Charge-state conditional operation of a spin qubit

We report coherent operation of a singlet-triplet qubit controlled by the spatial arrangement of two confined electrons in an adjacent double quantum dot that is electrostatically coupled to the qubit. This four-dot system is the specific device geometry needed for two-qubit operations of a two-electron spin qubit. We extract the strength of the capacitive coupling between qubit and adjacent double quantum dot and show that the present geometry allows fast conditional gate operation, opening pathways toward implementation of a universal set of gates for singlet-triplet spin qubits.     

Resonance backscattering in submicron rings

We discuss the rate of relaxation of the total spin in a two-electron droplet in the vicinity of the magnetic-field-driven singlet-triplet transition. The total spin relaxation is attributed to spin-orbit and electron-phonon interactions. The relaxation process is found to depend on the spin of ground and excited states. This asymmetry is used to explain puzzles in recent high source-drain transport experiments.     

Singlet-Triplet Transitions of a Pöschl-Teller Quantum Dot

We study the energy spectra of a two-dimensional two-electron quantum dot (QD) with Pöschl-Teller confining potential under the influence of perpendicular homogeneous magnetic field. Calculations are made by using the method of numerical diagonalization of Hamiltonian matrix within the effective-mass approximation. A ground-state behavior (spin singlet-triplet transitions) as a function of the strength of a magnetic field is found. We find that the dot radius R of a Pöschl-Teller potential is important for the ground-state transition and the feature of ground-state for a Pöschl-Teller QD and a parabolic QD is similar when R is larger. The larger the well depth, the higher the magnetic field for the singlet-triplet transition of the ground-state of two interacting electrons in a Pöschl-Teller QD.     

Universal set of quantum gates for double-dot spin qubits with fixed interdot coupling

We propose a set of universal gate operations for the singlet-triplet qubit realized by two-electron spins in a double quantum dot, in the presence of a fixed inhomogeneous magnetic field. All gate operations are achieved by switching the potential offset between the two dots with an electrical bias, and do not require time-dependent control of the tunnel coupling between the dots. We analyze the two-electron dynamics and calculate the effective qubit rotation angle as a function of the applied electric bias. We present explicit gate sequences for single-qubit rotations about two orthogonal axes, and a CNOT gate sequence, completing the universal gate set.     

Application of Tietz Potential to Study Singlet-Triplet Transition of a Two-Electron Quantum Dot

In this paper, we have studied electronic properties of a two-electron quantum dot using Tietz confining potential in the presence of an external magnetic field. In this regard, we have applied diagonalization procedure of Hamilonian matrix. We have calculated singlet-triplet ground state transitions as a function of the magnetic field. The obtained results show that the dot size of the Tietz potential has an important role in the ground state transition. The singlet-triplet transition of the ground state shifts towards lower magnetic field when the quantum size increases. Our results yield much less transitions than that of previous results [R.G. Nazmitdinov, N.S. Simonovic, and M.J. Rost, Phys. Rev. B 65 (2002) 155307].     

Effect of exchange interaction on spin dephasing in a double quantum dot

We measure singlet-triplet dephasing in a two-electron double quantum dot in the presence of an exchange interaction which can be electrically tuned from much smaller to much larger than the hyperfine energy. Saturation of dephasing and damped oscillations of the spin correlator as a function of time are observed when the two interaction strengths are comparable. Both features of the data are compared with predictions from a quasistatic model of the hyperfine field.     

Spectroscopy of spin-orbit quantum bits in indium antimonide nanowires

A double quantum dot in the few-electron regime is achieved using local gating in an InSb nanowire. The spectrum of two-electron eigenstates is investigated using electric dipole spin resonance. Singlet-triplet level repulsion caused by spin-orbit interaction is observed. The size and the anisotropy of singlet-triplet repulsion are used to determine the magnitude and the orientation of the spin-orbit effective field in an InSb nanowire double dot. The obtained results are confirmed using spin blockade leakage current anisotropy and transport spectroscopy of individual quantum dots.     

Experimental signature of phonon-mediated spin relaxation in a two-electron quantum dot

We observe an experimental signature of the role of phonons in spin relaxation between triplet and singlet states in a two-electron quantum dot. Using both the external magnetic field and the electrostatic confinement potential, we change the singlet-triplet energy splitting from 1.3 meV to zero and observe that the spin relaxation time depends nonmonotonously on the energy splitting. A simple theoretical model is derived to capture the underlying physical mechanism. The present experiment confirms that spin-flip energy is dissipated in the phonon bath.     

Application of Tietz Potential to Study Singlet-Triplet Transition of a Two-Electron Quantum Dot

In this paper, we have studied electronic properties of a two-electron quantum dot using Tietz confining potential in the presence of an external magnetic field. In this regard, we have applied diagonalization procedure of Hamilonian matrix. We have calculated singlet-triplet ground state transitions as a function of the magnetic field. The obtained results show that the dot size of the Tietz potential has an important role in the ground state transition. The singlet-triplet transition of the ground state shifts towards lower magnetic field when the quantum size increases. Our results yield much less transitions than that of previous results [R.G. Nazmitdinov, N.S. Simonovic, and M.J. Rost, Phys.Rev. B 65(2002) 155307].     

Two-electron quantum dot in tilted magnetic fields: Sensitivity to the confinement model

Semiconductor quantum dots are conventionally treated within the effective-mass approximation and a harmonic model potential in the two-dimensional plane for the electron confinement. The validity of this approach depends on the type of the quantum-dot device as well as on the number of electrons confined in the system. Accurate modeling is particularly demanding in the few-particle regime, where screening effects are diminished and thus the system boundaries may have a considerable effect on the confining potential. Here we solve the numerically exact two-electron states in both harmonic and hard-wall model quantum dots subjected to tilted magnetic fields. Our numerical results enable direct comparison against experimental singlet-triplet energy splittings. Our analysis shows that hard and soft wall models produce qualitatively different results for quantum dots exposed to tilted magnetic fields. Hence, we are able to address the sensitivity of the two-body phenomena to the modeling, which is of high importance in realistic spin-qubit design.     

