Experimental study of a broad-band XeCl double-pass amplifier with SBS mirror

An oscillator-amplifier XeCl laser system has been used to experimentally investigate the effectiveness of a liquid stimulated Brillouin scattering (SBS) mirror for correcting the spatial aberrations of broad-band laser radiation in a double-pass amplifier. It has been found that the SBS amplifier performance is strongly dependent on the intensity I _p exciting the Brillouin medium. A good beam reconstruction has been attained at I _p1GW/cm², whereas highly aberrated output beams have been delivered by the SBS amplifier for I _p>1 GW/cm². By comparing the broad-band SBS amplifier performance to that of the same amplifier with a dielectrically coated flat mirror at one end, it has been found that the use of a SBS mirror is advantageous to obtain lower divergence output beams only for low energy pump beams (<1 mJ).     

Threshold reduction of stimulated Brillouin scattering (SBS) using fiber loop schemes

SBS mirrors as self-pumped and easy to handle non-linear optical devices are frequently used in high-power laser systems for improving the beam quality based on optical phase conjugation. Because of the non-linear behaviour, a certain pulse energy or power of incident light is needed to generate enough reflectivity for practical purposes. Therefore, reducing this “threshold” is still a main topic in the development of new schemes for optical phase conjugation. In addition to the taper concept reported earlier, this paper deals with loop schemes for reducing the power requirements. A reduction of the so-called “threshold” by a factor of between two and four was obtained with the schemes investigated using liquids and fibers. Received: 4 September 2001 / Revised version: 22 October 2001 / Published online: 23 November 2001     

Study of second harmonic generation by non-linear crystals with phase conjugation

We present the correction of the phase distortion which occurs during the second harmonic generation by non-linear crystals, such as KDP and KTP at high average power laser. This is due to the optical quality and thicknesses of the crystals which in turn influence the quality of the incident laser beam. This phase distortion is corrected by reflecting back the laser beam into the crystal using a phase conjugate mirror. It is found that the conversion efficiency of second harmonic generation without phase conjugation is more than that with phase conjugation. Far field pattern shows that the distortion of the laser beam can be corrected by using the phase conjugate mirror. Fidelity of the beam profile increases significantly with phase conjugation in the case of KDP crystal.     

Influence of Temperature on Stimulated Raman Scattering in Single-Mode Silica Fibre

One piece of single-mode silica fibre is used to study of temperature characteristics of stimulated Raman scattering (SRS), additional peaks (double-humped) are observed at both sides of pump light and 1^st-order Stokes light in the experiment. The frequency shift of the double-humped is calculated by stimulated Four--Photon mixing (SFPM) phase matching theory, the result is consistent with the frequency shift of this experiment. Simultaneously, the experimental conditions accord with the theoretical calculation of effective coherence length. We indicate that the double-humped phenomenon is caused by SFPM. The intensity of double-humped is first increased, then decreased and finally disappeared as the temperature increases. This phenomenon has been explained theoretically.     

Self-focussing of CO2 laser radiation in SF6

Self-focussing of high-power TEA CO₂ laser pulses for a number of 10 m P-band lines is reported in SF₆ molecular gas. Application of this effect to estimating the intensity-dependent refractive index of the gas is demonstrated.     

SBS pulse compression to 200 ps in a compact single-cell setup

Received: 14 September 1998 / Published online: 24 February 1999     

Coexisting Raman- and Rayleigh-Enhanced Four-Wave Mixing in Femtosecond Polarization Beats

Based on the polarization interference of Raman- and Rayleigh-enhanced four-wave mixing processes, heterodyne detection of the Raman, Rayleigh and coexisting Raman and Rayleigh femtosecond difference-frequency polarization beats is investigated in the cw and the three Markovian stochastic models, respectively. These two processes exhibit asymmetric and symmetric spectra, respectively, and the thermal effect in them can be suppressed by field-correlation method. Such studies of coexisting Raman- and Rayleigh-enhanced four-wave mixing processes can have important applications in coherence quantum control, and quantum information processing.     

