裂变位垒参数的推荐和裂变位垒参数库

通过分析和计算锕系核裂变截面和全套中子反应截面获取了一组锕系核的裂变位垒参数.Fm)在此基础上,广泛收集实验裂变位垒参数,通过比对和评价,推荐了本组的129个核素(109Cd—255的实验裂变位垒参数.此外,对收集的不同裂变位垒参数作了分析与评价,推荐了7组实验和1组模型计算的裂变位垒参数,并组建了中国评价核参数库裂变位垒参数子库(CENPL FBPL). The fission barrier parameters for actinide nuclei were obtained by analysis and calculations of fission cross-sections and complete neutron reaction cross sections. A lot of experimental fission barrier parameters from different authors were collected. A set of fission barrier parameters for 129 nuclei ranging from~(109)Cd~( ) to~(255)Fm were recommended after performing comparisons, evaluations and systematics extrapolations for these extracted fission barrier parameters in model calculations of fissi...     

核裂变扩散模型Kramers定态解的理论分析

在核裂变动力学扩散模型理论的框架内,严格求解Fokker-Planck方程.用所得到的结果对Kramers定态解进行了分析,指出其成功之处和存在的局限性.     

基于双核模型对准裂变产物质量分布的研究

在双核模型基础上引入一维的Kramers公式，计算了⁴⁸Ca+²⁴⁴Pu，⁴⁸Ca+²³⁸U和⁵⁸Fe+²³²Th这三个反应准裂变碎片的质量分布，得到了与实验比较符合的结果.同时提取出了碎片质量分布随时间的演化关系，为理解熔合与准裂变竞争过程提供了非常有用的信息.由于准裂变在重离子熔合反应中起着重要作用，理论计算与实验结果的比较是对现有熔合模型的重要检验. 关键词： 超重元素 熔合反应 准裂变产物 质量产额     

合成Z=119, 120超重核的理论研究

合成Z=119,120超重核是当今各核物理实验室争相追逐的目标,理论预言可靠的弹靶组合、入射能等信息有助于超重核合成的实验设计和探测。本工作基于双核模型研究影响重离子核反应生成截面大小的反应机制,计算了$^{50}{\rm{Ti}}$+$^{249}{\rm{Bk}}$、$^{50}{\rm{Ti}}$+$^{249}{\rm{Cf}}$两个弹靶组合,预测$^{50}{\rm{Ti}}$+$^{249}{\rm{Bk}}$的生成截面为0.021 1 pb。考虑双核系统熔合与存活两个过程,重点关注$^{52-59}{\rm{Cr}}$+$^{243}{\rm{Am}}$、$^{54-62}{\rm{Mn}}$+$^{243}{\rm{Am}}$、$^{56-72}{\rm{Ni}}$+$^{238}{\rm{U}}$生成截面的同位素链依赖性,研究表明熔合几率随弹核质量数呈现强烈的依赖行为,直接影响蒸发剩余截面大小。     

基于ImIQMD模型对近垒重系统准裂变反应的研究

利用改进的同位旋相关的量子分子动力学(ImIQMD)模型程序,对能量在库仑位垒附近的48Ca+208Pb反应系统进行了模拟。 计算得到的俘获截面、 准裂变截面和碎片分布及其发生的时间分布等结果与实验数据符合较好。 同时还得到了准裂变过程中发射第三个较大碎片的截面, 并简单讨论了它们的发射机制。Based on the improved isospin dependent quantum molecular dynamics (ImIQMD) model,the reaction of 48Ca+208Pb at energies near the Coulomb barrier was investigated systematically. The capture cross section,the quasi fission cross section, the mass distribution of the quasi fission fragments and the time for quasi fission happened were obtained. According to the comparison with experimental data,the calculated capture cross sections and the fragment distributions of the quasi fission were reasonable. Additionally,we got the cross sections of the third largest fragment,and the emission mechanism was also discussed briefly.     

