Electric quadrupole and magnetic dipole moments of the first excited 2+ states of186Os and188Os

The spectroscopic quadrupole moments and the magnetic dipole moments of the lowest 2⁺ states in¹⁸⁶Os (137 keV) and¹⁸⁸Os (155 keV) have been determined by Mößbauer transmission experiments. The electric quadrupole momentsQ ₂₊(Os 186)=? (1.80±0.22) b andQ ₂₊(Os 188)=?(1.81±0.24) b as well as their ratioQ ₂₊(Os 188)/Q ₂₊(Os 186)=1.00±0.07 within the limits of error agree withB(E2) data, if a comparison on the basis of the rotational model is made. For the g-factors and their ratio g₂₊(Os 186)=0.281±0.008, g₂₊(Os 188)=0.305±0.015 andg ₂₊(Os 188)/g ₂₊(Os 186)=1.08±0.05 was obtained. All results are compared with recent model calculations.     

Mössbauer studies and nuclear quadrupole moments of186, 188, 189, 190 Os

Mössbauer transmission experiments with the 137, 155, 69 and 187 keV gamma rays of^{186, 188, 189, 190}Os, respectively, yielded the electric quadrupole splitting of these gamma resonance lines in OsO₂ and OsP₂. From the results the following ratios of quadrupole moments were derived:Q ₂ ⁺(¹⁸⁶Os, 137 keV):Q ₂ ⁺(¹⁸⁸Os, 155keV):Q ₂ ⁺(¹⁹⁰Os, 187 keV):Q _3/2 ^?(¹⁸⁹Os, g.s.)=(+1.100±0.020): 1.0:(+0.863±0.051): (?0.586±0.011) andQ _5/2 ^?(¹⁸⁹Os, 69 keV)/Q _3/2 ^?(¹⁸⁹Os, g.s.)=?0.735 ±0.012. The ratios for^{180, 188, 190}Os are, within their limits of error, in agreement with the expectation of the rotational model, indicating that the pairing-plusquadrupole model calculations of Kumar and Baranger predict too rapid a transition form rotational to vibrational nuclei. Applying this argument to¹⁸⁶Os in particular and using the measured ratios, one obtains a set of values for the quadrupole moments themselves, namelyQ ₂ ⁺ (¹⁸⁶Os)=?(1.50 ± 0.10)b,Q ₂ ⁺(¹⁸⁸Os)=?(1.36± 0.09) b,Q ₂ ⁺ (¹⁹⁰Os)=?(1.18 ± 0.08) b,Q _3/2 ^?(¹⁸⁹Os)=+ (0.80 ± 0.06) b, andQ _5/2 ^? (¹⁸⁹Os)=? (0.59 ± 0.05) b. For the electric field gradient at Os nuclei in Re metal a value ofV _zz=?(3.3 ± 0.6) · 10¹⁷ V/cm² was found. A measurement with a magnetically split source yielded δ=+ 0.685 ± 0.025 for theE2/M1 mixing parameter of the 69 keV transition of¹⁸⁹Os,g _5/2 ^?/g _3/2 ^?=0.895 ± 0.006 for the ratio of theg-factors of the 69 keV state and the groundstate, andH _i=?(1135 ± 20) kOe for the hyperfine field at Os nuclei in an iron matrix.     

The spin of the 2,198 keV level in74Ge and multipole mixing ratios of gamma transitions in the decay of74As

Directional-correlation measurements of several cascades in the⁷⁴As decay have been made with a NaI — Ge(Li) detectors system. In the⁷⁴Ge the following cascades were measured: 608–596 keV, 994–1,204 keV, 994-(608)-596 keV and 887-596 keV. The corresponding results give a unique spin assignment of 2 for the 2,198 keV level and determine theE2/M 1 mixing ratios ofδ(608)=3.4±0.4 andδ(994)=?(2.8 ± 0.2). In the⁷⁴Se it was measured the 635-635 keV cascade. The result obtained assigned the spin of the 1,270 keV level as 2 and fixed the E2/M1 mixing ratio of δ(635)=?(2.6 ± 0.2). Also aγ-intensity study has been made to determine the branching ratios of the transitions that deexcite the 1,270 keV level in⁷⁴Se. From these data aI(635)/I(1,270)=12.5 ± 5.0 is obtained.     