The interplay of thermal and pump fluctuations in stimulated Brillouin scattering

We present a experimental and theoretical investigation of spontaneously initiated stimulated Brillouin scattering in which the interplay of two independent noise sources (thermal and pump) can be studied by controlling the relative importance of each source. We vary the pump noise by adding a controlled amount of Gaussian noise to the input pulses, and we control the contribution of the thermal noise by examining the energy statistics of both entire scattered pulses and of temporal slices of the scattered pulses. We show that the energy of the whole Stokes pulses follow a Gaussian distribution but that the energy of the Stokes pulse slices do not.     

Stimulated Brillouin scattering in magnetized diffusive semiconductor plasmas

Using the hydrodynamical model and following the coupled mode approach, detailed analytical investigation of stimulated Brillouin scattering is performed in an electrostrictive semiconductor. The total induced current density including diffusion current density and the effective Brillouin susceptibility are obtained under off-resonant laser irradiation. The analysis deals with the qualitative behaviour of the Brillouin gain and transmitted intensity with respect to excess doping concentration and magnetic field. Efforts are directed towards optimizing the doping level and magnetic field to achieve maximum Brillouin gain at pump intensities far below the optical damage threshold level. It is found that by immersing a moderately doped semiconductor in a sufficiently strong magnetic field in transverse direction, one can achieve resonant enhancement of Brillouin gain provided the generated acoustic mode lies in the dispersionless regime.     

Investigation on the output energy characteristic of optical limiting based on stimulated Brillouin scattering

Stimulated Brillouin scattering (SBS) featuring sub-nanosecond response time takes place at a high power threshold, which enables its application at a high power density. When the intensity of input light excesses the SBS threshold, strong SBS process takes place through SBS medium, leading to a quick energy transfer from pump to the Stokes and thereby an optical limiting characteristic in the output energy. In this paper, the correlation between SBS output energy and input power density is numerically simulated and validated in the Nd: YAG Q-switch laser system. The results indicate that not only the output energy exhibits an optical limiting characteristic, but also the clamped value of output energy can be controlled by changing the medium or the focal length.     

Stimulated raman scattering of fuel droplets

The strong stimulated Raman scattering (SRS) from diesel fuel droplets has the potential of providing the relative concentration of multicomponent fuel and the absolute size of individual droplets. The morphology-dependent resonances (MDRs) of a sphere cause the droplet to act as an optical resonator which greatly lowers the SRS threshold. The number density, quality factor, and frequency shift of several MDRs are calculated as a function of the ratio of the index of refraction of the liquid and the surrounding gas, which approaches unity at the thermodynamic critical condition for the fuel spray. The SRS spectra of monodispersed droplets of toluene, pentane, Exxon-Aromatic-150, and Mobil D-2 are presented. The exponential growth region of the SRS intensity I _1S as a function of the input laser intensity I _input is investigated for the toluene carbon ring breathing mode v ₂ and the pentane C-H stretching region. The I _1S ratio of toluene and pentane is measured as a function of the ratio of the toluene and pentane concentration for monodispersed droplets. The reduced fluctuation in I _1S when I _input is changed from multimode to single-mode is displayed as a histogram of the I _1S of the v ₂ mode of toluene droplets.     

Transient conical parametric scattering of two orthogonally polarized waves in BaTiO3

The strength of the transient parametric scattering in BaTiO₃ is shown to be strongly dependent on the initial conditions of the sample illumination. It is shown that the effect can be explained by a considerable increase of the seeding radiation intensity after pre-exposure of the sample to the ordinarily polarized pump beam. Received: 27 March 2000 / Published online: 16 June 2000     

Threshold of oscillation in a ring-loop phase conjugator as a second-order optical phase transition

The threshold behavior is studied for a ring-loop coherent oscillator with a photorefractive strontium barium niobate (SBN) sample. A soft onset of oscillation is revealed and critical slowing down is observed in the temporal development of light-induced scattering below the threshold, thus pointing to a similarity with a second-order phase transition. Received: 10 July 2000 / Published online: 20 September 2000     

Photorefractive four-wave mixing in a high-contrast regime

The effect of high contrast in photorefractive four-wave mixing is studied using a recently proposed empirical formula for the grating amplitude. An analytical solution to the coupled-wave equation is obtained and its properties are discussed in the case of a double-phase-conjugate mirror and semilinear phase-conjugate mirror.     

