Precise atomic masses of neutron-rich Br and Rb nuclei close to the r-process path

The Penning trap mass spectrometer JYFLTRAP, coupled to the Ion-Guide Isotope Separator On-Line (IGISOL) facility at Jyv?skyl?, was employed to measure the atomic masses of neutron-rich ^85-92Br and ^94-97Rb isotopes with a typical accuracy less than 10keV. Discrepancies with the older data are discussed. Comparison to different mass models is presented. Details of nuclear structure, shell and subshell closures are investigated by studying the two-neutron separation energy and the shell gap energy.     

Beta Decay of 111Tc to 111Ru

The β-decay of the very neutron-rich ¹¹¹Tc nucleus has been observed. A partial decay scheme of ¹¹¹Ru is presented, complementing the high-spin levels earlier reported in spontaneous fission work. Received: 15 January 1998     

First decay scheme of 113Tc and identification of 113Ru m

Very neutron–rich fission products of the mass chain A=113 obtained from the IGISOL on–line mass separator have been investigated by γγ coincidence techniques and γ-spectra multiscaling. Gamma–rays following β–decay of ¹¹³Tc have been observed for the first time and a new 0.5 s isomeric state has been found in ¹¹³Ru. Received: 10 February 1998     

First observation of medium-spin excitations in the <Superscript>138</Superscript>Cs nucleus

The Penning trap mass spectrometer JYFLTRAP, coupled to the Ion Guide Isotope Separator On-Line (IGISOL) facility at Jyv?skyl?, was employed to measure the atomic masses of neutron-rich ^70-73Ni and ^{73, 75}Cu isotopes with a typical accuracy less than 5keV. The mass of ⁷³Ni was measured for the first time. Comparisons with the previous data are discussed. Two-neutron separation energies show a weak subshell closure at ⁶⁸ ₂₈Ni₄₀ . A well established proton shell gap is observed at Z = 28 .     

Decay study of neutron-rich zirconium isotopes employing a Penning trap as a spectroscopy tool

A new technique to produce isobarically pure ion beams for decay spectroscopy by using a gas-filled Penning trap was commissioned at the ion guide isotope separator on-line facility, IGISOL. β-decays of neutron-rich ¹⁰⁰Zr, ¹⁰²Zr and ¹⁰⁴Zr isotopes were studied with this technique. In addition, the values of ^100,102,104Zr β-decays were determined from the direct mass measurements of zirconium and niobium isotopes performed with a high-precision Penning trap. The mass of ¹⁰⁴Nb was directly measured for the first time and the obtained mass excess value for the longer-living (1⁺) state is -71823±10 keV. For the ground states of ¹⁰⁰Nb and ¹⁰²Nb the obtained mass excess values were -79802±20 keV and -76309±10 keV, respectively. The observed distribution of the β strength supports a prolate deformation assignment for ^100,102,104Zr isotopes.     

Penning-trap-assisted study of 115Ru beta decay

The beta decay of ¹¹⁵Ru has been studied by means of Penning-trap-assisted beta and gamma spectroscopy at the IGISOL facility. The level scheme of ¹¹⁵Rh has been substantially extended and compared with the level systematics of lighter rhodium isotopes. Tentative candidates for three states of the deformed K = 1/2 band have been suggested. The beta-strength distribution of the beta decay of ¹¹⁵Ru differs from the beta decays of ^{111, 113, 113m}Ru isotopes due to non-observation of the 3-quasiparticle states in ¹¹⁵Rh. The decay properties of ¹¹⁵Ru indicate a spin-parity of (3/2⁺ for its beta-decaying ground state. In addition, possible Nilsson states as well as the shape and spin transitions in odd neutron-rich ruthenium isotopes are discussed.     

Beta decay of very neutron-rich110Mo studied at the new IGISOL facility

The decay of the new activity¹¹⁰Mo (t_1/2=0.30(4).s) has been observed at the new IGISOL separator. Multiscaled singles,--t and -y-t coincidences were recorded. The decay scheme suggests I=2⁺ for the ground state of the daughter nucleus¹¹⁰Tc. Three 1⁺ levels are fed with logft values below 5, indicating no drastic change among Mo and Ru decays at the middle of the neutron shell. This experiment confirms the expectation that the new IGISOL facility will allow the identification of one or two new more neutron-rich isotopes per element in this region.Supported by the Academy of Finland.     

