The 16O(d, 3He)15N reaction at 29 MeV: Reaction mechanism and nuclear structure

The reaction ¹⁶O(d, ³He)¹⁵N has been investigated using 29 MeV deuterons, and angular distributions were obtained for levels in ¹⁵N up to 10 MeV excitation energy. The measured distributions were subjected to distorted-wave (DWBA), compound nucleus (Hauser-Feshbach) and coupled-channel (CCBA) analyses. Only the strong transitions to the $\text{1}\text{2}$^? ground state and the $\text{3}\text{2}$^? state at 6324 keV exhibit distributions which are well described by DWBA. The spectroscopic factors are in agreement with shell-model estimates. The weak transitions generally show little structure and the spectroscopic factors extracted for these transitions tend to be unreasonably large. Contributions from compound nucleus formation were estimated and found to vary between about 10 % and 100 % of the observed cross sections with an average of the order of 30 %. The CCBA analysis for the transitions to the $\text{5}\text{21}{}^{\mathrm{+}}$, $\text{5}\text{22}$⁺ and $\text{7}\text{2}$⁺ states at 5271, 7155 and 7566 keV, respectively, was performed using the spectroscopic amplitudes from weak coupling shell-model wave functions. Inelastic excitations to one-phonon states in the target and residual nuclei were included. The agreement between calculated and experimental distributions is good for both shape and magnitude, a conclusion which is not disturbed by the addition of small compound nucleus contributions. It is evident that spectroscopic factors extracted for the weak transitions on the basis of a direct one-step reaction mechanism alone are unreliable.     

Electronic transition dipole moments and excited-state alignment in linear molecules,with application to diatomic rare gas halides

The relationship between the direction of transition dipoles and the symmetry of electronic wavefunctions is investigated. In the case of $\text{Ω}\text{=}\text{1}\text{2}\text{?}\text{Ω′}\text{=}\text{1}\text{2}$ transitions, the dipole direction is not determined by symmetry alone. However, in all other cases the directions (parallel or perpendicular) are specified by simple selection rules based upon $\text{ΔΩ}$. In $\text{Ω}\text{=}\text{1}\text{2}\text{Ω′}\text{=}\text{1}\text{2}$ transitions, the transition dipole may accidentally have spherical symmetry, in which case a linearly polarized plane wave photon beam produces an unaligned excited-state distribution. These results are applied to the ultraviolet charge transfer transitions of the diatomic rare gas halides.     

The ground state of propynal

The millimeter wave spectrum of propynal, HCCCHO, has been studied in the ground vibrational state. A detailed centrifugal distortion analysis has been carried out on the combined data of newly assigned millimeter wave rotational transitions (up to 200 GHz) together with the microwave transitions reported earlier. A total of 90 transitions as high as J = 20 and K = 12 could be fitted with a standard deviation of 87 kHz. This analysis yielded a complete set of ground state rotational and centrifugal distortion constants. The rotational constants are in MHz:

$\text{A = 68 035.2994 ± 0.0429,}$

$\text{B =}\text{4826.3014 ± 0.0073,}$

$\text{C =}\text{4499.5107 ± 0.0069.}$

     

The interaction of nucleons with antinucleons. III. Photon and pion emission from bound states

We calculate widths and branching ratios for the emission of γ rays or pions from a bound state of the nucleon-antinucleon ($\text{N}\text{N}$) system, leading to another $\text{N}\text{N}$ bound state. We use a realistic potential model to describe the medium- and long-range parts of the $\text{N}\text{N}$ interaction, and parametrize the short-range behavior. The general features of γ and π transitions, based on the selection rules, are emphasized. We illustrate these features with typical results for several choices of the short-range cutoff. The observation of pions is a necessary supplement to the γ-ray experiments, in order to significantly constrain the possible quantum number assignments of final states. We investigate transitions between quasiatomic (QA) and more deeply bound quasinuclear (QN) states, and also QN to QN γ or π emission. The former may have been seen in experiments involving the $\text{p}\text{p}$ atom, while the latter are in some optimum cases accessible in $\text{p}\text{d}$ spectator experiments, although there is no evidence for these QN to QN transitions as yet. The role of isospin mixing in QA states is discussed, as well as the importance of maintaining orthogonality of the QA and QN wave functions.     

