Four-wave mixing and biphoton generation in a two-level system

We find that in a two-level system there are two kinds of four-wave mixing processes which destructively contribute to the third-order nonlinear susceptibility. In a paired-photon generation scheme by using a single retroreflected pump beam, these two processes occur with definite time orders. The biphoton temporal correlation, which is measured with a back-to-back geometry in a laser-cooled two-level atomic ensemble, shows a damped Rabi oscillation and photon antibunching. Without suppressing the background of Rayleigh scattering, the upper limit of Cauchy criteria is estimated.     

Magnetic-Field Dependence of Raman Coupling Strength in Ultracold ~(40)K Atomic Fermi Gas

We experimentally demonstrate the relation of Raman coupling strength with the external bias magnetic field in degenerate Fermi gas of ~(40)K atoms.Two Raman lasers couple two Zeeman energy levels,whose energy splitting depends on the external bias magnetic field.The Raman coupling strength is determined by measuring the Rabi oscillation frequency.The characteristics of the Rabi oscillation is to be damped after several periods due to Fermi atoms in different momentum states oscillating with different Rabi frequencies.The experimental results show that the Raman coupling strength will decrease as the external bias magnetic field increases,which is in good agreement with the theoretical prediction.     

Rabi oscillations and generalizations

A unified, quantum mechanical account of the behavior of a model atom with few relavant energy eigenstates and subject to intense monochromatic incoming radiation is given. The modifications of the standard application of quantum electrodynamics needed to include incoming fields of finite intensity are described. A projected Green's function method for evaluating either the time evolution or spectral properties of systems is developed and applied to a variety of systems, including: (1) An atom with two to four levels interacting with a radiation field of one or two modes, resulting in various forms of Rabi oscillation; (2)_An atom interacting with all modes of the radiation field in its vacuum state, resulting in the possibility of spontaneous radiation; (3) An atom interacting with all modes of the radiation field with one highly excited, resulting in damped Rabi oscillation, resonance fluorescence, optical pumping, and in a continuing sequence of photon emissions which are studied in some detail.     

Generation of Competitive and Coexisting Two Pairs of Biphotons in Single Hot Atomic Vapor Cell

The non-classical states of light serve as a potential candidate for emerging quantum information process. A processing trend to enhance its scalability is to integrate multiple nonlinear processes with the dressed-state picture into a single device, and therefore, are useful for quantum computations. Here, a novel method is proposed to experimentally achieve the generation of coexisting two pairs of narrow-band biphotons by two four-wave mixing processes in a single hot rubidium vapor cell. Based on the photon-atom nonlinear interfaces, the generated biphotons exhibits genuine entanglement in time–energy. Meanwhile, the nonlinear susceptibility with the dressed-state picture decides the temporal correlation of the biphotons wave packet as a damped periodic Rabi oscillation, suggesting the property of the high-dimensional time–energy entangled state. Such a high-dimensional entangled state also is an efficient way to enhance information carrying capacity. By alternating two nonlinear susceptibilities in a single device, respectively, there exists a competition of the generation rate between such two pairs of biphotons. Moreover, both generated two pairs of biphotons that violate the Cauchy–Schwarz inequality and show their non-classical behavior.     

Temporally Correlated Narrowband Biphoton Interference Based on Mach–Zehnder Interferometer

Since early 1990s, Mach–Zehnder interferometer has been used to investigate the interference of biphoton wave packets. Due to subpicosecond time coherence of biphoton generated by spontaneous parametric downconversion process, some physical processes are ignored in the interferometer, most likely the biphoton time‐domain interference. Here, the two‐photon interference phenomenon based on the Mach–Zehnder interferometer is theoretically studied, where the correlated photon pairs are produced by the four‐wave mixing in atomic system. In particular, the quantum interference effect to effectively control the coherent time of two‐photon by adjusting the input delay is used. In the damped Rabi oscillation regime, two‐photon bunching and antibunching effects are observed. In addition, in the group‐delay regime, the interference between biphoton precursor, slow‐light wave packets and also in between the precursor and the slow‐light wave packets is observed, which had never been reported before. These results may have potential applications in the fields of biphoton shaping and quantum information processing.     

