Broadband difference frequency mixing between visible and near-infrared pulses for few-cycle pulse generation with stable carrier-envelope phase

Difference frequency generation between broadband visible noncollinear optical parametric amplifier (NOPA) pulses and the fundamental pump laser pulses allows the generation of ultrashort infrared pulses with passively stabilized carrier-envelope phase. A simple prism compressor for the visible NOPA pulses is sufficient to generate few-cycle pulses in the infrared and no additional compression is needed. We theoretically investigate the concept, explain the principles, and demonstrate it for high repetition rate, long pulse durations, and various wavelengths by applying it to a Ti:sapphire and an Yb:KYW-based laser systems. For the latter sub-15 fs phase stable pulses around 1.8 μm with an energy of 100 nJ are obtained at 100 kHz repetition rate.     

Non-adiabatic transition in C2H5OH+ on a light-dressed potential energy surface by ultrashort pump-and-probe laser pulses

We experimentally investigate how parameters of ultrashort laser pulses such as the pulse width and wavelength could induce changes in the dynamics of vibrational wave packets on the light-dressed-potential energy surface (LD-PES) of C₂H₅OH⁺ using a pump-and-probe pulse excitation scheme. The probability of non-adiabatic transition at 800 nm from the singly ionized ground state to the repulsive excited state leading to C–O bond breaking is enhanced when a probe laser pulse is delayed by ～180 fs. At this pulse delay, on the other hand, C–C bond breaking is significantly suppressed. Therefore, the deformation of LD-PES is considered to change the direction of the wave packet traveling originally along the C–C stretching into the direction along the C–O stretching. This non-adiabatic transition leading to the redirection of the dissociating wave packet is found to occur more efficiently at the probe laser wavelengths at 400 nm than at 800 nm. The critical pulse delay is still ～180 fs even at 400 nm.     

A study of electron beams extracted from a plasma produced by laser interaction with a solid target

In this work, wave formation in laser-produced plasma is investigated by an analysis of time-of-flight signal of the electron pulse. Electrons are extracted from a non-equilibrium plasma, generated by pulsed laser ablation on a solid Ge target. The process is represented by ion-acoustic waves, which are generated from an external perturbation, given by the positive bias voltage of a Faraday cup. The characteristics of the waves depend substantially on the geometry of the plasma expansion chamber and on laser fluence, but are independent on bias potential. A KrF excimer UV laser was employed for plasma generation. Measurements were performed at two different laser fluences, 4 and 7 J/cm². The plasma created propagates with a mean velocity of about 1.1?×?10⁴ m/s. A movable Faraday cup was employed in order to collect electrons at different bias voltage values.     

Smith–Purcell free electron laser based on a semi-conical resonator

We investigate a Smith–Purcell free electron laser composed of an electron gun, a semi-conical resonator, a metallic grating and collector. The semi-conical resonator could reflect all Smith–Purcell radiation with emission angle θ, and with random azimuthal angles, back onto the electron beam and causes the electrons to be modulated. Tunable coherent far-infrared Smith–Purcell radiation with a high output peak power at millimeter wavelengths can be generated.     

The ALP-PALS project: optimal coupling for laser propulsion

Ablative laser propulsion (ALP) could revolutionize space travel by reducing the 30:1 propellant/payload ratio needed for near-earth orbit 50-fold. Experiments to date have demonstrated the necessary efficiency, coupling coefficient, and specific impulse for application, but were performed at pulse energies and spot sizes much smaller than required and at wavelengths not usable in the atmosphere. Prior experiments have also not simultaneously measured the properties of the ions produced or of the ablated surface, properties that would allow full understanding of the propulsion properties in terms of ion characteristics.

The first realistic measurements of laser propulsion parameters are proposed using PALS (Prague Asterix Laser System), the important parameters of which (pulse energy (～ 1 kJ), pulse length (400 ps), beam diameter (～ 29 cm), and flat beam profile) equal those required for application. The PALS wavelength is a little short (1.3 μ m vs.>1.5 μ m) but is closer than any other laser available and PALS’ 2ω/3ω capability should allow extrapolation to application values. The PALS’ proven infrastructure for measuring laser-driven ion properties means that only a ballistic pendulum for measuring momentum transfer will have to be added.     

