Decay of63Zn

Investigation of the 38.8 min decay of⁶³Zn has resulted in 31 gamma-ray transitions in⁶³Cu. New levels not earlier reported inΒ ⁺-decay of⁶³Zn, but found in nuclear reactions, are suggested at 2,010.9 and 3,101 keV. It is assumed that the excited core model generates a multiplet of levels at 669.75 keV (1/2^?), 962.1 keV (5/2^?), 1,327.1 keV (7/2^?) and 1,546.6 keV (3/2^?). Intensities for intramultiplet transitions were found to be: 219.4 keV, <0.004 (in units of 200 for annihilation radiation), 292.4 keV, <0.004, 365.0 keV, 0.03±0.03, 584.4 keV, <0.005, and 876.8 keV, <0.005.     

Der radioaktive Zerfall des Fe61

Fe⁶¹(T _1/2=5.95 min) was produced irradiating Ni⁶⁴ and natural nickelfoils with fast neutrons in the reaction Ni⁶⁴(n, α)Fe⁶¹; Fe was chemical seperated. The gamma and beta spectrum were investigated with Ge(Li)-counters, NaJ(Tl) and plastic scintillation spectrometers. Fe⁶¹ emits five gamma rays having the energies and intensities per Fe⁶¹ decay: 121 keV (0.064), 177 keV (0.027), 298 keV (0.293), 1025 keV (0.461), 1202 keV (0.539). Threeγγ-cascades could be identified: 121–177 keV, 121–1202 keV, 298–1025 keV. Inγ β-coincidence measurements the maximal beta energy was determined:E _βmax=2.86 MeV. A decay sceme Fe⁶¹-Co⁶¹ was constructed: Fe⁶¹, spin and parityJ ^π=3/2^?, decays by means of allowed beta decay to three excited states of Co⁶¹: 1323 keV (1/2^?), 1202 keV (3/2^?), 1025 keV (5/2^?). The energies and intensities per Fe⁶¹ decay of the three beta decay modes are: 2.56 MeV (0.367), 2.68 MeV (0.495), 2.86 MeV (0.138). — A 88 keV gamma ray (T_1/2=33 sec) was observed coming from the Co⁶³ decay.     

Der Zerfall des Ag106g und Ag106m

The decays of the 25 min-Ag^106g and 8.3 d-Ag^106m have been investigated using Ge(Li)- and Si(Li)-counters. Theγ-rays of 17 transitions in the Ag^106g -decay and of 42 transitions in the Ag^106m -decay have been observed and their energies and relative intensities have been determined. The intensities of theseγ-rays and the intensities of conversion-electrons known from earlier measurements allow the determination ofK-conversion-coefficients for 23 transitions. The present data are consistent with a level-scheme of Pd¹⁰⁶ having states at 0, 0⁺; 511.8, 2⁺; 1127.8, 2⁺; 1133.1, 0⁺; 1228.8, 4⁺; 1557.4, 3⁺; 1562, 2⁺; 1702.8, 4⁺; 1931.7, 3, 4⁺; 2002, 0⁺; 2040.4, 3, 4⁺; 2076.8, 3, 4⁺; 2084.2, 3^?; 2305.7, 4^?; 2324, 1, 2⁺; 2350.4, 3, 4⁺; 2365.3, 3, 4⁺; 2529, 1, 2⁺; 2756.3, 5⁺; 2951.3 keV, 5⁺. The level-scheme of Pd¹⁰⁶ is compared with the predictions of the vibrational model for spherical nuclei.     

Der Zerfall des Cu61

Theγ-ray-spectrum of Ni⁶¹ associated with the E.C. andΒ ⁺-decay of Cu⁶¹ has been measured with a Ge(Li)-counter. The observed 14 newγ-ray-transitions led to a new level-scheme for this decay with Ni⁶¹-Ievels at: 67.7, 282.9, 656.0, 907.9, 1099.8, 1132.7, 1186.8, 1610.6, 1730.8 and 2128.0 keV. Five of these levels were known from earlier investigations of Cu⁶¹-decay, but all of them could be identified with some of previously reported levels found in scattering experiments. As far as possible spin and parity assignments have been made and are compared with the results of scattering experiments.     

