New experimental results in proton radioactivity

A review of experimental data obtained recently on proton-radioactive nuclei is presented. The highlights include the observation of fine structure in proton emission, for the decays of ¹³¹Eu, ¹⁴⁵Tm and ¹⁴⁶Tm, and the studies of the excited states in proton-emitting nuclei. The observation limits are extended to few nanobarns cross-sections ( ¹⁴⁰Ho, ¹⁶⁴Ir and ¹³⁰Eu) and few microsecond half-lives (e.g., ¹⁴⁵Tm). Measured decay properties for thirty-nine proton-emitting ground and isomeric states contributed to the understanding of nuclear masses and evolution of single-particle states at and beyond the proton drip line. Experimental results have stimulated new theoretical approaches to proton emission and the structure of unbound narrow resonance states. Received: 21 March 2002 / Accepted: 16 May 2002 / Published online: 31 October 2002 RID="a" ID="a"e-mail: rykaczew@phy.ornl.gov     

Studies with one- and two-proton drip line nuclei

In recent experiments at GANIL, we studied nuclei at the one- and two-proton drip line. The production rates allowed to search for direct 2p emission in the drip line nuclei ⁴²Cr, ⁴⁵Fe, and ⁴⁹Ni. No evidence for this decay mode was found in ⁴²Cr and ⁴⁹Ni, whereas the situation stays unclear for ⁴⁵Fe due to the limited statistics. In the medium-mass region ( A = 50-70), the half-life was measured for all proton-rich nuclei in the range T _z = 0 to T _z = - 1 between Z = 27 and Z = 36. First half-lives were determined for ⁶⁰Ga, ⁶²Ge, ⁶⁴As and ⁶⁶Se. Finally, β-decay studies of the 0⁺ → 0⁺ decay of ⁶²Ga have been performed at IGISOL in Jyv?skyl?. Non-analog transitions have been observed and are compared to theoretical predictions. Received: 21 March 2002 / Accepted: 16 May 2002 / Published online: 31 October 2002 RID="a" ID="a"e-mail: blank@cenbg.in2p3.fr     

New insights into neutron-rich nuclei at high spin

With new high statistic data, new isotopes and new high-spin structures are observed in neutron-rich nuclei populated in the spontaneous fission of ²⁵²Cf. The ¹³⁵Te levels are extended, and many new levels in ^139,141Ba observed. The coexistence of collective and single particle-hole states is found in ¹³⁵Te. The N = 83 ¹³⁵Te and ¹³⁹Ba show marked differences associated with differences in their particle and hole states. New levels in ¹⁴¹Ba complete evidence for two opposite-parity doublets characteristic of stable octupole deformation. In ^114,116Pd a second backbend is observed for the first time in this mass region and the backbend in ¹¹⁸Pd occurs earlier than in ^112-116Pd because of a reduction in pairing. Gamma-type vibrational bands are seen up to 13⁺ to 15⁺ in ^104,106Mo, ^108-112Ru, and ^112-116Pd. Their behavior reflects prolate to triaxial shapes in these nuclei. The levels of ^162,164Gd are observed for the first time. As N increases toward mid-shell at 104, the moments of inertia in N = 100 ¹⁶⁴Gd show an unexpected decrease compared to N = 98 ¹⁶²Gd. The levels in ^162,164Gd form remarkable shifted identical bands with nuclei separated by 2n, 2p, α, and 2α. Received: 21 March 2002 / Accepted: 16 May 2002 / Published online: 31 October 2002 RID="a" ID="a"e-mail: j.h.hamilton@vanderbilt.edu     

Evidence for partial rotation alignment in proton emitting Pr

Using nonadiabatic quasiparticle calculations we reproduce the experimental half-life for proton radioactivity in ¹²¹Pr assuming that the decaying state has angular momentum Jπ=7/²⁻$J^{\pi }=7/2^{-}$, thus showing for the first time clear evidence for partial rotation alignment in a proton emitting nucleus. The treatment of the pairing interaction in the BCS approach produces profound changes in the ordering of energy levels, and at high deformation, the state 7/²⁻$7/2^{-}$ coming from the h_11/2${\mathrm{h}}_{11/2}$ spherical shell becomes the bandhead.     