Clock frequency estimation under spontaneous emission

We investigate the quantum dynamics of a driven two-level system under spontaneous emission and its application in clock frequency estimation. By using the Lindblad equation to describe the system, we analytically obtain its exact solutions, which show three different regimes: Rabi oscillation, damped oscillation, and overdamped decay. From the analytical solutions, we explore how the spontaneous emission affects the clock frequency estimation. We find that under a moderate spontaneous emission rate, the transition frequency can still be inferred from the Rabi oscillation. Our results enable potential practical applications in frequency measurement and quantum control under decoherence.     

Interplay of Rabi oscillations and quantum interference in semiconductor quantum dots

We investigated the manifestation of Rabi oscillation in the coherent dynamics of excitons in self-assembled semiconductor quantum dots. The Rabi oscillation phenomenon was directly observed as a function of the input pulse area. Furthermore, by performing wave packet interferometry in the nonlinear excitation regime, we discover a new type of quantum interference phenomenon, resulting from the interplay between Rabi oscillation and quantum interference.     

Dynamics of four-wave mixing on excitons in a quantum optical microcavity

A theory of degenerate four-wave mixing in a semiconductor optical cavity with quantum wells is constructed. The nonlinear response of a microcavity can be four to five orders of magnitude stronger than that of an isolated quantum well. For P ² E-and P ³-type nonlinearities the damped diffracted signal oscillates with a period determined by the Rabi splitting. For a biexcitonic mechanism of nonlinearity, the signal contains damped overtones of the Rabi splitting and the biexciton binding energy. Pis’ma Zh. éksp. Teor. Fiz. 64, No. 11, 749–754 (10 December 1996)     

方波电场驱动下的Rabi振荡

研究了方波电场驱动下的双Bloch带的紧束缚模型.借助Fourier分析,得到了在弱耦合极限下Rabi振荡及Rabi频率的解析解;这些结果均由电子的数值演化所证实.     

Temporal Behavior of Rabi Oscillation in Nanomechanical QED System with a Nonlinear Resonator

In nanomechanical QED system,consisting of a charge qubit and a nanomechanical resonator with intrinsic nonlinearity,we study the temporal behavior of Rabi oscillation in the nonlinear Jaynes-Cummings model.Using microscopic master equation approach,we solve time evolution of the density operator describing this model.Also,the probability of excited state of charge qubit is calculated.These analytic calculations show how nonlinearity parameter and decay rates of two different excited states of the qubit-resonator system affect time-oscillating and decaying of Rabi oscillation.     

Quantum state reduction and conditional time evolution of wave-particle correlations in cavity QED

We report measurements in cavity QED of a wave-particle correlation function which records the conditional time evolution of the field of a fraction of a photon. Detection of a photon prepares a state of well-defined phase that evolves back to equilibrium via a damped vacuum Rabi oscillation. We record the regression of the field amplitude. The recorded correlation function is nonclassical and provides an efficiency independent path to the spectrum of squeezing. Nonclassicality is observed even when the intensity fluctuations are classical.     

Energy Exchange Dynamics and Relaxation of Excitations upon Strong Exciton–Plasmon Interaction in a Planar Nanostructure of Molecular J-Aggregates on a Metal Substrate

The kinetics of energy exchange between the plasmonic and excitonic subsystems in a “metal–dielectric–molecular layer” is studied for a planar composite nanostructure with a strong exciton–plasmon interaction. It is shown that the time dependence of the energy transfer between the components of the system has the character of damped oscillations, which depend on the prepared initial state, a number of relaxation parameters, the Rabi frequency, and the detuning from resonance.     

Time-dependent dressed-states analysis of lasing without population inversion in a three-level ladder scheme

A dressed-state study of lasing without population inversion from a three-level atom interacting with a bichromatic laser field in the ladder configuration is being formulated. The system is allowed to be dressed by both laser-field photons (double dressing). The temporal behavior of the system under consideration is being explored numerically. Although the use of dressed-basis density matrix equations introduces major complexity into the equations, this procedure has crucial importance to the understanding of the atomic spectrum and the underlying physics of the processes involved. The system is found to possess a gain without population inversion, as well as a regular gain with inversion for various transitions, both in the transient and steady-state regimes. Enhancement of the refractive index accompanied by vanishingly small absorption was also found. The frequency response of various transitions is explored via numerical Fourier analysis. Some transitions are found to exhibit a dispersion-like line shape, clear evidence of a quantum-coherent interference effect. The spectrum consists of two distinct quintets centered about the coupling and probe-laser frequencies. The spectral features consisting of each quintet are located symmetrically (at resonance conditions only) around the line center at positions shifted from the center by the generalized Rabi and double Rabi frequencies.     