Radiative strength functions in odd-A spherical nuclei

The radiative strength functions for the partial γ-transitions from neutron resonances to the ground and low-lying states of odd-A spherical nuclei are calculated within the quasiparticle-phonon nuclear model. The fragmentation of one-quasiparticle and quasiparticle-plus-phonon states is calculated. This allowed one to calculate γ-transitions between the one-quasi-particle components (valence transitions) and γ-transitions between the quasiparticle-plus-phonon and one-quasiparticle components of the wave functions. The energy dependence of the strength functions $\text{C}$(E1, η) and $\text{C}$(M1, η) is calculated near the neutron binding energy B_n for ⁵⁵Fe and ^{59, 61}Ni. The corresponding experimental data are described qualitatively. The contribution of the valence E1 transitions to the strength function is shown to be from 20% to 90%, and M1 transitions about 1%. The influence of the M1 giant resonance is important for M1 transition probabilities.     

On the reactions pp ↔ dπ+

The total cross section for π⁺d → pp and the angular distribution and asymmetry parameters for the inverse reaction $\text{p}\text{p}\text{→ π}{}^{\mathrm{+}}\text{d}$ have been calculated with different models for the pion absorption (and production) operator and several sets of nuclear wave functions. The absorption operator includes both single-nucleon and two-nucleon operators. Fair agreement can be achieved with all empirical parameters at low energies, but significant discrepancies occur at high energies. The results are very sensitive to the model for the nucleon-nucleon interaction used to generate the wave functions.     

Coupling constants and the nonrelativistic quark model with charmonium potential

Hadronic coupling constants of the vertices including charm mesons are calculated in a nonrelativistic quark model. The wave functions of the mesons which enter the corresponding overlap integrals are obtained from the charmonium picture as quark-anti-quark bound state solutions of the Schrödinger equation. The model for the vertices takes into account in a dynamical way the SU₄ breakings through different masses of quarks and different wave functions in the overlap integrals. All hadronic vertices involving scalar, pseudoscalar, vector, pseudovector and tensor mesons are calculated up to an overall normalization constant. Regularities among the couplings of mesons and their radial excitations are observed: (i) Couplings decrease with increasing order of radial excitations; (ii) in general they change sign if a particle is replaced by its next radial excitation. The k-dependence of the vertices is studied. This has potential importance in explaining the unorthodox ratios in different decay channels (e.g. $\text{D}\text{D}\text{, D}\text{D}{}^1\text{, D}{}^1\text{D}{}^1$). Having got the hadronic couplings radiative transitions are obtained with the current coupled to mesons and their recurrences. The resulting width values are smaller than those conventionally obtained in the native quark model. The whole picture is only adequate for nonrelativistic configurations, as for the members of the charmonium- or of the γ-family and most calculations have been done for transitions among charmed states. To see how far nonrelativistic concepts can be applied, couplings of light mesons are also considered.     

Study of 39K levels via the 39K(α, α') reaction

The ³⁹K(α, α') reaction has been studied at E_α = 31 MeV. A number of hole-core coupled states were identified by their strong excitations with angular momentum transfers of L = 3 or 5. The L = 3 transitions showed fairly good agreement with strengths predicted from holecore coupled wave functions. However, agreement between experiment and theory for the states excited by L = 5 excitations $\text{(}\text{11}\text{2}{}^{\mathrm{?}}\text{and}\text{13}\text{2}{}^{\mathrm{?}}\text{levels}\text{)}$ requires accounting for the blocking effects in the wave functions for these levels.     

Opto-electronic properties of CuAlO2

CuAlCO₂ is a p-type semiconductor with an average hole mobility of $\text{1.1 × 10}{}^{\mathrm{?7}}\text{m}{}^2\text{Vs}$. From photoelectrochemical measurements its bandgap is found to be indirect allowed at 1.65 eV; other interband transitions are at 2.3 and 3.5 eV. The valence band is made up mainly from Cu-3d wave functions and lies 5.2 eV below the vacuum level.     

Inelastic processes and form factor effects in the 162, 164Dy(3He,d) reactions at 46.5 MeV

