Nuclear viscosity of hot rotating 240Cf

In a detailed investigation of giant dipole resonance (GDR) γ-ray yield from ²⁴⁰Cf populated in the ³²S + ²⁰⁸Pb reaction, the absolute γ-ray/fission multiplicities are extracted over a wide range of excitation energy and angular momentum. The enhanced yield of GDR decay γ rays has been analyzed within the framework of a modified statistical model containing the nuclear viscosity as a free parameter. The extracted nuclear dissipation coefficient is found to be independent of the temperature. Large constant dissipation during the saddle-to-scission path provides good fits to the γ-ray spectra.     

A study of charge,energy and angular momentum transfer in the 56Fe + 197Au and 56Fe + 107, 109Ag reactions at 7.2 and 8.3 MeV/nucleon

Kinetic energy spectra, charge and angular distributions have been measured for thirty elements produced in the reactions of 401 and 460 MeV ⁵⁶Fe + ¹⁹⁷Au and in the reaction of 470 MeV ⁵⁶Fe + ^{107, 109}Ag. In addition, γ-ray multiplicities were measured at the 470 MeV bombarding energy for both targets at a limited number of angles. The charge distributions for the deep-inelastic component of these systems increase monotonically with atomic number in the measured angular range, whereas, those for the quasielastic component are skewed toward Z-values below the projectile. The angular distributions for the Fe-induced reactions show a smooth evolution from a side-peaked to forward-peaked distributions with increasing mass transfer. This side peak is more intense and more persistent for mass transfers from the projectile to the target. In the quasielastic region the γ-ray multiplicity is observed to increase almost linearly with decreasing Q-value whereas for large negative β-values it is essentially constant and independent of the exit channel mass asymmetry. Finally, angular distributions, angle-integrated charge distributions and γ-ray multiplicities have been compared with a diffusion model in which the dynamics of shape evolution, N/Z equilibration, angular momentum and energy exchange occur via one-body forces.     

Gamma decay after heavy ion reactions studied by first and higher order multiplicity measurements

First and higher order multiple coincidence rates have been measured for the γ-rays from ¹⁶O induced reactions on targets of ^148,150Nd at various bombarding energies. Average values and shape parameters for the γ-ray multiplicity distributions have been extracted from the data. The multiplicities are connected to angular momentum through complete fusion cross sections, and conclusions are drawn on spin distributions of entry states in the final nuclei as well as on the decay pattern from these states.     

High-spin states and yrast isomerism in 153Er

Energy levels in ¹⁵³Er have been populated in the reaction ¹⁴⁴Sm(¹²C. 3n)¹⁵³Er. Isotopically enriched targets were bombarded with 53–65 MeV ¹²C ions and the emitted γ-ray and conversion electron spectra were investigated. From studies of excitation functions. γ- coincidences, γ-ray multiplicities, delayed γ-radiation and angular distributions, the level scheme of ¹⁵³Er has been constructed. The properties of the energy levels are discussed and compared with the results of calculations with a deformed shell model. The remarkable similarities and some important discrepancies of the level structure, when compared with adjacent, N = 85 nuclides, are emphasized.     

Investigation of giant E3 resonances by (N, γ) reactions

Effects related to the presence of giant E3 resonances are investigated by nucleon radiative capture according to the direct-semidirect model. The γ-ray angular distributions from the ²⁰⁸Pb(N, γ₀) reactions are calculated in the energy region above the giant dipole resonance and the influence of the E1–E3 and E2–E3 interferences is discussed. The results provide indications of an appreciable effect on the 90° photon emission when a collective isovector E3 excitation is present.     

Giant M1 resonance in the direct-semidirect model for nucleon radiative capture

The direct-semidirect model for nucleon radiative capture proceeding via giant E1 and E2 resonance states is extended to account for capture through collective M1 excitation. The ²⁰⁸Pb(N, γ₀) and ¹⁴⁰Ce(N, γ₀) reactions are investigated in the 2–10 MeV energy interval. For the M1 and isoscalar E2 neutron capture processes, calculations provide cross section values of the same order of magnitude, as well as comparable effects on γ-ray angular distributions. The model proves to be an appropriate framework for discussing the E1-M1 and E1-E2 interference processes, giving useful suggestions as to effects arising from the presence of the M1 and E2 collectivities.     

Étude des isotopes du plomb de masse 200, 198, 196 et 194 formés par réaction (ions lourds, xn)

The low-lying excited states of ^{194, 196, 198, 200}Pb have been studied through the de-excitation γ-rays following the reactions Os(¹²C, 4n), W(¹⁶O, 4n) and Re(¹⁴N, 5n). Prompt and delayed spectra, γ-γ coincidences, γ-ray angular distributions and γ-ray time distributions have been obtained. Half-lives were measured for the 12⁺ level in the four isotopes, for the 9^? level in ^{194, 196, 200}Pb, for the ^7? level in ²⁰⁰Pb and for the ^5? level in ^{196, 198}Pb. The results of microscopic calculations, performed with either a Gaussian interaction or a surface delta interaction, are compared to the experimental level schemes and transition probabilities, and discussed.     

