Fast optical preparation, control, and readout of a single quantum dot spin

We propose and demonstrate the sequential initialization, optical control, and readout of a single spin trapped in a semiconductor quantum dot. Hole spin preparation is achieved through ionization of a resonantly excited electron-hole pair. Optical control is observed as a coherent Rabi rotation between the hole and charged-exciton states, which is conditional on the initial hole spin state. The spin-selective creation of the charged exciton provides a photocurrent readout of the hole spin state.     

Coherent transfer of spin through a semiconductor heterointerface

Spin transport between two semiconductors of widely different band gaps is time resolved by two-color pump-probe optical spectroscopy. Electron spin coherence is created in a GaAs substrate and subsequently appears in an adjacent ZnSe epilayer at temperatures ranging from 5 to 300 K. The data show that spin information can be protected by transport to regions of low spin decoherence, and regional boundaries used to control the resulting spin coherent phase.     

All-optical manipulation of electron spins in carbon-nanotube quantum dots

We demonstrate theoretically that it is possible to manipulate electron or hole spins all optically in semiconducting carbon nanotubes. The scheme that we propose is based on the spin-orbit interaction that was recently measured experimentally; we show that this interaction, together with an external magnetic field, can be used to achieve optical electron-spin state preparation with a fidelity exceeding 99%. Our results also imply that it is possible to implement coherent spin rotation and measurement using laser fields linearly polarized along the nanotube axis, as well as to convert spin qubits into time-bin photonic qubits. We expect that our findings will open up new avenues for exploring spin physics in one-dimensional systems.     

Optically controlled initialization and read-out of an electron spin bound to a fluorine donor in ZnSe

Here we report photon antibunching and magneto-spectroscopy of a single electron spin bound to a fluorine donor in a ZnMgSe/ZnSe QW nanostructure. The results confirm the presence of an optically controllable lambda-system which allows the optical manipulation of the electron bound to the neutral fluorine donor as a spin qubit. Moreover, we achieved optical spin pumping of the qubit by resonant excitation of each of the four allowed transitions of the lambda system. We verified the spin transfer by detecting single photons when the bound electron decays into the opposite spin state. The results presented here constitutes an elegant initialization and the read-out procedure of the electron spin qubit bound to a fluorine donor which are prerequisite for coherent optical control of an impurity based solid-state spin qubit.     

All-electrical control of single ion spins in a semiconductor

We propose a method for all-electrical manipulation of single ion spins substituted into a semiconductor. Mn ions with a bound hole in GaAs form a natural example. Direct electrical manipulation of the ion spin is possible, because electric fields manipulate the orbital wave function of the hole, and through the spin-orbit coupling the spin is reoriented as well. Coupling ion spins can be achieved using gates to control the size of the hole wave function. Coherent manipulation of ionic spins may find applications in high-density storage and in scalable coherent or quantum information processing.     

Stimulated and spontaneous optical generation of electron spin coherence in charged GaAs quantum dots

We report on the coherent optical excitation of electron spin polarization in the ground state of charged GaAs quantum dots via an intermediate charged exciton (trion) state. Coherent optical fields are used for the creation and detection of the Raman spin coherence between the spin ground states of the charged quantum dot. The measured spin decoherence time, which is likely limited by the nature of the spin ensemble, approaches 10 ns at zero field. We also show that the Raman spin coherence in the quantum beats is caused not only by the usual stimulated Raman interaction but also by simultaneous spontaneous radiative decay of either excited trion state to a coherent combination of the two spin states.     

玻色凝聚的原子自旋链中的非线性自旋波

研究了囚禁在光晶格中的旋量玻色-爱因斯坦凝聚体(BEC)形成的原子自旋链中的相干非线性自旋波的激发与调制不稳定性.通过解析分析，得到了调制不稳定性的一般判据以及其对原子自旋的长程耦合的依赖关系.在蓝失谐和红失谐光晶格的情况下，分别具体分析了长程非线性自旋耦合，包括光诱导的和静磁诱导的偶极-偶极相互作用对相干自旋波调制不稳定性的影响.     