Multipole mixing ratios of γ-transltions in 182W

γ-γ directional correlation experiments were performed on 14 cascades in ¹⁸²W populated from the β^? decay of ¹⁸²Ta(115 d). Two Ge(Li) detectors were used in a coincidence arrangement, and the ¹⁸²Ta sources were dissolved in HF acid to minimize extranuclear perturbations. For the 1189keV, 2^? → 2⁺ transition, the measured directional correlation coefficients are consistent only with multipole mixing ratios $\text{δ}\text{(}\text{M}\text{2}\text{E}\text{1)}\text{= 0.45 ± 0.03}\text{and}\text{δ}\text{(E3}\text{E1)}\text{= ?0.67 ± 0.07}$. These mixing ratios are discussed and compared with the known conversion coefficients for the 1189keV transition. The E2/M1 multipole mixing ratios determined are (energy in keV): δ(66) = 0.15 ± 0.15, δ(85) = 0.31 ± 0.05, δ(114) = 0.31 ± 0.05, 0.56 ≦ δ(179) ≦ 1.36, δ(1121) = 12⁺²_?1, and δ(1231) = ?(32⁺¹⁴²_?15). The measured M2/E1 mixing ratios are: δ(68) = 0.03 ± 0.02, δ(152) = 0.014 ± 0.013 and δ(156) = ?0.13 ± 0.19.     

810.6–863.6 keV γγ-directional correlation in58Fe

The 810.6–863.6 keV γγ-directional correlation has been measured with an NaI(Tl)-Ge(Li) detector system. The NaI window was set on the 810.6+863.6 keV composite peak. From the (810.6 NaI gate) (863.6 Ge spectrum) data at 90 °, 135 °, and 180 °, we deducedA ₂=+0.51±0.03 andA ₄=+0.09±0.04. These results disagree with the values previously obtained from⁵⁸Co decay (with Nal-NaI detector systems) but agree with the values from γγ(θ) studies following thermal neutron capture by⁵⁷Fe.     

The charge radii of198Pt-183Pt

The reactions⁵⁸Ni+¹⁰²Pd→¹⁶⁰W and⁵⁸Ni+¹⁰⁶Cd→¹⁶⁴Os were investigated to search for new decay data of neutron deficient nuclei. Excitation energies of the compound nuclei covered a range from 47 to 89 MeV. Velocity separation of the evaporation residues and position time correlations with the a decays of the implanted nuclei were used. The following new decay data were measured:¹⁶²Os (E_α=(6611 ±30) keV, T_1/2=(1.9±0.7) ms);¹⁵⁸W (T_1/2=(0.9±0.3) ms);¹⁵⁸m_W (E=1.88 MeV, E_α=(8280±30) keV, T_1/2=(0.01-1) ms);^155mLu (E_α=(5575±10) keV); β decay of¹⁵⁶Ta (T_1/2 > 10 ms) to the 8⁺ yrast isomer in¹⁵⁶Hf. A cross section of 5μb was measured for the new isotope¹⁵⁶Ta produced in a p3n evaporation channel from¹⁶⁰W at 64 MeV excitation energy.     

Measurement of partial radiation widths of high energy transitions from keV capture resonances in56Fe and58,60Ni

High energyγ-ray transitions to low-lying states following neutron capture in⁵⁶Fe and^58,60Ni have been investigated for individual resonances in the neutron energy range 7–70keV using a 50cc Ge(Li)-detector. Partial radiation widths fors- and 1>0 wave resonances were determined. For the 1>0 wave resonance in⁵⁸Ni at 47.8 keV a spin of 3/2 was derived. Theγ-ray strength forM1 transitions was found to be (21±17)×10^?9 and (16±7)×10^?9MeV^?3 for⁵⁶Fe and⁵⁸Ni, respectively. The partial radiation widths of the studieds-wave resonances were compared with valence model calculations.     

Measurements of γ-γ and γ-electron directional correlations in119Sb

The directional correlations ofγ-γ andγ-electron cascades in¹¹⁹Sb are measured, in the decay of^119mTe. Bothγ-γ andγ-electron directional correlation coefficients are determined for the cascades (energies in keV): 153.5-1212.7, 942.3-270.5, (976.2+979.3)-270.5, 1095.7-270.5 and 1136.8-270.5. For the cascades 912.6-1366.2, 2013.4-270.5 and 2089.9-270.5γ-γ directional correlations are measured. The mixing ratios evaluated are:δ(M2/E1, 153.5 keV)=0.0003±0.0023,δ(E2/M1, 270.5 keV)=-0.39±0.29,δ(E2/M1, 942.3 keV)= ?0.26±0.12,δ(E3/M2,1095.7 keV)=?0.01±0.07, andδ(M3/E2,1212.7 keV) =0.004±0.007. The result is compared with theoretical predictions.     

