum-induced quantum interference, the absorption spectrum shows some new interesting features, which include ultranarrow absorption line, transparency, and a reverse-saturated absorption that is characterized by a larger absorption with increasing laser intensity.     

Practical spatial resolution of electron energy loss spectroscopy in aberration corrected scanning transmission electron microscopy

The resolution of electron energy loss spectroscopy (EELS) is limited by delocalization of inelastic electron scattering rather than probe size in an aberration corrected scanning transmission electron microscope (STEM). In this study, we present an experimental quantification of EELS spatial resolution using chemically modulated 2×(LaMnO(3))/2×(SrTiO(3)) and 2×(SrVO(3))/2×(SrTiO(3)) superlattices by measuring the full width at half maxima (FWHM) of integrated Ti M(2,3), Ti L(2,3), V L(2,3), Mn L(2,3), La N(4,5), La N(2,3) La M(4,5) and Sr L(3) edges over the superlattices. The EELS signals recorded using large collection angles are peaked at atomic columns. The FWHM of the EELS profile, obtained by curve-fitting, reveals a systematic trend with the energy loss for the Ti, V, and Mn edges. However, the experimental FWHM of the Sr and La edges deviates significantly from the observed experimental tendency.     

On the electromagnetic energy density and energy transfer rate in a medium with dispersion due to conduction

The simplest dispersion relation determined by dissipation due to conduction is considered; the electromagnetic energy density in a plane monochromatic wave and its (phase and group) velocity are determined, as well as the energy and momentum transfer rates. It is shown that the energy density at low frequencies in this case has the form of the electrostatic density, in which the permittivity is replaced by its real part, and the energy transfer rate in a plane electromagnetic wave is equal to the phase velocity. The group velocity may exceed the speed of light.     

Analysis of the spatial distribution of detector sensitivity in a multilayer randomly inhomogeneous medium with strong light scattering and absorption by the Monte Carlo method

The spatial distribution of sensitivity in the domain of detection of a fiber-optic sensor used for spectrophotometric studies of skin and other biological tissues is studied. The method and results of modeling the propagation of optical radiation in multilayer randomly inhomogeneous media with strong light scattering and absorption are presented. Owing to the small distances between the source and detector (100–800 μm), the propagation of radiation in the medium under study is modeled by the Monte Carlo method combining the calculation of true paths and the use of statistical weights. For the same reason, we represent the surface and interfaces of layers of skin as rough randomly periodic surfaces corresponding to the actual structure of human skin. The method presented can be recommended as a means for the optimum selection of an arrangement for radiation incoupling and outcoupling.     

On the relaxation of a medium after excitation with single fast heavy ions

A plasma model of relaxation of a medium in heavy-ion tracks in condensed matter has been proposed. The model is based on the solution of time-dependent equations of radiative-collisional kinetics. The state of the medium, which is described in the framework of the classical model of multiple ionization of target atoms by a field of fast multiply charged ions, is used as the initial condition. The relaxation in the plasma is investigated using molecular dynamics simulation. An analysis of the results of the calculations performed has made it possible to determine the range of material parameters at which the plasma model actually changes over to the atomic model and to establish the conditions where the atomic model is a very rough approximation. It is demonstrated that the plasma model adequately describes the X-ray spectra recorded upon interaction of ion beams with condensed targets. An X-ray spectral method based on the plasma model is proposed for diagnosing the plasma in fast-ion tracks. The results obtained can be useful in examining the initial stage of defect formation in solids under irradiation with single fast heavy ions.     

Optical absorption and electron energy loss spectra of carbon and boron nitride nanotubes: a first-principles approach

We present results for the optical absorption spectra of small-diameter single-walled carbon and boron nitride nanotubes obtained by ab initio calculations in the framework of time-dependent density-functional theory. We compare the results with those obtained for the corresponding layered structures, i.e. the graphene and hexagonal boron nitride sheets. In particular, we focus on the role of depolarization effects, anisotropies, and interactions in the excited states. We show that the random phase approximation reproduces well the main features of the spectra when crystal local field effects are correctly included, and discuss to what extent the calculations can be further simplified by extrapolating results obtained for the layered systems to results expected for the tubes. The present results are relevant for the interpretation of data obtained by recent experimental tools for nanotube characterization, such as optical and fluorescence spectroscopies, as well as polarized resonant Raman scattering spectroscopy. We also address electron energy loss spectra in the small-q momentum-transfer limit. In this case, the interlayer and intertube interactions play an enhanced role with respect to optical spectroscopy. PACS 71.45.Gm; 77.22.Ej; 78.20.Bh; 78.67.Ch