Trap-assisted studies of odd, neutron-rich isotopes from Tc to Pd

We review the present and future of trap-assisted structure studies of odd, neutron-rich Tc, Ru, Rh and Pd isotopes at the limits of present experimental techniques. These nuclei of refractory elements are produced in light-particle induced fission and filtered by their mass number with the IGISOL mass separator. Further mass separation with the JYFLTRAP Penning trap system provides a clean, monoisotopic beam perfectly suited for precise nuclear spectroscopy. Connecting the IGISOL and the JYFLTRAP facilities to the recently installed MCC30/15 cyclotron opens new prospects for post-trap spectroscopy of very exotic, neutron-rich nuclei.     

Decay of 1.643 h <Superscript>95</Superscript>Ru and its daughter's level structure

The decay of ⁹⁵Ru has been investigated by means of γ-ray spectroscopy. The ⁹⁵Ru nuclei were produced by the reaction ⁹²Mo( α, n) ⁹⁵Ru at a beam energy of 17MeV. High-purity Ge detectors have been used singly and in coincidence to study γ-rays in the decay of ⁹⁵Ru to ⁹⁵Tc. 132 γ-rays are reported, among them, energies and intensities for 127 transitions have been determined. A decay scheme of ⁹⁵Ru with 31 levels is proposed which accommodates 127 of these transitions. Spins and parities for three new levels are proposed from calculated log ft values, measured γ-ray branching ratios, and in-beam experiment results of the daughter nucleus ⁹⁵Tc. Combining with the high-spin states observed by in-beam γ-ray spectroscopy of previous decay works, the structure of the excited states of ⁹⁵Tc is discussed in the framework of the projected shell model.     

Low-spin structure of 113Ru and 113Rh

The ¹¹³Ru and ¹¹³Rh nuclei, produced in the spontaneous fission of ²⁴⁸Cm and in proton-induced fission of ²³⁸U , were studied by means of prompt gamma spectroscopy using the EUROGAM 2 array of Anti-Compton spectrometers and the IGISOL mass separator, respectively. For the 0.5s isomer, found in ¹¹³Ru in our recent study we propose the 7/2^-[523] configuration. The present data indicate spin and parity 1/2⁺ for the ground state in ¹¹³Ru . This and some new data on the excited levels in ¹¹³Rh allows reinterpretation and a better understanding of the β^- _{} decay scheme of ¹¹³Ru . The properties of ¹¹³Ru were studied in the frame of the Core-Quasiparticle Coupling model, which has well reproduced the experimental data.     

Mass measurements of neutron-deficient radionuclides near the end-point of the rp-process with SHIPTRAP

Direct mass measurements of nuclides near to the supposed end-point region of the astrophysical rp-process were performed at SHIPTRAP, the Penning trap mass spectrometer at GSI Darmstadt. The masses of 24 nuclides were measured with relative uncertainties between 5 ^. 10^-8 and 2 ^. 10^-7 . Three of them, ¹⁰⁷Sb , ¹¹¹I and ¹¹²I , were determined experimentally for the first time. The data analysis and mass evaluation are presented in detail.     

Shape coexistence near the double-midshell nucleus 111Rh

The decay of ¹¹¹Ru obtained from fast on-line chemical and mass separation has been investigated by β-γ-t and γ-γ coincidence techniques. Earlier spin and parity assignments of ¹¹¹Rh levels based on extrapolations of level systematics are confirmed. In particular, the K=1/2 intruder band is supported by the hindrance of E2 transitions between deformed and spherical states and enhancement of intraband E2 transitions. The excitation energies of intruder band members in Rh isotopes show a minimum at ¹⁰⁹Rh₆₄, with two neutrons less than ¹¹¹Rh at the N=66 midshell. This trend, which differs from the one in the higher-Z neighbouring elements Ag and Cd with minima at N=66, follows the evolution of deformation observed in the lower-Z elements Ru and Mo. Received: 25 June 1997 / Revised version: 10 September 1997     

Mass measurements of neutron-deficient nuclides close to A = 80 with a Penning trap

The masses of ^{80, 81, 82, 83}Y, ^{83, 84, 85, 86, 88}Zr and ^{85, 86, 87, 88}Nb have been measured with a typical precision of 7keV by using the Penning trap setup at IGISOL. The mass of ⁸⁴Zr has been measured for the first time. These precise mass measurements have improved S_p and Q_EC values for astrophysically important nuclides.     

