超短中红外参量放大过程的时空走离特性

计算了MgO:LiNbO3晶体中,共线与非共线相位匹配光参量放大产生超短中红外激光脉冲过程中的相位匹配曲线、有效非线性系数以及时间和空间走离情况。结果表明,采用非共线相位匹配方式,可以实现三波间群速度匹配;在抑制了泵浦光与信号光之间的空间走离的同时加大了泵浦光与闲频光之间的空间走离,但这种影响可以忽略;同时非共线角的引入使相位匹配角增大,提高了有效非线性系数。因此,非共线角的引入在不影响空间走离的情况下,有效补偿超短中红外参量放大过程中的时间走离,有利于参量放大转换效率的提高。     

BBOⅠ类相位匹配光参量放大中群速失配的补偿

描述了在BBOⅠ类相位匹配的飞秒光参量放大（OPA）中，利用非共线结构和倾斜抽运光的脉 冲波面来完全补偿三波群速失配的方法.理论计算了三波群速匹配时，非共线角、相位匹配 角、抽运光的脉冲波面倾斜角随信号光波长的变化，并分析了对抽运光光斑尺寸的要求和对 空间走离长度的影响.结果表明，利用该方法不仅能够实现最大的参量带宽，而且能够完全 补偿飞秒OPA中三波的群速失配.此外，选取合适的抽运光光斑尺寸和非线性晶体的长度对提 高参量增益也至关重要. 关键词： 群速匹配 非共线相位匹配 脉冲波面倾斜 飞秒光参量放大     

AgGaSe_2晶体差频产生可调谐太赫兹波的理论研究

基于单轴晶体中三波互作用的共线相位匹配技术,采用CO2激光器泵浦非线性晶体AgGaSe2,数值计算出在oee类和oeo类相位匹配条件下,差频产生太赫兹波的相位匹配角、走离角、允许角和有效非线性系数。计算结果表明:两类相位匹配太赫兹波可调谐的范围都非常宽,而且走离角都在1°以下,允许角足够大。在绝大部分太赫兹波区域,oee类匹配有效非线性系数远大于oeo类匹配,实验中适合采用oee类相位匹配方式。     

飞秒光参量放大中三波群速失配的补偿

为了消除群速失配对参量放大的不利影响，描述了利用脉冲波面倾斜与非共线相位匹配相结 合，完全补偿飞秒光参量放大（OPA）中三波群速失配的新方法.计算了在BBOⅠ类、Ⅱ类相 位匹配条件下， 三波实现群速匹配时，相位匹配角、脉冲波面倾斜角以及非共线角随信号 光波长的变化.并分析了三波群速匹配对空间走离长度、参量增益和参量带宽的影响.结果表 明，在BBOⅠ类、Ⅱ类相位匹配条件下，利用该方法均能实现飞秒OPA连续调谐时三波的群速 匹配，从而大大增加了三波的有效互作用长度，为能够获得高增益，窄脉宽的参量光脉冲提 供了理论依据和指导. 关键词： 群速匹配 脉冲波面倾斜 非共线相位匹配 飞秒光参量放大     

基于交叉泵浦的受激电磁耦子散射非共线相位匹配方法

提出一种基于交叉泵浦实现受激电磁耦子散射的非共线相位匹配的方法，获得频率可调谐的窄带Stokes光输出。根据参量放大理论，推导出交叉泵浦受激电磁耦子散射的单程放大增益效率表达式，揭示了交叉泵浦实现受激电磁耦子非共线相位匹配的物理机制。实验上采用泵浦光在晶体侧面全反射的方式构建交叉泵浦，通过旋转晶体改变泵浦光全反射角，实现相位匹配条件的改变和输出Stokes光频率的调谐。输出Stokes光线宽为0.17 nm，波长调谐范围为1 068～1 076 nm。在15 mJ的泵浦能量下的输出能量为1.07 mJ，能量转化效率为6.8%。本研究为非线性参量转换过程中的相位匹配方法提供一种方案参考，尤其适用于泵浦光脉宽小于纳秒量级的短脉冲情况。     

非共线相位匹配LBO晶体飞秒光参变放大器的研究

对非共线相位匹配LBO晶体飞秒光参变放大器进行了系统地分析和理论研究，用数值方法得出了非共线角、相位匹配角、增益和增益带宽之间的关系，给出了放大器设计的各种最优化参量。研究结果表明，这种参变放大器不仅可以实现较高的参变增益和获得极宽的增益带宽，还具有较大的参变允许角、较小的走离角和小的群速色散。因此这种参变放大器对于以纳秒级高功率激光作为抽运光，利用光参变啁啾脉冲放大（OPCPA）技术高效率参变放大飞秒脉冲产生10^12W甚至10^15W级的超强超短激光脉冲具有重要的意义。建立的理论模型具有普遍意义，也为其他类似的参变过程提供了重要的理论依据。     

