Decay of the neutron-rich isotope 113Ru to 113Rh

The decay of neutron-rich isotope ¹¹³Ru obtained as on-line mass separated product of proton-induced fission has been investigated by γγ coincidence and spectrum multiscaling measurements. Decay schemes for both low- and high-spin isomers of ¹¹³Ru have been constructed. The level scheme of ¹¹³Rh is considerably extended. Systematics of the lowest-lying rhodium levels is smooth. The picture of shape coexistence established for neutron-rich Rh isotopes near-neutron midshell is confirmed with the observation of a K = 1/2 deformed band, with its 3/2⁺ state at 600 keV being the lowest-lying level and of probable 7/2⁺ and 5/2⁺ band members. A large fraction of β feeding is found to populate high-lying levels in ¹¹³Rh. The GT strength in ¹¹³Ru^m decay is significantly larger than for the decay of ¹¹³Ru_g and of lighter rhodium isotopes. Received: 18 January 2001 / Accepted: 14 January 2002     

First decay scheme of 113Tc and identification of 113Ru m

Very neutron–rich fission products of the mass chain A=113 obtained from the IGISOL on–line mass separator have been investigated by γγ coincidence techniques and γ-spectra multiscaling. Gamma–rays following β–decay of ¹¹³Tc have been observed for the first time and a new 0.5 s isomeric state has been found in ¹¹³Ru. Received: 10 February 1998     

Intruder states in even-even neutron-rich Pd isotopes

The decays of ¹¹²Rh ^g and ¹¹²Rh ^m obtained as on-line mass separated fission products have been investigated by standard β and γ spectroscopic techniques and γ-γ angular correlations. Low-lying 0⁺ and 2⁺ states are identified in the daughter nucleus ¹¹²Pd. Systematics suggests the existence of an intruder band which is the lowest in ¹¹⁰Pd, i.e. two neutrons before the midshell. Received:13 March 1998     

Beta decay of neutron-rich 118Rh and the lowest excited states in 118Pd

Beta decay of a refractory isotope ¹¹⁸Rh produced in symmetric fission and mass separated by the ion guide technique has been applied for the study of low-lying excited states of ¹¹⁸Pd. The yrast band in ¹¹⁸Pd has been observed up to a 6⁺ state and the lowest states of the asymmetric γ-band have been identified. The measured half-life of ¹¹⁸Rh is (300±60)ms. The systematics of the excited states in neutron-rich Pd-isotopes implies the saturation towards an O(6) symmetry at N = 70. Received: 19 June 2000 / Accepted: 1 August 2000     

Decay of 1.643 h <Superscript>95</Superscript>Ru and its daughter's level structure

The decay of ⁹⁵Ru has been investigated by means of γ-ray spectroscopy. The ⁹⁵Ru nuclei were produced by the reaction ⁹²Mo( α, n) ⁹⁵Ru at a beam energy of 17MeV. High-purity Ge detectors have been used singly and in coincidence to study γ-rays in the decay of ⁹⁵Ru to ⁹⁵Tc. 132 γ-rays are reported, among them, energies and intensities for 127 transitions have been determined. A decay scheme of ⁹⁵Ru with 31 levels is proposed which accommodates 127 of these transitions. Spins and parities for three new levels are proposed from calculated log ft values, measured γ-ray branching ratios, and in-beam experiment results of the daughter nucleus ⁹⁵Tc. Combining with the high-spin states observed by in-beam γ-ray spectroscopy of previous decay works, the structure of the excited states of ⁹⁵Tc is discussed in the framework of the projected shell model.     

In-beam study of 145Tb

The high-spin states of ¹⁴⁵Tb have been studied in the ¹¹⁸Sn(³²S, 1p4n) reaction at ³²S energies from 161 to 175 MeV using techniques of in-beam γ-ray spectroscopy. Measurements of γ-ray excitation functions and γ-γ-t coincidences were performed with 12 BGO(AC)HPGe detectors. Based on the measured results of γ-γ coincidences, γ-ray anisotropies and DCO ratios, a level scheme for ¹⁴⁵Tb was established for the first time. The observed excited states show typical irregular pattern in a spherical nucleus, and the low-lying levels have been interpreted qualitatively with a particle-core coupling. Received: 21 September 2001 / Accepted: 9 November 2001     

New states in heavy Cd isotopes and evidence for weakening of the N = 82 shell structure

A chemically selective laser ion source has been used in a β-decay study of heavy Ag isotopes into even-even Cd nuclides. Gamma-spectroscopic techniques in time-resolving event-by-event and multiscaling modes have permitted the identification of the first 2⁺ and 4⁺ levels in ¹²⁶Cd₇₈, ¹²⁸Cd₈₀, and tentatively the 2⁺ state in ¹³⁰Cd₈₂. From a comparison of these new states in ₄₈Cd with the E(2⁺) and E(4⁺)/E(2⁺) level systematics of ₄₆Pd and ₅₂Te isotopes and several recent model predictions, possible evidence for a weakening of the spherical N = 82 neutron-shell below double-magic ¹³²Sn is obtained. Received: 13 July 2000 / Accepted: 12 October 2000     

