极化检测型铷原子磁力仪的研究

针对交变弱磁场的检测,研制了一种基于极化-检测双光束结构的激光抽运铷原子磁力仪.为了获得该磁力仪对磁场的响应特性,通过数值仿真分析了信号幅度随极化磁场强度、弛豫时间的变化关系,并进行了实验验证.最后通过选择合适的极化磁场使磁力仪对待测磁场的灵敏度最大.实验结果表明,优化后磁力仪灵敏度为0.2pT/(Hz)~(1/2),响应带宽3.5kHz,可用于弱磁场磁共振、高频异常物理现象等信号的检测.     

Structural,Spectroscopic and Vibrational Properties for Low-Lying Electronic States of LiCl

A multireference configuration interaction (MRCI) study has been carried out on the LiCl molecule. The potential energy has been calculated over a wide range of internuclear separation for the 21 low-lying electronic states of the LiCl molecule dissociating into Li (²S, ²P, ³S)+Cl(²P). The (4)¹Σ⁺, (3)¹Π, 1-3³Σ⁺, 1-3³Π, ^1,3Δ, ^1,3Σ^-, (5)¹Σ⁺, (4)³Σ⁺, (4)¹Π, (4)³Π excited states are studied for the first time in theory. Molecular spectroscopic constants (R_e, D_e, ω_e, ω_eχ_e, B_e and α_e) have been derived for the 9 bound states (X¹Σ⁺, (3)¹Σ⁺, (2)¹Σ⁺, ^1,3Δ, ^1,3Σ^-, (4)¹Π, (4)³Π) with a regular shape, and the spectroscopic constants of ground states X¹Σ⁺ are in good agreement with available experimental and theoretical values. The relative differences between experimental values and our values for R_e, D_e, ω_e, ω_eχ_e, B_e and α_e are 1.02%, 0.60%, 1.72%, 9.46%, 2.0%, and 0.75%, respectively. Moreover, vibrational levels of 9 bound states, which have not been investigated experimentally, are computed.     

Theoretical Study on the Low-Lying Electronic States of He2, He2+, and He2++

The equilibrium geometries, potential energy curves, spectroscopic dissociation energies of the ground and low-lying electronic states of He₂, He₂⁺ and He₂⁺⁺ are calculated using symmetry adapted cluster/symmetry adapted cluster-configuration interaction (SAC/SAC-CI) method with the basis sets CC-PV5Z. The corresponding dissociation limits for all states are derived based on atomic and molecular reaction statics. The analytical potential energy functions of these states are fitted with Murrell--Sorbie potential energy function from our calculation results. The spectroscopic constants B_e, α _e, ω _e, and ω _e χ _e of these states are calculated through the relationship between spectroscopic data and analytical energy function, which are in well agreement with the experimental data. In addition, the origin of the energy barrier in the ground state X¹Σ_g⁺ of He₂⁺⁺ energy curve are explained using the avoided crossing rules of valence bond model.     

