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1.
Oxy-fuel combustion is a promising alternative for power generation with CO2 capture, where the fuel is burned in an atmosphere enriched with oxygen and CO2 is used as a diluent. This type of combustion is characterised by uncommon characteristics in terms of thermal heat transfer budget as compared to air supported systems. The study presents experimental results of radiative heat flux along the flame axis and radiant fractions of non-premixed jet methane flames developing in oxy-fuel environments with oxygen concentrations ranging from 35% to 70%, as well as in air. The flames investigated have inlet Reynolds numbers from 468 to 2340. The data collected have highlighted the effects of the flame structure and thermo-chemical properties of oxy-fuel combustion on the heat flux radiated by the flames. It was first observed that peak heat flux increases considerably with oxygen concentration. More generally the radiant fraction increases with both increasing Reynolds number in the laminar regime and oxygen concentration. It was found that despite a difference in flame temperature, the radiative characteristics of the flames (heat flux distributions and radiant fraction) in air were similar to those with 35% O2 in CO2. The radiative properties of flames in oxy-fuel atmosphere with CO2 as diluents appear to be dominated by the flame temperature.  相似文献   

2.
One of the most promising methods for reducing NO x emissions of jet engines is the lean combustion process. For realization of this concept the percentage of air flowing through the combustor dome has to be drastically increased, which implies high volume fluxes in the primary zone of the combustion chamber and represents a substantial challenge in regard to the flame stabilization. Swirl motion is thus applied to the air flux by the swirl generator and decisively contributes to the flame stabilization. The current paper reviews an atmospheric investigation of a burner configuration in regard to the weak extinction limit, comprising a confined non-premixed swirl-stabilized flame. The burner can be supplied with either kerosene or after a small adaption with natural gas (methane). Therefore, a comparison of a kerosene-fuelled flame (spray flame) to a natural gas fuelled one (methane flame) can be performed. Both are realized by almost identical burner configuration and at identical conditions. The main idea of this work is to align the stability characteristics of both flames by means of similarity. However, fundamental differences regarding the flame structures of the flames are detected through in-flame measurements. This determines the limits of the current approach and motivates an appropriate choice of flame modeling.  相似文献   

3.
Oxy-fuel combustion has been proven to increase thermal efficiency and to have a potential for NOx emission reduction. The study of 25-kW turbulent diffusion flames of natural gas with pure oxygen is undertaken on a coaxial burner with quarl. The structural properties are analysed by imaging the instantaneous reaction zone by OH* chemiluminescence and measuring scalar and velocity profiles. The interaction between the flame front and the shear layers present in the coaxial jets depends on the momentum ratio which dictates the turbulent structure development. Flame length and NOx emission sensitivity to air leaks in the combustion chamber are also investigated. Received: 5 November 1999/Accepted: 29 April 2000  相似文献   

4.
Finite Rate Chemistry Effects in Highly Sheared Turbulent Premixed Flames   总被引:1,自引:0,他引:1  
Detailed scalar structure measurements of highly sheared turbulent premixed flames stabilized on the piloted premixed jet burner (PPJB) are reported together with corresponding numerical calculations using a particle based probability density function (PDF) method. The PPJB is capable of stabilizing highly turbulent premixed jet flames through the use of a small stoichiometric pilot that ensures initial ignition of the jet and a large shielding coflow of hot combustion products. Four lean premixed methane-air flames with a constant jet equivalence ratio are studied over a wide range of jet velocities. The scalar structure of the flames are examined through high resolution imaging of temperature and OH mole fraction, whilst the reaction rate structure is examined using simultaneous imaging of temperature and mole fractions of OH and CH2O. Measurements of temperature and mole fractions of CO and OH using the Raman–Rayleigh–LIF-crossed plane OH technique are used to examine the flame thickening and flame reaction rates. It is found that as the shear rates increase, finite-rate chemistry effects manifest through a gradual decrease in reactedness, rather than the abrupt localized extinction observed in non-premixed flames when approaching blow-off. This gradual decrease in reactedness is accompanied by a broadening in the reaction zone which is consistent with the view that turbulence structures become embedded within the instantaneous flame front. Numerical predictions using a particle-based PDF model are shown to be able to predict the measured flames with significant finite-rate chemistry effects, albeit with the use of a modified mixing frequency.  相似文献   

