波长锁定878.9nm激光二极管抽运内腔式YVO_4/BaWO_4连续波拉曼激光器

采用波长锁定878.9 nm激光二极管共振抽运复合Nd:YV04激光晶体,改善热效应的同时提高抽运吸收率,分别以YVO_4和BaWO_4晶体作为拉曼介质,实验和理论研究了晶体性能、谐振腔结构和稳定性对内腔分体式连续波拉曼激光器性能的影响.结果表明:由于内腔分体式拉曼激光器腔长较长,谐振腔稳定性对激光器性能影响较大,选择高增益的拉曼晶体,不仅可获得高拉曼转换效率,还能一定程度上减轻热效应.而平凹腔结构中输出镜的曲率半径越小,拉曼晶体中基频光的功率密度越大,腔的动态稳定区越宽,获得的拉曼激光输出功率更高.最终以30 mm的BaWO_4晶体作为拉曼介质,在抽运功率25.1 W时,获得了3.02 W的连续拉曼激光输出,光-光转换效率达到12%.     

Picosecond parametric Raman laser based on KGd(WO4)2 crystal

Simultaneous frequency up and down conversion using a biharmonically pumped parametric Raman laser (PRL) based on a KGd(WO₄)₂ (KGW) crystal has been demonstrated experimentally. Collimated beams have been generated for both the 1st anti-Stokes (1AS) at 511 nm and 2nd Stokes (2S) at 579 nm by four-wave parametric Raman interaction. To excite PRL biharmonically, we pumped the KGW crystal with 20 ps pulses at the fundamental 530 nm and its 1st Stokes component at 555 nm. The 1st Stokes pump beam was generated using stimulated Raman scattering in a separate KGW Raman oscillator. The energy conversion efficiencies reached experimentally were 10% for the 2S and 4% for the 1AS.     

YbVO4晶体的受激拉曼散射

采用腔外单次通过方式,研究了一种新型晶体YbVO₄的受激拉曼散射.当抽运激光为532 nm皮秒脉冲时获得了3级斯托克斯线(558.47 nm, 587.92 nm, 620.67 nm)和1级反斯托克斯线(507.58 nm),测得YbVO₄晶体1级斯托克斯受激拉曼散射的稳态增益系数为17.8±0.2 cm/GW,受激拉曼散射的整体转换效率达到37%.实现了YbVO₄晶体对355 nm皮秒激光的受激拉曼散射,观察到1级斯托克斯线(366.1 关键词： 受激拉曼散射 稳态增益系数 转换效率 4晶体')" href="#">YbVO₄晶体     

用受激拉曼泵浦方法高效制备v=2振动激发态氘分子

We report the preparation of D₂ molecules in v=2 level in molecular beam condition. A single longitudinal mode laser system was used for excitation of D₂ from (v=0, j=0) to (v=2, j=0) with the scheme of stimulated Raman pumping. An excitation efficiency of 25.2% has been achieved, which was determined by the scheme of resonance-enhanced multiphoton ionization. Dependence of relative excitation efficiency on laser energy has been measured. We found that the increasing rate of excitation efficiency became slower as pulse energy of Stokes laser increase, while the excitation efficiency still increases approximately linearly with pump pulse energies up to 60 mJ. The spectral line shapes of Raman transition was also measured at different laser energies and considerable dynamical Stark effect was observed. A single peak was found on the three dimension surface of relative excitation efficiency, indicating the process occurred in the present study is a process of stimulated Raman pumping instead of stimulated adiabatic Raman passage.     

High Efficient C6H12 Raman Laser Enhanced by DCM Fluorescence

We report the first-order Stokes output （wavelength of 627.6 nm） from C6H12 enhanced by DCM dye fluorescence with high energy conversion efficiency of 47.9%, quantum conversion efficiency of 56.5%. To our knowledge, it is the highest conversion efficiency of stimulated Raman scattering obtained from liquid Raman laser. A 532nm frequency doubled Nd：YAG laser with 8 Hz repetition rate is employed as the pump source, and the enhancement medium is DCM dye solution in ethanol. The conversion efficiencies at various pump energies and various pump repetition rates are measured and analysed. The enhancement mechanism of SRS together with its potential application is discussed.     