New states and γ-transitions in 209Bi observed in the (3He, d*γγ)-subcoulomb-reaction

High-spin states in ¹⁴³Pm have been investigated via the ¹²⁸Te(¹⁹F,4nγ)¹⁴³Pm reaction using techniques of in-beam γ-spectroscopy. γ-ray singles, γ-γ coincidences, γ-ray anisotropies and DCO ratios have been measured. Based on these measurements, the level scheme of ¹⁴³Pm has been extended up to an excitation energy of 10535.4 keV, including 48 new γ-rays deexciting 28 new levels. The yrast levels in ¹⁴³Pm can be understood qualitatively in the framework of a weak-coupling model. Received: 10 July 2000 / Accepted: 12 October 2000     

Beta Decay of 111Tc to 111Ru

The β-decay of the very neutron-rich ¹¹¹Tc nucleus has been observed. A partial decay scheme of ¹¹¹Ru is presented, complementing the high-spin levels earlier reported in spontaneous fission work. Received: 15 January 1998     

Decay study of neutron-rich zirconium isotopes employing a Penning trap as a spectroscopy tool

A new technique to produce isobarically pure ion beams for decay spectroscopy by using a gas-filled Penning trap was commissioned at the ion guide isotope separator on-line facility, IGISOL. β-decays of neutron-rich ¹⁰⁰Zr, ¹⁰²Zr and ¹⁰⁴Zr isotopes were studied with this technique. In addition, the values of ^100,102,104Zr β-decays were determined from the direct mass measurements of zirconium and niobium isotopes performed with a high-precision Penning trap. The mass of ¹⁰⁴Nb was directly measured for the first time and the obtained mass excess value for the longer-living (1⁺) state is -71823±10 keV. For the ground states of ¹⁰⁰Nb and ¹⁰²Nb the obtained mass excess values were -79802±20 keV and -76309±10 keV, respectively. The observed distribution of the β strength supports a prolate deformation assignment for ^100,102,104Zr isotopes.     

The modified decay width of the radioactive nucleus

It is reported that the width of the first excited state ( , 37.133keV) of ¹²¹ ₅₁Sb embedded in a ZnSb alloy can be modified by reabsorption of γ -rays scattered backward on the platinum (gold) reflector. Its dependence on the reflector shape is also investigated. The decay rate is reduced about 4.5% at a temperature of 4.2K by a platinum spherical reflector of 5mm radius.     

The low-spin structure of <Superscript>115</Superscript>Xe

The low-spin band structure of neutron-deficient ¹¹⁵ ₅₄Xe has been studied following a low-energy (212.3 MeV) ⁶⁰Ni(⁵⁸Ni,2pnγ) reaction performed at IReS, Strasbourg, with the Garel⁺ spectrometer. The relative excitation energies of νh_11/2 (isomeric), νg_7/2, and νd_5/2 bandheads have been established. Received: 23 March 2000     

Precision electron-gamma spectroscopic measurements in <Superscript>75</Superscript>As

The decay of ⁷⁵Se to levels of ⁷⁵As has been studied using an HPGe detector for gamma-ray and a mini-orange electron spectrometer for conversion electron measurements. We identify 38 transitions in this decay, including 18 gamma rays and 16 conversion electron lines reported for the first time. New results also include E2 multipolarity assignment for the 81 keV transition, M1 assignment to three newly observed transitions and M1 + E2 for the 617 keV transition. A revised ⁷⁵As level scheme is constructed using the Ritz combination principle through the computer code GTOL. While confirming the existence of 10 well-established levels, two levels at 587 and 859 keV are newly placed into the decay scheme of ⁷⁵Se. The interpretation of the observed levels in terms of various theoretical approaches is briefly discussed. The newly placed 586.8 keV 1/2^- and 859.9 keV 1/2⁺ levels are studied in the light of the Interacting Boson-Fermion Model.     

Gamma-ray spectroscopy of the nucleus 139Ce

Gamma-ray coincidence techniques are used to determine new level structures in the N = 81 nucleus ¹³⁹Ce, at low spins and excitation energies with the ¹³⁹La(p, nγ) reaction at 5.0 and 6.0MeV incident energy, and at high spins with the ¹³⁰Te(¹²C, 3nγ) reaction at 50.5MeV, respectively. Lifetime determinations are also made in the (p, nγ) reaction with the centroid DSA method. The observed level structures are discussed by comparison with existing calculations and with those in the neighbouring nucleus ¹⁴⁰Ce.     

