Comment on Lockerbie, N.A.: Gen. Rel. Grav. 36, 593 (2004)

We comment on the paper “ISLAND – Inverse-Square-Law Acceleration Measurement using Inertial Drift,” by Lockerbie, N.A.: Gen. Rel. Grav. 36, 593–600 (2004).     

Summation of electrostatic interactions in quasi-two-dimensional simulations

An error in our previous paper (Clark, A. T., Madden, T. J. and Warren, P. B., 1996 Molec. Phys., 87, 1063) is corrected. This brings the results into agreement with the recent work of Grønbech-Jensen et al. (Grønbech-Jensen, N., Hummer, G. and Beardmore, K. M., Molec. Phys., 1997, 92, 941).     

Identification of a TGBA liquid crystal phase via its defects

We have shown that cholesteryl nonanoate, a thermotropic compound which is well known to exhibit pretransitional effects at the smectic A (SmA) cholesteric (N*) transition (W.L. McMillan, Phys. Rev. A 4, 1238 (1971); 6, 936 (1972)), has in fact a TGBA phase in between. Our arguments rely on the observation of new TGBA defects, either in Robinson spherulites cooled from the N* phase or in free-standing films. The same new defects can be obtained in a well-documented TGBA phase of a tolane compound. We analyze qualitatively the TGBA defects in both geometries, in particular their relation to the disclination radius of the N* Robinson spherulites. Received 12 February 2001     

A wavelet-based method for multifractal image analysis. I. Methodology and test applications on isotropic and anisotropic random rough surfaces

We generalize the so-called wavelet transform modulus maxima (WTMM) method to multifractal image analysis. We show that the implementation of this method provides very efficient numerical techniques to characterize statistically the roughness fluctuations of fractal surfaces. We emphasize the wide range of potential applications of this wavelet-based image processing method in fundamental as well as applied sciences. This paper is the first one of a series of three articles. It is mainly devoted to the methodology and to test applications on random self-affine surfaces (e.g., isotropic fractional Brownian surfaces and anisotropic monofractal rough surfaces). Besides its ability to characterize point-wise regularity, the WTMM method is definitely a multiscale edge detection method which can be equally used for pattern recognition, detection of contours and image denoising. Paper II (N. Decoster, S.G. Roux, A. Arnéodo, to be published in Eur. Phys. J. B 15 (2000)) will be devoted to some applications of the WTMM method to synthetic multifractal rough surfaces. In paper III (S.G. Roux, A. Arnéodo, N. Decoster, to be published in Eur. Phys. J. 15 (2000)), we will report the results of a comparative experimental analysis of high-resolution satellite images of cloudy scenes. Received 8 July 1999     

Single-oscillator model and determination of optical constants of spray pyrolyzed amorphous SnO<Subscript>2</Subscript> thin films

It has recently been shown that growth of a multilayer structure with one or more delta-layers at high temperature leads to spreading and asymmetrization of the dopant distribution [see, for example, E.F.J. Schubert, Vac. Sci. Technol. A. 8, 2980 (1990), A.M. Nazmul, S. Sugahara, M. Tanaka, J. Crystal Growth 251, 303 (2003); R.C. Newman, M.J. Ashwin, M.R. Fahy, L. Hart, S.N. Holmes, C. Roberts, X. Zhang, Phys. Rev. B 54, 8769 (1996); E.F. Schubert, J.M. Kuo, R.F. Kopf, H.S. Luftman, L.C. Hopkins, N.J. Sauer, J. Appl. Phys. 67, 1969 (1990); P.M. Zagwijn, J.F. van der Veen, E. Vlieg, A.H. Reader, D.J. Gravesteijn, J. Appl. Phys. 78, 4933 (1995); W.S. Hobson, S.J. Pearton, E.F. Schubert, G. Cabaniss, Appl. Phys. Lett. 55, 1546 (1989); Delta Doping of Semiconductors, edited by E.F. Schubert (Cambridge University Press, Cambridge, 1996); Yu.N. Drozdov, N.B. Baidus', B.N. Zvonkov, M.N. Drozdov, O.I. Khrykin, V.I. Shashkin, Semiconductors 37, 194 (2003); E. Skuras, A.R. Long, B. Vogele, M.C. Holland, C.R. Stanley, E.A. Johnson, M. van der Burgt, H. Yaguchi, J. Singleton, Phys. Rev. B 59, 10712 (1999); G. Li, C. Jagadish, Solid-State Electronics 41, 1207 (1997)]. In this work analytical and numerical analysis of dopant dynamics in a delta-doped area of a multilayer structure has been accomplished using Fick's second law. Some reasons for asymmetrization of a delta-dopant distribution are illustrated. The spreading of a delta-layer has been estimated using example materials of a multilayer structure, a delta-layer and an overlayer.     