基于Fokker-Planck方程的电介质材料短脉冲激光破坏机制分析

基于Pokker-Planck方程,建立一个描述短脉冲激光作用下电介质材料中导带电子能量分布随时间变化的模型,用数值方法计算电子能量分布与电子数密度随时间的演化过程,根据临界等离子体密度准则得到了不同激光脉冲宽度和波长下电介质材料(以SiO<,2>为例)的破坏阈值.结果发现,尽管激光波长通过3种途径对材料破坏阈值的确定...     

Nonlinear absorption and optical damage threshold of carbon-based nanostructured material embedded in a protein

Physical processes in laser–matter interaction used to be determined by generation of fast electrons resulting from efficient conversion of the absorbed laser radiation. Composite materials offer the possibility to control the absorption by choice of the host material and dopants. Reported here strong absorption of ultrashort laser pulse in a composite carbon-based nanomaterial including single-walled carbon nanotubes (SWCNTs) or multilayer graphene was measured in the intensity range between 10¹² and 10¹⁶ W cm^?2. A protein (lysozyme) was used as the host. The maximum absorption of femtosecond laser pulse has reached 92–96 %. The optical damage thresholds of the coatings were registered at an intensity of (1.1 ± 0.5) × 10¹³ W cm^?2 for the embedded SWCNTs and at (3.4 ± 0.3) × 10¹³ W cm^?2 for the embedded graphene. Encapsulated variant of the dispersed nanomaterial was investigated as well. It was found that supernatant protein in the coating material tends to dominate the absorption process, independently of the embedded nanomaterial. The opposite was observed for the encapsulated material.     

High-peak-power,high-repetition-rate LD end-pumped Nd:YVO<Subscript>4</Subscript> burst mode laser

A compact high-peak-power, high-repetition-rate burst mode laser is achieved by an acousto-optical Q-switched Nd:YVO₄ 1064 nm laser directly pumped at 878.6 nm. Pulse trains with 10–100 pulses are obtained using acousto-optical Q-switch at repetition rates of 10–100 kHz under a pulsed pumping with a 1 ms duration. At the maximum pump energy of 108.5 mJ, the pulse energy of 10 kHz burst mode laser reaches 44 mJ corresponding to a single pulse energy of 4.4 mJ and an optical-to-optical efficiency of 40.5 %.The maximum peak power of ~468.1 kW at 10 kHz is obtained with a pulse width of 9.4 ns. The beam quality factor is measured to be M ² ~1.5 and the pulse jitter is estimated to be less than 1 % in both amplitude and time region.     

Development of narrow linewidth, micro-integrated extended cavity diode lasers for quantum optics experiments in space

We present a micro-integrated extended cavity diode laser module for experiments on rubidium Bose–Einstein condensates and atom interferometry at 780.24 nm onboard a sounding rocket. The micro-integration concept is optimized for space application. The laser chip, micro-lenses, a volume holographic Bragg grating, micro-temperature sensors and a micro-thermoelectric cooler are integrated on an aluminium nitride ceramic micro-optical bench with a foot print of only 50 × 10 mm². Moveable parts are omitted to allow for a very compact and robust design. The laser module provides an output power of more than 120 mW at a short term (170 μs) linewidth of 54 kHz, both full-width-at-half-maximum. The laser can be coarsely tuned by 44 GHz with a continuous tuning range of 31 GHz. The micro-integration technology presented here can be transferred to other wavelengths.     