The 162, 164Dy(³He, d) reactions at E_3He = 46.5 MeV are analyzed using the coupled channels Born approximation (CCBA) and improved form factors derived from a deformed Woods-Saxon potential. The latter are generated using the coupled channels procedure of Rost. The transitions considered populate the $\text{7}\text{2}$^?[523], $\text{1}\text{2}$⁺[411], $\text{3}\text{2}$⁺[411], $\text{1}\text{2}$^?[541] and $\text{5}\text{2}$⁺ orbitals in ^{163, 165}Ho. Indirect processes induced by inelastic scattering are found to have an influence on the cross sections comparable to that deduced for neutron transfer reactions on rare earth nuclei at lower energies. Considered alone, these can alter the cross sections even of strong transitions by a factor of two and of weaker ones by an order of magnitude. For the weaker transitions equally large changes can result when the improved form factors, rather than conventional spherical Woods-Saxon functions, are used in the calculations. In the examples considered these two effects tend to cancel, often, but not always, resulting in predicted cross sections similar in magnitude to the results of conventional DWBA calculations made with spherical Woods-Saxon form factors. The CCBA angular distributions are generally similar in shape to DWBA predictions, which usually give good fits to the experimental angular distributions over the 0–35° range of the data. Compared with DWBA predictions which use (he same optical parameters, but spherical Woods-Saxon form factors, the CCBA with deformed Woods-Saxon form factors is in better overall agreement with the experimental cross-section magnitudes. However there are a number of cases in which the CCBA, although usually predicting larger cross sections than the DWBA, still underestimates the experimental cross sections by nearly factor of two. These cases all occur in the $\text{71}\text{2}$^?[541] band or in the strongly Coriolis mixed $\text{1}\text{2}$⁺[411] and $\text{3}\text{2}$⁺[411] bands, and include the majority of transitions populating these orbitals. Since both nuclear structure and reaction mechanism effects are interwoven m the calculations, further data would be most useful in probing the origin of the discrepancy.     

Study of the 176Lu(n, γ)177Lu reaction using a gamma band-filter spectrometer

The γ-ray spectrum from the ¹⁷⁶Lu(n, γ)¹⁷⁷Lu reaction has been investigated in the energy range 450 to 1420 keV using a newly developed gamma band-filter spectrometer. A total of 153 transitions have been observed. Improvements to the ¹⁷⁷Lu scheme are suggested, and in particular the γ-decay of several levels of the $\text{1}\text{2}$^?[530↑] and $\text{3}\text{2}$^?[532↓] rotational bands is proposed. Special attention has been given to the Coriolis coupling between the two latter bands and the $\text{1}\text{2}$^?[541↓] band. Results on a complementary investigation of the ¹⁷⁵Lu(n, γ)¹⁷⁶Lu reaction are presented.     

Spectroscopy of 62Ni with the 61Ni(d, p) reaction

Differential cross sections, vector and tensor analysing powers have been measured for the ⁶¹Ni(d, p) reaction at a deuteron energy of 12.3 MeV. Most of the 30 transitions observed below 8.5 MeV excitation are dominated by a single j-value, which was determined from behaviour of the analysing power data. For a number of transitions it was possible to make unambiguous j-assignment relying on the established j-dependence of the T₂₂ tensor analysing power. The deduced spectroscopic factors indicate that the full strength of neutron transfer to the ($\text{2p, 1f}{}_{\mathrm{<mtext>5</mtext><mtext>2</mtext>}}$) and $\text{1}\text{g}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}$ orbits was found and seven $\text{5}\text{2}{}^{\mathrm{+}}$ transitions were located above 5.3 MeV. The separated strengths of the $\text{3}\text{2}{}^{\mathrm{?}}\text{,}\text{1}\text{2}{}^{\mathrm{?}}\text{and}\text{5}\text{2}{}^{\mathrm{?}}$ transitions are compared with shell-model calculations for the low-lying states of ⁶²Ni.     

The reaction 67Zn(t, α)66Cu

Levels of ⁶⁶Cu have been studied using the (t, α) reaction on ⁶⁷Zn at 18 MeV. Orbital and, in some cases, total angular momentum transfer were inferred from a comparison of differential cross sections with those measured for the same reaction on the even zinc isotopes. The quartet of levels corresponding to the p_{$\text{3}\text{2}$} proton pick-up from the $\text{5}\text{2}$^? target was identified. In addition, a strong set of l = 3 transitions was found corresponding to pickup from the f_{$\text{7}\text{2}$} proton shell.     

Spins and lifetimes of levels in 55Mn

The study of excited ⁵⁵Mn levels with the ⁵²Cr(α, pγ) reaction was extended to levels up to 3161 keV. With a Ge(Li) detector, DSA measurements in gold-backed targets were made, as well as angular correlations; both of these experiments were done in coincidence with protons detected near 180°. A multiple-detector NaI(Tl) array was also used in the same reaction geometry for better γ-ray detection efficiency. Mean lifetimes of 12 levels from 2727 to 3161 keV are reported. Spins and sometimes parities of the following levels were deduced from the angular-correlation analyses and lifetime results: 1885 keV, $\text{7}\text{2}$^?; 2199 keV, $\text{7}\text{2}$(^?); 2311 keV, ($\text{13}\text{2}$); 2366keV, $\text{5}\text{2}$^?; 2727 keV, $\text{7}\text{2}$; 2823 keV, $\text{9}\text{2}$. Multipole mixing ratios and M1 and E2 transition rates of the radiations from these and from the 1292 keV level are presented. The similarity of the low-lying level structure and of interlevel transitions in ⁵⁵Mn to those in certain other f_{$\text{7}\text{2}$}³ nuclei is examined.     