The β-decay of98Y and the level scheme of98Zr

Study of theβ-decay of⁹⁸Y and of the level scheme of⁹⁸Zr was undertaken by the use of the two recoil fission product separators JOSEF and LOHENGRIN. Twoβ-decay modes have been detected for⁹⁸Y, the half-lives of which are 0.65±0.05 s and 2.0±0.2 s. The spins and parities of the two states which undergoβ-decay are proposed to be 1⁺ and 4^?, respectively, with the configurations (π1g _9/2)(ν1g _7/2) and (π2p _1/2 (ν1g _7/2). The measuredQ _β -value is 7300±400 keV for the 0.65 s decay. The level scheme of⁹⁸Zr was deduced fromγ,γ-coincidence data. Absoluteγ-intensities were obtained from two independent measurements. The half-life of the first excited state of⁹⁸Zr at 853.0 keV with spin and parity 0⁺ was determined through delayedγ, e^?-measurements to be 63 ±7ns. No indication of the coexistence of two different nuclear shapes of⁹⁸Zr was found.     

Der Zerfall von Tm174 und Tm175

The radioactive isotopes Tm¹⁷⁴ and Tm¹⁷⁵ were produced by the reactions Yb¹⁷⁶ (γ, np) Tm¹⁷⁴ and Yb¹⁷⁶(γ,p) Tm¹⁷⁵ respectively, with bremsstrahlung of 54 MeV maximum energy. TheΒ- andγ-radiations from the decay of these isotopes were investigated using scintillation counters, solid state detectors and coincidence methods. The decay scheme proposed for Tm¹⁷⁴ is similar to those proposed by previous investigations. The spin assignment of the isomeric 1520 keV level was revised to beI=7. The decay of Tm¹⁷⁵, which was until now rather unknown, has a half-life of of 15.2±0.5 min. The suggested decay scheme shows excited levels at 105 (9/2^?), 511 (1/2^?), 553 (3/2^?), 598 (5/2^?), 643 (5/2^?, 7/2^?), 816 (3/2^?), 873, 990, 1454 (1/2⁺), 1496 (3/2⁺), 1505, 1810 and 1881 keV. The results are discussed using the Nilsson model.     

Die Zerfälle des Rh97g und des Rh97m

The decays of Rh^97g and Rh^97m were investigated using Ge(Li)- and Si(Li)-detectors and a Ge(Li)—Ge(Li)-coincidence circuit. The isomeric transition with an energy of 259 keV was identified by its conversion electrons and decays with a half-life of (48.0±0.8) min. Therefore, the half-lives (30.3±0.9) min and (47.9±0.6) min obtained from theγ-studies were attributed to the decays of Rh^97g and Rh^97m respectively. The proposed decay schemes have 31 excited states of Ru⁹⁷ and account for 84 of the 110 observedγ-transitions, especially for the 37 strongest ones. Twelve of the proposed levels having spins and parities 1/2^? or 3/2^? and excitation energies between 2200 keV and 3600 keV are interpreted as being due to 2p _1/2-neutron-hole-states.     

On theβ − decay of the 2s isomer in98Y and the existence of an intruder band in98Zr

The γ radiation from the ß^? decay of the high-spin isomer in⁹⁸Y has been studied at the separator JOSEF. A main goal was to get insight into the spins of levels in⁹⁸Zr which have been interpreted as members of an intruder band based on the 0₂ ⁺ state at 854 keV. The measuredγ-γ angular-correlations lead to the assignment of spins of 4 and 3 ? to the 2491 and 1844 keV levels, respectively, and contradict their interpretation as the 6⁺ and 4⁺ states of the proposed band. For the 2.0s isomer of⁹⁸Y, the ß{?}-decay properties suggest I=5 with a major configuration [πg_9/2,νs_1/2(g² _7/2)₀].     