GeS分子基态和低激发态的势能曲线与光谱性质

本文以aug-cc-pv5Z为基组, 采用考虑Davidson修正的多参考组态相互作用方法(MRCI+Q)得到了GeS分子基态(X¹Σ⁺)和5个低激发态(1¹Σ, 1¹Δ, A¹Π, 1⁵Σ⁺, 2⁵Σ⁺)的势能曲线. 计算结果表明: 2⁵Σ⁺态为排斥态, 其余5个态为束缚态; 6个态有着共同的离解通道, 离解极限均为Ge(³P)+S(³P). 利用计算得到的势能曲线得了X¹Σ⁺, 1¹Σ^-, 1¹Δ, A¹Π和1⁵Σ⁺态的垂直跃迁能T_e, 平衡键长R_e, 离解能D_e, 谐振频率ω_e, 非谐性常数ω_ex_e及平衡位置的电偶极矩. X¹Σ⁺态的R_e 为2.034 Å, D_e 为5.728 eV, ω_e为571.73 cm^-1, ω_ex_e为1.6816 cm^-1, 平衡位置的电偶极矩为1.9593 Debye. 激发态1¹Σ, 1¹Δ, A¹Π, 1⁵Σ⁺的T_e 依次为25904.81, 26209.22, 32601.19, 43770.26 cm^-1; R_e依次为2.313, 2.322, 2.188, 2.8790 Å; D_e依次为2.524, 2.487, 1.694, 0.3036 eV, ω_e依次为358.90, 353.08, 376.32, 134.96 cm^-1; ω_ex_e依次为1.2421, 1.2151, 1.6608, 1.9095 cm^-1; 平衡位置的电偶极矩依次为1.3178, 1.4719, 1.5917, -1.9785 Debye. 通过求解核运动的薛定谔方程得到了J=0时X¹Σ⁺, 1¹Σ^-, 1¹Δ, A¹Π和1⁵Σ⁺态前30个振动态的振动能级G_v和分子常数B_v, 得到的结果和已有的实验值及其他理论值符合较好.     

Acoustic double layers in multispecies plasma

Particle simulation in a one-dimensional bounded system is used to examine the formation of acoustic double layers in the presence of two ion species. Double-layer formation depends critically on the details of the distribution functions of the supporting ion populations, and their relative drifts with respect to the electrons. The effect of having two ion components, an H⁺ and an O⁺ beam, on double-layer evolution from ion acoustic turbulence driven by an electron drift relative to the H⁺ beam of ≈0.5u _e, where uu_e is the electron thermal speed, is examined. The ratio of ion drifts is taken to be consistent with acceleration by a quasi-static auroral potential drop (i.e. V _H/V_O=√M_O/ M_H=4.0). Acoustic double layers form in either ion species on the time scale τ≈100ω_ps^-1, where ω_ps is the ion plasma frequency for species `s' and s=H or O, and for drifts relative to the electrons lower than that required for double layer formation in simulations of single ion component plasma     

AsCl自由基的基态及激发态的势能函数与光谱常数的研究

利用原子分子反应静力学推导出AsCl自由基的基态及激发态的理解极限. 采用完全活性空间自洽场和含Davidson 修正的内收缩多参考组态相互作用理论方法, 在aug-cc-pV5Z基组下对AsCl自由基进行结构优化计算及单点能扫描计算. 在AsCl自由基基态势能曲线的基础上, 通过Molcas程序拟合出了AsCl的光谱常数D_e, R_e, ω_e, ω_eχ_e, B_e 和α_e. 通过求解双原子分子核运动的径向Schrödinger方程, 找到了J=0 时该分子基态存在的40个振动态. 针对每一振动态, 计算了其振动能级、转动惯量B_ν和离心畸变常数D_ν, 与现有的实验及其他理论相比较, 本文的光谱参数和分子常数结果更准确. 关键词： AsCl 势能函数 光谱常数     

Dark and Bright Solitons of Extraordinary Waves in Ferromagnetic Systems

It is shown that the slowly varying amplitudes of both high and low frequency extraordinary waves propagating perpendicular to the dc magnetic field in ferromagnetic systems are described by the nonlinear SchrEdinger equation. The extraordinary waves are modulationally stable (unstable) and may evolve as dark (bright) solitons as the frequency ω satisfies ω₀ < ω < ω_b or ω > ω₁(0 < ω < ω₀ or ω_a ≤ ω < ω₁), where ω_a, ω_b, ω₀ and w₁ are given in the text.     