5.
Confined short turbulent swirling premixed and non-premixed methane and heptane spray flames stabilized on an axisymmetric bluff body in a square enclosure have been examined close to the blow-off limit and during the extinction transient with OH* chemiluminescence and OH-PLIF operated at 5 kHz. The comparison of flames of different canonical types in the same basic aerodynamic field allows insights on the relative blow-off behaviour. The flame structure has been examined for conditions increasingly closer to blow-off. The premixed flame was seen to change from a cylindrical shape at stable burning condtions, with the flame brush closing across the flow at conditions close to blow-off. The PLIF images show that for the gaseous non-premixed flame, holes appear along the flame sheet with increasing frequency as the blow-off condition is approached, while the trend is less obvious for the spray flame. Non-premixed and spray flames showed randomly-occurring lift-off, which is further evidence of localised extinction. The mean lift-off height increased with increasing fuel jet velocity and decreased with increasing air velocity and approaches zero (i.e. the flame is virtually attached) just before the blow-off condition, despite the fact that more holes were evident in the flame sheet as extinction was approached. It was found that the average duration of the blow-off event, when normalised with the characteristic flow time d/U b (d being the bluff-body diameter and U b the bulk velocity) was in the range 9–38 with the spray flame extinction lasting a shorter time than the gaseous flames. Finally, it was found that correlations based on a Damköhler number collapse the blow-off velocity data for all flames with reasonable accuracy. The results can help the development of advanced turbulent combustion models.  相似文献   

6.
Dynamic processes in gas turbine (GT) combustors play a key role in flame stabilization and extinction, combustion instabilities and pollutant formation, and present a challenge for experimental as well as numerical investigations. These phenomena were investigated in two gas turbine model combustors for premixed and partially premixed CH4/air swirl flames at atmospheric pressure. Optical access through large quartz windows enabled the application of laser Raman scattering, planar laser-induced fluorescence (PLIF) of OH, particle image velocimetry (PIV) at repetition rates up to 10 kHz and the simultaneous application of OH PLIF and PIV at a repetition rate of 5 kHz. Effects of unmixedness and reaction progress in lean premixed GT flames were revealed and quantified by Raman scattering. In a thermo-acoustically unstable flame, the cyclic variation in mixture fraction and its role for the feedback mechanism of the instability are addressed. In a partially premixed oscillating swirl flame, the cyclic variations of the heat release and the flow field were characterized by chemiluminescence imaging and PIV, respectively. Using phase-correlated Raman scattering measurements, significant phase-dependent variations of the mixture fraction and fuel distributions were revealed. The flame structures and the shape of the reaction zones were visualized by planar imaging of OH distribution. The simultaneous OH PLIF/PIV high-speed measurements revealed the time history of the flow field–flame interaction and demonstrated the development of a local flame extinction event. Further, the influence of a precessing vortex core on the flame topology and its dynamics is discussed.  相似文献   

7.
Flow structure of premixed propane–air swirling jet flames at various combustion regimes was studied experimentally by stereo PIV, CH* chemiluminescence imaging, and pressure probe. For the non-swirling conditions, a nonlinear feedback mechanism of the flame front interaction with ring-like vortices, developing in the jet shear layer, was found to play important role in the stabilisation of the premixed lifted flame. For the studied swirl rates (S = 0.41, 0.7, and 1.0) the determined domain of stable combustion can be divided into three main groups of flame types: attached flames, quasi-tubular flames, and lifted flames. These regimes were studied in details for the case of S = 1.0, and the difference in the flow structure of the vortex breakdown is described. For the quasi-tubular flames an increase of flow precessing above the recirculation zone was observed when increased the stoichiometric coefficient from 0.7 to 1.4. This precessing motion was supposed to be responsible for the observed increase of acoustic noise generation and could drive the transition from the quasi-tubular to the lifted flame regime.  相似文献   