Low lying levels of Fe55

Angular distributions of 413 and 1,322keV gamma rays from the Mn⁵⁵(p,nγ)Fe⁵⁵ reaction and the (n-γ) angular correlation measurements have been measured at proton energies below 2.50 MeV. The experimental results show agreement with the Sheldon formula. The multipole mixture parameters for the 933 and 1,322 keV gamma rays in Fe⁵⁵ have been determined. The sum coincidence technique is used to give some information about the scheme of excited levels in the Fe⁵⁵ nucleus.     

Der Zerfall des125m Xe,des127m Xe und des127g Xe

The decay of^125m Xe produced by the reaction¹²²Te(α, n)^125m Xe using a target enriched in¹²²Te (95.4%) and the decay of^127m Xe produced by the reaction¹²⁷J(d, 2n)^127m Xe have been investigated: ^125m Xe decays with a half-life ofT _1/2=(56±3) sec by ayy- cascade withE _γ1=(140.4 ±0.5) keV andE _γ2=(110.5 ±0.5) keV. The experimental conversion coefficients yield multipolarities ofE3 for the 140.4 keV isomeric transition and predominantlyM1 for the 110.5 keV-transition. ^127m Xe decays with a half-life ofT _1/2=(71±2) sec. The decay also proceeds by aγγ-cascade with an isomeric E3 transition ofE _γ1=(172.5±0.3) keV and a predominantlyM1 transition ofE _γ2=(124.6±0.3) keV. In the decay of^127g Xe an additional branching of the electron capture to a level at (618.1±0.3) keV was observed. The relative probability forK-captureP _K618/P_K375=0.40 ±0.07 yields a total transition energyQ _EC=(664 ±4)keV. A spin of 1/2⁺ was assigned to the ground state.     

Der Zerfall des Mn52m

Mn^52m(T _1/2=21 m) was produced by irradiating iron-foiles with deuterons ofE _d =9 MeV. Coincidences ofγ-rays with the main 1434 keV-transition had been sought for with the aid of a scintillation fast-slow-coincidence circuit. There was no evidence ofγ-lines which had been found earlier byKatoh et al. atγ-energies 700, 940, 1020, 1150, 1370, 1520 keV. If these transitions exist, their relative intensities are less than 0.7% (700 keV) and 0.3% (all others) per decay of Mn^52m.     

High-spin states in48Ti

The⁴⁵Sc(α, p γ) reaction has been investigated atE ^α=11, 12 and 13MeV. Theγ-decay of 198 levels in⁴⁸Ti up to 8,323 keV excitation energy has been observed. High-spin states were investigated by proton-γ ray angular correlation measurements atE=11 and 13MeV and by DSAM lifetime measurements atE=11 MeV. From the combined evidence spin (-parity) assignments were obtained for the levels atE _x =8,323 keV (J= 10,8,6), 8,091(12, 10, 8, 6), 7,668(10, 8), 7,427(9, 7), 7,374(11, 9, 7), 6,906(10, 8, 6), 6,172(8⁺,6⁺), 6,102(10⁺,8⁺), 6,039(6), 6,034(9⁺, 7⁺), 5,630(7), 5,197(8⁺), 5,169(7⁺), 5,155(5), 4,404(5), 4,398(6⁺) and 4,046keV (5). Most of the ambiguous spin assignments become unique if the 8,091 keV level hasJ=12, an assumption which is favoured by its excitation function. The level spectrum thus obtained is well reproduced by shell model calculations in the pure (f _7/2)⁸ configuration space. Discrepancies exist in the reproduction ofγ-decay modes. The reason is found in low-lying high-spin intruder states which include the 7,427 and 8,323 keV levels. The spectrum of negative-parity states is understood qualitatively by a comparison with⁴⁶Ti and⁴²Ca.     

