未被俘获电子对多光子非线性Compton散射能量转换效率的影响

 应用单粒子理论和电子与光子非弹性碰撞模型，研究了未被俘获电子对多光子非线性Compton散射能量转换效率的影响。结果表明，未被俘获电子使该散射的频谱展宽随入射电子速度和与电子同时作用的光子数的增大而增大，随电子与光子非弹性碰撞成分的增大而减小，从而使能量转换效率近乎与电子入射速度正比降低。用低能电子入射，能有效地减小这种损失。     

Relativistic energy loss and induced photon emission in the interaction of a left-handed sphere with an external electron beam

Relativistic energy loss and photon emission in the interaction of a coated sphere containing a left-handed material with an external electron beam are studied based on the classical electrodynamics. Both of electric modes and magnetic modes are not only found in the spectra of energy loss and photon emission for different combinations of electron velocity and sphere radius, the new excitation modes can be also observed. Our results show that different excitation modes for the left-hand materials and the structure information of coated sphere can be explored by scanning transmission electron microscopy (STEM).     

多光子非线性Compton散射的能量转换

研究了多光子非线性Compton散射中电子与光子的能量转换及其转换效率.结果表明:散射光子频率随电子吸收光子数n的增大而增大,随碰撞非弹性成分ξ的增大而迅速减小.在超强激光场中,当极端相对论性电子与光子发生多光子非线性Compton散射且被光场俘获时,能量转换效率趋于无限大,即电子可以从超强激光场中获得巨大的加速能量.用高速电子束入射并与光子发生多光子非线性Compton散射,是提高非线性Compton散射能量转换效率的重要途径.     

高能闪光照相X射线能谱的理论研究

 用Monte-Carlo方法模拟球对称客体系统的闪光照相中X光光子的输运过程。分别在单客体情况和全系统情况下,给出了记录平面上各种光子谱及其在记录平面上的空间分布。结果表明：记录区边缘的谱形与源光子谱形很相似;深穿透区各点之间的谱形差别不大,谱平均光子能量近似相同,并且位于使高Z材料的光子线吸收系数最小的能量范围内。 结果还表明,高能闪光照相的光子能谱会因客体中光子的光程不同而有较大的差别。     

全光汤姆逊散射X光源数值模拟

 使用蒙特卡罗数值模拟程序研究了不同电子束和激光强度下,尾场电子束与超短脉冲激光发生汤姆逊散射获得的X光子能谱、角分布等,初步探索了180°散射下高质量X射线光源所需要的电子束与激光强度。数值模拟结果显示,为了尽量提高光子产额并抑制非线性效应,激光归一化强度应为1的量级。为了获得方向性和单色性好、亮度高的X射线脉冲,需要较高的电子能量和较小的电子能散,电子束脉冲尽量短,且发散角尽量小。     

Analysis of Two-Grid Methods for Nonlinear Parabolic Equations by Expanded Mixed Finite Element Methods

In this paper, we present an efficient method of two-grid scheme for the approximation of two-dimensional nonlinear parabolic equations using an expanded mixed finite element method. We use two Newton iterations on the fine grid in our methods. Firstly, we solve an original nonlinear problem on the coarse nonlinear grid, then we use Newton iterations on the fine grid twice. The two-grid idea is from Xu$'$s work [SIAM J. Numer. Anal., 33 (1996), pp. 1759-1777] on standard finite method. We also obtain the error estimates for the algorithms of the two-grid method. It is shown that the algorithm achieves asymptotically optimal approximation rate with the two-grid methods as long as the mesh sizes satisfy $h=\mathcal{O}(H^{(4k+1)/(k+1)})$.     

Energy dependence of electron energy loss processes in Ge 2s photoemission

Deep core Ge 2s photoelectron spectra from polycrystalline Ge films induced by monochromatic synchrotron radiation, of 4, 6 and 8 keV were measured and analysed using two different methods, the partial intensity analysis and the extended Hüfner method to determine the spectral contributions from different electron energy loss processes due to bulk extrinsic, intrinsic and surface excitations. The obtained photon energy dependence of the ratio of these contributions was compared as a function of the photoelectron kinetic energy. It was found that the relative contribution of intrinsic excitations increase with the photon energy.     

