Quadrupole Moments of Na Isotopes

The electric quadrupole coupling constants eqQ/h of ²⁰Na (I ^π = 2⁺, T _1/2 = 449.7 ms), ²¹Na (I ^π = 3/2, T _1/2 = 22.49 s) and ²⁵Na (I ^π = 5/2, T _1/2 = 59.6 s) in single crystal ZnO and TiO₂ were precisely measured by applying the β-NMR technique. The ratio of the quadrupole moments between ²⁰Na (²⁵Na) and ²¹Na was determined to be 0.728 ± 0.023 (0.011 ± 0.002).     

Quadrupole moment of the doubly closed shell +1 nucleon nucleus41Sc(Iπ=7/2−)

The nuclear electric quadrupole moment of⁴¹Sc(I^π=7/2⁻) was experimentally determined by use of the NMR detection in which the asymmetric β-ray distribution from spin polarized nuclei was monitored. The magnetic interaction of the state with high external magnetic field and the nuclear quadrupole interaction with the electric field gradient obtained in TiO₂ crystal were studied. The field gradient seen to the implanted⁴¹Sc was measured independently by the high field NMR detection on the stable isotope⁴⁵Sc located in the equivalent⁴¹Sc site with. |Q(⁴¹Sc;I^π=7/2⁻)|=(0.120±0.006) b was determined.     

A Possible Nuclear Spin Dewar. Hyperfine Interactions of Short-Lived β Emitter 8Li and 12B in TiO2

It was confirmed by detecting the β-NMR of ¹²B (I ^π=1⁺, T _1/2=20.2 ms) in a TiO₂ (rutile) crystal that the nuclear spin polarization of ¹²B was totally maintained in the crystal as produced through a nuclear reaction before implantation. Two locations, site 1 and site 2, were found with the relative populations 9 and 1, respectively, and the electric field gradients (EFGs) at those sites were obtained to be q(site 1)=+(37.1±0.5)10¹⁵ V/cm², η(site 1)<0.03, q(site 2)=+(185±5)10¹⁵ V/cm² and η(site 2)=0.62±0.02. We also found that about 30% of the initial polarization of ⁸Li (I ^π=2⁺, T _1/2=838 ms) was maintained in the crystal. Since the polarizations of other β emitting nuclei, ^12,16N, ^13,19O, and ⁴¹Sc were also totally maintained in the crystal, the crystal can be a “Spin Dewar” in which many short-lived nuclides can be implanted with their polarizations totally maintained during their lifetimes for the studies not only on the electronic structure of impurities in it but also on the nuclear properties. This revised version was published online in September 2006 with corrections to the Cover Date.     

Hyperfine Interactions of N Isotopes in TiO2 and Quadrupole Moment of 16N

Hyperfine interactions of ^12,14N in BN(hexagonal) crystal were studied by detecting β-NQR(¹²N) and FT-NMR(¹⁴N). A β-NMR of ¹⁶N (I ^π=2⁻,T _1/2=7.13 s) in MgO crystal was detected to determine the magnetic moment of ¹⁶N to be |μ(¹⁶N:2⁻)|=(1.986±0.001)μ_N. Also, the β-NQR of ^12,16N in TiO₂ crystal were detected to determine |Q(¹⁶N:2⁻)|=(17.9±1.7) mb. An abnormally small effective charge for neutrons is required to account for |Q(¹⁶N:2⁻)|. This revised version was published online in September 2006 with corrections to the Cover Date.     

Precise Quadrupole Moment of the Doubly Closed Shell Plus One Proton Nucleus 41Sc

In order to precisely determine the |eqQ(⁴¹Sc)/h| of ⁴¹Sc(I ^π=7/2⁻, T _1/2=0.596 s) implanted in a TiO₂ single crystal the electric field gradient tensor and anisotropic chemical shift were determined by detecting the Fourier Transformed Pulse-NMR of ⁴⁵Sc(I ^π=7/2⁻, stable) in the crystal at a high field of 7.0 T and 9.4 T. Combining the new |eqQ(⁴¹Sc)/h| value with the Q(⁴⁵Sc)=−(23.6±0.2) fm², also renewed by using the known atomic hyperfine interaction constants and Sternheimer polarization effect, the |Q(⁴¹Sc;I ^π=7/2⁻,T _1/2=0.596 s)|=(15.6±0.3) fm² has been precisely determined. The value is compared with the theoretical Q(⁴¹Sc) given by a shell model code. This revised version was published online in September 2006 with corrections to the Cover Date.     

