The decay of131Ba

The decay of¹³¹Ba has been studied by Ge(Li) detector supplemented by Ge(Li)-Ge(Li) fast-slow coincidence and NaI(Tl)-NaI(Tl) sum-coincidence spectrometer. The existence of 31 gamma rays and the levels at 78.8, 123.5, 133.4, 215.7, 373.0, 585.0, 620.0, 696.3 and 1084.4 keV have been confirmed. No evidences are found for the level at 1170 keV and 215.7?78.8 and 696.3?373.0 transitions. Some transitions are found to be connected with the impurities which were attributed to¹³¹Ba decay in earlier studies. The relative intensities and conversion coefficients have been determined and multipolarities of some of the transitions infered from the comparison of the conversion coefficients with the theoretical values.     

Levels and transitions in125Te

Gamma transitions and levels of¹²⁵Te following the decay of¹²⁵Sb have been studied using Ge(Li) detector and NaI(Tl)-NaI(Tl) sum-coincidence spectrometer incorporated with a fast-slow coincidence circuit. In all, twenty five gamma rays have been reported, out of which two weak gamma rays with energies 366·0 and 402·0 keV have been observed and confirmed for the first time. These gamma rays have been fitted by assigning a new level of 402 keV energy. An ambiguous transition of energy 122·1 keV has also been confirmed. No evidence was found for the existence of 145·9, 315·0, 489·8, and 497·4 keV transitions. The accurate intensities for various transitions have been determined.     

Der Zerfall des 1,5 min-Isomers Co54m

Co^54m (T _1/2=1.43 min) was produced in iron-foils by irradiation with_dE=19 MeV deuterons. The gamma ray spectrum was investigated using a NaJ(Tl) scintillation spectrometer, a coincidence circuit and a Ge(Li)-counter. There were observed three gamma rays having the following energies and intensities per Co_54m decay: 411 keV (0.97±0.07), 1130keV (0.98±0.05), 1407 keV (1.00±0.05). The directional correlation between the pairs of gamma rays were determined. These results correspond to spin and parityJ _π=2⁺ for the 1407 keV,J _π=4⁺ for the 2537 keV, andJ _π=6⁺ for the 2948 keV energy level of Fe⁵⁴. The last-mentioned level was not excited in previous scattering experiments. Our results are compatible withE=210keV andJ _π=6⁺ or 7⁺ of the isomeric state of Co^54m .     

Gamma-ray spectra and positive parity bands in 158Gd

A Ge(Li)-NaI(Tl) pair spectrometer and a Ge(Li)-NaI(Tl) anti-Compton spectrometer were used to measure γ-rays from the reaction ¹⁵⁷Gd(n, γ)¹⁵⁸Gd. A detailed decay scheme for levels of ¹⁵⁸Gd was constructed up to an excitation energy of 2504 keV. Branching ratios for transitions from members of the positive parity bands to members of the ground state band were determined. It is shown that a single band-mixing parameter is not sufficient to explain the experimental results, and that even a four-band-mixing calculation does not provide satisfactory agreement. The binding energy of the last neutron is determined to be 7937.4±0.7 keV.     

A high-resolution spectroscopic study of the gamma radiation from the decay of96Nb

The decay of 24h⁹⁶Nb has been studied with a Ge(Li) spectrometer and with a Ge(Li)-NaI(Tl) coincidence spectrometer. A total of 27 gamma-ray transitions were observed, their energies and intensities measured. All but one of these have been incorporated into the level scheme of⁹⁶Mo. The level at 1,625.9 keV reported recently in (n _th, γ) work on⁹⁵Nb has also been observed through the decay of⁹⁶Nb. No experimental evidence has been found for previously proposed levels at 2,657 and 2,791 keV in⁹⁶Mo.     

K conversion coefficients of transitions in87Sr

TheK conversion coefficients of the 388 and 483 keV transitions in⁸⁷Sr populated in the decay of⁸⁷Y have been measured with Ge(Li) and Si(Li) detectors by the NPG method. We find α _K values of 0.162 ± 0.010 and 0.00260 ± 0.00013 for the 388 and 483 keV transitions, respectively.     

Energy levels of174Yb populated in the decay of174Tm

The decay of the¹⁷⁴Tm activity has been studied with Ge(Li) detectors and with a Ge(Li)—NaI(Tl) coincidence arrangement. Gamma ray energies and relative intensities were determined. Five new gamma transitions are reported, four of which have been placed in the decay scheme in addition to the previously observed but unplaced 1305 keV transition. Five energy levels at 1557.7, 1762.1, 1781.1, 1877.5 and 2050.1 keV not earlier reported to be populated in the decay of¹⁷⁴Tm are suggested. Some spin and parity assignments are proposed and the intrinsic structure of several states is discussed in terms of two quasi-particle excitations. For the half-life of¹⁷⁴Tm a value 5.4±0.1 min was measured.     