BeC分子基态和低激发态光谱性质和解析势能函数

BeC是一个具有丰富低激发电子态的分子,本文基于动态权重完全活性空间自冾场方法获得的参考波函数,采用多参考组态相互作用方法对BeC分子进行高精度的从头计算,获得了BeC分子X~3Σ~-,A~3Π,b~1Δ,c~1Π和d~1Σ~+共5个电子态的势能曲线.为了获得精确的光谱结果,在计算中考虑了标量相对论效应修正,并把相互作用能外推至完全基组极限.在此基础上获得了这些态的光谱常数和偶极距,以及一些允许跃迁的跃迁偶极距、弗兰克-康登因子和辐射寿命.最后,通过扩展的Rydberg函数拟合获得了基态势能曲线精确的解析表达式.     

WKB solution for wave propagation in a time-varying magnetoplasmamedium: longitudinal propagation

The interaction of a right circularly polarized electromagnetic wave of frequency ω₀ with a switched-on-time-varying plasma medium, in the presence of a static magnetic field, is considered. Longitudinal propagation is assumed and ion motion is neglected. The electron density is assumed to vary slowly with time, and the solution is obtained through a WKB approximation. The main effect of switching the time-varying medium is the splitting of the original (incident) wave of frequency ω₀ into three new waves with time-varying frequencies. An exponentially increasing electron density profile is considered to illustrate the solution. The distinguishing feature of the presence of the static magnetic field is the creation of the third wave. The initial value of the instantaneous frequency ω₃ of this wave is equal to the gyrofrequency ω_b, and the final value depends on ω_b, ω₀, and the final value of the plasma frequency. ω₃ decreases with time for the profile under consideration     

Cold-Fluid Analysis of the Space-Charge Effects in an Electromagnetically Pumped Free-Electron Laser with an Axial-Guide Magnetic Field

The space-charge effects are analysed and five kinds of fluid waves are obtained in the e-beam density and the axial-current density for an electromagnetically pumped free-electron laser with an axial-guide magnetic field by using the cold-fluid theory. To enhance the gain, the guide field Bo must be in this regime: -2(ω_υ + cβ_x0k_ω) < Ω < -(ω_υ + cβ_x0k_ω), where Ω₀ = eB₀/mr₀ and ω_υ(k_ω) is the frequency (wave number) of the wiggler.     

Optimal configuration for vibration frequencies in a ring of harmonic oscillators: The nonidentical mass effect

The parameter diversity effect in coupled nonidentical elements has attracted persistent interest in nonlinear dynamics. Of fundamental importance is the so-called optimal configuration problem for how the spatial position of elements with different parameters precisely determines the dynamics of the whole system. In this work, we study the optimal configuration problem for the vibration spectra in the classical mass–spring model with a ring configuration, paying particular attention to how the configuration of different masses affects the second smallest vibration frequency (ω₂) and the largest one (ω_N). For the extreme values of ω₂ and ω_N, namely, (ω₂)min, (ω₂)max, (ω_N)min, and (ω_N)max, we find some explicit organization rules for the optimal configurations and some approximation rules when the explicit organization rules are not available. The different distributions of ω₂ and ω_Nare compared. These findings are interesting and valuable for uncovering the underlying mechanism of the parameter diversity effect in more general cases.     

On the effect of long-wavelength electron plasma waves onlarge-angle stimulated Raman scattering of short laser pulse in plasmas

Spectral features of a large-angle stimulated Raman scattering (LA SRS) of a short electromagnetic pulse in an underdense plasma, which are caused by the presence in a plasma of a given linear long-wavelength electron plasma wave (LW EPW), are investigated. It is shown that the LW EPW, whose phase velocity coincides with a group velocity of a pulse and a density perturbation normalized to a background electron density δn_LW/n₀ exceeds the ratio of the electron plasma frequency to the laser frequency ω_pe/ω₀ suppresses the well-known Stokes branch of the weakly coupled LA SRS. Under the same condition, the anti-Stokes band appears in the spectrum of the scattered radiation. Variation of a scattering angle and an electron temperature do not significantly modify qualitative features of the effect. In the case of strongly coupled LA SRS, the maximum of the increment is decreased by nearly one-half for δn_LW/n₀~(a₀ω_pe /ω₀)^2/3≫ω_pe /ω₀, where a₀ is an amplitude of an electron quiver velocity in the laser field normalized to a speed of light c, and it decreases further with an increase in plasma density perturbation in LW EPW     