Measurement of 2+ 1 level lifetimes in 162Yb and 162Er by fast electronic scintillation timing

Lifetime measurements for the 2⁺ ₁ levels of ¹⁶²Er and ¹⁶²Yb were obtained in β⁺/ɛ decay at the Yale Moving Tape Collector by fast electronic scintillation timing of β⁺γ coincidences. Received: 2 September 2002 / Accepted: 1 October 2002 / Published online: 4 February 2003 RID="a" ID="a"e-mail: mark.caprio@yale.edu Communicated by J. ?yst?     

High-resolution in-beam particle spectroscopy --New results on prompt proton emission from 58Cu

Prompt proton decay lines in ⁵⁸Cu have been studied by means of high-resolution in-beam particle-γ coincidence spectroscopy using the GAMMASPHERE Ge-detector array in conjunction with a dedicated set of ancillary detectors including four ΔE-E silicon-strip telescopes. High-spin states in ⁵⁸Cu have been populated via the heavy-ion fusion-evaporation reaction ²⁸Si(³⁶Ar, 1α1p1n) at 148 MeV beam energy. The full-width at half maximum for the proton peak could be reduced significantly compared to earlier experiments. The results indicate that only one prompt proton decay branch exists in the decay-out of the well-deformed band of ⁵⁸Cu. Received: 11 March 2002 / Accepted: 10 April 2002     

Lifetime measurements in 148Gd

Lifetimes of excited states in ¹⁴⁸Gd were measured using the recoil distance method with a plunger device coupled to the EUROBALL Ge detector array. The differential decay curve method in coincidence mode allowed the unambiguous determination of lifetimes of more than 20 excited states. The obtained transition strengths are in good agreement with the shell model calculations. The effect of the Z = 64 subshell closure on the B(E2 : 2⁺ → 0⁺) reduced strengths above the N = 82 magic number is discussed.-1 Received: 14 November 2002 / Accepted: 4 February 2003 / Published online: 29 April 2003     

First evidence for the two-proton decay of 45Fe

Decays of five ⁴⁵Fe atoms have been observed at the fragment separator of GSI. Whereas one event is consistent with the β-decay of ⁴⁵Fe accompanied by the emission of a 10 MeV proton, four decays are consistent with the emission of particle(s) of total energy 1.1±0.1 MeV. This observation represents the first evidence for two-proton ground-state radioactivity, a decay mode predicted for ⁴⁵Fe. The time distribution of the observed decay events corresponds to a half-life of 3.2^+2.6 _-1.0 ms. Received: 17 May 2002 / Accepted: 28 May 2002     

High-spin proton and alpha-particle emission as probes for nuclear structure

During recent years the nuclear decay modes of discrete prompt proton and α-particle emission from (super)deformed high-spin states have been discovered in nuclei in the vicinity of ⁵⁶Ni. The latest news from experiments performed at EUROBALL and GAMMASPHERE regarding these decays are presented and discussed. Published online: 31 October 2002 RID="a" ID="a"e-mail: dirk.rudolph@kosufy.lu.se     

Inelastic excitation of <Superscript>187</Superscript>Re

Excited states in ¹⁸⁷Re populated by inelastic scattering of a 500 MeV ⁸²Se beam have been studied by means of in-beam γ-ray spectroscopy. Levels built on the 5/2⁺[402] and 9/2^-[514] one-quasiparticle states were measured up to I ^π = (21/2⁺) and (21/2^-), respectively. In addition, several new levels including an isomer at 1682 keV with a half-life of 114(23) ns have been found. Quasiparticle configurations of the levels and the transition rates are discussed. Received: 12 December 2002 / Accepted: 13 March 2003 / Published online: 13 May 2003     

