Evidence for a transition in the pairing symmetry of the electron-doped cuprates La(2-x)Ce(x)CuO(4-y) and Pr(2-x)Ce(x)CuO(4-y)

We present measurements of the magnetic penetration depth, lambda(-2)(T), in Pr(2-x)Ce(x)CuO(4-y) and La(2-x)Ce(x)CuO(4-y) films at three Ce doping levels, x, near optimal. Optimal and overdoped films are qualitatively and quantitatively different from underdoped films. For example, lambda(-2)(0) decreases rapidly with underdoping but is roughly constant above optimal doping. Also, lambda(-2)(T) at low T is exponential at optimal and overdoping but is quadratic at underdoping. In light of other studies that suggest both d- and s-wave pairing symmetry in nominal optimally doped samples, our results are evidence for a transition from d- to s-wave pairing near optimal doping.     

Inhomogeneous electronic structure probed by spin-echo experiments in the electron doped high-Tc superconductor Pr1.85Ce0.15CuO4-y

63Cu nuclear magnetic resonance spin-echo decay rate (T-12) measurements are reported for the normal and superconducting states of a single crystal of Pr(1.85)Ce(0.15)CuO(4-y) in a magnetic field B(0)=9 T over the temperature range 2相似文献   

Magnetic penetration depth measurements of Pr2-xCexCuO4-delta films on buffered substrates: evidence for a nodeless gap

We report measurements of the inverse squared magnetic penetration depth, lambda(-2)(T), in Pr(2-x)Ce(x)CuO(4-delta) (0.115< or =x < or =0.152) superconducting films grown on SrTiO3 (001) substrates coated with a buffer layer of insulating Pr2CuO4. lambda(-2)(0), T(c), and normal-state resistivities of these films indicate that they are clean and homogeneous. Over a wide range of Ce doping, 0.124< or =x < or =0.144, lambda(-2)(T) at low T is flat: it changes by less than 0.15% over a factor of 3 change in T, indicating a gap in the superconducting density of states. Fits to the first 5% decrease in lambda(-2)(T) produce values of the minimum superconducting gap in the range of 0.29< or =Delta(min)/k(B)T(c)< or =1.01.     

Fermi-liquid ground state in the n-type Pr(0.91)LaCe(0.09)CuO(4-y) copper-oxide superconductor

We report nuclear magnetic resonance studies on the low-doped n-type copper-oxide Pr(0.91)LaCe(0.09)CuO(4-y) (T(c)=24 K) in the superconducting state and in the normal state uncovered by the application of a strong magnetic field. We find that when the superconductivity is removed the underlying ground state is the Fermi liquid state. This result is at variance with that inferred from previous thermal conductivity measurement and appears to contrast with that in p-type copper oxides with a similar doping level where high-T(c) superconductivity sets in within the pseudogap phase. The data in the superconducting state are consistent with the line-node gap model.     

Evidence for a quantum phase transition in Pr2-xCe(x)CuO4-delta from transport measurements

The doping and temperature dependences of the Hall coefficient, R(H), and ab-plane resistivity in the normal state down to 350 mK is reported for oriented films of the electron-doped high-T(c) superconductor Pr(2-x)Ce(x)CuO(4-delta). The doping dependences of beta (rho=rho(0)+ATbeta) and R(H) (at 350 mK) suggest a quantum phase transition at a critical doping near x=0.165.     

Specific heat of the electronic superconductor Pr1.85Ce0.15CuO4

We have investigated the specific heat of the ceramic Pr_1.85Ce_0.15CuO₄ in the temperature range 2–800K in magnetic fields up to 8 T. We have determined the magnitude of the specific-heat discontinuity at the superconducting transition ΔC/T _c and estimate the coefficient of the electronic specific heat. In the temperature interval 5–800K we have separated out the phonon contribution to the specific heat, determined the temperature dependence of the characteristic Debye temperature Θ, and calculated the mean frequencies (moments) of the phonon spectrum. We compare the parameter values obtained in this way with data for the compound La_1.85Sr_0.15CuO₄ having similar crystal structure, but hole conductivity. The magnitude of the specific-heat discontinuity and consequently the effective electron mass in the “electronic” superconductor Pr_1.85Ce_0.15CuO₄ is several times smaller than in the “hole” superconductor La_1.85Sr_0.15CuO₄. The phonon spectrum in Pr_1.85Ce_0.15CuO₄ in the low-energy region is somewhat “more rigid,” and in the high-energy region somewhat “softer” than in La_1.85Sr_0.15CuO₄. Fiz. Tverd. Tela (St. Petersburg) 41, 1154–1159 (July 1999)     

Direct observation of a nonmonotonic dx2-y2- wave superconducting gap in the electron-doped high-Tc superconductor Pr0.89LaCe0.11CuO4

We performed high-resolution angle-resolved photoemission spectroscopy on electron-doped high-Tc superconductor Pr0.89LaCe0.11CuO4 to study the anisotropy of the superconducting gap. The observed momentum dependence is basically consistent with the dx2-y2- wave symmetry, but obviously deviates from the monotonic dx2-y2- gap function. The maximum gap is observed not at the zone boundary, but at the hot spot where the antiferromagnetic spin fluctuation strongly couples to the electrons on the Fermi surface. The present experimental results suggest the spin-mediated pairing mechanism in electron-doped high-Tc superconductors.     