Anisotropic optical conductivity and electron–hole asymmetry in doped monolayer graphene in the presence of the Rashba coupling

In this study, the optical conductivity of substitutionary doped graphene is investigated in the presence of the Rashba spin orbit coupling (RSOC). Calculations have been performed within the coherent potential approximation (CPA) beyond the Dirac cone approximation. Results of the current study demonstrate that the optical conductivity is increased by increasing the RSOC strength. Meanwhile it was observed that the anisotropy of the band energy results in a considerable anisotropic optical conductivity (AOC) in monolayer graphene. The sign and magnitude of this anisotropic conductivity was shown to be controlled by the external field frequency. It was also shown that the Rashba interaction results in electron–hole asymmetry in monolayer graphene.     

Coherent spin precession of electrons and excitons in charge tunable InP quantum dots

Coherent spin precession of electrons and excitons is observed in charge tunable InP quantum dots under the transverse magnetic field by means of time-resolved Kerr rotation. In a quantum dot doped by one electron, spin precession of the doped electron in the quantum dot starts out of phase with spin precession of the doped electrons in a GaAs substrate just after a trion is formed and persists for more than 2 ns even after the trion recombines. Simultaneously spin precession of a trion (hole) starts. Observation of spin precession of both a doped electron and a trion (hole) confirms creating coherent superposition of an electron and a trion as the initialization process of spin of doped electrons in quantum dots. In a neutral quantum dot, the exciton spin precession starts out of phase with spin precession of the doped electrons in a GaAs substrate and the precession frequency does not converge to 0 at the zero field limit. It contains the electron–hole exchange interaction and corresponds to the splitting between bright and dark excitons under the transverse magnetic field.     

Spin coherence of holes in GaAs/(Al,Ga)As quantum wells

Carrier spin coherence in a p-doped GaAs/(Al,Ga)As quantum well with a diluted hole gas is studied by picosecond pump-probe Kerr rotation. For resonant optical excitation of the positively charged exciton the spin precession shows two types of oscillations: Electron spin beats decaying with the charged exciton radiative lifetime of 50 ps, and long-lived hole spin beats with dephasing times up to 650 ps, which decrease with increasing temperature, underlining the importance of hole localization. The mechanism of hole spin coherence generation is discussed.     

Hole burning—EIT studies of the NV centre in diamond

The negative nitrogen-vacancy centre in diamond is used to illustrate electromagnetically induced transparency features within a coherent hole. A hole is created in an inhomogeneously broadened electron spin transition and its spectrum modified by driving hyperfine transitions. The modified spectrum is discussed in terms of dressed states of the system, and the spectrum is shown to be in good correspondence with numerical solutions of the density matrix for the doubly driven system.     

Nuclear spins of ionized phosphorus donors in silicon

We demonstrate the coherent control and electrical readout of ionized phosphorus donor nuclear spins in (nat)Si. By combining time-programed optical excitation with coherent electron spin manipulation, we selectively ionize the donors depending on their nuclear spin state, exploiting a spin-dependent recombination process at the Si/SiO(2) interface, and find a nuclear spin coherence time of 18 ms for the ionized donors. The presented technique allows for spectroscopy of ionized-donor nuclear spins and enhances the sensitivity of electron nuclear double resonance to a level of 3000 nuclear spins.     

Spin squeezing and entanglement via hole-burning in atomic coherent states

We study the generation of spin squeezing via the hole burning of selected Dicke states out of an atomic coherent state prepared for a collection of N two-level atoms or ions. The atoms or ions of the atomic coherent state are not entangled, but the removal of one or more Dicke states generates entanglement, and spin squeezing occurs for some ranges of the relevant parameters. Spin squeezing in a collection of two-level atoms or ions is of importance for precision spectroscopy.     

Excitation of the spin density and current by coherent light pulses in quantum wells

We study the orbital and spin dynamics of charge carriers induced by non-overlapping linearly polarized light pulses in semiconductor quantum wells. It is shown that such an optical excitation with coherent pulses leads to a spin orientation of photocarriers and an electric current. The effects are caused by the interference of optical transitions driven by individual pulses. The distribution of carriers in the spin and momentum spaces depends on the crystallographic orientation of quantum wells and can be efficiently controlled by the pulse polarizations, time delay and phase shift between the pulses, as well as an external magnetic field.     

Magnons interaction of spinor Bose-Einstein condensates in an optical lattice

We study the interaction of magnons in dipolar spinor Bose-Einstein condensates in an optical lattice. By means of Holstein-Primakoff and Fourier transformations the energy spectra of the ground and the excited states is obtained analytically. Our results show that the collision of magnons is elastic which is expressed by the conservation of wave numbers in the process of collision. At last, we found that the interaction of magnons is attractive which tends to self-localization to form spin waves, i.e., a cluster of a macroscopic number of coherent magnons. Because of the attraction, the instability of spin wave brings about the existence of solitary wave.     