Isomeric states in proton-unbound 187, 189Bi isotopes

Prompt and delayed gamma-ray spectroscopy of very neutron-deficient bismuth isotopes ^{187, 189}Bi has been performed using the Recoil Decay Tagging (RTD) method. The isomeric i _13/2 states have been identified and their lifetimes have been measured. The systematics of these long-lived M2 isomers has been extended to the proton-unbound isotopes. The general behaviour of single-proton states is discussed within the systematics and interpreted within the shell-model framework. Received: 2 May 2002 / Accepted: 3 June 2002 / Published online: 19 November 2002 RID="a" ID="a"e-mail: wkorten@cea.fr RID="b" ID="b"Present address: GANIL, Caen, France. RID="c" ID="c"Present address: Radiation and Nuclear Safety Authority, P.O. Box 14, FIN-00881 Helsinki. Communicated by D. Schwalm     

Systematics of related high-spin isomers in 144Sm and other N = 82 nuclei

An in-beam experiment with the reaction ¹²²Sn(²⁷Al,4np) at 127 MeV was performed at the Nordball multi-detector array in Roskilde. It provided evidence for a new high-spin isomer in ¹⁴⁴Sm. This isomer with T _1/2= (2.6 ± 0.5) ns at an excitation energy E _x= 9232 keV seems to belong to a family of isomers of similar configuration in neighbouring N= 82 nuclei. Received: 16 November 1997     

High-spin states in odd-odd 168Lu

High-spin states in the odd-odd ¹⁶⁸Lu nucleus, populated in the ¹⁵⁴Sm(¹⁹F,5n) reaction at a beam energy of 96 MeV, were investigated using in-beam γ-ray spectroscopy techniques. The BC neutron crossing in the yrast band, based on πg _7/2[404]7/2⁺⊗νi _13/2[642]5/2⁺ configuration, occurs at ħω= 0.31 MeV. The two side bands, based on πh _11/2[514]9/2⁻⊗νi _13/2[642]5/2⁺ and πh _9/2[541]1/2⁻⊗νi _13/2[642]5/2⁺ configurations, show anomalous signature-splitting and signature-inversion in the first one, to occur at ħω= 0.24 MeV. A moderately delayed BC-crossing is anticipated in the second one. Received: 15 June 1998 / Revised version: 11 January 1999     

Shape-driving effect of the proton 1/2[541] band in 171Ta

High-spin states in ¹⁷¹Ta were populated through the heavy-ion fusion-evaporation reaction ¹⁵⁷Gd (¹⁹F, 5n)¹⁷¹Ta at 105MeV beam energy. Lifetimes of the levels of the πh_9/21/2[541] band have been measured by using the Doppler shift attenuation method. The transition quadrupole moments ( Q_t) and the quadrupole deformation (β₂) have been extracted. Both β₂ and Q_t values decrease slightly with increasing rotational frequency. The average β₂ value of 0.26 is 18% larger than that of the πh_11/2 9/2[514] band. Total Routhian Surface calculations have been performed with the non-axial deformed Woods-Saxon potential and the predicted values of the quadrupole deformation β₂ are in good agreement with that deduced from our lifetime measurement. The shape-driving effect is discussed.     

Observation of signature inversion in odd-odd 178Ir

High spin states in ¹⁷⁸Ir have been studied via the ¹⁵²Sm(³¹P, 5nγ)¹⁷⁸Ir reaction through excitation functions, X-γ and γ-γ-t coincidence measurements. According to the band structure characteristics and the measured intraband B(M1)/B(E2) ratios, two rotational bands are identified and assigned to be associated with the πh _9/2⊗νi _13/2 and πh _11/2⊗νi _13/2 configurations, respectively. Both bands show the signature inversion feature. Received: 23 March 2000 / Accepted: 31 July 2000     