中子诱发233,235,238U裂变机制的多通道理论研究

用改进的多通道和无规颈断裂模型,计算了能量E_n=0—6MeV的中子诱发²³³U、²³⁵U裂变和E_n=1.3—5.3MeV中子诱发²³⁸U裂变的碎片的质量分布、动能分布和瞬发中子数分布,理论计算在定量上与实验符合较好.     

n+233U裂变碎片质量分布的唯象模型研究

本模型基于裂变多通道无规颈断裂模型,考虑宏观液滴能、壳效应能以及壳效应与温度的关系,得到参数化的势能表示形式。通过拟合不同测量方法得到的实验数据(经过评价) 获得3 组模型参数。3 组参数计算的碎片质量分布均很好地再现了不同能点的实验数据,除了基于动能法实验数据得到的参数外,其14 MeV的计算结果与实验数据符合较差。研究发现,不同入射中子能量的裂变碎片质量分布有4 个主要交叉点,在叉点之上的产额随入射中子能量增加减少,之下的产额则随入射中子能量上升;内侧(或外侧) 的两个交叉点质量数之和近似等于裂变复合核的质量数;不同裂变系统的重峰左侧的交叉点都保持在132 附近。Present model was based upon Brosa model, where macro energy,shell effect energy and its decreasing with system temperature were considered and parameterized. 3 sets of model parameters were obtained by fitting to 3 groups of evaluated experimental data, respectively, where the groups were classified by measured method: radiochemistry (RA) method, double kinetic energy (KE) method, and both (ALL). All the 3 sets of parameters could well reproduce themeasured mass distributions on different energies, except the KE set on 14 MeV. The result shows the mass distributions mainly had 4 trend turning points, above which the yield decreasing and below which the yield increasing with energy.The sum of the 1st and 4th (or 2nd and 3rd) point positions was equal to the compound nuclei mass approximately. And the 3rd point was kept at ~132 constantly for different fission systems n+233 U, n+235U, n+233Pu.     

超重核292-310122同位素链的α衰变和自发裂变的竞争

基于推广的液滴模型(GLDM) 理论框架,计算了292-310122 同位素链的 衰变和自发裂变的半衰期。计算时的基本输入量为两子核的质量数和电荷数以及反应Q 值。GLDM能很好地描述重核和超重核的 衰变和自发裂变过程。计算结果表明,A < 308 时在同位素链上N = 176~184 的区域α衰变为主要衰变模式。A > 308 时在同位素链上自发裂变为主要衰变模式。308122 是α衰变和自发裂变的分界点,暗示着N = 184 为中子幻数。Based on the framework of the Generalized Liquid Droplet Model (GLDM), alpha decay and spontaneous fission half-lives for 292-310122 isotopes are studied. The calculation of the basic inputs which only need the two fragmentmass numbers, charge numbers and the Q value. GLDM can describe alpha decay and spontaneous fission the nuclei. It is found that the alpha decay is the dominant mode of decay for isotopes with mass number A < 308, and for those with A > 308 spontaneous fission is dominant. The demarcation between alpha decay and spontaneous fission is at 308122, which shows the presence of a spherical neutron shell closure at N = 184.     

裂变路径对断点前粒子发射的影响

用扩散模型研究了裂变系统从鞍点到断点的时间演化, 以及在此间的粒子发射与鞍点前粒子发射的比随着裂变系统质量的变化. 解释了实验上发现的断点前粒子多重性随裂变碎片质量不对称性的变化趋势. 结果表明上述两种变化趋势都可以归因于裂变演化路程长短的影响.     

