Single-beam homodyne SPIDER for multiphoton microscopy

We report a new version of spectral phase interferometry for direct electric field reconstruction (SPIDER) requiring only a single phase-shaped laser beam. A narrowband probe pulse is selected out of a broadband ultrafast laser pulse by a phase pulse-shaping technique and mixed with the original broadband pulse to generate a second-harmonic generation (SHG) signal. Using another SHG signal solely generated by the broadband pulse as a local oscillator, the spectral phase of the broadband laser pulse can be analytically retrieved by a combination of double-quadrature spectral interferometry and homodyne optical technique for SPIDER (HOT SPIDER). An arbitrary spectral phase at the sample position of a microscope can be compensated with a precision of 0.05 rad over the FWHM of the laser spectrum. It is readily applicable to a nonlinear microscopy technique with a phase-controlled broadband laser pulse.     

Generation of ten-cycle pulses from an ytterbium fiber laser with cubic phase compensation

We demonstrate the use of a prism-grating sequence to reduce third-order dispersion inside a mode-locked Yb fiber laser. This laser generates pulses as short as 33 fs with extremely clean temporal and spectral profiles. Nanojoule pulse energies are possible.     

Characterization of a broadband pulse for phase controlled multiphoton microscopy by single beam SPIDER

We present what we believe to be a new version of spectral phase interferometry for direct electric field reconstruction (SPIDER) using only a single-phase and polarization controlled laser beam. Two narrow pulses and one broadband pulse are selected out of an ultrafast laser pulse by a polarization and phase control technique to generate second harmonic generation (SHG) signals, which are equivalent to a spectral shear interferogram in the conventional SPIDER method. The spectral phase of the broadband laser pulse is extracted analytically with double quadrature spectral interferometry (DQSI). An arbitrary spectral phase can be retrieved with great precision and compensated in situ at the sample position of a microscope. This new method requires no separate reference beam and is suitable for nonlinear optical microscopy with a phase controlled laser pulse.     

用SPIDER法测量飞秒激光脉冲的光谱相位

介绍了用SPIDER测量光谱相位的实验装置和模拟计算飞秒激光特性参数的原理；提出了Ω 和τ等重要参数的确定方法.实验上用自建的SPIDER进行了掺钛蓝宝石飞秒振荡器输出脉 冲的相位测量，并以此为基础还原出了原输入脉冲的时域形式，模合计算所得的脉宽为107 fs，与利用二次相关法直接测量的结果十分一致. 关键词： 飞秒激光 SPIDER 光谱相位 光谱相干     

Long-cavity passively mode-locked fiber ring laser with high-energy rectangular-shape pulses in anomalous dispersion regime

We report on a long-cavity passively mode-locked fiber laser in the anomalous dispersion regime. The nonlinear polarization rotation technique is employed to achieve mode locking. The output pulse from the fiber laser has a rectangular shape and a corresponding gaussian-shape spectral profile. Stable mode-locked pulses at a repetition rate of 278 kHz with single pulse energy as high as 715 nJ are obtained under equal bidirectional pumping power of 500 mW in cavity. The experimental results demonstrate that the passively mode-locked fiber laser operating in the anomalous regime can also realize a high-energy pulse, which is different from the conventional low-energy soliton pulse.     

基于旋转相干光谱的整形飞秒激光转动动力学调控

我们实验上发展了基于飞秒激光旋转相干光谱的整形飞秒激光转动动力学调控方法,通过脉冲整形技术调控激发脉冲的光谱相位,从而实现对飞秒激光作用下转动态相干激发过程中复原信号及转动布居数的调控. 研究了飞秒激光旋转相干光谱对激光频谱相位的响应机制,突出了飞秒激光频谱相位在气相分子转动态相干激发中的重要作用. 为飞秒激光作用下生物大分子和团簇鉴别及结构探测研究提供了新的参考.     

Coherent measurement of short laser pulses based on spectral interferometry resolved in time

We propose a new method for measuring the phase and the amplitude of a short laser pulse that is based on shearing interferometry in the spectral domain combined with time gating. The method has several features in common with spectral interferometry for direct electric-field reconstruction, in particular, fast and direct reconstruction of the phase. Accurate measurement of the phase added to an 80-fs pulse by a block of F4 glass demonstrates the technique.     

Fourier transform spectral interferometric coherent anti-Stokes Raman scattering (FTSI-CARS) spectroscopy

A novel Fourier transform spectral interferometric (FTSI) multiplex coherent anti-Stokes Raman scattering (CARS) technique is developed to extract the vibrational spectrum equivalent to the spontaneous Raman scattering. The conventional FTSI method is modified to use the internal nonresonant CARS signal as a local oscillator to perform spectral interferometry. Utilizing the causality of the coherent vibration (i.e., there should be no signal before the laser excitation), this new FTSI method recovers the entire complex vibrational spectral parameters. We demonstrate this technique with a previously reported single-pulse multiplex CARS method that uses a single phase-controlled broadband ultrafast laser pulse.     