Theoretical analysis of a Brillouin switch for amplifier decoupling and prepulse suppression in short-pulse high-power laser systems

A switch suited for high-power amplifier chains emitting nanosecond pulses is theoretically investigated. It is based on a two-step Brillouin backscattering process. Gases like N₂ or SF₆ at high pressure are used as the scattering medium. The transmission efficiency is about 50%. The limitation is mainly due to gas breakdown. The capability for amplifier decoupling and prepulse suppression is excellent. Strong pulse steepening favors the generation of ultra-short laser pulses.     

Origin of low-frequency spectrum structure of four-photon scattering in liquid water

-1 has been found experimentally in liquid water. The theoretical interpretation relates these spectral features to an interference of strictional and orientational contributions to the scattered signal. Received: 16 October 1996     

Highly efficient Raman conversion in O2 pumped by a seeded narrow band second-harmonic Nd:YAG laser

The first-Stokes conversion efficiency for a stimulated Raman scattering (SRS) is usually very low in gaseous oxygen media. In 3.0 Mpa O₂, a single longitudinal mode second harmonic Nd:YAG laser pump source gives a typical vibrational first-Stokes conversion efficiency of only 2.5%, In comparison, the accompanying stimulated Brillouin scattering (SBS) attains a reflectivity of 67%. However, by seeding an OPO beam into the Raman cavity, the first-Stokes photon conversion efficiency now attains a peak value of 54%, while the SBS reflectivity reduces to 5% in a 6.1 Mpa 41:59 O₂/ He mixture. This 54% efficiency was obtained for a seeder laser pulse-width less than one half that of pump laser (6.8 ns). A first-Stokes peak power conversion efficiency as high as 88% has been obtained when the pump and seeder pulse peaks coincide. So, we may expect a higher first-Stokes photon conversion efficiency if the seeder pulse-width can be made equal to or larger than that of the pump pulse. On the other hand, the beam quality of the first-Stokes in an O₂/ He mixture excels that of the pump laser for a seeder energy of 5 mJ and pump energy of 50 mJ. However, at pump energies higher than 105 mJ and a pump laser repetition rate of 10 Hz, the thermal defocusing effect worsens the first-Stokes beam quality. This thermal defocusing effect is a result of the Raman heat release and could be eliminated by fast circulating and cooling the Raman gas medium.     

Study of beam-fanning hysteresis in photo- refractive SBN:Ce: light-induced and primary scattering as functions of polar structure

We study light-induced scattering (beam-fanning) in the photorefractive crystal SBN:Ce as a function of the polar structure of the crystal. The spatial structure of the beam-fanning is measured at different externally applied electric fields, and an optical hysteresis is found in the scattering. It is shown that the scattering hysteresis results from a polarization hysteresis typical for ferroelectrics in the polar phase. New information about primary scattering in SBN is obtained, and a corresponding model of its origin is proposed. It is shown that the intensity and angular distribution of the primary scattering strongly depend on the polar structure of the crystal and can be affected by the subsequent action of an external field and coherent illumination. Received: 27 August 2002 / Revised version: 19 December 2002 / Published online: 26 March 2003 RID="*" ID="*"Corresponding author. E-mail: mirco.imlau@uni-osnabrueck.de     

Nonlinearity of a response in photorefractive crystals with a square-wave applied field

The space-charge-field formation in a photorefractive crystal illuminated by a one-dimensional light pattern is studied when an alternating square-wave electric field is applied to the crystal. We derive the general nonlinear equation for the time-averaged distribution of the space-charge field and employ the simplified versions of this equation to analyze the space-charge-field formation in the case of a Gaussian beam and interference light pattern. The borders of the applicability of simplified equations and analytic expressions to describe a self-action of light beams and the large modulation effects under two-beam coupling are estimated from the numerical calculations. Received: 18 November 1998 / Revised version: 26 January 1999 / Published online: 12 April 1999     

Effects of dark soliton crystal temperature on the self-deflection of bright soliton in a biased serial photovoltaic photorefractive crystal circuit

Based on the theory of one-dimensional separate soliton pairs formed in a serial photovoltaic photorefractive crystal circuit, the effects of the dark soliton crystal temperature on the self-deflection of the bright one in a bright-dark soliton pair are investigated. The numerical results indicate that the spatial shift of the bright soliton can experience obvious increase in their self-deflection with the increase of the temperature of the dark soliton. The self-bending process is further studied using perturbation techniques and the results are found to be good agreement with that obtained by numerical method.