Polarization detection of trapped electrons via interaction with polarized atoms

Electrons were trapped in an electrostatic quadrupole trap with superimposed homogeneous magnetic field. The electrons were polarized by spin exchange with a polarized atomic beam. The free trapped electron polarization was converted to a change in the electron translational energy via spin-dependent inelastic collisions with the atomic beam, and the electron translational temperature was monitored. Discussed are the development of this variation of the measurement technique, characteristics of electron storage, and the electron-polarized atom inelastic interaction as a function of electron temperature and time. The method has been applied to the detection of the (g-2) resonance of free, stored electrons.     

Optically detected electron resonance in phosphorus-doped ZnTe

Samples of ZnTe showing near gap edge luminescence predominantly due to exciton recombination at shallow neutral acceptors and donor- acceptor pair recombination have been investigated using optically detected magnetic resonance (ODMR). Emission polarization changes at 2.318 eV were observed due to magnetic resonance of electrons at g_e = + 0.401 ± 0.004. The observations are consistent with the donor trapped electron resonance resulting from microwave induced changes in donor-acceptor pair photoluminescence.     

Effect of CDW and magnetic interactions on the electrons of the manganite systems

We address a model study which includes the co-existence of the charge density wave (CDW) and ferromagnetic interactions in order to explain the colossal magnetoresistance (CMR) in manganites. The Hamiltonian consists of the ferromagnetic Hund's rule exchange interaction between e_g and t_2g spins, Heisenberg core spin interactions and the CDW interaction present in the e_g band electrons. The core electron magnetization, induced e_g electron magnetization and the CDW gap are calculated using Zubarev's Green's function technique and determined self-consistently. The effect of core electron magnetization and the CDW interaction on the induced magnetization as well as on the occupation number in the different spin states of the e_g band electrons are investigated by varying the model parameters of the system like the CDW coupling, the exchange coupling, the Heisenberg coupling and the external field. It is observed that the induced magnetization exhibits re-entrant behaviour and exists within a narrow temperature range just below the Curie temperature. This unusual behaviour of the e_g band electrons will throw some new insights on the physical properties of the manganite systems.     

Spin resonance associated with itinerant electrons affected by the injected spin current

The effect of spin injection on the spin resonance associated with itinerant electrons in a nonmagnetic semi-conductor has been studied within the phenomenological approach. The power absorbed under the resonance conditions has been analyzed as a function of the frequency, effective g-factor, and magnetic field direction. It is shown that the power absorbed by the spin-polarized charge carriers under the resonance conditions can provide a tool for studying the spin injection.     

<Superscript>55</Superscript>Mn spin relaxation with the participation of mobile carriers in doped perovskites

Analytical expressions are derived for the rates of longitudinal and transverse nuclear spin relaxation under conditions of fast modulation of the magnitude and direction of a hyperfine field induced by unpaired electrons of an ion. The results obtained are used to explain the data available in the literature on the ⁵⁵Mn spin relaxation in the ferromagnetic metallic phase of doped perovskites, in which the modulation of the hyperfine field is caused by the hopping of e _g electrons between Mn³⁺ and Mn⁴⁺ ions. It is demonstrated that, within this model, the rates of longitudinal and transverse relaxation are characterized by the same temperature dependence and their ratio is independent of temperature, which is in agreement with the experimental data.     

Spin-wave dispersion softening in the ferromagnetic Kondo lattice model for manganites

Spin dynamics is calculated in the ferromagnetic (FM) state of the generalized Kondo lattice model taking into account strong on-site correlations between e_g electrons and antiferromagnetic (AFM) exchange among t_2g spins. Our study suggests that competing FM double-exchange and AFM super-exchange interaction lead to a rather nontrivial spin-wave spectrum. While spin excitations have a conventional Dq² spectrum in the long-wavelength limit, there is a strong deviation from the spin-wave spectrum of the isotropic Heisenberg model close to the zone boundary. The relevance of our results to the experimental data are discussed.     

