Investigation of the external-magnetic-field dependence of polarization transfer in a 8Li-6Li disordered nuclear system

Random walks in disorderedmedia are studied by considering the example of the delocalization of nuclear polarization in an ensemble of ⁸Li beta-active nuclei produced in (n, γ) reactions induced by polarized thermal neutrons in LiF single crystals. The process is initiated by magnetic dipole-dipole interactions. It consists in polarization transfer from a primarily polarized ⁸Li nucleus to the closest (stable) ⁶Li nuclei and in subsequent polarizationmigration over 6Li nuclei, the return of the polarization in question to the ⁸Li nucleus being possible. In order to obtain information about the polarization of ⁸Li nuclei, the asymmetry of beta radiation from them was measured with respect to the external magnetic field H ₀. The process was studied until it reached the diffusion asymptotic regime. The concentration of ⁶Li was varied between 3% and 10%, while the field strength H ₀ was changed from 200 to 1200 G. It is shown that microscopic theory is in satisfactory agreement with the experimental results obtained in the way outlined above. A comparison with the investigation of the mathematically allied process of the Förster electricdipole transfer of localized excitons is performed.     

Experimental investigation of highly excited states of the 5,6He and 5,6Li nuclei in the (6Li, 7Be) and (6Li, 7Li) one-nucleon pickup reactions

The (⁶Li, ⁷Be) and (⁶Li, ⁷Li) reactions on ⁶Li and ⁷Li nuclei were investigated in the angular interval 0°–20° in the laboratory system at a ⁶Li energy of 93 MeV. In addition to low-lying states of the ^5,6He and ^5,6Li nuclei, broad structures were observed near the t(³He)+d and t(³He)+t thresholds at the excitation energies of 16.75 (3/2⁺) and ～20 MeV (for ⁵He), 16.66 (3/2⁺) and ～20 MeV (⁵Li), 14.0 and 25 MeV (⁶He), and ～20 MeV (⁶Li). The angular distributions measured in the ⁷Li(⁶Li, ⁷Be)⁶He reaction for transitions to the ground state (0⁺) and excited states at E _x=1.8 MeV (2⁺) and 14.0 MeV of the ⁶He nucleus were analyzed by the finite-range distorted-wave method assuming the 1p-and 1s-proton pickup mechanism. The (⁶Li, ⁷Be) and (⁶Li, ⁷Li) reactions were shown to proceed predominantly through the one-step pickup mechanism, and the broad structures observed at high excitation energies are considered as quasimolecular states of the t(³He)+d and t(³He)+t types.     

Spin exchange polarization and measurement of the hyperfine splitting of short-lived8Li

Free⁸Li (T _1/2=0.84 sec) atoms were polarized by spin exchange with optically pumped rubidium vapour. The⁸Li nuclei were produced by the reaction⁷Li(d, p)⁸Li in a thin LiF target. They recoiled into helium which was used as a buffer gas for optical pumping as well. Nuclear polarization up to 2% was detected by β-decay asymmetry. Rf transitions between hfs levels of the atomic ground state yielded the hfs separation ΔW=382.543(7) MHz. The nuclear spin assignmentI=2 was confirmed.     

Single nucleon transfer reactions in6Li+6Li collisions at 156 MeV

Single nucleon transfer reactions in collisions of 156 MeV⁶Li ions with⁶Li nuclei, leading to unstable final nuclei (⁵Li,⁵He) have been experimentally studied. The measured⁶Li(⁶Li,⁷Li)⁵Li_gr and⁶Li(⁶Li,⁷Be)⁵He_gr differential cross sections have been analysed on the basis of a FR-DWBA procedure, looking to which extent the entrance channel optical potentials may account for the unknown exit channel potentials.     

β-delayed neutron decay of drip line nuclei 11Li and 14Be

Experimental studies of β-decay measurements of the neutron drip line nuclei ¹¹Li and ¹⁴Be are presented. β- decay schemes of these nuclei are determined by measuring β-rays, delayed neutrons and γ-rays in triple coincidence. The decay schemes of both ¹¹Li and ¹⁴Be associated with single neutron emission are unambiguously determined. New levels in their daughter nuclei, ¹¹Be and ¹⁴B, are found. In addition, the deduced level scheme of 14B indicates the lowering of 2s _1/2 single neutron orbital with respect to 1p _1/2 orbital in the N=9 isotones. Such behavior is known to exist in N=7.     

Quadrupole interaction of8Li and9Li in LiNbO3 and the quadrupole moment of9Li

The quadrupole interaction of nuclear spin polarized⁸Li (I=2) and⁹Li (I=3/2) in LiNbO₃ has been studied at room temperature. The polarization was achieved by optical pumping of a fast atomic beam with circularly polarized laser light. The atoms were implanted into a hexagonal LiNbO₃ single crystal and the quadrupole splitting ofβ-NMR spectra was measured. A ratio of ¦Q(⁹Li)/Q(⁸Li)¦=0.88(4) for the nuclear quadrupole moments was deduced, yielding a new value of ¦Q(⁹Li)¦=25.3 (9) mb for the quadrupole moment of⁹Li.     