Multipole mixing ratios of transitions in175Lu populated from the decay of175Hf

Electron capture decay of¹⁷⁵Hf(70 d) provides a possibility for unambiguous determination of the sign and magnitude of multipole mixing ratios for 89 keV and 114 keV transitions in¹⁷⁵Lu. This is because both gamma rays are in coincidence with the 230 keV transition which is of a pureE2 character. The results of theγ —γ directional correlation measurements, in terms ofE2/M1 mixing ratiosδ, areδ ₈₉ = 0.11±0.07 andδ ₁₁₄ = 0.465±0.005. In addition the directional correlation measurements of the 89γ- 343γ and 319γ-114γ cascades yieldδ ₃₄₃ = 0.08±0.07 andδ ₃₁₉ = ?0.152±0.015.Radioactivity ¹⁷⁵Hf from¹⁷⁴Hf(n, γ); measuredγ —γ(θ) deducedδ(E2/M1); Ge(Li) detectors.     

Nuclear structure effect on internal conversion ofl-forbidden transitions in139La,141Pr and203Tl

Accurate experimental internal conversion data have been used to study the effect of nuclear penetration in the case of thel-forbidden transitions in¹³⁹La (165.8 keV),¹⁴¹Pr (145.4 keV) and²⁰³Tl (279.2 keV). The nuclear penetration parameterλ and theE2/M 1 mixing ratioδ ² have been deduced by graphical analysis. Following results were obtained:λ=2.8±1.3,δ ² =(8.4 _?8.4 ^+14.0 )·10^?4 for¹³⁹La,λ=1.2±0.6,δ ²=(4.8±0.5)·10^?3 for¹⁴¹Pr, andλ=6.4±1.1,δ ²=1.36±0.12 for²⁰³Tl.     

Spins of the levels and multipole mixing ratios of transitions in 125Sb determined from γ-γ directional correlation and polarization-directional correlation measurements

In order to resolve several discrepancies in spin assignments to levels in ¹²⁵Sb, directional correlations and polarization-directional correlations have been measured for several γ-γ cascades in ¹²⁵Sb populated from the decay of ¹²⁵Sn. Earlier results obtained from using NaI and Ge(Li) and NaI detectors were difficult to interpret due to the complex structure of the decay scheme. To improve the experimental situation, we have used two coaxial Ge(Li) detectors for the angular correlation measurements and a coaxial Ge(Li)-planar Ge(Li) combination for the polarization-directional correlations. Combination of the results of these measurements give unique spin assignments of $\text{11}\text{2}$^?, $\text{11}\text{2}$^?, $\text{9}\text{2}$⁺, $\text{11}\text{2}$⁺ and $\text{9}\text{2}$⁺ to the 1982 keV, 1890 keV, 1420 keV, 1089 keV and 1067 keV levels, respectively. The determined E2/M1 mixing ratios are : δ(470) = 0.010±0.027, δ(1067) = ?0.86±0.18, and δ(916) = ?0.02±0.01.     

Suche nach dem Isomer74mAs

An activity with the decay propertiesT _1/2=(8.0±0.3)sec andE _γ=(283±5)keV has been produced bySchardt andGoodman by proton irradiation of thin layers of evaporated⁷³Ge and⁷⁴Ge on thick gold backings. This activity was interpreted as the new isomer^74mAs. In the present experiment a search for^74mAs was carried out using the reactions⁷⁵As(n, 2n),⁷¹Ga(α, n) and⁷⁴Ge(d, 2n).^74mAs could not be detected. Upper limits for the reaction cross sections were determined. It is discussed that the reported properties of^74mAs resemble the known properties of^197mAu.     