E.S.R. of sulphur-substituted purines and nucleosides; carbon-centred radicals in mercaptopurine crystals at 77 K

Single crystals of the sulphur-containing DNA-base analogue 6-methylmercaptopurine (6MeMP) and its riboside 6-methylmercaptopurine riboside (6MeMPR) have been prepared and irradiated by 4·0 MeV electrons at 77 K. Electron spin resonance techniques have been used to study the radiation-induced radicals at 77 K. The primary carbon-centred radical, common to both molecules, has been identified as a species formed by hydrogen atom abstraction from the methyl group. The principal values of the two α-proton hyperfine coupling tensors and the g-tensors were almost the same for both molecules and for 6MeMPR were: α1, -28·8, -17·9 and -6·4 G; α2, -28·2, -15·7 and -9·8 G; and g, 2·0063, 2·0024 and 2·0018. These data indicate a spin density of 0·77 on the methyl carbon atom. Molecular orbitals determined from CNDO/2 methods were used in calculations of the directions and magnitude of the g-tensor principal values. Comparison of these calculated values and experimental data suggests that contribution of spin density in d-orbitals on the sulphur atom is important in describing the g-tensor. Methyl H-abstraction radicals trapped in pairs were also detected in 6MeMP and the data are consistent with an effective interspin distance of 4·67 Å.     

The influence of phonons on the optical properties and the conductivity of quasi-one-dimensional metals

The frequency dependent conductivity σ(ω) completely taking into account the interaction between electrons is studied. The shape and the temperature dependence of optical absorption near the frequency of a molecular phonon activated due to the interaction with electrons are found. For a system with attractive sign of the e-e backward scattering amplitude g₁<0 an absorption edge near the gap 2Δ in the electronic spectrum is studied. A low frequency conductivity is discussed. The properties under consideration depend essentially on the magnitudes of e-e interactions and are critical to the sign of g₁.     

Resonant Bhabha scattering at MeV energies

We discuss, on a phenomenological level, the possible appearance of resonances ine ⁺+e ^? scattering at energies in the MeV region. The expected resonance cross section and angular distribution are examined. The observability depends crucially on the attainable energy resolution which is limit by the momentum distribution of the electrons contained in the target.     

Photoelectron spectra of substituted benzenes: II. Seven valence electron substituents

The He I photoelectron spectra of the isoelectronic series of substituted benzenes toluene, aniline, phenol, and fluorobenzene have been measured and the ionization bands in the low binding energy region of the spectra have been identified and assigned. The spectrum of pentafluoroaniline has also been obtained in order to use the “perfluoro effect” to identify the lowest energy σ ionization band. The photoelectron bands were assigned by using a “composite molecule” approach in which the known levels of benzene and the various substituents are correlated with those of the molecule, by using information supplied by vibrational analysis of the bands, and by reference to CNDO/2 and INDO MO calculations. The spectra of these composite molecules are consistent with the … 1a_2u(π), 3e_2g(σ), 1e_1g(π) MO configuration of benzene. The e_1g(π) orbital is split into two components in all of these substituted benzenes. Vibrational progressions in the ring CC stretching and the X-sensitive modes have been identified in these π ionization bands. Excitation of these two modes is evidence for delocalization of the π electrons over the composite molecule. The n (nonbonding) orbital of the substituents is shown to occur in the penultimate region along with the 1a_2u(π) and 3e_2g(σ) orbitals. The shifts in the n and π orbitals between the composite molecules and their constituent molecules are discussed in terms of resonance and inductive effects.     

Eine PrÄzisionsmessung des VerhÄltnisses der Spinresonanzfrequenz von Protonen zur Zyklotronfrequenz freier Elektronen im gleichen Magnetfeld

A new precision measurement of the ratio of the proton NMR frequency to the cyclotron frequency of free electrons in the same magnetic field, Ω _p /Ω_e=γ _p mc/e, has been performed. A cyclotron resonance linewidth of 5 ppm only and a reduction of the large space charge shifts, amounting up to the order of 50 ppm in earlier published measurements, enabled a high accuracy. The final result is Ω _p /Ω _e =1.5209945×10^?3±0.5 ppm, where the NMR is referred to a long cylindrical sample of H₂O, 0.2 m CuSO₄. Corrected to the free proton, we get Ω _p /Ω _e =1.5210329×10^?3±0.6 ppm. Combination of our result with an EPR-measurement ofLambe yields a free electrong-factor ofg=2(1+(α/2π)?(0.30±0.09) (α/π)²) in good agreement with the theoretical valueg=2(1+(α/2π)?0.328(α/π)²±...).     