Electromagnetic moments of short lived β emitters 21F, 23Mg, 27Si and 39Ca

The β-NMR spectra of ²¹F, ²³Mg, ²⁷Si and ³⁹Ca which were produced in heavy ion collisions and implanted in various crystals have been observed. The magnetic moments of ²¹F and ²⁷Si were determined to be |μ(²¹F)| = 3.9194 ± 0.0012 μ_N and |μ(²⁷Si)| = 0.8653 ± 0.0003 μ_N, respectively. The electric quadrupole coupling constants were determined for the first time to be |eqQ(²¹F in MgF₂)/h|= 9.94 ± 0.09 MHz, |eqQ(²³Mg in MgF₂)/h|= 1.96 ± 0.06 MHz, |eqQ(²⁷Si in Al₂O₃)/h|= 1.90 ± 0.12 MHz, |eqQ(³⁹Ca in CaCO₃)/h|= 0.60 ± 0.04 MHz. From the present eqQ/h, the Q moments were deduced as |Q(²¹F)|= 110 ± 22 mb, |Q(²³Mg)|= 114 ± 3 mb, |Q(²⁷Si)|= 60 ± 13 mb and |Q(³⁹Ca)|= 36± 7 mb. The present data were compared with the theoretical values obtained by the OXBASH shell model code. This revised version was published online in August 2006 with corrections to the Cover Date.     

Quadrupole moment of41Sc by use of new nuclear quadrupole resonance detection

Quadrupole effects in -NMR spectra of⁴¹Sc(I =7/2^–,T _1/2=0.596 s) implanted in a TiO₂ single crystal were detected by use of a modified -NMR technique. Using the field gradient in the crystal determined by the pulsed-Fourier-transformed NMR of⁴⁵Sc in TiO₂, the quadrupole moment of⁴¹Sc has been determined as |Q(⁴¹Sc; 7/2^–)|=166±8 mb.     

Hyperfine interactions of12B in BN (hexagonal)

Hyperfine interactions of¹²B(I =1⁺,T _1/2=21 ms) implanted in the substitutional site of B in BN (hexagonal) was studied by detecting -NMR. In order to measure the quadrupole coupling constant efficiently, we employed a newly developed quadrupole resonance technique (NNQR). The quadrupole moment of¹²B was determined to be |Q(¹²B)|=13.21±0.26 mb.     

Precise measurement of quadrupole moment of8B by use of a modified β-NMR

The nuclear quadrupole moment of⁸B(I =2⁺,T _1/2=769 ms) has been determined by use of a modified -NMR detection as |Q(⁸B)|=68.3±2.1 mb. A field gradient was obtained in a single crystal Mg at room temperature.     

Hyperfine Interaction of 140Ce(←140La) in CaB6

A ¹⁴⁰La(I ^π=3⁻, T _1/2=40.3 h)-doped layer has been produced in CaB₆ by means of radioactive isotope (RI) beam technique: ¹⁴⁰Cs(I ^π=1⁻, T _1/2=63.7 s) was implanted into CaB₆ and the radioactive equilibrium of ¹⁴⁰Ba–¹⁴⁰La was achieved. The concentration of La in CaB₆ was La/Ca ∼0.001. Obtained TDPAC spectra of the 2083 keV level of ¹⁴⁰Ce (I ^π=4⁺, T _1/2=3.4 ns, μ=+4.35±0.10 μ _N ) followed by the β decay of ¹⁴⁰La showed the existence of hyperfine magnetic fields: B _hyp=−15.0±0.5 T and −1.00±0.15 T. This revised version was published online in September 2006 with corrections to the Cover Date.     

Giant quadrupole moment andproton halo discovered in8B

The nuclear quadrupole moment of⁸B(I =2⁺,T _1/2=769 ms) has been determined by use of a modified -NMR detection as |Q(⁸B)|=68.3±2.1 mb, which is twice the prediction of the Cohen-Kurath shell model calculation. The anomalous quadrupole moment which is carried mainly by the protons in the nucleus, has been accounted for by the proton halo effect.     

Precise measurement of the quadrupole moment of β-emitting12B

Hyperfine interactions of¹²B(I ,T _1/2=21 ms) implanted in the substitutional site of B atoms (stable) in a (single crystal like) BN (hexagonal) was studied by use of a -NMR detection. For efficient and simple measurements, the conventional -NMR has been modified as a new nuclear quadrupole resonance technique (NNQR). For the present case with the nuclear spinI=1 the detection efficiency is improved about 30 times compared with the one with the old method. The quadrupole moment of¹²B was determined precisely as ¦Q(¹²B; 1⁺)¦=13.21±0.26 mb.     

