Computer simulation and observation of anomalous light emission from nonlinear photonic crystal with various geometry of its elements

Recently, in papers [1, 2] were described the effect of long-time emission of photonic crystal (synthetic opals) under the action of nanosecond laser pulse. The duration of the luminescence is of the order of seconds. Despite on the other phenomena, which were considered in these papers, below we focus our attention on possible explanation of long time emission from nonlinear photonic crystal. The basis of our consideration is papers [3, 4], those deal with soliton formation in several layers of 1D nonlinear photonic crystal. Because of this, the light wave can exist in photonic crystal a long time (in ideal case—infinite time interval). Taking into account a relation between soliton duration and its maximum intensity, the leaving of laser energy from the layer of photonic crystal takes place due not full reflection from boundaries of layer. The time of light emission for this case depends on nonlinear susceptibility of photonic crystal and the intensity of laser pulse. Hence, soliton formation inside the nonlinear elements of photonic crystal can be one of the reasons of long time emission. We got in computer simulation a long time emission of 1D (layered) and 2D (circular or rectangular elements) nonlinear photonic crystal under the action of laser pulse with femtosecond duration under the conditions of soliton formation in some elements of photonic crystal. Input intensity of laser pulse, at which a soliton appears in nonlinear photonic crystal, can be ten times less due to effects of enhancement of optical intensity in periodic structure [4, 5].     

Spontaneous emission spectrum of a three-level atom embedded in photonic crystal

The two models of three-level (one upper level and two lower levels, or two upper levels and one lower level) atom embedded in a double-band photonic crystal are adopted. The atomic transitions from the upper levels to the lower levels are assumed to be coupled by the same reservoir which are respectively the isotropic photonic band gap (PBG) modes, the anisotropic PBG modes and the free vacuum modes. The effects of the fine structure of the atomic ground state levels in the model with one upper level and two lower levels, and the quantum interferences in the model with two upper levels and one lower level on the spontaneous emission spectrum of an atom are investigated in detail. Most interestingly, it is shown that new spontaneous emission lines are produced from the fine splitting of atomic ground state levels in the isotropic PBG case. The quantum interferences induce additional narrow spontaneous lines near the transition from the empty upper level to the lower level.     

具有态守恒赝隙的光子晶体中两能级原子自发辐射的增强与抑制

论证了在赝带隙光子晶体中存在一个全频率域态总数守恒规则，在完全带隙光子晶体中还存在一个局域态总数守恒规则.态总数守恒规则指出，如果一个光子晶体的态密度在某些频率范围存在相对于等效介质态密度的谷，则一定由其他频率范围内相对于等效介质态密度的峰来补偿.使用符合态总数守恒规则的态密度模型，解释了态密度调制导致的自发辐射谱增强、抑制、变窄、红移、蓝移以及谱分裂等光子晶体中的量子光学现象.该理论比较适合研究在具有赝带隙的光子晶体中大量随机分布的发光原子或分子的自发辐射行为. 关键词： 光子晶体 自发辐射 态密度 光子赝带隙     

Controllable Photonic Band Gap and Defect Mode in a 1D CO2-Laser Optical Lattice

We propose a new method to form a novel controfiable photonic crystal with cold atoms and study the photonic band gap （PBG） of an infinite 1D CO2-laser optical lattice of SSRb atoms under the condition of quantum coherence. A significant gap generated near the resonant frequency of the atom is founded and its dependence on physical parameters is also discussed. Using the eigenquation of defect mode, we calculate the defect mode when a defect is introduced into such a lattice. Our study shows that the proposed new method can be used to optically probe optical lattice in situ and to design some novel and controllable photonic crystals.     