Surface plasmon assisted photoemission from Au nanoparticles on graphite

The resonant multiple excitation of collective modes in metallic nanoparticles using ultrashort laser pulses leads to an enhanced multiphoton photoemission from the particles. This effect is here demonstrated for the surface-plasmon resonance of Au nanoparticles on graphite. The shape of the photoemission spectra is explained by multiphoton photo-assisted thermionic emission from the nanoparticles and resonant emission via the image-potential state on graphite. Tuning the photon energy between 1.7 eV and 3.2 eV allows the identification of an enhancement of the photoemission yield at 2.1±0.1-eV photon energy that is attributed to the resonant excitation of the surface plasmon in the Au nanoparticles. This identification of the surface-plasmon excitation in this energy range is also supported by electron energy loss spectroscopy. Received: 8 August 2001 / Revised version: 13 September 2001 / Published online: 10 October 2001     

Element-selective mapping of magnetic moments in ultrathin magnetic films using a photoemission microscope

We combine X-ray magnetic circular dichroism (XMCD) and photoelectron emission microscopy to obtain locally resolved magnetic information on a microscopic scale. Scanning the photon energy across elemental absorption edges and recording microscopic images of the local secondary electron intensity for both photon helicities at each photon energy step allows to analyze local XMCD spectra at any position of the imaged area of the sample. With the help of magnetic sum-rules local quantitative information about magnetic moments can be extracted from such microspectroscopic measurements. The full power of XMCD as a spectroscopic tool is so maintained, while microscopic spatial resolution is added.     

Numerical Investigation Into the Highly Nonlinear Heat Transfer Equation with Bremsstrahlung Emission in the Inertial Confinement Fusion Plasmas

A highly nonlinear parabolic partial differential equation that models the electron heat transfer process in laser inertial fusion has been solved numerically. The strong temperature dependence of the electron thermal conductivity and heat loss term (Bremsstrahlung emission) makes this a highly nonlinear process. In this case, an efficient numerical method is developed for the energy transport mechanism from the region of energy deposition into the ablation surface by a combination of the Crank‐Nicolson scheme and the Newton‐Raphson method. The quantitative behavior of the electron temperature and the comparison between analytic and numerical solutions are also investigated. For more clarification, the accuracy and conservation of energy in the computations are tested. The numerical results can be used to evaluate the nonlinear electron heat conduction, considering the released energy of the laser pulse at the Deuterium‐Tritium (DT) targets and preheating by heat conduction ahead of a compression shock in the inertial confinement fusion (ICF) approach. (© 2015 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)     

Large Third-Order Optical Nonlinearity of Cadmium Sulphide Nanoparticles Embedded in Polymer Thin Films

A simple method for synthesis of well dispersed cadmium sulphide nanoparticles embedded in a polyethylene glycol matrix （PEG 400） in thin film form is presented. The large blue shift of the band gap energy of the CdS nanoparticles compared to the bulk semiconductors is observed via UV-vis absorption spectra. Photoluminescence spectra of CdS nanocomposite films show that the emission peaks shift towards the longer wavelength with the increase of annealing temperature. Transmission electron microscopic images as well as Raman scattering studies confirm the CdS nanometer size particle formation within the polymer matrix. The particle size is about 8 nm. Selected area electron diffraction （SAED） shows the cubic zinc blende polycrystalline rings. Third-order optical nonlinearity of the CdS nanopartieles embedded in polymer thin films is studied with the Z-scan technique under 1064 nm excitation. The results show that the CdS nanocomposite film exhibits negative nonlinear refraction index and positive absorption coefficient. The film shows large optical nonlinearity, and the magnitude of the third-order nonlinear susceptibility of the film is calculated to be 1.73 × 10^-9 esu. The corresponding mechanism is discussed.     