飞秒激光脉冲整形技术及其应用

通过频域上控制飞秒激光脉冲幅度、相位和偏振在时域上可以获得几乎任意形状的飞秒激光脉冲,这种飞秒激光脉冲整形技术可为研究光与原子分子非线性相互作用提供一种全新实验技术手段.本文介绍飞秒激光脉冲整形发展历史、技术方法、控制方式及其相关应用,并展望飞秒激光脉冲整形技术未来的发展方向.     

Single-shot measurement of the spectral envelope of broad-bandwidth terahertz pulses from femtosecond electron bunches

We present a new approach (demonstrated experimentally and through modeling) to characterize the spectral envelope of a terahertz (THz) pulse in a single shot. The coherent THz pulse is produced by a femtosecond electron bunch and contains information on the bunch duration. The technique, involving a single low-power laser probe pulse, is an extension of the conventional spectral encoding method (limited in time resolution to hundreds of femtoseconds) into a regime only limited in resolution by the laser pulse length (tens of femtoseconds). While only the bunch duration is retrieved (and not the exact charge profile), such a measurement provides a useful and critical parameter for optimization of the electron accelerator.     

The deformable mirror method of adaptive phase correction

In this paper, a simple method of phase correction by using a micromachined deformable mirror (MMDM)is demonstrated. With correction of high-order phases due to propagating through medium, we obtaineda clean pulse shape, flattened spectral phase and decreased the femtosecond laser pulse duration. It isshown by our experiment that the deformable mirror is an effective and easy method for adaptive phasecorrection.     

14-fs high temporal quality injector for ultra-high intensity laser

We present a chirped pulse amplification (CPA) Ti:Sa laser generating sub-15 fs pulses with expected high temporal quality. Gain-narrowing in the pre-amplifier is balanced by a variable spectral reflectivity mirror and by a fine adaptation of the saturation conditions. A crossed polarized wave generation (XPW) filter is introduced to enhance the contrast, reduce the pulse duration and improve the spectral quality. The pulses are generated at 10 Hz repetition rate, with pulse energy of 110 μJ and very clean Gaussian spectrum. The temporal contrast is evaluated by a measurement before the XPW filter and calculations of the enhancement by the filter. The potential temporal incoherent contrast is 10¹² and the coherent contrast 10¹⁰. The performance of the system makes it suitable as an injector for petawatt lasers operating in the double-CPA scheme.     

Cleaning of artificially soiled paper with 532-nm nanosecond laser radiation

Cleaning of paper is a challenging task due to the fact that a contamination should be removed and a fragile organic original material has to be preserved. Pulsed laser cleaning of artificially soiled Whatman© filter paper samples serving as models for historical paper was performed. Different cleaning strategies employing 8-ns laser pulses at 532 nm wavelength were applied to clean paper avoiding undesired effects like discoloration (yellowing) and mechanical deterioration of the substrate. Multi shot experiments with low-energy pulses were compared with single pulse investigations utilizing high pulse energies achieving a constant energy load incident on the samples in both cases. The cleaning efficiency and possible yellowing effects were evaluated by means of a multi spectral imaging system. An extensive microscopic analysis of the cleaned parts of the samples provided insight into the remaining soiling on the surface and in the bulk of the paper material after laser treatment. As a reference, a hard and a soft eraser were used to clean the samples.     

Stimulated Raman spectroscopy using chirped pulses

We present a detailed theoretical and experimental characterization of a new methodology for stimulated Raman spectroscopy using two duplicates of a chirped, broadband laser pulse. Because of the linear variation of laser frequency with time (‘chirp’), when the pulses are delayed relative to one another, there exists a narrow bandwidth, instantaneous frequency difference between them, which, when resonant with a Raman‐active vibration in the sample, generates stimulated Raman gain in one pulse and inverse Raman loss in the other. This method has previously been used for coherent Raman imaging and termed ‘spectral focusing’. Here, gain and loss signals are spectrally resolved, and the spectrally integrated signals are used to determine the spectral resolution of the measured Raman spectrum. Material dispersion is used to generate a range of pulse durations, and it is shown that there is only a small change in the magnitude of the signal and the spectral resolution as the pulse is stretched from 800 to 1800 fs in duration. A quantitative theory of the technique is developed, which reproduces both the magnitude and linewidth of the experimental signals when third‐order dispersion and phase‐matching efficiency are included. The theoretical calculations show that both spectral resolution and signal magnitude are severely hampered by the third‐order dispersion in the laser pulse, and hence, a minimal amount of chirp produces the most signal with only a slight loss of spectral resolution. Copyright © 2014 John Wiley & Sons, Ltd.     