Position Dependent Spontaneous Emission Spectra of a Λ-Type Atomic System Embedded in a Defective Photonic Crystal

We investigate the position dependent spontaneous emission spectra of a Λ-type three-level atom with one transition coupled to the free vacuum reservoir and the other one coupled to a double-band photonic band gap reservoir with a defect mode in the band gap.It is shown that,for the atom at the defect location,we have a two-peak spectrum with a wide dark line due to the strong coupling between the atom and the defect mode.While,when the atom is far from the defect location(or in the absence of the defect mode),the spectrum has three peaks with two dark lines due to the coupling between the atom and the photonic band gap reservoir with the largest density of states near the band edges.On the other hand,we have a four-peak spectrum for the atom at the space in between.Moreover,the average spontaneous emission spectra of the atoms uniformly embedded in high dielectric or low dielectric regions are described.It is shown that the atoms embedded in high(low) dielectric regions far from the defect location,effectively couple to the modes of the lower(upper) photonic band.However,the atoms embedded in high dielectric or low dielectric regions at the defect location,are coupled mainly to the defect modes.While,the atoms uniformly embedded in high(low) dielectric regions with a normal distance from the defect location,are coupled to both of defect and lower(upper) photonic band modes.     

Thermal emission properties of 2D and 3D silicon photonic crystals

We present measurements of the thermal emission properties of 2D and 3D silicon photonic crystals with and without substrate heated resistively as well as passively with an aluminium hotplate. The out-of-plane and in-plane emission properties were recorded and compared to numerical simulation. It turned out that for the in-plane 2D photonic crystal and out-of-plane 3D photonic crystal emission a photonic stop gap effect is visible. For the out-of-plane 2D photonic crystal emission, no photonic bandgap effect is observable but instead strong silicon oxide emission from native oxide inside the pores of silicon are observable. A model for the modified thermal emission is presented.     

具有复介电常量二维光子晶体的特性研究

采用平面波展开法,通过数值模拟研究了具有复介电常量的二维光子晶体的能带结构和光传输特性,重点讨论介电常量的虚部为负值情形时对传输特性的影响。研究表明由于光子带隙的存在有效地抑制了频率位于带隙内光的自发辐射。当在介质中掺入具有增益特性的杂质时,即使两种介质的介电常量相差很小,在靠近光子带隙边缘,出现了较强的受激辐射放大。通常在带隙的边缘处,光子晶体的群速度较小,而激光阈值正比于群速度的平方,当群速度很小时,激光阈值将大大减小。这为实现零阈值激光器提供了基础,也为制作光放大微器件提供了一个有益的理论参考。     

Effect of atomic initial phase difference on spontaneous emission of an atom embedded in photonic crystal

<正>We investigate the effect of initial phase difference between the two excited states of a V-type three-level atom on its steady state behaviour of spontaneous emission.A modified density of modes is introduced to calculate the spontaneous emission spectra in photonic crystal.Spectra in free space are also shown to compare with that in photonic crystal with different relative positions of the excited levels from upper band-edge frequency.It is found that the initial phase difference plays an important role in the quantum interference property between the two decay channels.For a zero initial phase,destructive property is presented in the spectra.With the increase of initial phase difference,quantum interference between the two decay channels from upper levels to ground level turns to be constructive.Furthermore, we give an interpretation for the property of these spectra.     

Entanglement of a two-level atom and its spontaneous emission near the edge of a photonic band gap

The entanglement of a two-level atom and its radiation field near the edge of a photonic band gap is studied by using the quantum entropy. Unlike the free space case, there is a steady-state entanglement between the atom and its spontaneous emission field even when the atomic transition frequency lies outside the band gap. Moreover, the degree of entanglement, which is due to the formation of atom–photon bound dressed state, depends on the detuning of the atomic transition frequency from the photonic band edge and can be controlled by a controllable photonic band gap crystal.     