800 mW/1484 nm highly efficient two-cascaded phosphosilicate Raman fiber laser pumped by Nd:YVO4 solid-state laser

Using 1064 nm CW Nd:YVO₄ solid-state laser as a pump, 1-km phosphosilicate fiber and cascaded cavities with two pairs of fiber Bragg grating mirrors for 1239 and 1484 nm, we obtained a CW 800 mW/1484 nm Raman fiber laser (RFL) for an actual incident pump power of about 2 W (Nd:YVO₄ power of 6.90 W). The conversion efficiency is as high as 40%. To the best of our knowledge, this is the highest conversion efficiency of RFL pumped by solid-state laser. The output power instability at 1484 nm in half an hour is less than 3%. In addition, the numerical simulations are also performed. Good agreement between the results of numerical simulation and the results of the experiment has been demonstrated.     

Tuning characteristics of a high pressure CO2 laser pumped CH3F Raman laser

Conclusion We described a CH₃F Raman laser pumped by a two stage 20 atmospheres CO₂ laser. The emission spectrum of the CH₃F laser at 11 Torr extends from 23 cm^–1 to 45 cm^–1 when the CO₂ laser is scanned over the 9R emission branch at a fixed pump power of 180 mJ. The emission spectrum shows a strong structure with large parts where the FIR energy decreases to zero. This fact makes the use of such a laser for spectroscopic scanning experiments in the FIR difficult. The laser is, however, very suited for working at fixed but adjustable FIR frequencies. The pulse energy in the maxima of the emission characteristics at a pump energy of 180 mJ exceeds 300 J, which corresponds a photon conversion coefficient of more than 6%.     

波长锁定激光二极管共振泵浦Nd:YVO_4晶体连续波自拉曼激光器的设计与研究

对波长锁定878.9 nm的激光二极管共振泵浦Nd:YVO_4晶体的全固态连续波自拉曼激光器进行了理论研究.考虑了激光晶体在共振泵浦时的热透镜效应,采用ABCD传输矩阵法和等效G参数法,计算了当采用不同曲率半径输出镜时腔内振荡激光的腔模参数,通过比较抽运光与振荡激光模式匹配的情况和拉曼晶体中基频光功率密度的大小,分析了不同腔结构对拉曼激光输出功率的影响,给出了实验结果的理论解释,并进一步优化设计了谐振腔结构.最终获得了5.3 W的高功率1175 nm连续拉曼激光输出,光光转换效率达到20%.     

碘激光的H2振动受激拉曼阈值研究

首次实现了脉冲光解碘激光作为基频光的氢气振动受激拉曼变频,对碘激光的波长转换有着重要意义。在碘激光单脉冲能量100~130 mJ(脉宽100 ns)的条件下, 采用双次聚焦技术降低了高压氢气的振动受激拉曼变频的阈值,获得了波长为2900 nm中红外激光,光子转化效率最高达到8.7%。实验发现当拉曼介质氢气气压大于1 MPa后,一级斯托克斯光的拉曼转化效率不再随气压变化,并对这一现象进行了理论分析和归属。     

探测大气中CO2的Raman激光雷达

基于大气激光后向散射光谱，研究和设计了探测大气CO₂浓度的Raman激光雷达,其发射机采用Nd∶YAG激光的三倍频354.7nm作为工作波长,发射的单脉冲能量350mJ,重复频率20Hz；接收机采用了光电倍增管(量子效率25%)和光子计数器(计数速率200MHz),探测CO₂的Raman散射371.66nm(频移1285cm^-1)信号,(1小时累加)近地面2.5km以内信噪比不小于8.采用组合滤光片来抑制强的354.7nm Mie-Rayleigh后向散射和氧气375.4nm Raman后向散射对信号的严重干扰. 比较分别来自大气CO₂和参考气体N₂的Raman后向散射回波,可反演出大气中CO₂的相对浓度. 关键词： 大气光学 激光雷达 Raman散射光谱 参考气体 Mie-Rayleigh散射     