Shape-driving effect of the proton 1/2[541] band in 171Ta

High-spin states in ¹⁷¹Ta were populated through the heavy-ion fusion-evaporation reaction ¹⁵⁷Gd (¹⁹F, 5n)¹⁷¹Ta at 105MeV beam energy. Lifetimes of the levels of the πh_9/21/2[541] band have been measured by using the Doppler shift attenuation method. The transition quadrupole moments ( Q_t) and the quadrupole deformation (β₂) have been extracted. Both β₂ and Q_t values decrease slightly with increasing rotational frequency. The average β₂ value of 0.26 is 18% larger than that of the πh_11/2 9/2[514] band. Total Routhian Surface calculations have been performed with the non-axial deformed Woods-Saxon potential and the predicted values of the quadrupole deformation β₂ are in good agreement with that deduced from our lifetime measurement. The shape-driving effect is discussed.     

On-line Time Differential Perturbed Angular Correlation with Light Probe Nucleus 19F

An on-line time differential perturbed angular correlation technique has been developed with the light probe nucleus ¹⁹F. The first on-line TDPAC measurement was carried out to determine the field gradient in Cd and quadrupole moment of ¹⁹F (0.197 MeV: I ^π = 5/2⁺, T_1/2 = 89 ns). This revised version was published online in September 2006 with corrections to the Cover Date.     

Nuclear Spin Alignment of 12,13B Produced in Heavy Ion Collisions

The nuclear spin alignments of the β-emitting fragments ¹²B(I ^π=1⁺, T _1/2=20.2 ms) and ¹³B(I ^π=3/2⁻, T _1/2=17.4 ms) produced in the 100A-MeV ¹³C, ¹⁵N + ⁹Be collisions respectively have been observed for the first time detecting asymmetric β-ray emission from these nuclei. By means of the spin manipulation technique based on the hyperfine interaction of B isotopes in TiO₂, both the polarization P and the alignment A were determined reliably. The obtained P and A were significantly smaller than the expectation from the kinematical model. From the fact that the quenching factors for P and A are almost the same, there may be some depolarization mechanism in the collision process itself. This revised version was published online in September 2006 with corrections to the Cover Date.     

Precise measurement of magnetic moment of short-lived β-emitting nuclei12B ( I π=1+, T 1/2=20.18 ms)

The spin polarized β-emitting nuclei¹²B (I ^π=1⁺,T _1/2=20.18 ms) were produced by the nuclear reaction¹¹B(d, p)¹²B and by the selection technique of the incident deuteron energy and the¹²B recoil angle following the nuclear reaction. The nuclear magnetic moment of the short-lived nuclei¹²B was measured by β-NMR with the β-NMR and β-NQR setup established for the first time in China. The nuclear magnetic moment of¹²B was determined to be μ=0.99993±0.00048 nm org=0.99993±0.00048 after the precise correction of the Knight shift.     

Magnetic moment of beta-emitting41Sc(Iπ=7/2−) and knight shift in Pt metal

The nuclear magnetic moment of⁴¹Sc(I^π=7/2⁻, T_l/2=0.59sec) was remeasured, and the precision of the value was improved about 10 times compared with the previously known one. The value was determined to be |μ(⁴¹Sc;I^π=7/2)|=(5.4305±0.0018) nm. Comparing the value with the previously known NMR of the nuclei in Pt, the knight shift, K=−(0.4±5.3)·10⁻⁴ was determined.     

Diffusion study of 18O implanted into α-Hf using the nuclear resonance technique

The diffusion of ¹⁸O in α-Hf was studied in the 723–923 K temperature range by using ion implantation and nuclear resonance techniques. The measurements show that the diffusion coefficients follows an Arrhenius behavior D(T)=D₀e^(-Q/RT), where D₀=(5±3)×10^-9 m²s^-1 and Q=162±5 kJ/mol. A comparison of the present results with previous ones is also done. PACS 66:30 Jt; 85:40 Ry     

New determination of quadrupole coupling constants of Li isotopes in single crystals LiIO3 andLiNbO3

Quadrupole effects in NMR spectra of⁸Li(I =2⁺;T _1/2=0.84 s) in LiIO₃ andLiNbO₃ single crystals have been detected by use of a modified -NMR. The coupling constants for both crystals are in agreement with known ones. Field gradients in the crystals were measured by detecting pulsed-Fourier transformed NMR of⁷Li. The quadrupole moments deduced from both samples agree, and|Q(⁸Li; 2⁺)|=32.7±0.6 mb has been determined.     

The β-decay of 22Al

In an experiment performed at the LISE3 facility of GANIL, we studied the decay of ²²Al produced by the fragmentation of a ³⁶Ar primary beam. A β-decay half-life of T_1/2 = 91.1±0.5ms was measured. The β-delayed one- and two-proton emission as well as β-α and β-delayed γ-decays were measured and allowed us to establish a partial decay scheme for this nucleus. New levels were determined in the daughter nucleus ²²Mg. The comparison with model calculations strongly favours a spin-parity of I^π = 4⁺ for the ground state of ²²Al.