High-repetition-rate femtosecond optical parametric chirped-pulse amplifier in the mid-infrared

We discuss a dual-stage optical parametric chirped-pulse amplifier generating sub-100-fs pulses in the mid-infrared at a repetition rate of 100 kHz. The system is based on a 1064 nm pump laser and a 3–4 μm difference frequency generation seed source derived from the output of a femtosecond fiber laser amplifier. Both lasers are commercially available, are diode-pumped, compact, and allow for turn-key operation. Here, we focus our discussion on the design and dimensioning of the optical parametric chirped-pulse amplifier. In particular, we review the available gain materials for mid-infrared generation and analyze the impact of different stretching scenarios. Timing jitter plays an important role in short-pulse parametric amplifier systems and is therefore studied in detail. The geometry of the amplifier stages is optimized through a full 3-dimensional simulation with the aim of maximizing gain bandwidth and output power. The optimized system yields output pulse energies exceeding 1 μJ and an overall gain larger than 50 dB. The high repetition rate of the pump laser results in an unprecedented average power from a femtosecond parametric system at mid-infrared wavelengths. First experimental results confirm the design and the predictions of our theoretical model.     

The Spectrum of Ne-Like Ar and the 4d-4p Transition of Kr7+ at 45 nm in Capillary Discharge Experiment

Capillary discharge soft X-ray laser, which is always called “table-top soft X-ray laser,” is one of the effective methods for miniaturization. The method is deemed to have experimental facility with practicable value. With capillary discharge mechanism, Ne-like Ar at 46.9 nm soft X-ray laser has been obtained, and the experimental results and the analyses are reported in this paper. Experimentally, a current pulse with the amplitude of 20 kA was used to excite three different gases: Ar, Kr, and N₂. The signals were detected by an X-ray diode (XRD), and the emission spectra were monitored with a Rowland spectrograph. The J = 0–1 line and one 3d-3p transition of Ne-like Ar were detected, with wavelengths of 46.9 nm and 48.5 nm, respectively. Adjusting the pure Ar to the appropriate pressure, the authors found that the J = 0–1 line gains amplification, while 3d-3p does not. When the Ar pressure was 26 Pa, the J = 0–1 line completely dominated the spectrum. N₂ and Kr were used as the materials of capillary discharge respectively. The spike signal was obtained by XRD, then the spectrum was detected by Rowland spectrograph, and the spectrum of Kr⁷⁺ was found.     

Dynamics of the formation of laser-induced periodic surface structures on dielectrics and semiconductors upon femtosecond laser pulse irradiation sequences

The formation of laser-induced periodic surface structures (LIPSS) upon irradiation of fused silica and silicon with multiple (N _DPS) irradiation sequences consisting of linearly polarized femtosecond laser pulse pairs (pulse duration ～150 fs, central wavelength ～800 nm) is studied experimentally. Nearly equal-energy double-pulse sequences are generated allowing the temporal pulse delay Δt between the cross-polarized individual fs-laser pulses to be varied from ?40 ps to +40 ps with a resolution of ～0.2 ps. The surface morphologies of the irradiated surface areas are characterized by means of scanning electron and scanning force microscopy. Particularly for dielectrics in the sub-ps delay range striking differences in the orientation and spatial characteristics of the LIPSS can be observed. For fused silica, a significant decrease of the LIPSS spatial periods from ～790 nm towards ～550 nm is demonstrated for delay changes of less than ～2 ps. In contrast, for silicon under similar irradiation conditions, the LIPSS periods remain constant (～760 nm) for delays up to 40 ps. The results prove the impact of laser-induced electrons in the conduction band of the solid and associated transient changes of the optical properties on fs-LIPSS formation.     

超强飞秒激光与固体靶产生的超热电子加热机制

 在SILEX-1激光器上测量了超强飞秒激光与Ta靶相互作用产生的出射超热电子能谱及角分布,研究了出射超热电子加热机制。激光脉宽为 30 fs,激光功率密度为8.5×10¹⁸ W/cm²。靶前法线方向超热电子温度为550 keV。从实验结果可知：共振吸收是靶前法线方向超热电子主要加热机制,这与靶前存在大密度标长预等离子体的实验条件吻合。靶厚为6～50 μm时,靶后超热电子沿法线方向出射;靶厚为2 mm时,该发射峰消失。     

Radiation effects on poly(methyl methacrylate) induced by pulsed laser irradiations