Fabrication of three‐dimensional photonic crystals in quantum‐dot‐based materials

Controlling spontaneous emission (SE) is of fundamental importance to a diverse range of photonic applications including but not limited to quantum optics, low power displays, solar energy harvesting and optical communications. Characterized by photonic bandgap (PBG) property, three‐dimensional (3D) photonic crystals (PCs) have emerged as a promising synthetic material, which can manipulate photons in much the same way as a semiconductor does to electrons. Emission tunable nanocrystal quantum dots (QDs) are ideal point sources to be embedded into 3D PCs towards active devices. The challenge however lies in the combination of QDs with 3D PCs without degradation of their emission properties. Polymer materials stand out for this purpose due to their flexibility of incorporating active materials. Combining the versatile multi‐photon 3D micro‐fabrication techniques, active 3D PCs have been fabricated in polymer‐QD composites with demonstrated control of SE from QDs. With this milestone novel miniaturized photonic devices can thus be envisaged.     

Decay distribution of spontaneous emission from atoms in one-dimensional photonic crystal

Spontaneous emission behavior from atoms (or molecules) in one-dimensional photonic crystal with a defect is investigated. Taken all the TE and TM modes into account, the normalized spontaneous emission rate of the atom is calculated as a function of the position of the atom in the crystal. Results for both nonabsorbing dielectric structure and absorbing dielectric structure are presented. With the increase of the thickness of the defect in which the atoms are embedded, the oscillations of the spontaneous emission rate versus the position of the atom become dense and the lifetime distribution becomes narrow and sharp. The PC effect may lead to the coexistence of both accelerated and inhibited decay processes.     

Modification of the spontaneous emission of quantum dots near the surface of a three-dimensional colloidal photonic crystal

This paper demonstrates experimentally and numerically that a significant modification of spontaneous emission rate can be achieved near the surface of a three-dimensional photonic crystal.In experiments,semiconductor core-shell quantum dots are intentionally confined in a thin polymer film on which a three-dimensional colloidal photonic crystal is fabricated.The spontaneous emission rate of quantum dots is characterised by conventional and time-resolved photoluminescence (PL) measurements.The modification of the spontaneous emission rate,which is reflected in the change of spectral shape and PL lifetime,is clearly observed.While an obvious increase in the PL lifetime is found at most wavelengths in the band gap,a significant reduction in the PL lifetime by one order of magnitude is observed at the short-wavelength band edge.Numerical simulation reveals a periodic modulation of spontaneous emission rate with decreasing modulation strength when an emitter is moved away from the surface of the photonic crystal.It is supported by the fact that the modification of spontaneous emission rate is not pronounced for quantum dots distributed in a thick polymer film where both enhancement and suppression are present simultaneously.This finding provides a simple and effective way for improving the performance of light emitting devices.     

Specific features of the resonance interaction of a coherent wave with an ensemble of impurity atoms of a photonic crystal

Two-quantum relaxation transitions in an impurity atom that are activated by its resonance interaction with a monochromatic wave lead to hole burning in the distribution of atoms populating the lower energy level over detunings from the resonance. In this case, the levels of an impurity atom lying within the gap or the pseudogap in the density of photon states of a photonic crystal act as a trap. The impurity atoms change to these levels in the process of interaction of a monochromatic wave with the atomic transition that is not influenced by specific spectral features of a photonic crystal.     

Quantum theory of atom-surface scattering: Debye-Waller factor

The Debye-Waller factor, introduced historically for X-rays, was used later for electrons, neutrons, and atoms as well. In this process of extension, however, the assumptions on which the Debye-Waller theory rested became more and more questionable until in the case of atoms (whose scattering from surfaces is both strong and slow) serious modifications are necessary. In the present article four models are discussed in order. In Model 1 a fast atom impinges on a surface whose atoms all vibrate deviating from their equilibrium positions by the same vector displacement ?. In Model 2 again the impinging atom is fast, but the atoms in the surface vibrate incoherently rather than coherently. It is shown that both Models 1 and 2 yield the conventional Debye-Waller result in the infinite crystal atom mass limit (for Model 2 Einstein oscillators have also to be assumed) and it is also shown how corrections to this result can be built. Turning then to slow impinging atoms, in Model 3 a slow atom impinges on a hard crystal surface, interacting with the rapidly varying potential of the vibrating solid. Model 3 is discussed in detail and it is shown that the Debye-Waller exponent can be written in terms of a time integral of the product of two correlations: the force correlation and the displacement correlation. The result is a dramatic increase of diffraction of relatively heavy atoms (with respect to the conventional theory). Finally, in Model 4 the impinging atom is again slow but the crystal is soft rather than hard. This case is more difficult to treat but a preliminary analysis again indicates a dramatic increase of diffraction since the soft solid adjusts itself to the instantaneous atom position leading to elastic scattering. The experimental implications of the present theory, especially for neon scattering from surfaces, are discussed.     