N2 laser frequency conversion by stimulated Raman scattering in H2

High-efficiency frequency conversion in H₂ of a nitrogen laser oscillator-amplifier system is described. The laser system provides about 1 MW output power with a very low intrinsic divergence. Up to 3 Stokes lines at 392, 468, and 581 nm and 3 Anti-Stokes at 296, 263, and 237 nm, respectively, have been observed at the output of the 60 cm long H₂ Raman cell. Peak power values of 500, 300, and 70 kW have been measured for the first 3 Stokes, respectively, corresponding to a 56% pump energy conversion efficiency.A comparison between free and guided propagation (in a hollow dielectric waveguide) is also reported, for various values of the pump intrinsic divergence.     

Effect of buffer gas on the generation of eye-safe 1.54 μm radiation using the stimulated Raman scattering technique in CH4

Experimental results on the generation of 1.54 μm eye-safe radiation in pure CH₄, CH₄:He and CH₄:Ar mixtures pumped by the fundamental of an Nd:YAG laser, using the stimulated Raman scattering (SRS) technique, are described. A decrease in the energy conversion efficiency and degradation in the beam quality of S₁ was observed in pure CH₄ at high pump energies. This problem was overcome in CH₄:He and CH₄:Ar mixtures. Compared with the first Stokes (1.54 μm) energy conversion efficiency in pure CH₄, at a pump energy of 126 mJ, an enhancement of 50% in energy conversion efficiency was observed in the CH₄:Ar mixture (60% argon concentration) and as much as 100% in the CH₄:He mixture (60% helium concentration). The use of these buffer gas mixtures improved the spatial beam quality of the Stokes radiation considerably and also resulted in raising the pump threshold for optical breakdown of the Raman gain medium.     

Side-pumped crystalline Raman laser

A crystalline Raman laser is pumped at 90° to the Raman laser axis by a single pass from a line-focused 532 nm pump laser of pulse duration 10 ns. The Raman laser threshold was 6.1 mJ, and at 12 mJ pump energy, a maximum output energy of 2.7 mJ was obtained with a slope efficiency of 46%. The threshold pump intensity is within a factor of 2 of the same device when end-pumped. The results highlight significant potential for coherent beam conversion and combination with enhanced degrees of flexibility and increased power.     

Continuous-wave high-power Nd:YAG-KNbO3 laser at 473 nm

A continuous-wave high-power Nd:YAG laser operating on the ⁴F_3/2→⁴I_9/2 transition at 946 nm and intracavity frequency-doubled to 473 nm by a KNbO₃ nonlinear crystal at room temperature is reported. The Nd:YAG laser outputs a randomly polarized beam of 3.8 W maximum power (38% optical-to-optical efficiency and 44% slope efficiency with respect to the absorbed pump power) at the 946 nm fundamental wavelength. Intracavity frequency-doubling with a 2.0-mm thick KNbO₃ crystal in a linear resonator yielded 159-mW single-ended blue-output with 4.8% optical-to-optical conversion efficiency versus the absorbed pump power. The 473-nm maximum power of 418 mW with 11.6% optical-to-optical conversion efficiency in absorbed power was obtained from a V-type resonator; the overall optical-to-optical conversion efficiency was 6.7%, while the conversion of the available infrared power reached 50%.     

Nd:YAG陶瓷与单晶4F3/2–4I13/2跃迁的弱谱线多波长激光性能对比

报道了基于半导体激光端面抽运Nd:YAG的⁴F_3/2–⁴I_13/2 跃迁的弱谱线多波长激光输出. 实验对比了透明陶瓷与单晶材料的激光输出特性, 表明透明陶瓷和单晶材料荧光谱强度的略微差异, 导致了多波长输出时相同两个波长之间的激光强度比在两种材料中的差异. 基于两种耦合输出镜片, 激光阈值都在2 W左右. 在13.5 W的抽运功率下, 基于Nd:YAG透明陶瓷获得了输出功率4.05 W、强度比1 :2的1338与1356 nm双波长激光和输出功率3.65 W、强度比13 : 1的1356与1414 nm 双波长激光, 斜率效率分别达33.9% 和31.9%.     