Volume form of coupling interaction in semi-direct (n, γ) and (p, γ) reactions

A coupling interaction between the nucleon and the nuclear E1 mode having a volume radial form instead of the usual surface one is used in the semi-direct nucleon radiative-capture theory. The calculated cross sections for the ²⁰⁸Pb(n,γ) and ¹⁴²Ce(p,γ) reactions in the giantresonance region reproduce the measured ones both in shape and magnitude. Satisfactory agreement is achieved in comparing the predicted and detected γ-ray spectra following neutron capture by ²⁰⁸Pb. A detailed analysis of the energy and angular-momentum dependence of the matrix elements when the volume and surface form factors are used, is performed.     

Energy and angular momentum transfers in equilibrium and pre-equilibrium 158Gd(α, xn) reactions

Neutron time-of-flight spectra and γ-ray multiplicities were measured in coincidence with discrete γ-rays for specific exit channels in the ¹⁵⁸Gd(α, xn) reactions at E_α = 70 MeV. The neutron energy spectra and angular distributions were analysed in terms of equilibrium and non-equilibrium decay processes. Significant emission of non-equilibrated neutrons was found, amounting to about 40 %, 25 % and 15 % of the total neutron emission in the 4n, 5n and 6n exit channels, respectively. The corresponding average kinetic energies in this precompound phase were around 12, 8 and 4.5 MeV. The angular momentum carried away by the neutrons was found to be rather constant for all exit channels and on the average about 3? units. It is found that the total energy and angular momentum removed by the neutrons and γ-rays agrees within the experimental errors with the calculated values for the compound nucleus.     

The level structure of the 153Gd nucleus studied in the 150Sm(α, n)153Gd reaction

The level structure of ¹⁵³Gd has been studied by means of the ¹⁵⁰Sm(α, n)¹⁵³Gd reaction. The experiment included measurements of γ-γ coincidences, γ-angular distributions, γ-ray yield at 17 MeV and 19 MeV beam energy, and γ-ray multiplicities. Favoured and unfavoured members of the positive-parity i_13,2, band were identified. States belonging to the h_9,2 and f_7,2 band structures have been located.Surprisingly low multiplicity numbers were deduced for ₁₅₃Gd γ-rays. This may indicate that the (α, n) reaction is not a pure compound reaction. The level structure of ¹⁵³Gd has been compared to the known structure of other odd-mass N = 89 nuclei, and a close similarity is found.The positive-parity band structure has been compared to calculations with the pairing-plus-recoil model. Good agreement is obtained without any ad hoc Coriolis attenuation.     

Limitation to complete fusion in the reactions 12,13C+48Ti and 30Si+30Si

Excitation functions of the reactions ^{12, 13}C+⁴⁸Ti and ³⁰Si+³⁰Si were measured by in-beam γ-ray spectrometry in the energy ranges 20–60 MeV for the ^{12, 13}C induced reactions and 55–126 MeV for the ³⁰Si+³⁰Si reaction. Light-particle angular distributions were measured at 46 MeV and 47.5 MeV for the ¹³C and ¹²C induced reactions. Measurements of elastic scattering angular distribution and particle-γ coincidences were carried out for the system ¹³C+⁴⁸Ti at 46 MeV. The limitation to complete fusion detected for the system ³⁰Si+³⁰Si appears to be related to entrance channel effects and is well reproduced by a barrier penetration calculation using the KNS potential. The angular distribution measurements carried out for the ¹²C+⁴⁸Ti and ¹³C+⁴⁸Ti systems allowed to identify an incomplete fusion mechanism with emission of direct α-particles before the formation of a fully equilibrated system.     

Evidence for quasi-fission in40Ar+208Pb collisions near the coulomb-barrier

Fission-fragment angular distributions were measured in the reaction of⁴⁰Ar with²⁰⁸Pb near the fusion barrier. For nearly symmetric mass-/charge splits we find angular distributions symmetric around θ=90 degrees, however, with unusually large anisotropies. These develop gradually into forward-backward asymmetric distributions as one moves away from mass-/charge symmetry. This indicates that non-compound fission (‘quasi-fission’) competes with true fusion-fission. The relative contribution of quasi-fission to the total fission cross section is somewhere between 51 and 85%. In the framework of the extra-push model this is equivalent to an extra-extra push energy for compound-nucleus formation inside the true fission saddle point of 4<E _xx <9 MeV in agreement with a recent empirical parametrization of fusion-barrier shifts based on fusion-fission cross sections. On the basis of cross sections for fusion-evaporation residues it had previously been concluded that fusion of⁴⁰Ar with Pb isotopes occurs unhindered. Possible reasons for this apparent discrepancy are discussed.     

