飞秒激光诱导有机薄膜自组装微结构

通过改变辐照激光脉冲数、激光的平均功率、显微镜物镜倍数/数值孔径等研究微皇冠结构形成与加工条件的关系,并借鉴激光熔池形成和液滴溅射的模型对其进行理论分析。当激光脉冲数达到一定数量后,烧蚀区域会出现微皇冠结构。烧蚀区域尺寸的改变是由于形成的液体区域中热毛细作用和化学毛细作用共同所致;微皇冠结构溅射个数的改变是由于形成的气体因多光子吸收体积迅速膨胀所致。     

飞秒激光诱导有机薄膜自组装微结构

通过改变辐照激光脉冲数、激光的平均功率、显微镜物镜倍数/数值孔径等研究微皇冠结构形成与加工条件的关系,并借鉴激光熔池形成和液滴溅射的模型对其进行理论分析。当激光脉冲数达到一定数量后,烧蚀区域会出现微皇冠结构。烧蚀区域尺寸的改变是由于形成的液体区域中热毛细作用和化学毛细作用共同所致;微皇冠结构溅射个数的改变是由于形成的气体因多光子吸收体积迅速膨胀所致。     

Femtosecond filamentation induced fluorescence technique for atmospheric sensing

Recent progress in filament-induced atmospheric sensing is reviewed.Self-guided propagation of ultrashort laser pulses in air induces laser filamentation.All molecules in the path of a filament can be dissociated into highly excited fragments,resulting in emission of characteristic fluorescence spectra.The fluorescence spectra provide information about the various molecules in the filaments.By using a filament-induced"fingerprinting"fluorescence technique,molecules in the atmosphere can be identified.     

基于飞秒激光的一维速度场测量方法

飞秒激光诱导氰基化学发光利用飞秒光丝标记流场中的气体分子,通过观测被标记分子在固定时间内的位移可获得流场的速度信息.一维的光丝在实验结果中包含了一维的速度场信息,但由于无法将光丝移动前后的位置信息精确关联,因此只能给出中心一点的速度.针对此问题,我们提出了一种一维速度场反演算法,可根据移动后光丝的位置及其线型反演出整条...     

飞秒激光诱导水光学击穿阈值

为了研究飞秒激光诱导水光学击穿阈值随激光脉冲参数的变化关系,采用四阶Runge-Kutta方法对飞秒激光诱导水光学击穿的椭球体模型进行了不同脉宽（40~540 fs）、波长(400~1 200 nm)和光斑尺寸（0~200 μm）下的数值模拟。通过控制变量法得出阈值光强与这些激光脉冲参数的关系曲线图,据此定性分析了阈值光强与激光脉冲参数的变化特征趋势。应用光强与功率、能量、辐照曝光量和电场强度之间的关系,得到了它们随激光脉冲参数脉宽、波长和光斑尺寸的动态关系,这为进一步研究飞秒激光与水和含水介质的相互作用提供了理论依据。     

飞秒激光诱导水光学击穿阈值

为了研究飞秒激光诱导水光学击穿阈值随激光脉冲参数的变化关系,采用四阶RungeKutta方法对飞秒激光诱导水光学击穿的椭球体模型进行了不同脉宽(40～540fs)、波长(400～1200nm)和光斑尺寸(0～200μm)下的数值模拟。通过控制变量法得出阈值光强与这些激光脉冲参数的关系曲线图,据此定性分析了阈值光强与激光脉冲参数的变化特征趋势。应用光强与功率、能量、辐照曝光量和电场强度之间的关系,得到了它们随激光脉冲参数脉宽、波长和光斑尺寸的动态关系,这为进一步研究飞秒激光与水和含水介质的相互作用提供了理论依据。     