Excited states in neutron-rich 188W produced by an 18O-induced 2-neutron transfer reaction

Excited states in neutron-rich ¹⁸⁸W have been populated using a ¹⁸⁶W(¹⁸O,¹⁶O) reaction. In-beam γ-rays were measured in coincidence with scattered particles detected by a high-resolution ΔE-E Si telescope. In this experiment, the ground-state band has been identified up to I ^π = 8⁺. The γ band, the K ^π = 2^- octupole band, and a 2-quasiparticle state were also observed. The results are compared with predictions of self-consistent HFB cranking calculations and blocked-BCS multi-quasiparticle calculations.     

High-spin levels based on the 11/2- isomer in 135Ba

High-spin states in the ¹³⁵Ba nucleus have been studied with the reaction ¹³⁰Te(⁹Be, 4n) at a beam energy of 45 MeV. The level scheme based on the h _11/2 isomer has been expanded with spins up to 35/2 ℏ. At low spins, the yrast collective structure built on the ν h _11/2 ^-1 multiplet may show a transitional shape with γ > 30^° according to the systematical behavior observed in neighboring nuclei as well as the calculations of the triaxial rotor-plus-particle model. The configurations for several high-spin states have been discussed from a systematical comparison with neighboring isotones.     

High-spin structure of the neutron-rich 107,109 45Rh isotopes: the role of triaxiality

The ^107,109Rh nuclei have been produced as fission fragments following the fusion reaction ²⁸Si +¹⁷⁶Yb at 145 MeV bombarding energy and studied with the Eurogam2 array. In both nuclei three new rotational bands with the odd proton occupying the πg_9/2, πp_1/2 and π(g_7/2/d_5/2) sub-shells have been observed. In ¹⁰⁷Rh, two other bands involving strong M1 transitions have been identified at excitation energy larger than 2 MeV. They can be interpreted in terms of three quasiparticle excitations. In addition new structures consisting of four transitions, built on states located at low excitation energy (680 keV in ¹⁰⁷Rh and 642 keV in ¹⁰⁹Rh), point out the importance of triaxial deformation in these two isotopes. Received: 1 September 1999     

The 130Nd↦130Pr↦130Ce decay chain revisited

An investigation of low-lying energy levels of ¹³⁰Pr and ¹³⁰Ce has been made via β-decay. The radioactive parent nuclei were produced via ^94,96Mo + ⁴⁰Ca reactions at 6.8 MeV/nucleon and transported by a He-jet system. Gamma-γ-t, γ-X-t, γ-e^--t coincidence measurements were performed. Internal conversion coefficients have been measured with a magnetic spectrometer. The new β-decay half-life of ¹³⁰Nd has been determined to be 21(3) s. A partial level scheme of ¹³⁰Pr at low-spin has been constructed. The β-decay of ¹³⁰Pr to ¹³⁰Ce suggests the existence of three β-instable isomeric states in ¹³⁰Pr, while only one half-life T _1/2 = 40(4) s has been measured. Based on the present work and low-lying excited states in neighbouring odd-mass nuclei, the spins and parities of isomeric states in ¹³⁰Pr are proposed to be 2⁺, (4,5)⁺ and (7,8^±). The ground state in ¹³⁰Pr is still undetermined. Received: 20 August 2001 / Accepted: 6 November 2001     

Low-spin structure of 113Ru and 113Rh

The ¹¹³Ru and ¹¹³Rh nuclei, produced in the spontaneous fission of ²⁴⁸Cm and in proton-induced fission of ²³⁸U , were studied by means of prompt gamma spectroscopy using the EUROGAM 2 array of Anti-Compton spectrometers and the IGISOL mass separator, respectively. For the 0.5s isomer, found in ¹¹³Ru in our recent study we propose the 7/2^-[523] configuration. The present data indicate spin and parity 1/2⁺ for the ground state in ¹¹³Ru . This and some new data on the excited levels in ¹¹³Rh allows reinterpretation and a better understanding of the β^- _{} decay scheme of ¹¹³Ru . The properties of ¹¹³Ru were studied in the frame of the Core-Quasiparticle Coupling model, which has well reproduced the experimental data.     

Shapes of the neutron-rich 88-94Kr nuclei

Neutron-rich, ^88-94Kr nuclei, populated in spontaneous fission of ²⁴⁸Cm, have been studied with EUROGAM 2, by measuring prompt γ-rays. Many new excited states in even-even Kr isotopes have been identified. For the first time spins and parities were determined experimentally in these nuclei. Our results indicate that the quadrupole deformation of Kr isotopes will appear only above N = 58, as observed in Sr and Zr nuclei. The newly found 3^- level at 1506.4 keV in ⁹⁰Kr suggests the exsistence of a new region of increased octupole correlations, probably associated with the ν(d _5/2 h _11/2) pair of Δl = Δj = 3 orbitals. Received: 18 September 2000 / Accepted: 18 October 2000