Rabi oscillations and long-time behaviour in resonance fluorescence from vibronic systems

The resonance fluorescence from a vibronic system is studied for the case of a strong pump field. For a system with slow vibrational relaxation the Rabi oscillations are damped less than in the case of a two-level atom and additionally the intensity substantially decreases. The long time behaviour is characterized by the increase of the intensity towards its stationary value.     

Gate control of quantum dot-based electron spin–orbit qubits

We investigate theoretically the coherent spin dynamics of gate control of quantum dot-based electron spin–orbit qubits subjected to a tilted magnetic field under electric-dipole spin resonance (EDSR). Our results reveal that Rabi oscillation of qubit states can be manipulated electrically based on rapid gate control of SOC strength. The Rabi frequency is strongly dependent on the gate-induced electric field, the strength and orientation of the applied magnetic field. There are two major EDSR mechanisms. One arises from electric field-induced spin–orbit hybridization, and the other arises from magnetic field-induced energy-level crossing. The SOC introduced by the gate-induced electric field allows AC electric fields to drive coherent Rabi oscillations between spin-up and -down states. After the crossing of the energy-levels with the magnetic field, the spin-transfer crossing results in Rabi oscillation irrespective of whether or not the external electric field is present. The spin–orbit qubit is transferred into the orbit qubit. Rabi oscillation is anisotropic and periodic with respect to the tilted and in-plane orientation of the magnetic field originating from the interplay of the SOC, orbital, and Zeeman effects. The strong electrically-controlled SOC strength suggests the possibility for scalable applications of gate-controllable spin–orbit qubits.     

Electrical detection of spin coherence in silicon

Experimental evidence is presented showing that photocurrents in silicon can be used as highly sensitive readout probes for coherent spin states of localized electrons, the prime candidates for quantum bits in various semiconductor based quantum computer concepts. Conduction electrons are subjected to fast Rabi oscillation induced by means of pulsed electron spin resonance. The collective spin motion of the charge carrier ensemble is reflected by a spin-dependent recombination rate and therefore by the sample conductivity. Because of inhomogeneities, the Rabi oscillation dephases rapidly. However, a microwave induced rephasing is possible causing an echo effect whose intensity contains information about the charge carrier spin state and the coherence decay.     

Strongly driven exciton resonances in quantum wells: light-induced dressing versus coulomb scattering

The nonequilibrium dynamics of a two-dimensional electron-hole gas is studied in the regime of strong and resonant pumping of the exciton resonance. The Coulomb collision rates are consistently determined by taking into account the light-induced coherence of the two-band system that leads to a dressing of the carrier spectral functions. The light dressing dramatically reduces the Coulomb scattering efficiency. Results are presented for Rabi oscillations in the time domain and dynamical Stark splitting in the pump-probe absorption spectra.     

非简并拉曼过程中交流斯塔克位移对原子反转的影响

利用修正后的有效哈密顿量计算非简拉曼过程中原子反转的演化，并研究交流斯塔克位移对拉比振荡崩溃和再生的影响。结果发现：交流斯克位移的存在使得非简并拉曼过程中原子反转的崩溃与再生现象呈现较好的周期性，并且拉比振荡的频率和幅均受交流斯塔克位移的影响。     

五能级原子开放系统中的多波混频共存特性

研究了受强缀饰场作用的五能级原子系统所产生的多波混频共存特性.研究发现,通过调节激光束方向,沿同一方向出射的八波混频、双缀饰四波混频和单缀饰六波混频信号因共用能级的原子相干产生而出现竞争现象,通过控制缀饰场减弱四波混频和六波混频信号强度,可以达到增强八波混频信号的目的.还对级联和并联两种不同缀饰方式下双缀饰四波混频过程的差别进行了详细分析. 关键词： 双缀饰四波混频 单缀饰六波混频 八波混频 抑制增强     

Two-color two-photon Rabi oscillation of biexciton in single InAs/GaAs quantum dot

A two-photon absorption resonance is observed when the sum-frequency of two laser pulses equals the creation energy of a biexciton in a single InAs/GaAs semiconductor quantum dot. Resonant excitation of the two-color two-photon transition results in a coherent oscillation that is remarkably similar to a single-color two-photon Rabi oscillation of the crystal-ground to biexciton optical transition. A model explaining the coherent two-photon absorption is presented.