Cavity Mode, Q Value and the Photon′s Lifetime in a Cavity Formed by Defected 2-Dimensional Photonic Crystal

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Simulation of interstitial atoms in two-dimensional nanocrystals

The molecular-dynamics method is used to study the emergence of interstitial atoms at a free face of a 2D nanocrystal. Two new types of coordination of the interstitial defect are discovered: a symmetric trifolium coordination and a linear coordination of compressed atoms. It is shown that, in the case of linear coordination, a dislocation dipole is formed in the 2D crystal lattice; the dipole is characterized by a high mobility facilitating the arrival of an interstitial atom at a free face of the crystal. The cases of transition of an interstitial atom from one type of coordination to another, depending on the crystal temperature, are studied in a computer experiment.     

Cavity Mode, Q Value and the Photon′s Lifetime in a Cavity Formed by Defected 2-Dimensional Photonic Crystal

A complex frequency method to calculate the lifetime, Q value and field distribution of cavity mode in a defected 2D photonic crystal cavity is presented. Using this method, we analyze the cavity mode formed by a 2D photonic crystal with an interval “atom”. This method is also applicable to the defected 2D photonic crystal cavity of other structures. Cavity formed by a 2D random photonic crystal is discussed.     

The influence on atomic decay by inserting a LHM layer into an ordinary one dimensional multi-layer structure

Inserting left-handed material (LHM) layers into a one dimensional structure can influence the spontaneous emission (SpE) of a two-level atom. This has been investigated, starting from the simplest case of a three-layer system, where we find the reflected field (atom can “see”) passing through LHM layer is stronger than that through the corresponding normal layer. Indeed the induced decay is more strongly influenced by reflected field passing through LHM layer. Based on this and after further analysis of reflectivity, we find that, a quarter photonic crystal (PC) composed of alternately LHM and RHM can inhibit the atomic spontaneous emission more intensely compared to an ordinary PC.     

Spontaneous emission from a microwave-driven four-level atom in an anisotropic photonic crystal

The spontaneous emission from a microwave-driven four-level atom embedded in an anisotropic photonic crystal is studied. Due to the modified density of state(DOS) in the anisotropic photonic band gap(PBG) and the coherent control induced by the coupling fields, spontaneous emission can be significantly enhanced when the position of the spontaneous emission peak gets close to the band gap edge. As a result of the closed-loop interaction between the fields and the atom,the spontaneous emission depends on the dynamically induced Autler–Townes splitting and its position relative to the PBG.Interesting phenomena, such as spectral-line suppression, enhancement and narrowing, and fluorescence quenching, appear in the spontaneous emission spectra, which are modulated by amplitudes and phases of the coherently driven fields and the effect of PBG. This theoretical study can provide us with more efficient methods to manipulate the atomic spontaneous emission.     

Robust Preparation of Atomic Concatenated Greenberger–Horne–Zeilinger States via Shortcuts to Adiabaticity

Here, a protocol for robust preparation of an atomic concatenated Greenberger–Horne–Zeilinger (C‐GHZ) state via shortcuts to adiabaticity (STA) is proposed. The devices for implementing the protocol consist of atoms, cavities, and the optical fibers, which are feasible with current technology. The atoms are trapped in the separated cavities allowing individual control over each atom with classical fields. STA helps to design Rabi frequencies of classical fields so that the atoms can be driven from the initial states to the target states. The numerical simulations show that the protocol holds robustness against atomic spontaneous emissions and photonic leakages. Thus, the protocol may be realized by experiments in the near future.