非线性晶体散射及吸收光谱的测量

利用PE-Lambda900分光光度计，测量了非线性晶体的散射及吸收光谱，实验中避免了大块双轴晶体镜面反射作用引起的测量误差．实验结果表明，随光子能量增加，晶体材料的光吸收在400nm以外波段显著增加。对散射谱进行分析，来源于晶体结构内部的缺陷。如位错、包裹体的尺寸主要分布在lOOnm以上,这些缺陷在短波段的光散射作用有上升的趋势。     

The bremsstrahlung induced by 0.3–2 keV electron scattering by Ar atoms

The differential spectra of a bremsstrahlung resulting from a 0.3–2 keV electron scattering by Ar atoms are studied. Photon energies within the ultrasoft X-ray band from 124 to 190.8 eV, which is characterized by the low dynamic polarizability of the Ar atom, are considered. For the entire spectrum of photon energies (124–190.8 eV), the intensity of the bremsstrahlung differential spectra first grows with an increase in the electron energy from 0.3 to 0.7 keV and then decreases as the electron energy increases from 0.7 to 2 keV. The increase in intensity is directly proportional, and the decrease is inversely proportional to the square root of the energy of the scattered electrons. Within the context of a "low-energy" approximation, the increase in the number of photons with the electron energy is due to the contribution of the atomic excitation and ionization channels being available during the bremsstrahlung process.     

Spatially resolved Raman spectroscopy evaluation of residual stresses in 3C-SiC layer deposited on Si substrates with different crystallographic orientations

Raman scattering studies were performed on hot-wall chemical vapor deposited (heteroepitaxial) silicon carbide (SiC) films grown on Si substrates with orientations of (1 0 0), (1 1 1), (1 1 0) and (2 1 1), respectively. Raman spectra suggested that good quality cubic SiC single crystals could be obtained on the Si substrate, independent of its crystallographic orientation. Average residual stresses in the epitaxially grown 3C-SiC films were measured with the laser waist focused on the epilayer surface. Tensile and compressive residual stresses were found to be stored within the SiC film and in the Si substrate, respectively. The residual stress exhibited a marked dependence on the orientation of the substrate. The measured stresses were comparable to the thermal stress deduced from elastic deformation theory, which demonstrates that the large lattice mismatch between cubic SiC and Si is effectively relieved by initial carbonization. The confocal configuration of the optical probe enabled a stress evaluation along the cross-section of the sample, which showed maximum tensile stress magnitude at the SiC/Si interface from the SiC side, decreasing away from the interface in varied rate for different crystallographic orientations. Defocusing experiments were used to precisely characterize the geometry of the laser probe in 3C-SiC single crystal. Based on this knowledge, a theoretical convolution of the in-depth stress distribution could be obtained, which showed a satisfactory agreement with stress values obtained by experiments performed on the 3C-SiC surface.     

Effect of Laser Field and Mechanical Force on Deoxyribonucleic Acid Melting

We propose a physics method to study the effect of laser field and mechanical force on the melting process of double-stranded deoxyribonucleic acid （DNA）. A two-dimensional lattice model is established for DNA molecules stuck on the surface, and the stretching energy of the hydrogen bond and stacking energy for each DNA molecule are calculated by using a nonlinear potential. A real-time algorithm is employed to deal with the dynamics process of DNA melting. Numerical results explain the experimental observations. The spatial distribution of the laser field determines the sequences of DNA melting. The simulation has shown the dependence of the final number of melted DNA on the laser field and mechanical force.     

Accuracy of spectrum estimate in fluorescence spectral microscopy with spectral filters

We establish the accuracy of the spectrum that is estimated with an inexpensive fluorescence spectral microscope utilizing a small set of spectral filters [Soriano et al, Opt. Exp. 10, 1458–1464 (2002)]. The spectrum at an arbitrary image location of the fluorescent sample is estimated as a linear superposition of basis spectra that are derived by singular value decomposition (SVD) or principal component analysis (PCA) from a spectral library of fluorescence spectra. Estimation performance is analyzed as a function of library statistics, filter selection and sequencing, minimum negativity constraint and signal to noise ratio (SNR) of fluorescence image. We consider image SNR degradations that arise from weakening of image intensity, additive Gaussian noise, intensity-dependent Poisson noise and quantization errors. The recovery of specific spectral features like spectral resolution, general similarity and peak alignments, is assessed using Linfoot’s criteria of fidelity, structural content, and correlation. We found that estimation with SVD basis spectra is more robust against image noise than that with PCA basis spectra. However for high SNR images, accurate estimation is achieved more quickly with PCA basis spectra and with better response to the application of minimum negativity constraint.     