Gain-guided soliton in a positive group-dispersion fiber laser

We report on the operation of a passively mode-locked fiber ring laser made of purely normal dispersive fibers. Self-started mode locking can still be achieved in the laser by use of the nonlinear polarization rotation technique, and the mode-locked pulse has large pulse energy, strong frequency chirp, and a mode-locked spectral width limited by the effective laser gain bandwidth. Furthermore, we show that the operation of the laser can be well described by an extended Ginzburg-Landau equation model that governs the soliton dynamics of fiber lasers.     

Tunable light source for coherent anti-Stokes Raman scattering microspectroscopy based on the soliton self-frequency shift

We present a photonic crystal fiber (PCF)-based light source for generating tunable excitation pulses (pump and Stokes) that are applicable to coherent anti-Stokes Raman scattering (CARS) microspectroscopy. The laser employed is an unamplified Ti:sapphire femtosecond laser oscillator. The CARS pump pulse is generated by spectral compression of a laser pulse in a PCF. The Stokes pulse is generated by redshifting a laser pulse in a PCF through the soliton self-frequency shift. This setup allows for probing up to 4000 cm(-1) with a spectral resolution of approximately 25 cm(-1). We characterize the stability and robustness of CARS microspectroscopy employing this light source.     

Impact of spectral filtering on a weak breathing laser based on AS-Yb-PBGF with large net normal dispersion cavity

We have investigated numerically the effects of the spectral filtering on the temporal and spectral properties of the pulse with large net normal cavity dispersion in a weak breathing passively mode-locked ring laser based on all-solid Yb-doped photonic bandgap fiber (AS-Yb-PBGF), which gives the laser gain and anomalous dispersion simultaneously. The specific range of spectral filter bandwidth is indispensable for obtaining high-peak-power pulse in a given highly chirped pulse laser system under a fixed pump level. The shortening of the pulse durations and the shaving of the sharp peaks at the steep edges of the spectrum by the spectral filter are demonstrated. Moreover, the advantage of the weak breathing fiber laser by introducing the AS-Yb-PBGF for scaling up the peak power and shortening the pulse width is investigated, and the effect of third-order dispersion induced by AS-Yb-PBGF on the pulse shape is also discussed.     

Investigation of passively mode-locked erbium doped fiber ring laser due to nonlinear polarization rotation

Passively mode-locked erbium doped fiber ring laser was investigated. We present optimization of laser configuration where nonlinear polarization rotation was used for modes synchronization. Simulations of pulse propagation inside a laser cavity were applied in order to confirm the optimisation technique. Experimental results are presented and more than 32-nm spectral width of the output frequency comb was obtained.     

High-rate pulse-train generation by phase-only filtering of an electrooptic frequency comb: Analysis and optimization

We investigate the generation of high-rate optical pulse trains by spectral phase-only filtering of a frequency comb derived from an electrooptically phase-modulated continuous-wave laser. The technique is initially analyzed as a two-step filtering process. First, a fundamental pulse-train with repetition-rate equal to the modulation frequency is obtained by line-by-line phase-cancellation of the electrooptic frequency comb. Second, the temporal Talbot-effect is considered so that the output pulse repetition-rate is an integer multiple of the electrooptic modulation frequency. Nonidealities found in the fundamental train lead, in general, to multiplied trains with important degradations. We numerically analyze optimum modulation conditions for generation of output pulse trains with minimum peak-to-peak variations and/or maximum extinction level. On the other hand, a genetic algorithm is considered to numerically find optimum line-by-line phase-only filters that generate output multiplied trains with minimized degradations. Numerical simulations show that, in general, this second approach allows for improvement in the quality of the resultant multiplied trains, in terms of the uniformity degree and/or noise-level, compared with the pulse trains resulting from the Talbot-effect-based approach.     

Influence of spectral phase on cross-polarized wave generation with short femtosecond pulses

In this paper we present the first comprehensive study of the role of spectral phase on cross-polarized wave (XPW) generation using sub-30 femtosecond (fs) laser pulses. XPW generation improves the temporal contrast and shortens the pulse duration of fs chirped pulse amplification (CPA) lasers. For Ti:Sa lasers, compression below 30?fs is non-trivial and therefore never perfect. We therefore systematically analyze the effect of an arbitrary input spectral phase on the output spectrum and efficiency of the XPW process, both theoretically and experimentally. We derive the maximum acceptable value of residual phase for a given initial pulse duration in order to efficiently drive the XPW process for pulse shortening and contrast improvement.