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Stephen Sproules 《Angewandte Chemie (International ed. in English)》2019,58(30):10043-10047
A recent Communication in this journal reported the stabilization of low‐valent iron(I) in a fully oxidized polyoxovanadate. With no ligand‐field argument to support such an assignment, a re‐evaluation of the data accompanied by detailed computational analysis reveals the redox chemistry is localized to the polyoxovanadate, and when reduced, instigates a spin transition at iron. 相似文献
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