Optical properties of fullerene and non-fullerene peapods

Single-wall carbon nanotubes (SWNTs) encapsulating fullerenes, so-called fullerene peapods, were synthesized in high yield by using diameter-selected nanotubes as pods. Transmission electron microscopy revealed high-density fullerene chains inside the nanotubes. X-ray-diffraction measurements indicate 85% filling for C₆₀ and 72% filling for C₇₀ molecules as a total yield. Interestingly, C₆₀ peas do not show any thermal expansion while C₇₀ peas show normal behavior. Room-temperature Raman spectra show one-dimensional photopolymerization of C₆₀ inside nanotubes by blue-laser irradiation, suggesting molecular rotation inside them. In C₇₀ peapods, no photopolymerization was observed but the relative Raman intensity of each peak is different from the C₇₀ 3D crystal. This is probably caused by mixing of two different crystal structures in C₇₀ peas. Furthermore, we synthesized Zn-diphenylporphyrin peapods. Optical absorption and Raman spectra suggest that the encapsulated molecules are deformed by interaction with the SWNT. Received: 12 November 2001 / Accepted: 3 December 2001 / Published online: 4 March 2002     

Crystal growth, thermal and optical studies of nonlinear optical material: Glycine potassium sulphate

A new nonlinear optical material glycine potassium sulphate (GPS) has been synthesized and optical quality crystals were grown from aqueous solution. This material has positive temperature coefficient revealed from the solubility studies. The grown crystals were characterized by employing several techniques such as single crystal and powder X-ray diffraction, thermo gravimetric analysis, FTIR and UV-vis-NIR spectra. The etching studies have been done on the (1 0 0) plane of the grown crystal. Preliminary measurements to find second harmonic generation efficiency of GPS has been carried out.     

On choosing a nonlinear initial iterate for solving the 2-D 3-T heat conduction equations

The 2-D 3-T heat conduction equations can be used to approximately describe the energy broadcast in materials and the energy swapping between electron and photon or ion. To solve the equations, a fully implicit finite volume scheme is often used as the discretization method. Because the energy diffusion and swapping coefficients have a strongly nonlinear dependence on the temperature, and some physical parameters are discontinuous across the interfaces between the materials, it is a challenge to solve the discretized nonlinear algebraic equations. Particularly, as time advances, the temperature varies so greatly in the front of energy that it is difficult to choose an effective initial iterate when the nonlinear algebraic equations are solved by an iterative method. In this paper, a method of choosing a nonlinear initial iterate is proposed for iterative solving this kind of nonlinear algebraic equations. Numerical results show the proposed initial iterate can improve the computational efficiency, and also the convergence behavior of the nonlinear iteration.     

Time resolved studies on X-rays and charged particles emission from a low energy plasma focus device

The time resolved studies on soft X-ray, hard X-ray, electron beam and ion beam emissions from a low energy plasma focus device are carried out simultaneously by employing a photodiode X-ray spectrometer, a scintillator photomultiplier tube, a combination of Faraday cup and Rogowski coil assembly and a biased Faraday cup, respectively. The soft X-ray is seen to be emitted in short multiple pulses corresponding to different pinch stages where as it is a single for hard X-ray, which corresponds to only maximum pinch stage. Similarly, multiple pulses of electron beam is found, which also corresponds to different pinch stages and these pulses are analogous with the soft X-ray pulses. The effective hard X-ray photon energy is estimated by foil absorption technique and found to be around 110 keV, which is consistent with the observed electron beam energy distribution. The simultaneous investigation of the electron and ion beam shows that both are accelerated by the same local field generated during the pinching process. The detailed results of time resolved studies on various radiations are incorporated in this Letter.