Second harmonic stimulated Raman scattering of laser radiation in aplasma

A high-power linearly polarized laser propagating through a plasma produces oscillatory electron velocity at the second harmonic due to-the ν&oarr;×B&oarr; force, This velocity couples a Langmuir wave (ω, k&oarr;) and an electromagnetic wave (ω₁, k&oarr;₁), where ω₁=ω-2ω₀ , k-2k&oarr;₀ and ω₀, k&oarr;₀ are frequency and wavenumber of the laser pump, causing second harmonic Raman scattering. The growth rate is maximum for side scattering. This process can occur above the quarter critical density, unlike the first harmonic stimulated Raman scattering which occurs below the quarter critical density     

Oscillating two-stream instability of a plasma wave in a plasmachannel

A long wavelength Langmuir wave (ω₀, k₀), propagating through a parabolic plasma density channel, can decay into a low-frequency mode (ω,k&oarr;) and two short wavelength Langmuir wave sidebands (ν_1,2,k&oarr;_1,2 ), via two-stream instability where ω_1,2=ω∓ω₀ and k&oarr;_1,2=k&oarr;∓k&oarr;₀. Depending on the mode number n, the growth rate maximizes in the range γ_max≃0.1ω_pi-0.4ω_pi for the range of k from 0.1(ω_pi/c_s) to 0.2(ω_pi/c_x) for ν₀~ν_th where ν₀ and ν_th are the oscillatory and thermal velocities of electrons, ω_pi is the ion plasma frequency on the axis, and c_s is the sound speed. The growth rate increases with the width a of the plasma density channel. It decreases with the mode number. The instability may be relevant to laser based charged particle accelerators     

Analysis of the deflection system for a magnetic-field-immersedmagnicon amplifier

A linear analysis of the electron-beam deflection system in a magnicon amplifier is presented. The system consists of identical cavities, one driven and the remainder passive, separated by a drift space and immersed in an axial magnetic field. The cavities contain a rotating TM₁₁₀ mode. The length of each cavity is πν _z/ω, and that of the drift space is πν_z/ω_c, where ω is the RF frequency, ω_c is the relativistic gyrofrequency in the guide field, and ν_z is the mean axial velocity of the beam electrons. The linearized electron orbits are obtained for arbitrary initial axial velocity, radial coordinate, and magnetic field. The small-signal gain and the phase shift are determined. The special case where ω_c/ω=2 has unique features and is discussed in detail. For the NRL magnicon design, a power gain of 10 dB per passive cavity is feasible. Results from numerical modeling of a magnicon with two passive cavities are presented. Operation of the output cavity at the fundamental and higher harmonics of the input drive frequency is briefly discussed     

Constraining a New Type of Dark Energy Model from Present Observations

We propose a new type of dark energy (DE) model, in which the equation of state of DE ω de is a simple function of the fractional energy density de instead of the redshift z. We assume three DE models of this type, and fit them with present observations to get constraints of DE, which are also compared with the CPL model. It is shown that a suitable ω de (Ωde ) model can give smaller χ2 or smaller errors of ω de than that of the CPL model. This new type of DE model can help to study the essential properties and nature of DE.     