The beta decay of 18N and T = 2 states of mass 18

The ¹⁸N(β^?)¹⁸O decay was observed via the ⁹Be(¹⁸O, p2α)¹⁸N reaction, utilizing helium-transport techniques and Ge(Li) spectroscopy. In addition to the previously reported β-decay to the ¹⁸O 4456 keV level (J^π = 1^?) branches were observed to levels at excitation energies (in keV) of 1982 (J^π = 2⁺). 5530(2^?), 6198(1^?). 6350(2^? or 1⁺), 6880(0^?), and 7771(2^?). The percentage β-branches, in order of increasing excitation energy, are 3.9 ± 1.5, 54.6 ± 1.0, 3.1 ± 0.4, 1.4 ± 0.2, 2.2 ± 0.3, 14.8 ± 0.8 and 5.0 ± 0.5. respectively, with 15 % assumed on the basis of calculations to proceed to non-γ-emitting states. These measurements allow definite assignments J^π = 1^? for the ¹⁸N ground state and J^π = 0^? for the ¹⁸O 6880 keV state. Additional measurements determine the ¹⁸N half-life to be T_{1 2} = 624 ± 12 ms. A shell-model calculation for mass 18 was carried out in a full 1?ω basis. The predictions for the T = 2 energy level spectrum and for ¹⁸N β-decay are discussed.     

Über die selbständige Polarisierung des Spins der Elektronen durch Ausstrahlung bei der Bewegung auf einer Spiralbahn im Magnetfeld

The nuclear half-life of the 287 keV second excited state of⁷⁵Se, populated by the reaction⁷⁵As(p, n)⁷⁵Se^* has been measured by the delayed coincidence technique. NaJ(Tl)- and Ge(Li)-detectors were used for measuringγ-energies and time-spectra. By slope analysis of the time-spectra we obtained a half-life of T_1/2(⁷⁵Se, 287 keV)=(30.0±0.4) ns. Possible spin assignments for the 287 keV state in⁷⁵Se from logft-values derived fromβ ⁺-decay data of⁷⁵Br to this level byBaskova et al are 3/2^? and 1/2^?. Application of an external magnetic field of 24 kG to the target nuclei yielded no measurable perturbation of the time-spectra, thus a spin value of 1/2^? for this level seems to be more probable.     

Der Spin des Grundzustandes von F20

The spin of the F²⁰-ground-state has been determined by means of a circularpolarisation correlation measurement on theΒ-γ-cascade of F²⁰. The experimental result gives spin 2 for the ground-state of F²⁰. Within the statistical error of the experiment theΒ-decay of F²⁰ has pure Gamow-Teller-interaction.     

EPR study of Fe3+ and Mn2+ in CeO2 and ThO2

Attempts were made to grow CeO₂ and ThO₂ single crystals doped with transition metal ions. Only Fe³⁺ and Mn²⁺ could be detected by the EPR technique. The EPR spectrum of Fe³⁺ in CeO₂ exhibits the well-known fine structure in cubic fields. The parameters areg=2.0044(1) anda=15.6(1)·10^?4 cm^?1. The hyperfine constantA for⁵⁷Fe in hexahedral coordination was found to be 8.9(1)·10^?4 cm^?1. The EPR spectrum of Mn²⁺ in CeO₂ reveals two cubic Mn²⁺ centers. The parameters for center 1 areg=1.9999(1) andA=86.9(1)·10^?4 cm^?1 and for center 2g=1.9984(1) andA=87.0(1)·10^?4 cm^?1. Heating the Mn doped CeO₂ samples in hydrogen, the Mn²⁺ centers transform from cubic into trigonal centers with approximate values ofg=1.9988(2),A=84.5(6)·10^?4 cm^?1 andD=203(1)·10^?4 cm^?1. The two observed Mn²⁺ centers in ThO₂ exhibita priori axial symmetry with approximate values ofg=2.0006(2),A=88.9(4)·10^?4 cm^?1 andD=33(3)·10^?4 cm^?1.     