Simple and efficient H2 Raman conversion of a XeCl laser with a variable numerical aperture coupling geometry

A simple combination of a lens-based unstable resonator and an inverted telescope coupling geometry working in a XeCl laser pumped H₂ Raman cell are presented. Raman spectrum optimization is achieved by varying the pump beam numerical aperture. 70% pump depletion and energy conversion efficiencies as high as 66% and 7.8% have been obtained for S₁, S₂ and S₃ respectively.     

1064nm纳秒激光脉冲激发的外腔式PbWO4拉曼激光器

研究了外腔式PbWO4拉曼激光器在纳秒脉冲抽运下的输出特性。利用主动调Q的Nd:YAG激光器产生的脉冲宽度为31.4ns,最大输出能量为200mJ的1064nm激光作为抽运源。拉曼激光谐振腔采用的是平凹腔设计。测量了输出的拉曼光脉宽与抽运能量的关系,分析了输出的拉曼光脉冲波形图和光谱图,测量了输出的拉曼光脉冲能量与抽运能量的关系,计算了转换效率与抽运能量的关系。当注入抽运光能量达到42mJ时,得到了一阶斯托克斯光脉冲的最大能量和转换效率分别为10mJ和24%,获得外腔式PbWO4拉曼激光器的一阶斯托克斯光脉冲波长为1177.6nm,典型的一阶斯托克斯光脉冲脉宽为20ns。     

Cs 5D_(5/2)-6F 728 nm Laser Spectroscopy with Single Pumping Laser

The sub-Doppler absorption laser spectroscopy at 728 nm transition from the 5D5/2 state to the 6 F state of cesium with linewidth near 10 MHz is first experimentally performed with indirect pumping from the ground state 6S_(1/2)to the state 7P_(3/2)by a 455.5 nm diode laser.Using a 455.5 nm diode laser as an indirect pump laser,several excited states will be populated due to spontaneous decay from the 7P state.We first implement the sub-Doppler absorption laser spectroscopy at 728 nm from the 5D_(5/2)state to the 6F state when Cs atoms within thermal glass cell decay to the 5D_(5/2) state.Due to velocity transfer effect,the hyperfine structure of 5D_(5/2)shows a mixed and complicated pattern but very clear structure when the 455.5 nm pumping laser is counter-propagating(or co-propagating)with the 728 nm probing laser.     

532 nm激光泵浦硝酸钡晶体产生外腔拉曼激光

 由于硝酸钡晶体具有很强的对称振动(频率1 047 cm^-1)和较高的拉曼增益,可以用来产生受激拉曼激光。采用单端泵浦的外置拉曼振荡腔与双棱镜分光装置进行了硝酸钡晶体拉曼激光实验,泵浦源为倍频Nd: YAG的532 nm激光,硝酸钡晶体通过水溶液降温法生长,尺寸为10 mm×10 mm×48 mm,采用特殊镀膜的腔镜对各阶斯托克斯光进行优化选择。在泵浦源达到65 mJ时,获得21 mJ一阶斯托克斯光,输出波长为563 nm,以及16 mJ的二阶斯托克斯光,输出波长为599 nm,受激拉曼散射SRS最大的整体转换效率（包含一阶、二阶斯托克斯光之和）为56.3%。     

28.2 W波长锁定878.6 nm激光二极管共振抽运双晶体1064 nm激光器

报道了一种由波长锁定878.6 nm半导体激光器共振抽运两块不同掺杂浓度Nd:YVO4晶体串接的1064nm激光器,并与使用单块的低掺杂浓度晶体和高掺杂浓度晶体情况进行比较,实验表明利用波长锁定878.6nm半导体激光器共振抽运双晶体串接的方式,有利于降低晶体的热效应,提高光光转换效率.当抽运功率为40 W时,获得了28.2 W的1064 nm激光输出,光光转换率为70.5%,斜率效率为70.6%,相对吸收光的光光转换率76%,斜率效率为76.4%,同时该激光器在10?C—40?C的温度变化范围内具有极好的温度稳定性.