Two Electrons with Spin-Orbit Interactions in InAs Coupled Quantum Dots

We theoretically study the spin properties of two interacting electrons confined in the IhAs parallel coupled quantum dots （CQDs） with spin-orbit interactions （SOI） by exact diagonalization method. Through the SOI induced spin mixing of the singlet and the triplet states, we show the different spin properties for the weak and strong SOI. We investigate the coherent singlet-triplet spin oscillations of the two electrons under the SOI, and demonstrate the detailed behaviors of the spin oscillations depending on the SOI strengths, the inter-dot separations and the external magnetic fields. To better understand the underlying physics of the spin dynamics, we introduce a four-level model Hamiltonian for both weak and strong SOI, and find that the SOI induced in plane effective magnetic fields can be quantitatively extracted from the two-electron excitation energy spectra.     

Theoretical analysis of the MCD spectra of some singlet-triplet transitions in formaldehyde

A recently developed theoretical treatment of the magneto-optical activity of singlet-triplet transitions in molecules which are near-symmetric rotors is employed in simulation of the MCD spectra associated with some singlet-triplet transitions in formaldehyde. The theoretical results are compared with the relevant experimental data, and the agreement between theory and experiment is found to be satisfactory.     

Singlet-triplet splitting of geminate electron-hole pairs in conjugated polymers

The singlet-triplet splitting of geminate polaron pairs in a ladder-type conjugated polymer has been studied by the thermally stimulated luminescence technique. The energy gap separating the singlet and triplet states of the geminate pairs is measured to be in the range of 3-6 meV, depending on the polymer morphology. The results of correlated quantum-chemical calculations on a long ladder-type oligomer are fully consistent with the observed values of the geminate polaron pair singlet-triplet gap. Such low splitting values have important implications for the spin-dependent exciton formation in conjugated polymers.     

Attosecond pulse generation from two-electron harmonic emission spectrum

In this paper, we theoretically investigate the high-order harmonic generation and attosecond pulse generation when a two-electron He atom is exposed to the intense laser pulse. It shows that due to the two-electron double recombination mechanism, an extended plateau beyond the classical single-electron harmonic has been obtained on the two-electron harmonic spectrum. Further by using this two-electron harmonic extension scheme combined with the two-color field, two supercontinuum bandwidths with 200 e V have been obtained. As a result, a series of sub-60 as extreme ultraviolet(XUV)pulses have been directly generated.     

The effect of lead cations on the fluorescence characteristics of bovine serum albumin in aqueous solution

The effect of lead (heavy metal) cations on the fluorescence characteristics and photophysical parameters (fluorescence intensity and anisotropy, absorption cross section, excited state lifetime, and rates of singlet-triplet conversion and reversible photobleaching) of tryptophan in an aqueous solution of bovine serum albumin (two-tryptophan protein) is studied and compared with the effect in the aqueous solution of tryptophan. It is demonstrated that the effect of lead on the fluorescence characteristics of the protein is manifested at a molar concentration ratio of metal cations and protein macromolecules of greater than 10 and related to the dynamic quenching of the excited state, protein aggregation, and an increase in the rate of singlet-triplet conversion (the effect of a heavy atom) in tryptophan molecules.     

Numerical simulation of the ionization dynamics of a two-electron quantum system in a femtosecond pulse

The ionization of a simple two-electron model system, viz., the one-dimensional negative hydrogen ion, is investigated using direct numerical integration of the time-dependent Schrödinger equation. The one-and two-electron ionization probabilities as functions of frequency and radiation intensity are obtained. It is shown that two-electron ionization is mediated by both direct and sequential mechanisms. The stabilization of the two-electron system against the ionization process is investigated. The data obtained are compared with calculations performed within the one-dimensional single-particle model of H^?. The photoelectron spectrum is analyzed in the region of parameters corresponding to the single-electron ionization regime.     

Evolution from quasielastic to deep-inelastic transfer in the system132Xe+natFe§

The pronounced isotope shift of⁸⁷Sr versus⁸⁷Sr observed recently in 5sns¹S₀ Rydberg states reflects the singlet-triplet mixing solely caused by magnetic hyperfine interaction. Using semiempirical estimates for the hyperfine coupling constant a_{5 s} and the singlet-triplet splitting ΔE_ST (n) excellent agreement between experimental and calculated values is obtained.     

双电子复合逆过程的多通道理论

我们提出一个关于双电子复合逆过程(即共振辐射复合逆过程)的多通道理论。具体地分析了最近Safinya和Gallagher所完成的关于激发态钡原子的高分辨激光光谱。说明精确的实验光谱数据可以用来评定双电子复合逆过程理论计算的精确度;通过细致平衡关系,相当于评定双电子复合过程理论计算的精确度——这将是以分波展开的方式,对每一个适当的分波对称块进行基本的检验。 关键词：     

Spin-orbit matrix elements for internally contracted multireference configuration interaction wavefunctions

An efficient method for the calculation of Breit-Pauli spin-orbit matrix elements for internally contracted multireference configuration interaction wavefunctions is presented. Instead of taking all two-electron contributions of the wavefunction explicitly into account, the most important two-electron contributions of the spin-orbit operator are incorporated by means of an effective one-electron Fock operator. As a further refinement, explicit two-electron contributions can be reinstated for the dominant all-internal parts of the wavefunctions.