Direct and sequential Coulomb break-up of 7Li

Direct and sequential break-up of ⁷Li projectiles in the field of heavy target nuclei are studied on the basis of the Coulomb excitation approach. It is found that the experimental data observed for forward emission angles are fairly well described by Coulomb effects and that for angles more forward than 12° the direct (E1) break-up or 70 MeV⁷Li scattered from ¹²⁰Sn exceeds considerably the resonant (E2) break-up mode via the 7⁻/2 state in ⁷Li at E_x = 4.63 MeV.     

Vector analyzing power of π+7Li scattering in the region of the Δ33 resonance

Within Glauber diffraction theory, the vector analyzing power iT ₁₁ is calculated at three energies of positively charged pions, 134, 164, and 194 MeV, incident to ⁷Li nuclei. These energy values lie in the region of the Δ₃₃ resonance in π^± N interaction, the resonance maximum being at 180 MeV. The calculation of iT ₁₁ was performed with several model ⁷Li wave functions, including the αt-cluster and shell-model ones. The properties of π⁺⁷Li scattering are found to be sensitive to the structural features of the target nucleus. A comparison of the results of the calculations with experimental data shows that the wave functions in question and the potentials used to calculate them are quite appropriate.     

β NMR on8Li in the superiqnic conductor Li3N

Polarized⁸Li nuclei were produced in a Li₃N single crystal by irradiation with polarized neutrons, Β-ray detected NMR signals and spin-lattice relaxation of⁸Li were observed between B and 300 K. In Li₃N there are two non-equivalent Li sites. The corresponding two quadrupole split NMR spectra could be resolved. From the measured relaxation rates activation enthalpies for two diffusion processes were deduced.     

NMR study of 6Li in LiNbO3

An experimental NMR study of the ⁶Li isotope in single crystals of lithium niobate has been performed, along with a computer simulation of ⁶Li NMR spectra for a crystal of congruent composition, containing defects in the cation sublattice. It is found that the mean value of the principal component of the electric field gradient tensor at the ⁶Li nuclei is 1.48 times larger than at the ⁷Li nuclei. It is surmised that there is a substantial difference in the character of the mobility of the ⁶Li and ⁷Li nuclei in the LiO₆ octahedra at room temperature. Fiz. Tverd. Tela (St. Petersburg) 40, 122–125 (January 1998)     

Multiple quantum NMR transitions of8Li (T 1/2=0.84 s) in single crystals and powders of LiTaO3, and the quadrupole moment of8Li

Multiple quantum nuclear magnetic resonance (NMR) transitions were observed on polarized⁸Li nuclei, which were produced by capture of polarized neutrons in a single crystal of LiTaO₃. The asymmetric⁸Liβ-radiation distribution was used for the detection of NMR. A quadrupole moment ratio ¦Q(⁸Li)/Q(⁷Li)¦=0.78(1) was determined. Saturation of multiple quantum transitions in nuclear radiation detected NMR may lead to a reduction in measuring time of up to two orders of magnitude, as compared to single quantum detection methods. The measured spectra agree well with an exact lineshape calculation. The same measurements were also performed on a LiTaO₃ powder sample. This was done to test a method to obtain quadrupole coupling constants from high field NMR multiple quantum powder patterns, which are easily detectable, also for higher nuclear spins. This latter method may be applicable also to conventional NMR detection techniques.     

Five-nucleon transfer in the12C(d,7Li)7be reaction atE lab=78.0 MeV

Angular distributions of the¹²C(d,⁷Li)⁷Be reaction to the ground and to the unresolved first excited states of⁷Li or⁷Be nuclei were measured in the entire angular region in the centre of mass system atE _lab=78.0 MeV. Both the one-step five-nucleon cluster transfer as well as two-step sequential transfers were considered in the theoretical analysis. The former mechanism was found to dominate, but the latter is also not negligible.     

Li and K NMR relaxation study of a LiKSO4 single crystal

The ⁷Li and ³⁹K NMR relaxations in a LiKSO₄ single crystal grown by the slow evaporation method were investigated by employing a pulse NMR spectrometer. From the experimental data, the quadrupole coupling constant and asymmetry parameter were determined at the temperatures of 180 and 300 K. The relaxation processes of ⁷Li and ³⁹K were studied for the LiKSO₄ crystal, and the relaxation times for the ⁷Li and ³⁹K nuclei exhibit remarkable changes near T_c2 (=190 K). The activation energies for ⁷Li and ³⁹K were determined in phases I and III. The large change in the activation energy at 190 K indicates that the Li and K ions are significantly affected during this transition. The correlation time of the ⁷Li calculated from the spin-lattice relaxation time and quadrupole parameters was larger than that of the ³⁹K calculated using the same method. The reason for this is that the Li ion undergoes molecular motion as in the LiO₄ groups.     