Third-Order Optical Nonlinearity in Two-Dimensional Transition Metal Dichalcogenides

We present a detailed calculation of the linear and nonlinear optical response of four types of monolayer twodimensional (2D) transition-metal dichalcogenides (TMDCs), having the formula MX₂ with M=Mo, W and X=S, Se. The calculations are based on 6-band tight-binding model of TMDCs, and then performing a semi-classical perturbation analysis of response functions. We numerically calculate the linear χ_μν⁽¹⁾ (-ω;ω) and nonlinear surface susceptibility tensors χ_μνζη⁽³⁾(-ω_Σ; ω_r; ω_s; ω_t) with ω_Σ=ω_r+ω_s+ω_t. Both non-degenerate and degenerate cases are studied for thirdharmonic generation and nonlinear refractive index, respectively. Computational results obtained with no external fitting parameters are discussed regarding two recent reported experiments on MoS₂, and thus we can confirm the extraordinarily strong optical nonlinearity of TMDCs. As a possible application, we demonstrate generation of a π/4-rotated squeezed state by means of nonlinear response of TMDCs, in a silica micro-disk resonator covered with the 2D material. Our proposed method will enable accurate calculations of nonlinear optical response, such as four-wave mixing and highharmonic generation in 2D materials and their heterostructures, thus enabling study of novel functionalities of 2D photonic integrated circuits.     

Accurate Analytic Potential Energy Function and Spectroscopic Study for G^1Ⅱg State of Dimer ^7Li2

The reasonable dissociation limit for the G^1Ⅱg, state of dimer ^7Li2 is determined. The equilibrium internuclear distance, dissociation energy, harmonic frequency, vibrational zero energy, and adiabatic excitation energy are calculated using a symmetry-adapted-cluster configuration-interactlon method in complete active space in Gaussian03 program package at such numerous basis sets as 6-311 ＋＋G, 6-311 ＋＋G（2df,2pd）, 6-311 ＋＋G（2df, p）, cc-PVTZ, 6- 311＋＋G（3df,3pd）, CEP-121G, 6-311＋＋G（2df, pd）, 6-311＋＋G（d,p）,6-311G（3df,3pd）, D95（3df,3pd）, 6-311＋＋G（3df,2p）, 6-311＋＋G（2df）, 6-311＋＋G（df, pd） D95V＋＋, and DGDZVP. The complete potential energy curves are obtained at these sets over a wide internuclear distance range and have least squares fitted to Murrell-Sorbie function. The conclnsion shows that the basis set 6-311＋＋G（2df, p） is a most suitable one for the G^1Ⅱg state. At this basis set, the calculated spectroscopic constants Te, De, Eo, Re, ωe, ωeXe, ae, and Be are of 3.9523 eV, 0.813 06 eV, 113.56 cm^-1, 0.320 15 nm, 227.96 cm^-1, 1.6928 cm^-1, 0.004 436 cm^-1, and 0.4689 cm^-1, respectively, which are in good agreement with measurements whenever available. The total 50 vibrational levels and corresponding inertial rotation constants are for the first time calculated and compared with available RKR data. And good agreement with measurements is obtained.     

Equilibrium dynamics of the sub-Ohmic spin-boson model under bias

Using the bosonic numerical renormalization group method, we studied the equilibrium dynamical correlation function C(ω) of the spin operator σ_z for the biased sub-Ohmic spin-boson model. The small-ω behavior C(ω) ∝ω~s is found to be universal and independent of the bias ε and the coupling strength α(except at the quantum critical point α = αc and ε = 0). Our NRG data also show C(ω) ∝χ~2ω~s for a wide range of parameters, including the biased strong coupling regime(ε = 0 and α α_c), supporting the general validity of the Shiba relation. Close to the quantum critical point αc,the dependence of C(ω) on α and ε is understood in terms of the competition between ε and the crossover energy scale ω_0~*of the unbiased case. C(ω) is stable with respect to ε for ε《ε~*. For ε》ε~*, it is suppressed by ε in the low frequency regime. We establish that ε~*∝(ω_0~*)~(1/θ)holds for all sub-Ohmic regime 0≤s 1, with θ = 2/(3s) for 0 s≤1/2 and θ = 2/(1 + s) for 1/2 s 1. The variation of C(ω) with α and ε is summarized into a crossover phase diagram on the α–ε plane.