Failure of the collinear expansion in the calculation of the induced gluon emission

The collinear expansion is demonstrated to fail in the case of the gluon emission from a fast quark produced in eA deep inelastic scattering. In this approximation, the N = 1 rescattering contribution to the gluon spectrum vanishes. It has been shown that the higher-twist approach by X. N. Wang and X. Guo, Nucl. Phys. A 696, 788 (2001) and B. W. Zhang and X. N. Wang, Nucl. Phys. A 720, 429 (2003) based on the collinear expansion is wrong. The nonzero gluon spectrum obtained in those works is a consequence of an unjustified neglect of some important terms in the collinear expansion. The text was submitted by the authors in English.     

Application of conformal mapping to the determination of magnetic moment distributions in typical antidot film nanostructures

There has been an increasing technological interest on magnetic thin films containing antidot arrays of hexagonal or square symmetry. Part of this interest is related to the possibility of domain formation and pinning at the antidots boundaries. In this paper, we develop an accurate method for the simulation of the magnetic moments distribution for such arrays. The method concentrates the calculations on the immediate vicinity of each antidot. For each antidot distribution (square or hexagonal) a suitable system of coordinates is defined to exploit the shape of the unit-cells of the overall nanostructure. The Landau-Lifshitz-Gilbert-Brown equations that govern the distribution of moments are rewritten in terms of these coordinates. The moments orientation is calculated as a function of time until equilibrium is reached, in a Cartesian grid defined for these new coordinate systems. A conformal transformation is applied to insert the moment vectors into the actual unit-cell. The resulting vector maps display quite clearly regions of different moment orientation around the antidots, which can be associated with nanoscale domains. The results are similar to the ones obtained by other authors [C.C. Wang, A.O. Adeyeye, N. Singh, Nanotechnology 17, 1629 (2006); C.C. Wang, A.O. Adeyeye, N. Singh, Y.S. Huang, Y.H. Hu, Phys. Rev. B 72, 174426 (2005); C.T. Yu, H. Jiang, L. Shen, P. Flanders, G. Mankey, J. Appl. Phys. 87, 6322 (2000); E. Mengotti, L.J. Heyderman, F. Nolting, B.R. Craig, J.N. Chapman, L.L. Diaz, R.J. Matelon, U.G. Volkman, M. Klaui, U. Rudiger, C. Vaz, J. Bland, J. Appl. Phys. 103, 07D509 (2008)] using the NIST oommf method, but obtained in a much simpler and direct way.     

The mechanism of producing energy-polarization entangled photon pairs in the cavity-quantum electrodynamics scheme

We investigate theoretically two photon entanglement processes in a photonic-crystal cavity embedding a quantum dot in the strong-coupling regime. The model proposed by Johne et al. (Johne R, Gippius N A, Pavlovic G, Solnyshkov D D, Shelykh I A and Malpuech G 2008 Phys. Rev. Lett. 100 240404), and by Robert et al. (Robert J, Gippius N A and Malpuech G 2009 Phys. Rev. B 79 155317) is modified by considering irreversible dissipation and incoherent continuous pumping for the quantum dot, which is necessary to connect the realistic experiment. The dynamics of the system is analysed by employing the Born–Markov master equation, through which the spectra for the system are computed as a function of various parameters. By means of this analysis the photon-reabsorption process in the strong-coupling regime is first observed and analysed from the perspective of radiation spectrum and the optimal parameters for observing energy-entangled photon pairs are identified.     

Shaping of the electron distribution function in a striated solution

Numerous papers have been devoted to the investigation of striations in inert gases at low pressures (p⩽2 Torr) and small currents (i<100 mA) [A. V. Nedospasov, Sov. Phys. Usp. 11, 174 (1968); L. Pekarek, Sov. Phys. Usp. 11, 188 (1968); N. L. Oleson and A. W. Cooper, Adv. Electron. Electron Phys. 24, 155 (1968); P. S. Landa, N. A. Miskinova, and Yu. V. Ponomarev, Sov. Phys. Usp. 23, 813 (1980)]. Since the nature of striations is determined under these conditions by the nonlocal kinetics of the electrons in spatially periodic fields [L. D. Tsendin, Sov. J. Plasma Phys. 8, 228 (1982)], an investigation of the electron distribution function in space and time would be very interesting. The purpose of the present work is to experimentally investigate the potential profiles and distribution functions in S and P striations and to analyze the mechanism which shapes the distribution functions for striations of these types. Zh. Tekh. Fiz. 67, 14–21 (September 1997)     