角动量对基于裂变截面探测核耗散的影响（英文）

核耗散降低了裂变截面值(σdrop f)。基于Langevin模型,研究了角动量对σdrop f作为鞍点前摩擦强度β函数的影响。发现在低自旋,摩擦对σdrop1f的影响显著增强。通过考察系统95Bi,201Bi和207Bi的σdrop f随β的演化,发现摩擦效应随着Bi核中质比(N/Z)的增加而变大。这些结果建议,为了更好地在实验上用裂变截面探测β,应产生那些具有低自旋、高N/Z的热核系统。     

重离子周边碰撞和中心碰撞引起的不同裂变行为

本实验同时研究了4 0Ar+209Bi反应中周边碰撞和中心碰撞两者产生的关联裂变碎片,以及其与α粒子的再关联.对裂变碎片质量分布和能量分布随热裂变核初始温度演化的系统分析,发现中心碰撞和周边碰撞所形成的热核存在着不同的裂变行为. Correlated fission fragments from the 40Ar+209Bi reaction and their further correlation with α particles have been studied for peripheral and central collisions simultaneously. The existence of different fission behavior of hot nuclei formed in central and peripheral collisions was found from the systematic analysis of the mass and energy distributions of fission fragments as a function of the initial temperature of hot fissioning nuclei.     

推广的液滴模型及其应用

简单介绍了近年来在研究重核和超重核衰变性质及熔合反应方面取得的理论成果和面临的挑战,着重阐述推广的液滴模型(GLDM) 理论框架及其应用。基于原子核的质量数、质子数以及反应Q 值,GLDM考虑了质量和电荷的不对称性、形状演化、亲近势和温度等,很好地描述了重核和超重核的质子放射性、 衰变、重离子放射性、自发裂变的半衰期和重离子熔合反应截面,同时也研究了原子核的粒子(质子、 、重离子) 放射性与自发裂变的竞争。Recent theoretical achievements and challenges about the fusion and decay properties of heavy and superheavy nuclei are generally introduced. Especially, the Generalized Liquid Drop Model(GLDM) as well as its application are emphatically described. Based on the mass number, proton number and the reaction Q value, the GLDM has taken the mass and charge asymmetry, the shape evolution, the proximity potential, as well as the temperature of nucleus into account, well described the proton radioactivity, the decay, the heavy particle radioactivity, the half life of spontaneous fission of heavy nuclei and superheavy nuclei, and the cross-sections of heavy ion fusion. The competitions between the spontaneous fission and other decay modes such as proton and heavy particle radioactivity, the alpha decay, and so on are also studied.     

锕系原子核自发裂变性质的理论研究

运用推广的液滴模型（GLDM）来确定锕系原子核的自发裂变势垒, 采用量子力学中的WKB近似方法对相应自发裂变的半衰期进行了研究。 在GLDM中, 首次考虑了微观Strutinsky壳修正对裂变势垒的影响。 理论计算的锕系区重核自发裂变半衰期与实验值符合得很好, 表明包括微观壳修正的GLDM可以成功研究重核的自发裂变性质。 The spontaneous fission half lives of the actinides are calculated by the WKB approximation and the potential barriers are constructed by a General Liquid Drop Model (GLDM) including the proximity energy, the mass and charge asymmetry, and an accurate nucleus radius. The microscopic shell correction which plays a key role for the spontaneous fission barrier is considered for the first time. The two parameter quasi molecular shape and the proximity are described in details within the GLDM. The effects of the microscopic shell correction and proximity energy for fission barrier are discussed separately. The calcula ted spontaneous fission half lives for the actinides reasonably accord with the experimental data, implying the present GLDM combined with the microscopic shell correction can be used to study the spontaneous fission properties of heavy nuclei successfully.     

裂变碎片动能和质量分布的三维朗之万研究

采用一个具有协变形式的朗之万方程组来描述不对称热核裂变.基于核表面｛c,h,α｝三参数模型,用数值方法模拟了核系统从鞍点到断点的扩散过程,从而完成了碎片动能和质量分布的计算.研究了核的两体摩擦或一体耗散机制以及有限颈部作为核断裂条件对裂变碎片输出量的影响.     