深紫外和频晶体CLBO产生193 nm激光的频率变换

 简述了深紫外和频晶体CLBO的光学特性。根据相位匹配角公式、非线性有效系数公式、走离角公式和允许角公式,详细计算了CLBO晶体和频产生193 nm激光时的相位匹配角、非线性有效系数、和频时谐波走离角、允许角的具体数值。根据这些数值,并考虑产业化的要求,对目前几种和频方式进行了比较,最终选定波长为λ₁=2 100 nm的o光和波长为λ₂=213 nm的e光作为基频光进行和频的匹配方式。此方式相位匹配角为51.6°,具有大的非线性有效系数0.97,小的走离角3.7°,大的允许角1.9×10^-6 rad·mm,是非常理想的产生193 nm激光的匹配方式。     

基于BiB3O6晶体的飞秒光参量变换特性

对基于新型非线性晶体BiB₃O₆(BIBO)的飞秒光参量变换过程的参量特性进行了研究. 计算了BIBO晶体三个光学主平面内的相位匹配条件和有效非线性系数,确定了克尔透镜锁模钛宝石激光器的基频光与倍频光抽运时最佳的光学主平面和相位匹配方式,并分析了三波的时间走离和空间走离,以及信号光的参量增益和带宽. 为利用基于BIBO晶体的飞秒光参量技术获得高能量、宽调谐、窄脉宽的光源提供理论依据和实验指导. 关键词： 3O₆')" href="#">BiB₃O₆ 光参量变换 共线相位匹配 光学主平面     

新型光学晶体KABO的非线性频率变换特性

简述了新型非线性晶体KABO的光学特性.根据相位匹配角公式、非线性有效系数公式、走离角公式和允许角公式,详细计算了KABO晶体倍频时的相位匹配角、非线性有效系数、倍频时谐波走离角、允许角随波长变化的理论曲线.特别是对LD泵浦掺钕的全固态激光器532 nm输出时,得到了KABO晶体采用I类相位匹配进行四倍频的相位匹配角、非线性有效系数、倍频时谐波走离角、允许角分别为:58.1°、0.254×10^-12m/V、2.8°、1.8233 mrad·mm;并将该晶体与目前可应用于紫外倍频的晶体比较,在考虑走离效应的情况下,研究了四倍频转换效率随KABO晶体长度、基频光光斑半径的变化规律.     

第Ⅰ类BBO晶体中的参量荧光空间特性理论研究

 采用第Ⅰ类相位匹配BBO晶体的放大传递函数方法,分别对光参量放大过程中单波长信号光注入和多波长信号光注入出现的参量荧光的空间特性进行了详细的理论研究。结果表明:一方面单波长信号光注入时,在某一特定的非共线角和相位匹配角下,它是以泵浦光为中心,呈锥形分布的,而在其它相位匹配区域内,则呈环形分布;另一方面,在多波长信号光入射情况下,参量荧光的光谱在某一特定的相位匹配角下集中分布在很宽的范围内,而在其余相位匹配区域内,参量荧光光谱呈分散分布状态。该结论对于光参量放大中三波群速失配的补偿,高增益和窄脉冲宽度的参量光的产生以及对于参量荧光的控制提供了理论依据,并且对于近年来量子图像处理和量子通讯等领域所关注的纠缠光场的产生也具有参考价值。     

利用LiNbO3晶体的拉曼散射获得太赫兹辐射的研究

对利用LiNbO3晶体拉曼活性的E对称模(ωTO=236 cm-1≈7.08 THz)产生太赫兹辐射进行了研究, 采用输出波长为1.064 μm 的Nd:YAG脉冲激光器作为泵浦源, 根据光学参量振荡的基本原理, 推导计算了非共线第二类相位匹配条件下的晶体长度、有效非线性系数、相位匹配角等技术参量, 最后根据所计算的各技术参量设计了太赫兹光学参量振荡器(TPO)。     

Measurement of ultrashort laser pulses using single-crystal films of 4-aminobenzophenone

Single-crystal thin-film of an organic second-order nonlinear optical material, 4-aminobenzophenone (ABP), is used to measure the pulsewidth of a Ti-Sapphire laser producing 45 fs pulses at 1 kHz repetition rate, by the non-collinear second-harmonic generation (SHG) intensity autocorrelation technique. These films are suitable for measurements over a broad wavelength range, down to 780 nm, due to their wide optical transparency. The single-crystal film with thickness (3 μm) less than the coherence length requires no phase-matching for efficient broadband SHG. Pulse walk-off due to group-velocity mismatch (GVM) and temporal broadening of the pulses due to group-velocity dispersion (GVD) are found to be negligible. These effects have been estimated for pulse width down to few-cycle pulses (10 fs), and the analyses show that these films can be used to characterize such ultrashort optical pulses.     