Reply to the Comment by A. Rabhi on “Energies of the ground state and first excited 0<Superscript> + </Superscript> state in an exactly solvable pairing model”

It is pointed out that the exact solutions given in the recent Comment by A. Rabhi on the paper by N. Dinh Dang Energies of the ground state and first excited 0⁺ state in an exactly solvable pairing model (Eur. Phys. J. A 16, 181 (2003)) do not correspond to the standard exact solution of the well-known two-level pairing model. Other issues raised in the Comment reiterate the discussions already published in the original paper by N. Dinh Dang.Received: 21 July 2003, Published online: 17 February 2004PACS: 21.60.Jz Hartree-Fock and random-phase approximations - 21.60.-n Nuclear-structure models and methods     

Resonance Raman excitation and electronic structure of the single bonded dimers (C ¯60)2 and (C 59N)2

Raman spectra are presented for the single bonded dimeric fullerene (C ₆₀ ^- ) ₂ and compared to optical spectra and Raman spectra of the isostructural and isoelectronic heterofullerene (C₅₉N)₂. The spectra of both materials exhibit strong correlations with respect to splitting, line position, and line intensity. This holds for non resonant excitation with blue and green lasers as well as for the strong resonances observed with red lasers. The latter observation is consistent with a downshift for the electronic transition energies as compared to C₆₀. The absorption edge of thin films of (C₅₉N)₂ was found at 1.4 eV. The three intercage modes were observed at 82, 103, and 111, and at 88, 98, and 106 cm^-1 for (C₅₉N)₂ and (C ₆₀ ^- ) ₂ , respectively. A surprising difference was found for the position of the pentagonal pinch modes in the two materials as they were observed at 1461 and at 1451 cm^-1, for (C₅₉N)₂ and (C ₆₀ ^- ) ₂ , respectively. This is interpreted as a consequence of some characteristic differences in the electronic structure of the two compounds. Received 25 January 2000 and Received in final form 10 April 2000     

关于Airy光束衍射及自加速性质的研究

对Airy光束的特性做进一步探讨, 一方面对无限宽Airy光束的重心问题给出新的理论说明, 另一方面着重对有限宽情形下的Airy光束的奇特性质进行探讨. 文中采用反证法给出无衍射的讨论, 同时结合数值模拟给出高斯函数及矩形函数限定下的有限宽Airy光束的场分布, 并由此得到其重心位置的轨迹: 重心位置是不变的, 不可能整体自由加速. 最终得到有限宽Airy光束既不可能在自由空间加速, 也不可能是无衍射光束. 关键词： Airy光束 无衍射 自加速 数值模拟     

Bound and unbound rovibrational states of the methane-argon dimer

ABSTRACT

Peculiarities of the intermolecular rovibrational quantum dynamics of the methane-argon complex are studied using a new, ab initio potential energy surface [Y.N. Kalugina, S.E. Lokshtanov, V.N. Cherepanov, and A.A. Vigasin, J. Chem. Phys. 144, 054304 (2016)], variational rovibrational computations, and detailed symmetry considerations within the molecular symmetry group of this floppy complex as well as within the point groups corresponding to the local minimum structures. The computed (ro)vibrational states up to and beyond the dissociation asymptote are characterised using two limiting models: the rigidly rotating molecule's model and the coupled-rotor model of the rigidly rotating methane and an argon atom orbiting around it.     

SYNTHESIS AND SPECTROSCOPIC PROPERTIES OF HIGHLY PURE PERYLENE FLUORESCENT DYES

Two new perylene dye, N, N′-bis-(aminododecyl)-3, 4, 9, 10-perylenebis (dicarboximide) (1) and N, N′-bis-(4-chlorophenyl)-3, 4, 9, 10-perylenebis (dicarboximide) have been synthesized. Because the solubility of perylene derivatives is very low, their synthesis and purification are difficult. The imides 1 and 2 are easily prepared with high yield. Dye 2 has a lower density than the density of air. They are highly fluorescent and very photostable dyes. With high fluorescent quantum yield they are suggested as new convenient standards for the fluorescence quantum yield measurements in 500–650 nm region. The report includes the electronic absorption and emission spectra, extinction coefficients and fluorescence quantum yields. Applications of the dyes are discussed.     