近垒及垒下能区28Si+174Yb体系的裂变碎片质量分布

使用两块大面积平行板雪崩计数器,测量了近垒及垒下28Si+174Yb熔合裂变碎片质量-角度关联分布及质量分布。质量-角度二维图显示在该反应能量区间内并没有发现明显的准裂变成分。运用单高斯曲线拟合了裂变碎片的质量分布并抽取了质量宽度。结果表明:在库仑势垒以上,质量宽度随着反应能量的升高而增大;在库仑势垒以下能区,发现质量宽度随着反应能量的降低而呈现轻微增大的趋势。运用鞍点统计模型对本次实验数据拟合发现,需用比文献给出的更大的刚度系数才能重现实验结果,其物理原因还需要进一步研究。In order to study the fission mechanism, the mass distributions and mass-angle distributions of the fission fragments for 28Si+174Yb were measured near the Coulomb barrier. The mass-angle correlations do not indicate any possible quasi-fission events in this bombarding energy range. The mass distributions were fitted by the single Gaussian distribution and then the mass widths were extracted. At above-barrier energies, the mass widths were found to increase with the energy. However, the mass widths show slight increase with decreasing energy below the barrier. Additionally, the mass widths can not be reproduced in the framework of the saddle statistic model with the given parameter, so further study is still needed.     

40,48Ca+90,96Zr融合反应的动力学模型研究

应用改进的量子分子动力学模型,在严格挑选初始核考虑弹靶结构效应的基础上,研究了近垒和垒上融合反应^40,48Ca+^90,96Zr. 研究表明: 4个反应的理论计算截面与实验值很好符合; 丰中子反应⁴⁰Ca+⁹⁶Zr的垒下融合截面比其他3个反应有明显增强的现象.为了理解丰中子反应⁴⁰Ca+⁹⁶Zr与⁴⁰Ca+⁹⁰Zr相比垒下融合截面增强,而Ca+⁹⁶Zr垒下融合截面没有明显增强的原因, 进一步分析了484个反应的融合位垒,中子转移与融合位垒的关系、中子转移与Q值的关系,结果表明: 正反应Q值会引起核子(特别是中子)转移的增强,从而导致动力学融合位垒的下降和垒下融合截面增强.     

质子与裂变核238U反应的理论计算

利用球型光学模型、耦合道理论、核内级联、激子模型、蒸发模型、带宽度涨落修正的Hauser-Feshbach模型,Bohr-Wheeler裂变理论,对入射能量从阈能到200 MeV的p+²³⁸U各种反应进行了计算,计算结果和实验符合较好.     

利用改进的Glauber模型对非奇异核核反应总截面数据的拟合

在对反应总截面的理论计算中,现有的理论计算值与实验数据在高能区可以很好的符合，但在中能区理论值低于实验值约10％—20％.通过对计算核反应总截面的Glauber模型加入有限程修正，并对输入的核物质密度分布采用双参数的费米密度分布形式.计算结果表明，理论计算值对于没有奇异结构的核在低中能区和高能区，都与实验数据很好符合.     

反应窗理论的适用性研究

基于低能离子与原子碰撞的分子库仑过垒模型，简要描述了与入射离子速度相关的反应窗理论.根据这一理论，计算了不同碰撞速度时O⁸⁺-H，Ar⁸⁺-H，Ar⁸⁺-He，Ne¹⁰⁺-He及Ar¹⁸⁺-He等碰撞体系单电子俘获过程的微分截面，还计算了碰撞速度为0.53 a.u.时¹⁵N⁷⁺-Ne碰撞体系单电子、双电子及三电子俘获过程的微分截面，并与他人的实验结果作了比较.研究发现，反应窗理论预言的末态电子分布与实验结果符合较好.理论和实验研究表明，随着碰撞速度的增加反应窗变宽；反应窗理论所预言的微分截面，当Q值较小时比实验结果偏大，当Q值较大时比实验结果偏小. 关键词： 反应窗理论 态选择微分截面 分子库仑过垒模型 离子与原子碰撞