飞秒激光作用下光学与激光玻璃的暗化阈值测量

报道了各种商用光学玻璃和激光玻璃在800nm、120fs、1kHz钛宝石脉冲激光作用下,产生光致暗化的阈值。     

飞秒激光诱导玻璃内析出BaTiO3晶体

使用800nm、120fs、200kHz的高重复频率超短脉冲激光照射BaO-TiO2-SiO2系玻璃，玻璃经飞秒激光照射数秒钟后，激光会聚点的发光由800nm波长的红色突然转变为非常强的400nm的蓝色，对激光辐照点的发光光谱和X射线衍射分析表明，具有倍频效应的BaTiO3晶体已经产生。     

Femtosecond pulse laser-induced self-organized nanostructures on the surface of ZnO crystal

This paper reports self-organized nanostructures observed on the surface of ZnO crystal after irradiation by a focused beam of a femtosecond Ti：sapphire laser with a repetition rate of 250kHz. For a linearly polarized femtosecond laser, the periodic nanograting structure on the ablation crater surface was promoted. The period of self-organization structures is about 180 nm. The grating orientation is adjusted by the laser polarization direction. A long range Bragglike grating is formed by moving the sample at a speed of 10μm/s. For a circularly polarized laser beam, uniform spherical nanoparticles were formed as a result of Coulomb explosion during the interaction of near-infrared laser with ZnO crystal.     

Femtosecond laser-induced long-lasting phosphorescence in Pr^3＋-doped ZnO-B2O3-SiO2 glass

This paper studies the phenomenon of long-lasting phosphorescence induced by a femtosecond laser in Pr3 -doped ZnO-B2O3-SiO2 glass. With the glass irradiated by a focused femtosecond laser for a short time, the emission of strong reddish long-lasting phosphorescence from the irradiated part of the glass can be observed. The emission peaks are located at 495 and 603 nm in wavelength, showing that the long-lasting phosphorescence originates from the emission of Pr^3 . The intensity of the phosphorescence decreases in inverse proportion to time after the removal of the laser. By analysing the absorption and electron spin resonance spectra of the glass, we find that colour-centres are induced in the glass matrix after the irradiation of the femtosecond laser. A possible mechanism has been provided to account for the generation of long-lasting phosphorescence.     

对飞秒激光等离子体中成丝现象的研究

采用光学阴影法和散射光成像,对飞秒激光等离子体中的局域密度涨落进行了研究.在实验中观察到了成丝不稳定性现象.从理论上对有质动力引起的局域密度涨落进行了分析.分析表明,这种成丝不稳定性主要是由有质动力造成的.     

The photosensitive effect of Ce on the precipitation of Ag nanoparticles induced by femtosecond laser in silicate glass

This paper studies the photosensitive effect of cerium oxide on the precipitation of Ag nanoparticles after femtosecond laser irradiating into silicate glass and successive annealing. Spectroscopy analysis and diffraction efficiency measurements show that the introduction of cerium oxide may increase the concentration of Ag atoms in the femtosecond laser-irradiated regions resulting from the photoreduction reaction Ce³⁺ + Ag⁺ \to Ce³⁺ + Ag⁰ via multiphoton excitation. These results promote the aggregation of Ag nanoparticles during the annealing process. It is also found that different concentrations of cerium oxide may influence the Ag nanoparticle precipitation in the corresponding glass.     

飞秒脉冲激光1维强度调制的传输特性

实验研究了飞秒激光干涉条纹在CS2介质中传输的增长率与条纹间隔以及增长率与中心峰值强度的关系。结果发现,在非线性介质中传输的1维干涉调制特别是当其调制频率位于中心光强对应的最快增长频率附近时,随着传输距离的增加调制场迅速获得增长,将高斯光束分裂成多根峰值强度很高的带状细丝。相应的数值模拟与实验结果具有较好的一致性。     

飞秒激光对氟化镁烧蚀机理研究

用扫描电镜(SEM)研究了氟化镁在800nm超短脉冲激光作用下的单枪表面烧蚀形貌.根据烧蚀斑面积与激光脉冲能量间的对数关系，测得烧蚀阈值与激光脉宽的关系曲线(55—750fs).计算了导带电子的双光子吸收，改进了多速率方程模型，很好地解释了实验结果. 关键词： 飞秒激光 氟化镁 烧蚀机理 双光子吸收     