基于光束偏转的扫描式宽带光参量啁啾脉冲放大

光参量啁啾脉冲放大(OPCPA)是超短激光脉冲领域的重要技术之一,增大增益带宽对提高OPCPA的转换效率、实现宽带光参量放大具有重要的意义.本文将光束偏转和非共线OPCPA有机结合,提出了基于光束偏转的扫描式宽带OPCPA模型.分析了通过光束偏转来时刻改变非共线角,以保证各频率成分的相位匹配,从而增大增益带宽的基本原理.采用提出的扫描式宽带OPCPA,针对800 nm中心波长、带宽约为100 nm信号光的光参量放大进行了数值计算.结果表明:经过扫描式OPCPA后,信号光的带宽与放大之前几乎相同,光谱没有窄化;扫描式OPCPA比固定非共线角方式的放大极大地增加了增益带宽和转换效率,实现了宽带的光参量放大;要满足信号光各频率成分的相位匹配,达到最大的增益带宽和转换效率,需要尽量减小加载到钽铌酸钾(KTa_(1-x) Nb_xO_3, KTN)电光晶体上的电压抖动和电压延时.     

最优的双轴晶体非共线匹配频率升频转换效应

研究了双轴晶体的非共线相位匹配参量放大的升频转换效应.计算表明p,r,s三波位于同一子午平面上时是好的非共线匹配.选择适当的入射角α,所有光线的离散效应能够获得补偿,晶体的有效长度增加和能量转换效率能较大地提高.     

Theorie der parametrischen Vier-Photonen-Wechselwirkung. III. Verstärkung und Oszillation bei Berücksichtigung der Rückwirkung auf die Pumpwelle

The processes of parametric amplification and oscillation in a medium with cubic polarization are investigated theoretically taking into consideration the depletion of the pump wave. We suppose that phase-matching is realized exactly (a possible nonlinear detuning of the exact phase-matching should be compensated by a suitable subsequent adjustment of the frequencies). A consequence of linear losses is the appearance of a threshold for the parametric amplification. There exist a maximum length, a minimum length and an optimum length of the nonlinear medium for the process of parametric amplification. The threshold intensity, the optimum length of the nonlinear medium and the optimum reflection coefficient for outcoupling are determined for two arrangements of the double resonant parametric four-photon oscillator (ring resonator, FABRY -PEROT resonator). It is shown that for the above mentioned arrangements of the single resonant and the double resonant four-photon oscillator the efficiency is a monotonous function of the threshold excess. On the contrary in case of the three-photon oscillator there exists an optimum value of the threshold excess.     

Fiber optical parametric oscillator for sub-50 fs pulse generation: optimization of fiber length

We demonstrate generation of 48fs pulses with linear chirp using a short (27mm) fiber optical parametric oscillator (FOPO), which is synchronously pumped by a mode-locked ytterbium-doped fiber laser. We also study the pulse quality for both the short- and long-wavelength operation where the fiber length inside of the oscillator varies from 17 to 61mm. The optimal pulse duration is observed only in the short-wavelength operation. Furthermore, we model the FOPO system as a single-pass parametric amplifier including dispersive pulse broadening and walk-off between the pump and output. The optimal condition arises from the minimization of the walk-off and dispersion. When walk-off is large, the parametric amplification process is most efficient over some reduced effective fiber length, leading to an upper limit in the amount of the observed pulse broadening.     

Broadband non-collinear double QPM optical parametric amplification in mid-infrared wave

The properties of optical parametric amplification (OPA) based on non-collinear double quasi-phase matching (NDQPM) with single periodically poled KTP (PPKTP) have been investigated theoretically. The NDQPM includes two different non-linear processes: one is optical parametric generation (OPG) and the other is difference frequency generation (DFG). The investigation of our numerical simulation focuses on the gain bandwidth of dependence upon non-collinear angle, grating period and crystal temperature. At a certain non-collinear angle and grating period with fixed temperature, there exists a broadest gain bandwidths of output mid-infrared pulse at 526 nm pump wavelength and certain signal wavelength in PPKTP. These are an optimal values of non-collinear angles and grating period. By accurately tuning the non-collinear angle or temperature near the optimal non-collinear angle, broadband mid-infrared tuning is obtained and an optimal operation of NDQPM can be realized. In this paper, the solutions of the coupled equations of the cascaded processes were discussed, and the spatial-temporal frequency (STF) band of the output idler pulse is analyzed by taking angular dispersion of amplified pulse beam into account. The idler pulse with a certain angular dispersion can improve the OPA bandwidth significantly. So, optical parametric chirped-pulse amplification can be realized in this configuration. For a broadband NDQPM both the acceptance angles and the acceptance temperature are smaller and the gain bandwidth is sensitive to non-collinear angles and temperature, it is important to control the precision of the non-collinear angles and the temperature in experiment.