Dynamics of Two-Photon Lasers with A Atomic Level Configuration

We derive the dimensionless dynamic equations of two-photon lasers with A atomic level configuration by using the quantum Langevin equation method with the considerations of atomic coherence and injected classical fields. Then we analyze the stability and the chaotic dynamics of the two-photon laser by calculating the bifurcation diagram and the maximum Lyapunov exponent （MLE）. Our results show that the Lorenz strange attractors and one-focus strange attractors can exist in this system, and the chaos can be induced or inhibited by the injected classical fields via Hopfbifurcations or crises, while the atomic coherence induces chaos via crises, and inhibit chaos via Hopf bifurcation or crises.     

Effects of Atomic Coherence and Injected Classical Field on Chaotic Dynamics of Non-degenerate Cascade Two-Photon Lasers

Based on the cascade two-photon laser dynamic equation derived with the technique of quantum Langevin operators with the considerations of coherently prepared three-level atoms and the classical field injected into the cavity, we numerically study the effects of atomic coherence and classical field on the chaotic dynamics of a two-photon laser. Lyapunov exponent and bifurcation diagram calculations show that the Lorenz chaos and hyperchaos can be induced or inhibited by the atomic coherence and the classical field via crisis or Hopf bifurcations.     

Effects of Atomic Coherence and Injected Classical Field on Chaotic Dynamics of Non-degenerate Cascade Two-Photon Lasers

Based on the cascade two-photon laser dynamic equation derived with the technique of quantum Langevin operators with the considerations of coherently prepared three-level atoms and the classical field injected into the cavity, we numerically study the effects of atomic coherence and classical field on the chaotic dynamics of a two-photon laser. Lyapunov exponent and bifurcation diagram calculations show that the Lorenz chaos and hyperchaos can be induced or inhibited by the atomic coherence and the classical field via crisis or Hopf bifurcations.     

Self-pulsing Instability in Two-PhotonLasers of the Class B

1.IntroductionLasersystemshavebccnkno`"ntounderg0stabiIitychangesunderccrtainconditi0ns.Inthesingle-m0de1asers,forexampIc,thereisasecondthresh0Idvalueabovewhichafurtherinstability,namely,sclf-pulsing,sctsin[1'2J.H0\\'cver,inthccaseof0nc-ph0tonlasersoftheclassB,n0self-pulsinginstabilityoccursf0rthefrcc-runningandatresonance.Instabili-tiesin'tx"o-ph0t0nlasersystc112shavcals0bceninvcstigatcdthe0rctically.Inrecentyears,two-phQtonlaser0scillationhasbccnobscrvedinaFabry-Per0tcavityfil1edx"ithrub…     

羟基自由基双光子激发解离动力学

本文利用高里德堡态氢原子飞行时间探测技术,研究了羟基自由基的双光子激发解离动力学. H(²S)+O(¹D)和H(²S)+O(¹S)解离通道是由于羟基在经由A²Σ⁺(v''=2, J''=0.5-2.5)中间态通过双光子激发最终到排斥性的激发态势能曲线2²Ⅱ和B²Σ⁺上产生. 这两种解离通道产物都具有各向异性的角向分布,其中H(²S)+O(¹D)产物角分布异向因子β为-0.97,H(²S)+O(¹S)产物角分布异向因子β为1.97. 各向异性的角向分布与OH自由基在排斥性的激发态势能曲线上直接解离机理相吻合. 此实验观测到羟基自由基的解离能为35580±15 cm^-1.     

共振简并双光子激光近阈行为的理论研究

采用量子理论讨论共振简并双光子激光的小偏谐近阈行为，在一定条件下，系统能够呈现无反转激光，在另一条件下，系统则以于现无激光反转。     

飞秒激光在可饱和吸收体中的动力学特性

从激光动力学的自洽理论出发，推导出适用于含有可饱和吸收体的激光系统动力学方程组，研究了激光振荡的稳定性与系统参数的依赖关系，包括激励强度参数、饱和系数和能级寿命，并讨论了满足激光振荡稳定性的条件下B类激光的弛豫振荡特性。结果表明，增大激励强度与饱和系数有利于系统形成稳定的振荡输出，而且当激励强度超过一定阈值时，B类激光会产生弛豫振荡行为。     

Molecular Dynamics of Biological Probes by Fluorescence Correlation Microscopy with Two-Photon Excitation

We report on the application of fluorescence correlation microscopy under two-photon excitation of fluorophores of biological interest: FITC–dextran (MW, from 20 to 150 kDa), green fluorescent protein (MW, 27 kDa), and fluorescein (MW, 330 Da). Under these experimental conditions, the translational diffusion coefficients of these molecules in aqueous solutions derived from the fluorescence intensity autocorrelation function were determined for the first time and were found to be 24 × 10^–7, 8.2 × 10^–7, and 3 × 10^–7 cm² s^–1 for 150-kDa FITC–dextran, green fluorescent protein, and fluorescein, respectively. These results are discussed in connection with previously reported results obtained by different methods. The great sensibility of the system has been applied to single-molecule detection of the smaller fluorophore, fluorescein.     