8.
Quantitative hydroxyl time-series measurements from a set of stable and extinguishing turbulent opposed-flow partially premixed CH4/air flames are used to investigate the effect of Reynolds number and fuel-side equivalence ratio on the structure of turbulent partially premixed flames. The hydroxyl (OH) integral time scale, computed from the autocorrelation function, is used to characterize OH fluctuations and is found to reach a minimum at the axial location of peak OH. Analyses of the duration of and period between bursts in the OH time series are used to examine the dynamics of flame-front motion. In general, with increasing Reynolds number (Re), the distribution in OH burst times shifts towards smaller time scales. A hydroxyl intermittency parameter is also defined from the bursts to quantify the presence or absence of OH. For flames with the same fuel-side equivalence ratio, the hydroxyl intermittency at peak OH remains almost constant when going from stable to extinguishing flames. However, histograms portray an increase in burst separation times for flames displaying occasional extinction events. Hydroxyl time series for a partially premixed flame at a fuel-side equivalence ratio of 2.0 and Re = 6650 are synthesized by using mixture-fraction simulations based on calculated state relationships for OH versus mixture fraction (f). The laminar-flamelet model is employed to explore relations between OH and f so as to predict trends in mixture-fraction time scales.“Time-Series Measurements in Turbulent Opposed-Jet Flames" is submitted for consideration as a full length article to Flow Turbulence and Combustion.  相似文献   

9.
Numerical simulations of the Sandia flame CHNa and the Sydney bluff-body stabilized flame HM1E are reported and the results are compared to available experimental data. The numerical method is based on compressible URANS formulations which were implemented recently in the OpenFOAM toolbox. In this study, the calculations are carried out using the conventional compressible URANS approach and a standard k- ?? turbulence model. The Eddy Dissipation Concept with a detailed chemistry approach is used for the turbulence-chemistry interaction. The syngas (CO/H2) chemistry diluted by 30 % nitrogen in the Sandia flame CHNa and CH4/H2 combustion in the Sydney flame HM1E are described by the full GRI-3.0 mechanism. A robust implicit Runge-Kutta method (RADAU5) is used for integrating stiff ordinary differential equations to calculate the reaction rates. The radiation is treated by the P1-approximation model. Both target flames are predicted with the Steady Laminar Flamelet model using the commercial code ANSYS FLUENT as well. In general, there is good agreement between present simulations and measurements for both flames, which indicates that the proposed numerical method is suitable for this type of combustion, provides acceptable accuracy and is ready for further combustion application development.  相似文献   

10.
An investigation of the leading edge characteristics in lifted turbulent methane-air (gaseous) and ethanol-air (spray) diffusion flames is presented. Both combustion systems consist of a central nonpremixed fuel jet surrounded by low-speed air co-flow. Non-intrusive laser-based diagnostic techniques have been applied to each system to provide information regarding the behavior of the combustion structures and turbulent flow field in the regions of flame stabilization. Simultaneous sequential CH-PLIF/particle image velocimetry and CH-PLIF/Rayleigh scattering measurements are presented for the lifted gaseous flame. The CH-PLIF data for the lifted gas flame reveals the role that ``leading-edge' combustion plays as the stabilization mechanism in gaseous diffusion flames. This phenomenon, characterized by a fuel-lean premixed flame branch protruding radially outward at the flame base, permits partially premixed flame propagation against the incoming flow field. In contrast, the leading edge of the ethanol spray flame, examined using single-shot OH-PLIF imaging and smoke-based flow visualization, does not exhibit the same variety of leading-edge combustion structure, but instead develops a dual reaction zone structure as the liftoff height increases. This dual structure is a result of the partial evaporation (hence partial premixing) of the polydisperse spray and the enhanced rate of air entrainment with increased liftoff height (due to co-flow). The flame stabilizes in a region of the spray, near the edge, occupied by small fuel droplets and characterized by intense mixing due to the presence of turbulent structures. This revised version was published online in July 2006 with corrections to the Cover Date.  相似文献   