激光诱导玻璃内部金纳米颗粒的析出及光谱

使用钛宝石飞秒激光引发和热处理相结合，实现了在含有金离子的硅酸盐玻璃内部，有空间选择性地析出金纳米颗粒。对吸收光谱的研究表明，随着热处理温度的升高，吸收峰强度增大且红移；随着激光功率密度的增大，金纳米颗粒也增大。在特定的激光和热处理条件作用下，可以在玻璃内部有空间选择性的使金离子还原后聚集，形成金纳米颗粒，具有量子尺寸效应。改变激光功率和热处理温度可以控制所析出的金属纳米粒子的尺寸，从而实现多色显示，飞秒激光诱导金纳米颗粒具有稳定性，颜色具有持久性。     

Optical studies of two dimensional gratings in fused silica, GE 124, and Foturan glasses fabricated using femtosecond laser pulses

Herein we present results on the femtosecond laser direct writing and optical characterization studies of two dimensional gratings in fused silica, GE 124, and Foturan^™ glasses. Varieties of structures were achieved with varying input energy and spatial orientation of the samples. Various characterization techniques including fluorescence spectroscopy, micro-Raman spectroscopy, and laser confocal microscopy were employed to analyze the structural and physical modifications at the focal volume resulting in change of refractive index. Diffraction efficiencies of 9–12% were observed from the grating structures. A broad-band emission was observed in the laser-modified region of the Foturan glass. The obtained results are analyzed in the light of recent work in similar glasses and exploring the applications of such structures in the fields of photonics.     

飞秒激光器的相位薄膜

论述了飞秒激光器的相位补偿特点，讨论了采用位薄膜作为补偿晶体的色散和相位自调制的飞秒激光器，并对相位薄膜进行了理论设计。     

Femtosecond laser-induced damage in reflector

We have investigated the damage for ZrO₂/SiO₂ 800 nm 45° high-reflection mirror with femtosecond pulses. The damage morphologies and the evolution of ablation crater depths with laser fluences are dramatically different from that with pulse longer than a few tens of picoseconds. The ablation in multilayers occurs layer by layer, and not continuously as in the case of bulk single crystalline or amorphous materials. The weak point in damage is the interface between two layers. We also report its single-short damage thresholds for pulse durations ranging from 50 to 900 fs, which departs from the diffusion-dominated scaling. A developed avalanche model, including the production of conduction band electrons (CBE) and laser energy deposition, is applied to study the damage mechanisms. The theoretical results agree well with our measurements.     

各阶克尔非线性折射率对强激光大气传输的影响

用数值方法研究了各阶克尔非线性折射系数对强激光传输的影响,结果显示第7阶克尔非线性系数和第9阶克尔非线性系数协同影响激光传输,当第7阶克尔效应起作用时,忽略第9阶克尔效应的作用会导致光强随传输距离震荡剧烈,传输非常不稳定。要得到稳定传输需要第7阶克尔非线性系数和第9阶克尔非线性系数同时起作用或同时不起作用。在自聚焦阶段第3阶非线性折射率对折射率改变起主要作用,在稳定光丝传输阶段第7阶克尔非线性系数,第9阶克尔非线性系数起主要作用。第5阶克尔系数在整个传输过程中对折射率的改变一直比较小。     

飞秒激光相干场诱导材料功能微结构

飞秒激光在整个脉冲宽度内具有极好的相干性，因而当从同一光束分出的两束或两束以上的光束时间与空间上实现相互叠加时将会形成强度周期性调制的电磁场．这种周期调制的电磁场与材料产生相互作用，能诱导出相应的周期微结构．最近通过两束或两束以上飞秒激光干涉诱导功能微结构得到了广泛研究．文章综合了国内外飞秒激光研究小组在干涉诱导微结构方面的一些最新成果以及作者在这方面开展的工作，对飞秒激光干涉技术的原理及其在诱导微结构方面的应用进行了介绍．