Low-lying 134Cs excited states from the (n, γ) reaction

Low-energy γ-ray and conversion electron spectra from the ¹³³Cs(n,γ)¹³⁴Cs reaction have been investigated with a bent cyrstal spectrometer, β-speetrometer, Ge(Li) and Si(Li) detectors. Gamma-gamma coincidence measurements were made with the Ge(Li)-Ge(Li) arrangement. Gamma-gamma delayed coincidences have been studied with the use of the Ge(Li)-NaI(Tl) coincidence set-up. The decay of 2.9 h ^134mCs has been investigated with the prism β-spectrometer and Ge(Li) detector. The half-lives of the 176.403 and 257.112 keV levels have been measured to be 49.7 ± 0.8ns and 12.3 ± 1.1 ns respectively. The neutron binding energy B_n have been calculated to be 6891.4 ± 1.3 keV. Spin and parity assignments have been made for almost all the levels. The possible structure of the levels deduced is discussed.     

Anomalous conversion in the decay of197mHg

The total andK-shell conversion coefficients of the 165 keV transition in the decay of^197mHg are determined from intensity balance considerations and a coincidence technique using a Ge(Li)—NaI (Tl) system respectively. The resultant values area _T =274.8±19.2 anda _K =47±12, whil the corresponding theoretical values are 344 and 77 respectively, indicating anomalous conversion. The gamma ray transition probability however, shows a hindrance of only about 6 and cannot be correlated with the present anomalous conversion data. TheK/L ratio of the 130 keV transition, determined using a summing method with a Ge(Li) detector, yielded 0.090±0.012, while the corresponding theoretical value is 0.048, indicating anomalous conversion. The corresponding gamma transition probability shows a hindrance of about 3000, in correlation with anomalous conversion.     

Der Zerfall des Zn63

The decay of the 38.4 min-Zn⁶³ has been investigated using Ge(Li)-counters and a Ge(Li)-NaJ(Tl)-coincidence circuit. 43γ-transitions in the energy range from 364.5 keV to 3100.9 keV have been found and their relative intensities have been determined. A level scheme for Zn⁶³→Cu⁶³ having 24 levels is proposed. This accounts for all observedγ-transitions except one.     

A Si(Li) detector system for conversion coefficient measurements and application to the decays of51Cr and87Y

An electron detector system with a 3 mm × 100 mm² Si(Li) detector with a cooled FET and vacuum air lock for changing sources was constructed. The absolute efficiency was measured as a function of energy for use in the measurement ofK conversion coefficients. With the Si(Li) and a Ge(Li) detector, theK conversion coefficient of the 320 keV transition in⁵¹V was measured to be 0.00156 ± 0.00008 where theK conversion coefficients of the 661 and 279 keV transitions in¹³⁷Ba and²⁰³Tl were used as standards. From absolute detection efficiency measurements, theK conversion coefficients of the 388 and 483 keV transitions in⁸⁷Sr were measured to be 0.16 ± 0.02 and 0.0024 ± 0.0003, respectively.     

Decay of78Br

The decay of⁷⁸Br was investigated with a Ge(Li) spectrometer and Ge(Li)-NaI(Tl) coincidence methods. Accurate energy and intensity determinations of 14 gamma rays have been performed. A level scheme with levels at 614.0, 1,308.1, 1,498.4, 1,758.5, 1,993.7, 2,334.4, 2,538, 3,090 and 3,253 keV is deduced. Spin and parity indications for most of the observed levels are given from electron capture and positon decay considerations and gamma branches.     

The electron capture decay of 85gsr

In order to resolve the controversy concerning the existence of an 868 keV γ-transition in the decay of 65d ^85sSr and to determine the electron capture decay energy, radiochemically separated sources, Ge(Li), Ge(Li)-NaI(Tl), and NaI(Tl)-NaI(Tl) spectrometers have been used for singles and (X-ray-γ and γ-γ coincidence measurements. A γ-ray at 868.5±0.5 keV decaying with a 65±5 d half-life was conclusively identified in ^85gSr decay. From measurements of the ratio $\text{P}{}_{\mathrm{\kappa (868.5)}}\text{P}{}_{\mathrm{\kappa (514)}}$ of K-capture probabilities by (KX-ray-γ coincidences, a value of Q_EC was determined for the EC decay feeding the 868.5 keV transition. Thus, a level in ⁸⁵Rb is established at 868.5 keV, and an upper limit of 0.45 μsec is set on its lifetime.     