Dirty superconductivity in the electron-doped cuprate Pr(2-x)Ce(x)CuO(4-delta): tunneling study

We report a tunneling study between Pr(2-x)Ce(x)CuO(4-delta) and lead as a function of doping, temperature, and magnetic field. The temperature dependence of the gap follows the BCS prediction. Our data fit a nonmonotonic d-wave order parameter for the whole doping range studied. From our data we are able to conclude that the electron-doped cuprate Pr(2-x)Ce(x)CuO(4-delta) is a weak-coupling BCS dirty superconductor.     

Evidence for two energy scales in the superconducting state of optimally doped (Bi,Pb)2(Sr,La)2CuO6+delta

We use angle-resolved photoemission spectroscopy to investigate the energy gap(s) in (Bi,Pb)2(Sr,La)2CuO6+delta. We find that the spectral gap has two components in the superconducting state: a superconducting gap and pseudogap. Differences in their momentum and temperature dependence suggest that they represent two separate energy scales. Spectra near the node reveal a sharp peak with a small gap below T(c) that closes at T(c). Near the antinode, spectra are broad with a large energy gap of approximately 40 meV above and below T(c). The latter spectral shape and gap magnitude are almost constant across T(c), indicating that the pseudogap state coexists with the superconducting state below T(c), and it dominates spectra around the antinode. We speculate that the pseudogap state competes with the superconductivity by diminishing spectral weight in antinodal regions, where the superconducting gap is largest.     

Phase-sensitive order parameter symmetry test experiments utilizing Nd(2-x)Ce(x)CuO(4-y)/Nb zigzag junctions

Phase-sensitive order parameter symmetry test experiments are presented on the electron-doped high-T(c) cuprate Nd(2-x)Ce(x)CuO(4-y). These experiments have been conducted using zigzag-shaped thin film Josephson structures, in which the Nd(2-x)Ce(x)CuO(4-y) is connected to the low-T(c) superconductor Nb via an Au barrier layer. For the optimally doped as well as for the overdoped Nd(2-x)Ce(x)CuO(4-y), a clear predominant d(x2-y2)-wave behavior is observed at T=4.2 K. Both compounds were also investigated at T=1.6 K, presenting no indications for a change to a predominant s-wave symmetry with decreasing temperature.     

稀土元素(Ce/Pr/Nd)掺杂Mn_4Si_7的第一性原理计算

利用第一性原理,对稀土元素Ce、Pr或Nd掺杂Mn_4Si_7前后的几何结构、电子结构和光学性质进行了计算与分析.结果表明,掺杂后Mn_4Si_7晶格常数变大,禁带宽度明显减小,由于稀土元素特殊的4f层电子的影响,在费米能级附近出现了杂质能级.掺杂后Mn_4Si_7的介电函数虚部、吸收系数的主峰均出现红移,红外光区的光跃迁强度明显增强,光吸收系数和光电导率均增大.说明掺杂稀土元素Ce、Pr或Nd后改善了Mn_4Si_7在红外光区的光电性能.     

Crossing the gap from p- to n-type doping: nature of the states near the chemical potential in La(2)-(x)Sr(x)CuO(4) and Nd(2-x)Ce(x)CuO(4-delta)

We report on an x-ray absorption and resonant photoemission study on single crystals of the high-T(c) cuprates La2-xSrxCuO4 and Nd(2-x)Ce(x)CuO(4-delta). Using an intrinsic energy reference, we find that the chemical potential of La2-xSrxCuO4 lies near the top of the La2CuO4 valence band whereas in Nd(2-x)Ce(x)CuO(4-delta) it is situated near the bottom of the Nd2CuO4 conduction band. The data clearly establish that the introduction of Ce in Nd2CuO4 results in electrons being doped into the CuO2 planes. We infer that the states closest to the chemical potential have a Cu 3d(10) singlet origin in Nd(2-x)Ce(x)CuO(4-delta) and a 3d(9)L singlet origin in La2-xSrxCuO4.     

Magnetic field effect on the superconducting magnetic gap of Nd1.85Ce0.15CuO4

Inelastic neutron-scattering measurements on the archetypical electron-doped material Nd1.85Ce0.15CuO4 up to a high relative magnetic-field strength, H/H(c2) approximately 50%, reveal a simple linear magnetic-field effect on the superconducting magnetic gap and the absence of field-induced in-gap states. The extrapolated gap-closing field value is consistent with the upper critical field H(c2), and the high-field response resembles that of the paramagnetic normal state.