Production of heavy neutron-rich nuclei “south" of lead

The production of heavy neutron-rich nuclei is investigated using cold-fragmentation reactions. More than 25 new heavy neutron-rich nuclei were produced in the fragmentation of ²⁰⁸Pb projectiles at 1 A GeV impinging a beryllium target. The precise measurement of their production cross sections enables to benchmark the predictive power of different model calculations and make reliable predictions of the production rates expected in future radioactive beam facilities.     

Excited states in neutron-rich 188W produced by an 18O-induced 2-neutron transfer reaction

Excited states in neutron-rich ¹⁸⁸W have been populated using a ¹⁸⁶W(¹⁸O,¹⁶O) reaction. In-beam γ-rays were measured in coincidence with scattered particles detected by a high-resolution ΔE-E Si telescope. In this experiment, the ground-state band has been identified up to I ^π = 8⁺. The γ band, the K ^π = 2^- octupole band, and a 2-quasiparticle state were also observed. The results are compared with predictions of self-consistent HFB cranking calculations and blocked-BCS multi-quasiparticle calculations.     

Observation of M3 isomeric transition from <Superscript>156m</Superscript>Pm through the βdecay of <Superscript>156</Superscript>Nd

An M3 transition in a doubly odd nucleus of ¹⁵⁶Pm was identified by internal conversion electron measurement through the β-decay of ¹⁵⁶Nd which was separated from the fission products of ²³⁵U using the on-line mass separator KUR-ISOL. The isomeric state at 150.3keV de-excites to the ground state with the M3 transition, and the spin-parity is considered to be 1^-. Nilsson configurations are also discussed on the basis of the systematics.     

Mass measurements and evaluation around A = 22

Frequency ratio measurements with different combinations of the singly charged ions from ^{21, 22, 23}Na , ^{22, 24}Mg , and ^{37, 39}K were performed at the on-line Penning trap mass spectrometer ISOLTRAP, CERN, Geneva. The masses and mass differences were deduced with a relative uncertainty of about or even below one part in 10⁸ for the ions of interest using a least-squares analysis of all measured relations. The results have direct consequences for weak-interaction study as they give additional input to the test of CVC, and for nuclear astrophysics, because they help to establish the minimum observable signal for a NeNa cycle in a nova burst. We report here about the measurements and the detailed evaluation.     

Precise half-life measurement of the 26Si ground state

The β-decay half-life of ²⁶Si was measured with a relative precision of 1.4·10^?3. The measurement yields a value of 2.2283(27) s which is in good agreement with previous measurements but has a precision that is better by a factor of 4. In the same experiment, we have also measured the non-analogue branching ratios and could determine the super-allowed one with a precision of 3%. The experiment was done at the Accelerator Laboratory of the University of Jyväskylä where we used the IGISOL technique with the JYFLTRAP facility to separate pure samples of ²⁶Si.     

Beta decay of 101Sn

The β decay of the very neutron-deficient isotope ¹⁰¹Sn was studied at the GSI on-line mass separator using silicon detectors for recording charged particles and germanium detectors for γ-ray spectroscopy. Based on the β-delayed proton data the production cross-section of ¹⁰¹Sn in the ⁵⁰Cr + ⁵⁸Ni fusion-evaporation reaction was determined to be about 60nb. The half-life of ¹⁰¹Sn was measured to be 1.9(3)s. For the first time β-delayed γ-rays of ¹⁰¹Sn were tentatively identified, yielding weak evidence for a cascade of 352 and 1065keV transitions in ¹⁰¹In. The results for the ¹⁰¹Sn decay as well as those from previous work on the ¹⁰³Sn decay are discussed by comparing them to predictions obtained from shell model calculations employing a new interaction in the ⁸⁸Sr to ¹³²Sn model space.