Spontaneous-fission decay properties and production cross-sections for the neutron-deficient nobelium isotopes formed in the 44, 48Ca + 204, 206, 208Pb reactions

Heavy-ion fusion reactions ⁴⁸Ca + ²⁰⁴Pb and ⁴⁴Ca + ²⁰⁸Pb leading to the same compound nucleus ²⁵²No^* were run in attempts to produce new neutron-deficient spontaneous-fission isotopes of ^249,250No using the electrostatic separator VASSILISSA. Production cross-sections for the spontaneous-fission activities with the half-lives 5.6 and 54 μs observed in these reactions are compared with the measured ones for the well-known isotopes of ^{251 - 255}No formed in the heavy-ion fusion reactions ⁴⁸Ca + ²⁰⁶Pb and ⁴⁸Ca + ²⁰⁸Pb. The obtained excitation functions for the reaction products formed after the evaporation of 1-4 neutrons from the corresponding compound No nuclei have been compared with similar data obtained earlier and results of statistical model calculations. Received: 26 July 2002 / Accepted: 5 November 2002 / Published online: 18 March 2003 RID="a" ID="a"e-mail: eremin@sunvas.jinr.ru Communicated by J. ?yst?     

Angular anisotropy of the fusion-fission and quasifission fragments

The anisotropy in the angular distribution of the fusion-fission and quasifission fragments for the ¹⁶O + ²³⁸U , ¹⁹F + ²⁰⁸Pb and ³²S + ²⁰⁸Pb reactions is studied by analyzing the angular-momentum distributions of the dinuclear system and compound nucleus which are formed after capture and complete fusion, respectively. The orientation angles of the axial symmetry axes of the colliding nuclei relative to the beam direction are taken into account for the calculation of the variance of the projection of the total spin onto the fission axis. It is shown that there is a large contribution of the quasifission fragments in the ³²S + ²⁰⁸Pb reaction to the deviation of the experimental angular anisotropy from the statistical model results. Enhancement of anisotropy at low energies in the ¹⁶O + ²³⁸U reaction is connected with the quasifission of the dinuclear system having low temperature and relatively small effective moment of inertia.     

Finite-range nucleon-nucleon interaction in the radiative capture of fast nucleons

The direct-semidirect model for nucleon radiative capture has so far been formulated assuming a zero-range nucleon-nucleon interaction. An extension of the theory to finite-range forces is proposed here. The usual δ-function in the interaction is replaced by a range-dependent gaussian function and then the radial form factor in the particle-vibration coupling (responsible for excitation of the E1 and E2 giant resonance states) is derived. Calculations are performed for the ¹⁴²(p, γ) reaction in the 5–30 MeV energy region. A detailed analysis provides indications on effects related to the interaction range as regards both the E1 and E2 integrated cross sections and the forward-backward asymmetry of the γ-ray angular distributions. Sensitivity to the interaction range shows connections with the proton final-level spin.     

Investigation of the fusion-fission reaction 12C+208Pb

For the first time the cross section and angular distributions of fission fragments have been measured for the compound nucleus 220 Ra produced in the reaction 12 C+ 208 Pb at three energy values in the range from 0.5 to 8.0 r MeV below the fusion barrier calculated in terms of the Bass model. In the investigated energy range there is a plateau characterized by the relation W (180°)/ W (90°)=1.2 in the angular anisotropy of fission fragments.     

Quantum molecular dynamics approach to estimate spallation yield from<Emphasis Type="Italic">p</Emphasis> +<Superscript>208</Superscript>Pb reaction at 800 MeV

The spallation yield of neutrons and other mass fragments produced in 800 MeV proton induced reaction on²⁰⁸Pb have been calculated in the framework of quantum molecular dynamics (QMD) model. The energy spectra and angular distribution have been calculated. Also, multiplicity distributions of the emitted neutrons and kinetic energy carried away by them have been estimated and compared with the available experimental data. The agreement is satisfactory. A major contribution to the neutron emission comes from statistical decay of the fragments. For mass and charge distributions of spallation products the QMD process gives rise to target-like and projectile-like fragments only.     

Gamma-ray multiplicities in α-induced compound and precompound reactions

Measurements of γ-ray multiplicities from the¹⁵⁰Sm(α, xn) reactions at beam energies from 40–140 MeV show that the maximum angular momentum transfer occurs at an energy between 12 and 18 MeV higher than that of the maximum of the excitation function for the respective exit channel. At still higher bombarding energies, where precompound processes dominate, a decrease of the multiplicity is observed.