Ionic Pathways in Li13Si4 investigated by 6Li and 7Li solid state NMR experiments

Local environments and dynamics of lithium ions in the binary lithium silicide Li₁₃Si₄ have been studied by ⁶Li MAS-NMR, ⁷Li spin-lattice relaxation time and site-resolved ⁷Li 2D exchange NMR measurements as a function of mixing time. Variable temperature experiments result in distinct differences in activation energies characterizing the transfer rates between the different lithium sites. Based on this information, a comprehensive picture of the preferred ionic transfer pathways in this silicide has been developed. With respect to local mobility, the results of the present study suggests the ordering Li6/Li7>Li5>Li1>Li4 >Li2/Li3. Mobility within the z=0.5 plane is distinctly higher than within the z=0 plane, and the ionic transfer between the planes is most facile via Li1/Li5 exchange. The lithium ionic mobility can be rationalized on the basis of the type of the coordinating silicide anions and the lithium-lithium distances within the structure. Lithium ions strongly interacting with the isolated Si⁴⁻ anions have distinctly lower mobility than those the coordination of which is dominated by Si₂⁶⁻ dumbbells.     

Contributions of excited 6Li and 7Li nuclei to the production of 4He+2H and 4He+3H systems in 16O p collisions at a momentum of 3.25 GeV/c per nucleon

New experimental data on the cross sections for the yield of excited ⁶Li* and ⁷Li* nuclei and on their contributions to the production of ⁴He + ²H and ⁴He+³H light dinuclear systems in ¹⁶O _p collisions at a momentumof 3.25 A GeV/c per nucleon are presented.     

Measurement of the excitation function for the <Superscript>7</Superscript>Li(t,p)<Superscript>9</Superscript>Li reaction using detection of delayed neutrons

The excitation function for the ⁷Li(t, p)⁹Li reaction is measured at the EGP-10 electrostatic tandem accelerator (VNIIEF) at the incident triton energies E _t = 5–11.3 MeV. The measurements were based on detection of delayed neutrons resulting from the decay of ⁹Li nuclei. The neutrons were detected by the 4π detector consisting of ³He counters enclosed in a polyethylene moderator. A pulsed mode was used for irradiating the LiF target (210 μg cm^?2) of natural isotopic composition on the tantalum backing. Absolutization of the excitation function was performed against the ⁷Li(p, n) reaction cross sections.     

Channel coupling and exchange of an alpha-particle cluster in deuteron scattering on 6Li nuclei

Existing experimental data on elastic and inelastic deuteron scattering on ⁶Li nuclei in the energy range from 8 to 50 MeV were analyzed within the approach of coupled reaction channels. The coupling of elastic scattering and inelastic scattering accompanied by the transition to the 3⁺ state at E _x = 2.186 MeV and the mechanism involving the exchange of an alpha-particle cluster were taken into account in respective calculations. The phenomenological potentials obtained from the present analysis describe well experimental angular distributions at all energies and in full angular ranges. The depths of the real and imaginary parts of the potentials in question depend smoothly on energy at fixed values of the remaining parameters. The energy dependence of relevant volume integrals agrees well with similar data for the p + ⁶Li, ?? + ⁶Li, and ¹²C + ¹²C systems and with the predictions of a microscopic theory.     

The quadrupole moment of the neutron-halo nucleus11Li

The quadrupole moment ratio of⁹Li and¹¹Li was measured by a combination of in-beam laser induced nuclear polarization and Β-NMR in LiNbO₃. The result ¦Q(¹¹Li)/Q(⁹Li)¦=1.14(16) is consistent with cluster models describing¹¹Li as composed of a⁹Li core and a far extended halo of two loosely bound neutrons.     

Quasielastic deuteron and triton knockout from lithium isotopes by intermediate-energy pions

Quasielastic deuteron and triton knockout from ⁶Li and ⁷Li nuclei that was induced by a π ^?-meson beam of momentum p ₀ = 0.72 and 0.88 GeV/c was studied under conditions of full kinematics. The experiment was performed at the Institute of Theoretical and Experimental Physics (ITEP, Moscow) by using a 3-m magnetic spectrometer equipped with spark chambers. The distributions with respect to the momenta of quasideuteron and quasitriton internal motion, the excitation-energy spectra of residual nuclei, and the effective numbers of quasideuterons in ⁶Li and ⁷Li nuclei were obtained.