Electric monopole component in the 2+' → 2+ transition in 192Pt

Angular correlation measurements of K- and L-conversion electrons following the decay ¹⁹²Ir → ¹⁹²Pt have been made using a spectrometer with Ge(Li) and Si (Li) detectors. Absolute and relative internal conversion coefficients of transitions in ¹⁹²Pt were measured, using an ICC and prism β-spectrometers, to ≈ 2 % and values of δ_γ determined from the relative ICC. The experimental values measured in the study, A₂₂(K296γ316) = 0.138 ± 0.010, A₂₂(L296γ316) = 0.125 ± 0.013, α_K(296) = 0.0711 ± 0.0011, K/L_III = 9.65 ± 0.13. With δ_γ = + 5.4 ± 0.2, were employed for determining the E0/E2 amplitude ratios of conversion transitions, q(E0/E2), and the penetration parameter λ of the Ml component for the 2⁺' → 2⁺ (296 keV) transition in ¹⁹²Pt. The angular correlation measurements of L-conversion electrons enabled the elimination of one of two ranges of values of q and λ usually obtained. For the first time in our work, analysis of the e_Lγ angular correlation for the determination of the E0 component in the transition was carried out. As a result, q = +0.04 ± 0.05 with λ = ?4.5 ± 3.5 was obtained for the 296 keV transition. In this case, _ρ(E0) = 0.004 ± 0.005 agrees with _ρ(E0) = +0.006 determined theoretically by Kumar and Baranger for the 2⁺' → 2⁺ transition     

Der Zerfall des 1,5 min-Isomers Co54m

Co^54m (T _1/2=1.43 min) was produced in iron-foils by irradiation with_dE=19 MeV deuterons. The gamma ray spectrum was investigated using a NaJ(Tl) scintillation spectrometer, a coincidence circuit and a Ge(Li)-counter. There were observed three gamma rays having the following energies and intensities per Co_54m decay: 411 keV (0.97±0.07), 1130keV (0.98±0.05), 1407 keV (1.00±0.05). The directional correlation between the pairs of gamma rays were determined. These results correspond to spin and parityJ _π=2⁺ for the 1407 keV,J _π=4⁺ for the 2537 keV, andJ _π=6⁺ for the 2948 keV energy level of Fe⁵⁴. The last-mentioned level was not excited in previous scattering experiments. Our results are compatible withE=210keV andJ _π=6⁺ or 7⁺ of the isomeric state of Co^54m .     

Nuclear resonance fluorescence in94Mo,95Mo and96Mo

Using gaseous sources of Tc₂O₇ containing the radioactive isotopes⁹⁴Tc,⁹⁵Tc and⁹⁶Tc, levels at 871.0keV (⁹⁴Mo), 765.8, 820.6, 947.8, 1074.0keV (⁹⁵Mo) and 778.3keV (⁹⁶Mo) have been excited. From the effective cross sections for nuclear resonance scattering and from the lifetimes of the 947.8, 1074.0 and 778.3keV levels known from Coulomb excitation experiments the profiles of theγ-lines have been determined. A broadening of theγ-lines due to Coulomb explosion of the molecules has been observed. Making use of the line profiles, lifetimes ofΤ=(6.4±1.0) ps andΤ=(0.90 ± 0.20) ps have been determined for the 765.8 and 820.6keV levels, respectively. The angular distribution of the resonantly scattered radiation yields an amplitude ratioδ for the mixed M1 E2 765.8keV transition ofδ=0.14 _?0.009 ^+0.08 . TheB(E2) from a Coulomb excitation experiment and the lifetimeΤ from the present experiment yield ¦δ¦=0.07±0.01 for the 820.6keV transition.     

Nuclearg-factors of the first excited states in Ir191 and Ir193

Mössbauer experiments were performed to determine the nuclearg-factor of the 82 keV 1/2⁺ state in Ir¹⁹¹ (g=+1.083±0.009) and the 73 keV 1/2⁺ state in Ir¹⁹³ (g=+0.9400±0.0019). TheE2/M1 mixing parameters of the corresponding (1/2⁺) (E2/M1) (3/2⁺) transitions were found to be ¦δ¦ (Ir¹⁹¹, 82 keV)=0.80±0.06 andδ(Ir¹⁹³, 73 keV)=?0.558±0.005.     