Decay of149Gd and directional correlations of gamma cascades in149Eu

The decay of¹⁴⁹Gd(9.4d) to the levels of¹⁴⁹Eu has been studied using large volume high resolution Ge(Li) and NaI(Tl) detectors,γ-γ coincidence and directional correlation experiments have been performed. Newγ-rays at energies 131.9, 278.6, 384.7, 415.7, 599.2, 726.5, 734.7, 956.4 and 1,231.1 keV in¹⁴⁹Eu have been observed. Three new levels in¹⁴⁹Eu have been placed at 956.4, 1,082.0 and 1,231.1 keV. Spin-parity assignments have been made to some of the levels in¹⁴⁹Eu. Multipolarity assignments have been made for most of the electromagnetic transitions from the conversion coefficients obtained through the knowledge of ourγ-transition intensities and the published conversion-electron intensities. Based on the newγ-transitions observed in the singles and coincidence spectra, a revised level scheme has been proposed for¹⁴⁹Eu and compared with previously published level schemes. Radioactivity¹⁴⁹Gd; measuredT _1/2,T _γ,γγ coin, γγ(θ), I.C.C.,¹⁴⁹Eu deduced levels,J,γ-mixing,π. Enriched targets, Ge(Li) detectors.     

The decay of208Tl. Gamma-ray measurement

The gamma rays following the decay of²⁰⁸Tl have been studied using a separated²⁰⁸Tl-source and a Ge(Li)-detector. A decay scheme is proposed, with levels in²⁰⁸Pb at 3,920, 4,126 and 4,180 keV in addition to previously well-established levels. No support was found forΒ-branching to levels above 4.2 MeV.     

The levels of144Pr from the decay of144Ce

The level scheme of¹⁴⁴Pr has been studied from the decay of¹⁴⁴Ce. The intensities and energies of gamma rays have been determined with a X-ray Ge(Li) detector. TheK-shell internal conversion coefficients for γ-rays have been measured with theK X-ray/γ-ray ratio method using NaI(Tl)—X-ray Ge(Li) coincidence techniques.     

Der radioaktive Zerfall des Fe61

Fe⁶¹(T _1/2=5.95 min) was produced irradiating Ni⁶⁴ and natural nickelfoils with fast neutrons in the reaction Ni⁶⁴(n, α)Fe⁶¹; Fe was chemical seperated. The gamma and beta spectrum were investigated with Ge(Li)-counters, NaJ(Tl) and plastic scintillation spectrometers. Fe⁶¹ emits five gamma rays having the energies and intensities per Fe⁶¹ decay: 121 keV (0.064), 177 keV (0.027), 298 keV (0.293), 1025 keV (0.461), 1202 keV (0.539). Threeγγ-cascades could be identified: 121–177 keV, 121–1202 keV, 298–1025 keV. Inγ β-coincidence measurements the maximal beta energy was determined:E _βmax=2.86 MeV. A decay sceme Fe⁶¹-Co⁶¹ was constructed: Fe⁶¹, spin and parityJ ^π=3/2^?, decays by means of allowed beta decay to three excited states of Co⁶¹: 1323 keV (1/2^?), 1202 keV (3/2^?), 1025 keV (5/2^?). The energies and intensities per Fe⁶¹ decay of the three beta decay modes are: 2.56 MeV (0.367), 2.68 MeV (0.495), 2.86 MeV (0.138). — A 88 keV gamma ray (T_1/2=33 sec) was observed coming from the Co⁶³ decay.     

A coincidence study of the decay of 35.8y150m Eu

The decay of 35.8y^150m Eu was studied with a Ge(Li) counter and a Ge(Li)-NaI(Tl) coincidence spectrometer. A total of 64 gamma rays were observed, their energies and intensities measured. A partial level scheme for¹⁵⁰Sm containing 24 energy levels was constructed from the coincidence data. Radioactivity ^150mEu (from¹⁵⁰Sm(d,2n))γγ coincidence; measuredE _y I _y ; deduced levels, decay scheme. Enriched target, Ge(Li) and NaI(Tl) detectors.     

Search for weak transitions in the decay of125Sb and accurate gamma intensities

The weak transitions in the decay of¹²⁵Sb have been investigated through gamma ray measurements with high resolution X-ray and with large volume Ge(Li) detectors. The 172.6, 178.8 and 198.5 keV gamma rays are confirmed, while others previously reported were not. Accurate intensities were obtained for the stronger transitions. The weighted averages of these intensities which cover the range of 116 to 670 keV are useful for calibration of Ge(Li) systems.     

Der Zerfall des122Xe (T 1/2=20,l h) und des122J (T 1/2=3,6min)

Theγ spectra emitted in the decay of¹²²Xe and¹²²I have been investigated using Ge(Li) detectors and a Ge(Li)-NaI coincidence apparatus. 14γ transitions with energies between 61.8 and 416.9 keV have been identified in the decay of¹²²Xe, 44 transitions between 564.0 and 3,291.0 keV in the decay of¹²²I. Level schemes having 7 excited levels for¹²²I and 21 excited levels for¹²²Te are proposed.