11.
2D Direct Numerical Simulations of methane/air turbulent premixed flames at initial Karlovitz numbers ranging from 600 to 9500 are performed. Instantaneous results are then extracted and analyzed with a focus on the inner flame structure. Snapshots reveal that the distributed reaction zone regime, theoretically reached around Ka?≈?100, is not attained before Ka?≈?2000. A correction of the definition of Ka is proposed in order to account for gas expansion across the flame, and is found to be consistent with the previous observations. The fuel-consumption zone is shown to be highly affected by turbulence and the characteristics of flames developing at lower Ka cannot be seen: the reaction zone is indeed strongly stretched and curved by intense turbulence leading to the formation of large protruding structures. In addition, the heat release rate layer is found to be broader and more distributed than at lower Ka as small turbulent eddies are able to survive inside it. No local flame quenching is however noticed. A statistical analysis of the distributed flame highlighted three major features characterizing this regime: significant broadening of the whole flame results from the presence of small eddies inside the reaction zone, temperature evolves linearly with respect to the progress variable and minor species peak mass fractions are lower than in a laminar flame. These results have important consequences for turbulent combustion modelling of flames in the distributed combustion regime.  相似文献   

12.
Song  Erzhuang  Lei  Qingchun  Chi  Yeqing  Fan  Wei 《Flow, Turbulence and Combustion》2022,109(1):125-142

The flame pocket formation, including reactant pocket, product pocket, soot pocket, and fluid parcel, is a common phenomenon in turbulent combustion occurred as a response of the flame to flow straining and shearing. Understanding pocket behavior is vital to study the flames in such a regime. This work addresses the research need to experimentally measure and track multiple flame pockets in 3D. For this purpose, volumetric measurements were performed to measure the high-speed turbulent flame structure at 15 kHz based on emission tomography. With the 3D flame structures, a new tracking algorithm was developed to identify and track the multiple flame pockets simultaneously in 3D. The instantaneously tracked 3D flame pockets enabled the extraction of key properties of pocket dynamics, including the favorable formation location, 3D3C movement speed, and pocket expanding/shrinking speed. The developed methods were evidently able to resolve the detailed behavior of flame pockets in highly turbulent flames.

  相似文献   

13.
This paper presents planar imaging of laser induced fluorescence (LIF) from key reactive species in the auto-ignition region of dilute turbulent spray flames of methanol. High-speed (5?kHz) LIF-OH imaging as well as low speed (10?Hz) imaging of joint LIF-OH-CH2O is performed. The product of the OH and CH2O signals is used as a qualitative indicator of local heat release. The burner is kept intentionally simple to facilitate computations and the spray is formed upstream of the jet exit plane and carried with air or nitrogen into a hot co-flowing stream of vitiated combustion products. The studied flames are all lifted but differ in the shape of their leading edge and heat release zones. Similarities with auto-ignition of gaseous fuels, as well as differences, are noted here. Formaldehyde is detected earlier than OH implying that the former is a key precursor in the initiation of auto-ignition. Growing kernels of OH that are advected from upstream, close in on the jet centreline and ignite the main flame. The existence of double reaction zones in some flames may be due to ignitable mixtures formed subsequent to local evaporation of droplets and subsequent mixing. When air is used as spray carrier, reaction zones broaden with distance, possibly due to increased partial premixing and regions of intense heat release occur near the flame centreline further downstream. With nitrogen as carrier, the flame maintains a nominal diffusion-like structure with reaction zones of uniform width and substantially less concentration of heat release on the flame centreline.  相似文献   

14.
An experimental study has been carried out to investigate the interaction between propagating turbulent premixed flames and solid obstacles. The experimental rig was configured specifically to allow detailed measurements with laser-based optical diagnostics. A wall-type solid obstacle was mounted inside a laboratory-scale combustion chamber with rectangular cross-section. The flame was initiated, by igniting a combustible mixture of methane in air at the center of the closed end of the combustion chamber. The flame front development was visualized by a high-speed (9000 frame/s) digital video camera and flame images were synchronized with ignition timing and chamber pressure data. The tests were carried out with lean, stoichiometric and rich mixtures of methane in air. The images were used to calculate highly resolved temporal and spatial data for the changes in flame shape, speed, and the length of the flame front. The results are discussed in terms of the influence of mixture equivalence ratio on the flame structure and resulting overpressure. The reported data revealed significant changes in flame structure as a result of the interaction between the propagating flame front and the transient recirculating flow formed behind the solid obstacle. Combustion images show that the flame accelerates and decelerates as it impinges on the obstacle wall boundaries. It is also found that the mixture concentrations have a significant influence on the nature of the flame/solid interactions and the resulting overpressure. The highest flame speed of 40 m/s was obtained with the unity fuel–air equivalence ratio. Burning of trapped mixture behind the solid obstruction was found to be highly correlated with the flame front length and the rate of pressure rise.  相似文献   