Exciton-Boson Formalism in the Theory of Laser-Excited Semiconductors and Its Application in Coherent Four-Wave-Mixing Spectroscopy

By the use of a bosonization transformation and group-theoretical arguments, the Hamiltonian of an electron–hole–photon system in a laser-excited direct two-band semiconductor is transcribed into that of an exciton–photon system with the particle spins rigorously taken into consideration. It is shown that the third-order optical nonlinearities in the spectral region below the band edge have their microscopic origin in two-exciton correlations, which are expressed in terms of the effective exciton–exciton and anharmonic exciton–photon interactions. The dependence of the interparticle interactions on the spin states of quasiparticles is behind the polarization dependence of the semiconductor nonlinear optical response. On the example of the system of heavy hole excitons in quantum wells, grown from compounds with the zinc blende type of symmetry, it is demonstrated that the effective exciton–exciton interaction in two-exciton states with nonzero total spin is repulsive, while in zero-spin states it is attractive, which may result in the biexciton formation. The derived Heisenberg equations of motion for the exciton and biexciton operators form the basis for a theoretical study of the coherent four-wave-mixing in GaAs and ZnSe quantum wells. It is readily apparent from the equations that in different polarization configurations the coherent four-wave-mixing is generated by different ingredients of two-exciton Coulomb correlations: in the co-circular configuration, it is the interexciton repulsion, in the cross-linear configuration, the formation of the biexciton and its coupling to excitons, and in the collinear configuration, both of them jointly. The obtained expressions for the time-resolved and frequency-resolved four-wave-mixing signals adequately describe the main characteristics and various details of wave mixing phenomena, including a biexciton signature in the appropriate polarization configurations. Results of the work clarify the microscopic mechanism of the polarization dependence in coherent four-wave-mixing spectroscopy in semiconductor quantum wells.     

Surface Plasmon Mediated Controllable Spin‐Resolved Transmission in Meta‐Hole Structures

Chiral responses are optical responses involving circular polarizations. Controlling the chiral response in a flexible way is very important in optical manipulations. Chiral metamaterials have thus drawn enormous interest due to their flexible designing feature. However, most of the previous studies are mainly realized by designing the structure of the individual meta‐atom. Meanwhile, to enhance the response, complex design and fabrication processes are typically required. Here, by introducing spin‐dependent propagating surface plasmons and spin‐selective interference, giant spin‐resolved transmission is achieved in a simple meta‐hole structure. In this interaction process, spin‐orbital angular momentum conversion plays an essential role. By controlling the phase difference between the interference components, controllable spin‐resolved transmission is achieved. Furthermore, such method can also be applied to realize spin‐resolved excitation of surface plasmons. The proposed controlling strategy offers a versatile platform for a variety of promising applications, such as polarization control, asymmetric transmission, surface plasmon excitation, and on‐chip chiral manipulation.     

Tuning of exciton states in a magnetic quantum ring

The exciton states in a CdTe quantum ring subjected to an external magnetic field containing a single magnetic impurity are investigated. We have used the multiband approximation which includes the heavy hole–light hole coupling effects. The electron–hole spin interactions and the s, p–d interactions between the electron, the hole and the magnetic impurity are also included. The exciton energy levels and optical transitions are evaluated using the exact diagonalization scheme. We show that due to the spin interactions it is possible to change the bright exciton state into the dark state and vice versa with the help of a magnetic field. We propose a new route to experimentally estimate the s, p–d spin interaction constants.     

Negative circular polarization of InP QD luminescence: Mechanism of formation and main regularities

The spectrum and kinetics of the circular polarization of InP quantum dot (QD) photoluminescence have been experimentally investigated under different conditions of optical excitation and at different bias voltages applied to the sample. It is established that, at a bias of about ?0.1 V, the degree of photoluminescence polarization is negative and reaches ?50% in limiting cases. It is concluded that the negative polarization is formed in QDs containing one recident electron per dot and is mainly caused by the optical orientation of the electron spin. It is shown that all experimentally observed regularities are well described in the framework of the model assuming the energy relaxation of photogenerated electron-hole pairs accompanied by the electron- hole spin flip-flop process.