锁模光纤激光器时变动力学

锁模激光器除了可以产生稳定的超短脉冲以外,还可产生一系列重要的非平衡态动力学过程.这些快速变化的动力学过程有助于理解超快激光器和相关非线性系统的动力学,也对超快激光器的稳定性设计有重要指导意义.随着超快探测技术的发展,锁模激光器超快动力学的研究取得了一系列突破.介绍了锁模激光器几个典型的非平衡态动力学过程,包括锁模启动...     

Dynamic Equations and Nonlinear Dynamics of Cascade Two-Photon Laser

We derive equations and study nonlinear dynamics of cascade two-photon laser, in which the electromagnetic field in the cavity is driven by coherently prepared three-level atoms and classical field injected into the cavity. The dynamic equations of such a system are derived by using the technique of quantum Langevin operators, and then are studied numerically under different driving conditions. The results show that under certain conditions the cascade two-photon laser can generate chaotic, period doubling, periodic, stable and bistable states. Chaos can be inhibited by atomic populations, atomic coherences, and injected classical field. In addition, no chaos occurs in optical bistability.     

Carrier Dynamics in Quantum Well Lasers

A fully microscopic theory is used to perform an analysis of carrier–carrier and carrier-LO phonon scattering in semiconductor quantum wells, focussing on the high-density case relevant for laser structures. A large variance of scattering times is observed depending on the material parameters, apparently contradicting popular belief in some cases. For instance, carrier–carrier scattering may slow down when the carrier density is increased. Electron-hole scattering times are found to be on the same order of magnitude as carrier-phonon scattering, making the introduction of a separate electron and hole temperature necessary. Heating by optical pumping is investigated and plasma cooling is shown to be possible by optical pumping of the laser structure.     

Round-Trip-Time Nonlinear Dynamics of Electro-Optically-Controlled Solid State Lasers

We show numerically and analytically that the technique using a combination of optoelectronic feedback loops allows one to realize new time scale regimes in solid state lasers. In a self mode-locked laser, the combination of negative and positive feedback enables the realization of nonlinear dynamics similar to the logistic map. In quasi-CW mode, the combination leads to a laser output in the form of a square wave with a period of two cavity-round-trip times. The proposed approach paves the way to a regular pulsation with a period of three or four cavity-round-trip times as well.     

Dynamics of Semiconductor Lasers with Optical Feedback from Photorefractive Phase Conjugate Mirror

The dynamics of semiconductor lasers with photorefractive phase conjugate optical feedback are experimentally studied. Photorefractive fringes considered here are rather static compared with time fluctuations of laser output power. Therefore, it is expected that a semiconductor laser with photorefractive feedback shows similar dynamics to those with conventional optical feedback. We examine relaxation oscillation and external cavity modes of laser output power in the presence of photorefractive phase conjugate feedback. It is proved that the dynamics of photorefractive phase conjugate feedback are fundamentally the same as those of conventional optical feedback.     

Two-Photon Fluorescence Property and Ultrafast Dynamics of Two Dipolar Compounds with Dipicolinate as Electron Acceptor

Linear and nonlinear photophysical properties of two novel dipolar compounds named as trans- dimethyl-4-[4＇-（N,N-dimethylamino）-styry1]-pyridin-2,6-dicarboxylate （Xiao-1） and trans-dimethyl-4-[4＇-（N,N-diphenylamino）-styry1]-pyridin-2,6-dicarboxylate （Xiao-2） are investigated by steady-state absorption and fluorescence spectroscopy, Z-scan and two-photon excited fluorescence measurements. Strong two-photon fluorescence emission and the pronounced positive solvatochromism are observed from two compounds. The two-photon absorption cross section of Xiao-2 is about 1.5 times larger than that of Xiao-1. One-color and two-color femtosecond pump-probe experiments are employed to investigate the excited state dynamics of two compounds. The relaxation lifetime of the intra-molecular charge transfer state is determined to be in the hundreds of picosecond domain for both the compounds in THF, and several tens of picosecond in DMSO solutions.     

Influence of Atomic Phase Fluctuations on Field Squeezing and Brightness of Many Two-Photon Correlat ed-Spont aneous-Emission Lasers

We show in this paper that phase fluctuations of active atoms in many twephoton correlatedspontaneous-emission lasers will reduce field squeezings and brightness of the squeezed light. But, under certain conditions of laser operation, the fluctuations of atomic phases between lower almost degenerate atomic levels could increase the squeezings and the brightness. We also show that, even for large phase fluctuations of the active atoms, almost perfect field squeezings and substantial brightness of the squeezed light can be obtained.     

Modelling of Threshold and Extraction Efficiency in Pr3+ ZBLAN Upconversion Fibre Lasers Using Two-Photon Pumping

We model the steady-state threshold and extracted power of a two-photon incoherently pumped upconversion fibre laser. Our threshold analysis is entirely analytic, and along with this derivation we obtain an analytic threshold cutback formula. This takes a particularly simple form when the ground state pump absorption follows exponential absorption. We also numerically simulate the extracted laser power. The experiment which we simulate is upconversion in Pr³⁺ doped ZBLAN fibre lasing at 491 nm and pumped with 1017 nm and 835 nm diode lasers. Our formulas and simulations are mutually consistent and agree with the experiment to within 10%.     

飞秒超短脉冲的双光子干涉

利用钛宝石飞秒激光超短脉冲抽运BBO晶体,产生Ⅰ型自发光参量下转移的双光子对,在实验上得到双光子对的四阶干涉现象,证明了双光子纠缠态的关联特性。