15.
Three-dimensional Direct Numerical Simulations (DNS) in canonical configuration have been employed to study the combustion of mono-disperse droplet-mist under turbulent flow conditions. A parametric study has been performed for a range of values of droplet equivalence ratio ?d, droplet diameter ad and root-mean-square value of turbulent velocity u. The fuel is supplied entirely in liquid phase such that the evaporation of the droplets gives rise to gaseous fuel which then facilitates flame propagation into the droplet-mist. The combustion process in gaseous phase takes place predominantly in fuel-lean mode even for ?d>1. The probability of finding fuel-lean mixture increases with increasing initial droplet diameter because of slower evaporation of larger droplets. The chemical reaction is found to take place under both premixed and non-premixed modes of combustion: the premixed mode ocurring mainly under fuel-lean conditions and the non-premixed mode under stoichiometric or fuel-rich conditions. The prevalence of premixed combustion was seen to decrease with increasing droplet size. Furthermore, droplet-fuelled turbulent flames have been found to be thicker than the corresponding turbulent stoichiometric premixed flames and this thickening increases with increasing droplet diameter. The flame thickening in droplet cases has been explained in terms of normal strain rate induced by fluid motion and due to flame normal propagation arising from different components of displacement speed. The statistical behaviours of the effective normal strain rate and flame stretching have been analysed in detail and detailed physical explanations have been provided for the observed behaviour. It has been found that the droplet cases show higher probability of finding positive effective normal strain rate (i.e. combined contribution of fluid motion and flame propagation), and negative values of stretch rate than in the stoichiometric premixed flame under similar flow conditions, which are responsible for higher flame thickness and smaller flame area generation in droplet cases.  相似文献   

16.
Large scale dynamic behavior of buoyant diffusion flames were studied experimentally. It was found that buoyant diffusion flames originating from circular nozzles exhibit two different modes of flame instabilities. The first mode results in a sinuous meandering of the diffusion flame, characteristic of flames originating from small diameter nozzles. This instability originates at some distance downstream of the nozzle exit in the contraction region of the buoyant flame envelope and develops into a sinuous motion of the flame. The second mode is the varicose mode which develops very close to the nozzle exit as axisymmetric perturbations of a contracting flame surface. In this mode, flame oscillations result in the formation of toroidal vortical structures that convect through the flame and cause periodic burn out at the flame top resulting in the observed flame height fluctuations. The average flame heights are found to be typically shorter for these flames. The oscillation frequencies and their scaling for the two modes are also different with the sinuous mode having higher frequencies than the varicose mode. It was also observed that the instability can switch from one mode to the other and the probability of observing the varicose mode appears to increase with increasing Richardson number. Additionally, the feasibility of altering the behavior of buoyant diffusion flames was explored through variation of the oxidizer medium density. It was found that the flame oscillations can be completely suppressed for flames burning in helium rich helium–oxygen mixtures. At lower helium concentrations, the oscillation frequency can be significantly reduced. In order to enhance the buoyancy effect, CO2–O2 mixtures were also studied. However, the density increase and its effects on flame oscillation frequency were found to be small compared to those flames burning in air. These experiments point towards the feasibility of altering buoyant flame behavior under earth gravity and studying the large scale dynamical aspects of buoyant flames without the need of variable gravity environment. Received: 2 March 1999/Accepted: 6 August 1999  相似文献   

17.
CH double-pulsed PLIF measurement in turbulent premixed flame   总被引:1,自引:0,他引:1  
The flame displacement speeds in turbulent premixed flames have been measured directly by the CH double-pulsed planar laser-induced fluorescence (PLIF). The CH double-pulsed PLIF systems consist of two independent conventional CH PLIF measurement systems and laser beams from each laser system are led to same optical pass using the difference of polarization. The highly time-resolved measurements are conducted in relatively high Reynolds number turbulent premixed flames on a swirl-stabilized combustor. Since the time interval of the successive CH PLIF can be selected to any optimum value for the purpose intended, both of the large scale dynamics and local displacement of the flame front can be discussed. By selecting an appropriate time interval (100–200 μs), deformations of the flame front are captured clearly. Successive CH fluorescence images reveal the burning/generating process of the unburned mixtures or the handgrip structures in burnt gas, which have been predicted by three-dimensional direct numerical simulations of turbulent premixed flames. To evaluate the local flame displacement speed directly from the successive CH images, a flame front identification scheme and a displacement vector evaluation scheme are developed. Direct measurements of flame displacement speed are conducted by selecting a minute time interval (≈30 μs) for different Reynolds number (Re λ = 63.1–115.0). Local flame displacement speeds coincide well for different Reynolds number cases. Furthermore, comparisons of the mean flame displacement speed and the mean fluid velocity show that the convection in the turbulent flames will affect the flame displacement speed for high Reynolds number flames.  相似文献   