Spin dependent surface recombination in silicon p-n junctions: The effect of irradiation

We present the results of an investigation of spin dependent recombination in (100) oriented, gate controlled Si diodes irradiated by 30 keV electrons. After irradiation, recombination at the SiSiO₂ interface is increased, and saturation of the spin resonance increases the diode forward current by 5 parts in 10⁴. The results cannot be described by a conventional Shockley-Read recombination model. An alternative picture is proposed involving recombination between trapped electrons and trapped holes.     

Quantum interference effects in a multi-driven transition Fg = 3 ↔ Fe = 2

We calculated and studied the quantum coherence effects of a degenerate transition F_g = 3 ↔ F_e = 2 system interacting with a weak linearly polarized (with σ_± components) probe light and a strong linearly polarized (with σ_± components) coupling field. Due to the competition between the drive Rabi frequency and the Zeeman splitting, electromagnetically induced transparency (EIT) and electromagnetically induced absorption (EIA) are appeared at the different values of applied magnetic field in both cases that the Zeeman splitting of excited state Δe is smaller than the Zeeman splitting of ground state Δg (i.e., Δe < Δg) and Δe > Δg. It is shown that the resonance is broader and contrasts are higher for Δe < Δg than that for Δe > Δg at the same Rabi frequencies of probe and coupling fields.     

Temperature-dependent photoluminescence in La2/3Ca1/3MnO3

Visible photoluminescence and its temperature dependence of La_2/3Ca_1/3MnO₃ in the temperature range 138-293 K were measured. It was observed that the main broad band centered at ∼1.77 eV with the shoulders at ∼1.57 and ∼1.90 eV existed in the entire temperature range. It can be well fitted by three Gaussian curves B₁, B₂ and B₃ centered at ∼1.52, ∼1.75 and ∼1.92 eV, respectively. The intensities of the peak B₁ and B₂ vary as temperature increases. In the entire temperature range, the intensity of B₁ increases with increasing temperature, whereas that of B₂ decreases. The photoluminescence mechanisms for La_2/3Ca_1/3MnO₃ are presented based on the electronic structures formed by the interactions among spin, charge and lattice, in which B₁ was identified with the charge transfer excitation of an electron from the lower Jahn-Teller split e_g level of a Mn³⁺ ion to the e_g level of an adjacent Mn⁴⁺ ion, B₂ is assigned to the transition between the spin up and spin down e_g bands separated by Hund's coupling energy E_J and B₃ is attributed to the transition, determined by the crystal field energy E_C, between a t_2g core electron of Mn³⁺ to the spin up e_g bands of Mn⁴⁺ by a dipole allowed charge transfer process.     

Vector boson in the constant electromagnetic field

The propagator and the complete sets of in-and out-solutions of the wave equation, together with the Bogoliubov coefficients relating these solutions are obtained for the vector W-boson (with the gyromagnetic ratio g=2) in a constant electromagnetic field. When only the electric field is present, the Bogoliubov coefficients are independent of the boson polarization and are the same as for the scalar boson. For the collinear electric and magnetic fields, the Bogoliubov coefficients for states with the boson spin perpendicular to the field are again the same as in the scalar case. For the W ^? spin parallel (antiparallel) to the magnetic field, the Bogoliubov coefficients and the one-loop contributions to the imaginary part of the Lagrange function are obtained from the corresponding expressions for the scalar case by the substitution m ² → m ²+2eH (m ² → m ²-2eH). For the gyromagnetic ratio g=2, the vector boson interaction with the constant electromagnetic field is described by the functions that can be expected by comparing the scalar and Dirac particle wave functions in the constant electromagnetic field.     