Multipole solutions of the wave equation

The wave equation is solved by the operator separation method proposed in V. V. Zashkvara and N. N. Tyndyk, Zh. Tekh. Fiz. 61(4), 148 (1991) [Sov. Phys. Tech. Phys. 36, 456 (1991)]. Solutions describing the evolution of circular-multipole fields are obtained in a cylindrical coordinate system. Zh. Tekh. Fiz. 68, 9–14 (June 1998) Deceased.     

Theoretical study on the influence of different NˆN ligands on the electronic structures and optoelectronic properties of heteroleptic Iridium(III) complexes

DFT/TDDFT calculations were carried out to investigate the electronic structures, absorption and phosphorescence properties of a series of heteroleptic Ir(III) complexes consisting of two N-heterocyclic carbene ligands and a conjugated bicyclic N,N′-heteroaromatic (N?N) ligand. On the basis of the results reported herein, we attempt to explain the experimental observations according to which complex (mpmi)₂Ir(pybi) (1) [Hmpmi = 1-(4-tolyl)-3-methyl-imidazole; Hpybi = 2-(pyridin-2-yl)-1H-benzo[d]imidazole] emits green light with an extremely high-quantum phosphorescence efficiency (Φ _PL ) of 79.3%, while a relatively lower Φ _PL (only 11%) was measured for (fpmi)₂Ir(tfpypz) (2) [fpmi = 1-(4-fluorophenyl)-3-methylimdazolin-2-ylidene-C, C^2′; tfpypz = 2-(3-(trifluoromethyl)-1H-pyrazol-5-yl)pyridinato] emitting blue light by tuning the N?N ligands. Besides, we also designed (fpmi)₂Ir(pyN3) (3) [pyN3H = 2-(5-(trifluoromethyl)-2H-1,2,4-triazol-3-yl)pyridine] and (fpmi)₂Ir(pyN4) (4) [pyN4H = 2-(1H-tetrazol-5-yl)pyridine] to explore the influence of electron-withdrawing substituents on N?N ligands on the electronic and optical properties of these Ir(III) complexes. The results revealed that electron-withdrawing substituents can stabilise both HOMOs and LUMOs and induce HOMO–LUMO energy gap change. Moreover, the emission properties can be significantly tuned by introducing different N?N ligands. While new insights were gained on structural and electronic properties, the extremely high Φ _PL of 1 was found to be not inherent to spin-orbital coupling effects, but determined by its large transition dipole moment (μ_{S 1}) upon S ₀–S ₁ transition compared with that of 2. On the basis of these results, the designed complexes 3 and 4 are considered to be the promising candidates for blue-emitting phosphorescence materials with higher Φ _PL than the complex 2.     

Energy loss from metallic systems during ion implantation

Abstract

Temperature evolution during Ar - and N -implantation in a silver electrodeposited copper bar has been experimentally recorded. A theoretical model calculation for the target heating and cooling reproduces very well the experimental results. It is shown that N ions are more efficient than Ar ions in the sample heating.     

Fredholm Modules on P.C.F. Self-Similar Fractals and Their Conformal Geometry

The aim of the present work is to show how, using the differential calculus associated to Dirichlet forms, it is possible to construct non-trivial Fredholm modules on post critically finite fractals by regular harmonic structures (D, r). The modules are (d _S , ∞)–summable, the summability exponent d _S coinciding with the spectral dimension of the generalized Laplacian operator associated with (D, r). The characteristic tools of the noncommutative infinitesimal calculus allow to define a d _S -energy functional which is shown to be a self-similar conformal invariant. Thiswork has been supported by the project “Teoria ellittica e forme di Dirichlet su spazi frattali” G.N.A.M.P.A. 2008 and by the G.R.E.F.I.-G.E.N.C.O. French-Italian Research Group.     

Comparative Studies of Phase-Cycling Schemes for Multiple π-Pulse Sequences

Recently, a new phase cycling scheme was introduced by this laboratory for use in biological solid-state NMR experiments involving multiple π-pulses with characteristics that suggested it may enhance the sensitivity of these kind of experiments (Y. Li and J. N. S. Evans, 1995,Chem. Phys. Lett.241,79 and Erratum, 1995,ibid.246,527; Y. Li and J. N. S. Evans, 1996,J. Magn. Reson. B111,296). The new sequence followed the supercycled concept proposed a decade ago for heteronuclear decoupling experiments. In this paper, more detailed experiments demonstrate that the claim of enhanced sensitivity was unfounded, and in fact the supercycle proposed differs little from the established XY-8 and XY-16 based supercycles.