A particle-gamma correlation study in the 52Cr(d,pγ) reaction

Particle-gamma angular correlations for states populated in the ⁵²Cr(d, p) reaction have been measured. States in ⁵³Cr for which data are presented are the $\text{5}\text{2}$^?, 1.01 MeV, the $\text{7}\text{2}$^?, 1.29 MeV, the $\text{7}\text{2}$^?, 1.54 MeV, and the $\text{3}\text{2}$^?, 2.32 MeV levels. The DWBA is found to give a good representation of the data for strongly populated levels when the particle detector is located near the stripping peak. The data for the 1.29 MeV level confirm the previously suggested particle-excited core wave function.     

States in 163Dy and 169Er populated in the (t,p) reaction

Angular distributions of protons from the ¹⁶¹Dy(t, p)¹⁶³Dy and ¹⁶⁷Er(t, p)¹⁶⁹Er reactions were studied, using 15 MeV and 17 MeV tritons from the McMaster University tandem Van de Graaff accelerator. The reaction products were analyzed with a magnetic spectrograph and detected with nuclear emulsions. Since the ¹⁶¹Dy target ground state is the $\text{5}\text{2}$⁺[642] orbital, a strong L = 0 transition was observed to the $\text{5}\text{2}$⁺[642] bandhead in ¹⁶³Dy, which was previously assigned at 251 keV. Also transitions to the $\text{7}\text{2}$, $\text{9}\text{2}$ and $\text{11}\text{2}$ band members were observed. Similarly, a strong L = 0 transition was observed to the $\text{7}\text{2}$⁺[633] bandhead at 244 keV in ¹⁶⁹Er, with the other band members only weakly populated. The angular distributions to the various members of these two bands can be described when higher-order reaction processes are taken into account. In ¹⁶³Dy, surprisingly strong L = 0 transitions were observed to levels at 1831 keV, 1937 keV and 2053 keV, with strengths of 23%, 30% and 37% of that for the $\text{5}\text{2}$⁺[642] bandhead. In ¹⁶⁹Er, the 905 keV level was populated with an L = 0 transition that had 31% of the strength observed for the strong L = 0 transition to the 244 keV level. The nature of these states is at present not understood.     

Gamma-rays from an incomplete fusion reaction induced by 95 MeV 14N

Gamma-rays from the ${}^{159}\text{Tb}\text{(}{}^{14}\text{N}\text{, αx}\text{n}\text{)}{}^{\mathrm{169?x}}\text{Yb}$ reaction, in which non-evaporation α-particles are emitted, have been identified. Yields of E2 cascade transitions suggest that the angular momentum distribution of the entrance channel leading to this reaction is localized just above the critical angular momentum for complete fusion.     

The adsorption of benzene and naphthalene on the Rh(111) surface: A LEED,AES and TDS study

The adsorption of benzene and naphthalene on the Rh(111) single-crystal surface has been studied by low-energy electron diffraction (LEED), Auger electron spectroscopy (AES) and thermal desorption spectroscopy (TDS). Both benzene and naphthalene form two different ordered surface structures separated by temperature-induced phase transitions: benzene transforms from a ($\text{3}\text{1}\text{1}\text{3}$) structure, which can also be labelled c($\text{2}\text{3}\text{× 4}$)rect, to a (3 × 3) structure in the range of 363–395 K, while naphthalene transforms from a ($\text{3}\text{3}\text{× 3}\text{3}$)R30° structure to a (3 × 3) structure in the range 398–423 K. Increasing the temperature further, these structures are found to disorder at about 393 K for benzene and about 448 K for naphthalene. Then, a first H₂ desorption peak appears at about 413 K for benzene and 578 K for naphthalene and is interpreted as due to the occurrence of molecular dissociation. All these phase transitions are irreversible. The ordered structures are interpreted as due to flat-lying or nearly flat-lying intact molecules on the rhodium surface, and they are compared with similar structures found on other metal surfaces. Structural models and phase transition mechanisms are proposed.