18.
Planar laser induced fluorescence imaging (PLIF) is shown to be a quantitative method of measuring average values, rms fluctuations, and probability density functions of OH concentration in laboratory scale, H2-air diffusion flames. When compared with single-pulse laser saturated fluorescence (LSF) data, PLIF data show agreement (within a factor of two) for average and rms values in laminar, transitional, and turbulent flames. The unknown temperature dependence of the H2 quenching cross section introduces a factor of two uncertainty in PLIF measurements in rich flame zones. Extensions of PLIF to other molecules and other combustion systems are discussed.A version of this paper was presented at the ASME Winter Annual Meeting of 1984  相似文献   

19.
Experimental Characterization of Gelled Jet A1 Spray Flames   总被引:1,自引:0,他引:1  
Gelled propellants provide energetic performance similar to conventional liquid propellants and safety during storage and handling like a solid propellant. Experiments on unconfined gelled Jet A1 spray flames and the comparison with ungelled spray flames are reported for the first time in this paper in terms of the global features, burning regimes, stability limits, visible flame height, emission spectra, natural luminosity, and CH ? chemiluminescence. Propellants were atomized by an internally impinging two-fluid atomizer, developed specifically for efficient atomization of non-Newtonian gels. Swirling and non-swirling spray flames were successfully stabilized on a burner incorporating bluff body and annular jet of combustion air over a wide range of operating parameters. Structural features of the atomizer impart high momentum to the (central) spray jet, such that the recirculation zone could be penetrated under all conditions. Long-exposure smoke and high-speed visualizations were employed to study cold flow structures and droplet-vortex interactions. Short-exposure direct and backlit imaging were used to observe global features of spray flames. Stability limits and visible flame heights were mapped for different thermal inputs, swirl numbers, and flow rates of atomizing and combustion air jets. Non-swirling stable anchored, partially blown off, and neck-blown off flames were observed. Lifted, and a transition regime, in which the flame could burn in stable and lifted mode repetitively, were observed for the swirling flames. Interactions between central and annular jets are important in these regimes, determining flame shape, symmetry, and flame height. Jet-like propagation zone determines the flame height through its dependence on momentum of spray jet. The length of this zone is affected by variations in thermal input, gas-liquid ratio, and air-fuel ratio. The gelled Jet A1 flames are remarkably shorter despite having a larger average droplet size than ungelled Jet A1. This experimental observation directly supports theoretical predictions reported in literature. These flames are more luminous than ungelled Jet A1, especially at the base and the neck regions. While, majority of the heat is released in the jet-like propagation zone for both the flames, significant heat is released in the neck zone of ungelled Jet A1 spray flame in comparison to ungelled Jet A1 spray flame due to intense turbulence and smaller droplet size.  相似文献   

20.
Phase-resolved measurements of the velocity field in acoustically forced, flickering laminar co-flowing methane/air diffusion flames were made. Identical flames have been studied extensively in the past in order to characterize the effects of the vortical structures responsible for the flicker on the flame structure, but the initial velocity perturbation and the velocity fields have not been reported previously. Phase-locked measurements of the instantaneous two-dimensional velocity field at ten phases within a full excitation cycle were made using particle image velocimetry. The velocity measurements were complemented by phase-resolved shadowgraphs recorded in the vicinity of the flame base. Measurements are reported for the two forcing conditions that have most often been studied for this burner. When integrated with the results of previous studies, these measurements provide a clearer picture of the interactions between the buoyancy-induced vortical structures and the flame sheets, as well as providing the initial conditions required for realistic modeling of these flames.  相似文献   

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