Der Zerfall des Ruthenium 95

Theγ-spectrum of Tc⁹⁵ associated with the E.C.- and β⁺-decay of Ru⁹⁵ has been measured with a Ge(Li)-counter and a NaJ-crystal. 12 newγ-ray transitions have been found in these spectrums. To propose a new level-schemeγ-γ-coincidences have been taken with 2 NaJ-crystals in a two-dimensional device. Besides this the total conversion coefficient of the 336 keV transition was measured by detecting the electrons in a Si(Li)-counter and theγ-rays in a NaJ-crystal.     

Das magnetische Moment des 2,083 MeV-Zwei-Protonen-Niveaus des gerade-gerade-Kerns Ce140

The nuclearg-factor of the 2·083 MeV-state of Ce¹⁴⁰ has been determined as:g=1·11±0·04 This value suggests the interpretation of the level as the (g7/2,d5/2)₄ two proton shell model configuration. The investigation implies an integral measurement as well as a time dependent differential measurement (spin rotation method) of the rotation of the 329 keV-487 keVγγ-angular correlation in strong external magnetic fields. Liquid sources of lanthanum nitrate solved in 3n HNO₃ were used in these experiments. Some cerium (IV)nitrate was added to make sure that the 4f;-electronic shell remained empty after theβ ^?-decay. This prevented paramagnetic effects. Additional runs were performed without adding cerium (IV)nitrate and finally by using liquid sources of lanthanum chloride solved in 2n HCl with some iron (II)-chloride added. It was expected that the Fe⁺⁺ ions would reduce the primarily formed Ce⁺⁺⁺⁺ ions into the Ce⁺⁺⁺ state. The Ce⁺⁺⁺ shell is paramagnetic and enlarges the effective magnetic field at the position of the nucleus by about 36%. As no definitely faster rotation could be observed, one has to conclude that the ion reaction Ce⁺⁺⁺⁺+Fe⁺⁺?Ce⁺⁺⁺+Fe⁺⁺⁺ takes more than about 10^?8s. The half life of the 2·083 MeV state has been redeterminded asT _1/2=(3·41±0·04)·10^?9s. Differential measurements of the angular correlation of the 329 keV-487 keV cascade as a function of the time delay showed that perturbations by internal fields were very small. The coefficientsA ₂ andA ₄ of the angular correlation and the attenuation parameterλ ₂ were determined from measurements with sources of the first type as:A ₂=?0·105±0·003A ₄=?0·001±0·002 andλ ₂=(0·0065±0·0040)·10⁹S^?1=(0·032±0·020)·λ A comparison with the theoretical coefficients of a (3-4-2)-cascade shows that the multipolarity of the 329 keV radiation is a mixture of 99·83%M1 and (0·17±0·03) %E2.     

Magnetic rotation of levels of 53Mn and 54Mn following the 53, 54Cr(p,n) and 51V(α, n) reactions

The low-lying levels of ⁵³Mn and ⁵⁴Mn have been studied using the ^{53, 54}Cr(p, nγ) and ⁵¹V(α, nγ) reactions. Angular distributions of γ-rays have been measured and their integral rotations in iron alloy targets studied. The g-factor of the 377 keV, $\text{5}\text{2}{}^{\mathrm{?}}$ level of ⁵³Mn is g = + 1.15±0.17. Products gτ have been found for the 55, 156, 368, 408 and 1072 keV levels of ⁵⁴Mn to be 124±42, 360±60, 75±25, > 10 and 150±80 ps respectively. Using shell model estimates for the g-factors, the lifetimes of the levels have been deduced. An interpretation of the results in terms of shell model wave functions is given.     

Der Zerfall des Co56

Theγ-ray-spectrum of Fe⁵⁶ associated with the E.C.- andβ ⁺-decay of Co⁵⁶ has been measured with Ge(Li)-crystals. 6 newγ-ray-transitions have been found in this spectrum deexciting 3 new levels in Fe⁵⁶. The intensities of these transitions have been estimated and a new level-scheme is proposed. The new levels could be identified with some of previously reported levels found in Fe⁵⁶(p, p′)-measurements.