Investigation of neutron deficient nuclei in the region 28<N,Z <50 with the help of heavy ion compound reactions

In-beamγ ray spectroscopy withγ singles spectra,γγ coincidences andγ ray angular distributions has been performed with several target-projectile combinations:^natCa +³²S,^natCa +⁴⁰Ca,⁵⁴Fe +¹⁴N,⁵⁸Ni +¹²C,⁵⁸Ni +¹⁴N,⁶⁶Zn +¹⁶O,⁶⁸Zn +¹⁶O. Level schemes of⁶⁶Ge,⁶⁸Ge,⁶⁹As,⁷⁰Se,⁷⁴Kr,⁸⁰Sr and⁸²Sr have been deduced. The following level energies and spin-parity assignments have been found:⁶⁶Ge: 957.4 keV, 2⁺; 1693.7; 2174.7, (4⁺); 3685.7; 4207.5;⁶⁸Ge: 1015.8, 2⁺; 1777.9, 2⁺; 2267.9, 4⁺; 2428.8, 3(⁺); 2649.1, 3^?; 3582.3, (5^?); 3649.3, (5^?); 3696.2, (6⁺); 3883.3, (6^?); 4054.4, (7^?); 4454.6; 4837.3;⁶⁹As: 98.2; 164.6;789.6;863.2; 1306;2160;2210.4;2831.5;3258.3;3263.5;3991.1;5195.7;⁷⁰Se: 945.4, 2⁺; 1600.9; 2039.4, (4⁺);⁷⁴Kr: 455.7, 2⁺; 1013.5, (4⁺); 1781.5;⁸⁰Sr: 385.4, 2⁺; 980.2, (4⁺); 1763.2, (6⁺);⁸²Sr: 573.4, 2⁺; 1328.5,(4⁺); 2229.6,(6⁺). γ ray activity spectra have been measured after the bombardment of natural Ca with³²S. The half-life of the new isotope⁶⁹Se has been found to be 27±3 sec. Recoil distance Doppler-shift measurements have been performed with the reactions^62,64Ni,⁶⁶zn(¹⁶O, 2n)^{76, 78} Kr,⁸⁰Sr. The following half-lives have been determined:⁷⁶Kr: 423.8 keV, 2⁺, 37±5 psec; 1034.2,4⁺, 5.7±1.6;⁷⁸Kr: 455.3, 2⁺, 25±3; 1120.0, 4⁺, 3.8±1;⁸⁰Sr: 385.4, 2⁺, 44±6. The energy and half-life systematics of the first excited state of even-even nuclei suggest a maximum of nuclear deformation in the region 28≦N, Z≦50 near ₃₈ ⁷⁶ Sr₃₈ or ₄₀ ⁷⁸ Zr₃₈.     

Nuclearg factors of the first and second 2+ states in192,194Pt

Theg factors of the first and second excited 2⁺ states in¹⁹²Pt and¹⁹⁴Pt have been measured using γ-γ angular correlations perturbed by the hyperfine field in an iron lattice. Bulk magnetizations of sources were examined with special care for different shapes of alloys and different magnetizing conditions. The following results have been obtained:¹⁹²Pt: 316 keV stateg=0.346±0.024, 612 keV stateg=0.455±0.089.¹⁹⁴Pt: 328 keV stateg=0.354±0.031, 622 keV stateg=0.316±0.029. These values are the largest ones which have been reported so far. The discrepancies between the present and previous data are discussed especially in terms of magnetizing conditions for the sources used. It is suggested that the difference ing factor between the first and second 2⁺ states may be in a certain correlation with M1 matrix element connecting these two states.     

g-Faktoren und Multipol-Mischungsverhältnisse in156Gd

By integral perturbedγ-γ-angular correlation the gyromagnetic ratios of a 2-quasi-particle state at 1,513 keV and the 4⁺ state of the ground state rotational band in¹⁵⁶Gd were measured, using sources prepared by¹⁵⁹Tb(γ, 3n) and¹⁵⁶Gd(d, 2n) reactions:g _{1;513 keV} ⁴⁺ =0.78±0.05;g _R ⁴⁺ =0.37±0.05. In addition we obtain the multipole mixing ratiosδ _{535 keV}(M2/E1)=?0.09±0.01;δ _{1,225 keV}(E2/M1)=+1.83±0.10 for the 535 keV and 1,225 keVγ-rays. The classification of the 1,513 keV state is discussed. The internal field of Gd in Tb metal at 77 °K was found to beH=(?192±16)kOe.     

Measurement of thes-wave contribution to 2p-level shifts in pionic atoms

Energies and widths of pionic 3d-2p transitions of₃₀Zn,₃₂Ge, and₃₃As have been measured with a Ge detector. The values of the 2p shifts obtained from the measurementε _2p (Zn)=7.0±1.4keV,ε _2p (Ge)=5.5±0.9keV, andε _2p (As)=4.6±0.9keV show a decreasing behaviour for largeZ, which is caused by an increasings-wave contribution as predicted by theory.