In-beam studies of very neutron-deficient heavy nuclei

The JYFL gas-filled recoil separator RITU, combined with Ge detector arrays and a SACRED magnetic solenoid spectrometer, has been successfully employed in recoil-decay-tagging (RDT) experiments in order to probe structures of very neutron-deficient heavy nuclei. The present contribution focuses on the light Pb region where the new data extend the systematics of shape-coexisting yrast states towards the proton dripline. Similarities between band structures and their relation to possible multi-particle multi-hole intruder excitations will be discussed. Received: 21 March 2002 / Accepted: 16 May 2002 / Published online: 31 October 2002 RID="a" ID="a"e-mail: rauno.julin@phys.jyu.fi     

Decay studies of N ≈ Z nuclei from 75Sr to 102Sn

Neutron deficient nuclei near ¹⁰⁰Sn have been produced by fragmentation of a 1 ^. AGeV ¹¹²Sn beam. The fragments were separated, identified and stopped in a highly segmented silicon strip detector stack. This detector measured the total energy of emitted β⁺-particles. γ-radiation was measured with surrounding detectors. The half-lives for many nuclides have been determined for the first time and give important information for the following topics: For the heaviest particle-stable odd-odd nuclei ⁹⁰Rh, ⁹⁴Ag and ⁹⁸In we observed for the first time fast β-decays, compatible with superallowed Fermi transitions and confirmed such decays for ⁷⁸Y, ⁸²Nb and ⁸⁶Tc. We have also observed long-lived T = 0 states in some of these nuclei. We measured the half-lives of all rp-process waiting-point nuclei from ⁸⁰Zr up to ^{92, 93}Pd. In addition we find the proton drip line nucleus ⁷⁷Y to decay dominantly via β-decay. To study the Gamov-Teller strength in the β-decay near the doubly magic ¹⁰⁰Sn we measured the half-life, β- and γ-spectrum of ¹⁰²Sn. We propose a level scheme for the daughter nuclide ¹⁰²In and deduce the Gamov-Teller strength (B _GT = 4.0±0.6). This is one of the largest values known. Received: 21 March 2002 / Accepted: 16 May 2002 / Published online: 31 October 2002 RID="a" ID="a"e-mail: thomas.faestermann@ph.tum.de     

Mirror decay of 75Sr

The β-decay of ⁷⁵Sr to its mirror nucleus ⁷⁵Rb was studied at the ISOLDE PSB facility at CERN by means of β-delayed γ and proton spectroscopy. The decay Q-value and β-delayed γ intensity were measured for the first time. These results, 10.60±0.22 MeV and 4.5^+1.9 _-0.7%, together with accurate measurements of the β-decay half-life and β-delayed proton branching ratio yielded the Gamow-Teller strength 0.35±0.05 for the mirror transition. Implications of the results on studies of deformation effects and on the path of the rapid proton capture process are discussed. Received: 26 September 2002 / Accepted: 30 October 2002 / Published online: 18 February 2003 RID="a" ID="a"e-mail: jussi.huikari@phys.jyu.lfi Communicated by D. Schwalm     

(EC + β<Superscript>+</Superscript>) decays of the 11/2<Superscript>-</Superscript> isomer and 1/2<Superscript>+</Superscript> ground state of <Superscript>143</Superscript>Dy

The 1/2⁺ ground state and a 11/2^- isomer of very neutron-deficient isotope ¹⁴³Dy were produced by irradiation of an enriched target of ¹⁰⁶Cd with ⁴⁰Ca and studied by using a helium-jet fast tape-transport system in combination with proton-γ, X-γ and γ-γ coincidence measurements. A simple ( EC + β⁺) decay scheme of ^143mDy with a half-life of 3.0(3) s and a tentative ( EC + β⁺) decay scheme of ^143gDy with a half-life of 5.6(10) s are proposed. As a by-product, the 347- and 545-keV γ transitions in ¹³⁸Sm following the β-delayed proton emission of ¹³⁹Gd decay and the 323-keV γ transition in ¹³⁹Eu following the β-delayed proton emission of ¹⁴⁰Tb decay could be observed for the first time. Received: 20 August 2002 / Accepted: 28 October 2002 / Published online: 11 February 2003 RID="a" ID="a"e-mail: xsw@ns.lzb.ac.cn Communicated by D. Schwalm