Photoproduction of Triplets on Free Electrons and the Search for the Dark Photon

We have investigated the photoproduction of triplets on free electrons, γe^– → e⁺e^–e^–, in which dark photon A′ can be formed as an intermediate state with subsequent decay into an e⁺e^– pair. This effect appears as a result of the so-called kinetic mixing and is characterized by the small parameter describing the intensity of the interaction of the dark photon with charged Standard Model (SM) particles in terms of electric charge e. The search for a manifestation of A′ in this process is advantageous since the background to the A′ signal is purely electrodynamic and, hence, can be calculated with the required accuracy. We calculate this background taking into account the identity of final electrons. As regards A′, its contribution is taken into account only in Compton-type diagrams (of virtual Compton scattering) in which a virtual dark photon is a time-like particle and its propagator has the form of a Breit–Wigner resonance. It is only in the vicinity of resonance that A′ can be manifested. We calculate the invariant mass distribution of both e⁺e^– pairs formed in the process and analyze the kinematic region in which relatively small squares of momenta transferred from the target electron to the formed electrons are excluded. In these conditions, the contribution to the differential cross section from Compton-type diagrams is not suppressed relative to the contribution of the remaining (Borsellino) diagrams. A number of limitations on parameter depending on the dark photon mass and the statistics (number) of events are obtained for a special method of gathering events in which the invariant mass of one e⁺e^– pair remains fixed and of the other pair is scanned.     

Paramagnetic resonance in irradiated Sr(NO3)2 single crystal

Paramagnetic resonance absorption of centres with spin 1/2 centered aboutg=2 is reported in gamma-irradiated single crystals of Sr(NO₃)₂. At room temperature four centres are detected which appear to exhibit axial symmetry about the [111] crystal direction. Two of the observed centres have a resolved hyperfine structure of N¹⁴. This hyperfine structure and axial symmetry of the centres indicate that they could be irradiation products of the nitrate ion. To find the number of trapped electrons, a simplified calculation of the molecular orbitals of planar and pyramidal NO₃ is carried out. Centres with a resolved hyperfine structure are then identified as pyramidal NO ₃ ^? and a NO₂ molecule rotating about the [111] direction. Two centres without hyperfine structure are not identified exactly.     

Simple model for spin-crisis

Starting from the additive quarkSU(6) model and taking into account the pion and kaon (η) emission during the initial stage of evolution (fromq ²～m _quark ² toq ²～1 GeV²) we convert the main fraction of the proton spin into the orbital momentum of the pseudoscalar mesons. The results are in a good agreement with the experimental data. We get ∫g ₁(x)dx=0.152 for proton and +0.007 for the Λ hyperon (i.e. the quarks carry out only about 39% of the Λ spin). In the same model we explain the violation of the Gottfried sum rule ?∫(F ₂ ^p(x)?F ₂ ⁿ(x))dx=0.23 due to the charged meson exchanges at the beginning of the evolution. The Gribov-Lipatov relation between the polarized structure functions in DIS ande ⁺ e ^?-annihilation is discussed. It gives the possibility to study the spin structure of Λ hyperon produced through the decay of the jet originated by a polarized quark ine ⁺ e ^?-annihilation or in DIS.     

Interface contributions to the spin-orbit interaction parameters of electrons at the (001) GaAs/AlGaAs interface

One-body mechanisms of spin splitting of the energy spectrum of 2D electrons in a one-side doped (001) GaAs/Al _x Ga_{1 ? x} As quantum well have been studied theoretically and experimentally. The interfacial spin splitting has been shown to compensate (enhance) considerably the contribution of the bulk Dresselhaus (Bychkov-Rashba) mechanism. The theoretical approach is based on the solution of the effective mass equation in a quasi-triangular well supplemented by a new boundary condition at a high and atomically sharp hetero-barrier. The model takes into account the spin-orbit interaction of electrons with both bulk and interfacial crystal potential having C _2v symmetry, as well as the lack of inversion symmetry and nonparabolicity of the conduction band in GaAs. The effective 2D spin Hamiltonian including both bulk and interface contributions to the Dresselhaus (α_BIA) and Rashba (α_SIA) constants has been derived. The analytical relation between these constants and the components of the anisotropic nonlinear g-factor tensor in an oblique quantizing magnetic field has been found. The experimental approach is based, on one hand, on the detection of electron spin resonance in the microwave range and, on the other hand, on photoluminescence measurements of the nonparabolicity parameter. The interface contributions to α_BIA and α_SIA have been found from comparison with the theory.