Poly(methyl methacrylate) (PMMA) was irradiated using a medical UV-ArF excimer laser operating at the fundamental wavelength of 193 nm. Characterized by a beam diameter of 1.8 mm and energy of 180 mJ with a Gaussian energy profile, it operates in a single mode or at 30 Hz repetition rate. Mechanical profilometry was carried out on ablation craters in order to study the rugosity and the ablation yield in the various operative conditions. Optical transmission and reflection measurements at six wavelengths were conducted in order to characterize the optical properties of the irradiated surfaces. Measured crater depths in PMMA were lower with respect to the forecasted ones in corneal tissue, while the lateral crater aperture was maintained. The rugosity produced at the crater bottom after irradiation was about 0.3 μm, and the ablation yield was about 10¹⁵ molecules/laser pulse, while etching depth and diameter show a roughly linear dependence on the number of laser shots. These experiments constitute a base for deeper clinical investigations.     

Generation of MoS<Subscript>2</Subscript> quantum dots by laser ablation of MoS<Subscript>2</Subscript> particles in suspension and their photocatalytic activity for H<Subscript>2</Subscript> generation

MoS₂ quantum dots (QDs) have been obtained in colloidal suspensions by 532 nm laser ablation (7 ns fwhp/pulse, 50 mJ/pulse) of commercial MoS₂ particles in acetonitrile. High-resolution transmission electron microscopy images show a lateral size distribution from 5 to 20 nm, but a more homogeneous particle size of 20 nm can be obtained by silica gel chromatography purification in acetonitrile. MoS₂ QDs obtained by laser ablation are constituted by 3–6 MoS₂ layers (1.8–4 nm thickness) and exhibit photoluminescence whose λ_PL varies from 430 to 530 nm depending on the excitation wavelength. As predicted by theory, the confinement effect and the larger periphery in MoS₂ QDs increasing the bandgap and having catalytically active edges are reflected in an enhancement of the photocatalytic activity for H₂ generation upon UV–Vis irradiation using CH₃OH as sacrificial electron donor due to the increase in the reduction potential of conduction band electrons and the electron transfer kinetics.     

Eye-safe Raman laser based on BaTeMo2O9 crystal

An eye-safe Raman laser is realized with BaTeMo₂O₉ (BTM) nonlinear crystal for the first time. By using a diode-end-pumped acousto-optically Q-switched Nd:YVO₄ laser as the pumping source, the BTM crystal converts the fundamental laser at 1,342 nm to first-Stokes laser at 1,531 nm successfully. With an incident power of 10.8 W and a pulse repetition rate of 25 kHz, the average output power at 1,531 nm is obtained to be 0.83 W, corresponding to a diode-to-Stokes conversion efficiency of 7.7 %. The pulse width is 11 ns, and the peak power is 3.0 kW.     

Dense pair plasma generation by two laser pulses colliding in a cylinder channel

An all-optical scheme for high-density pair plasmas generation is proposed by two laser pulses colliding in a cylinder channel. Two dimensional particle-in-cell simulations show that, when the first laser pulse propagates in the cylinder,electrons are extracted out of the cylinder inner wall and accelerated to high energies. These energetic electrons later run into the second counter-propagating laser pulse, radiating a large amount of high-energy gamma photons via the Compton back-scattering process. The emitted gamma photons then collide with the second laser pulse to initiate the Breit–Wheeler process for pairs production. Due to the strong self-generated fields in the cylinder, positrons are confined in the channel to form dense pair plasmas. Totally, the maximum density of pair plasmas can be 4.60 × 10~(27)m~(-3), for lasers with an intensity of 4×10~(22)W·cm~(-2). Both the positron yield and density are tunable by changing the cylinder radius and the laser parameters. The generated dense pair plasmas can further facilitate investigations related to astrophysics and particle physics.     

Characteristics of laser and current pulses in a He–SrCl2 vapor laser

An experimental investigation on the characteristics of laser and current pulses in a He–SrCl₂ vapor laser is carried out. The temporal dependences of the discharge current pulse on the laser pulses at the 1.09 μm, ～3 μm and 6.45 μm lines in strontium atoms and ions are measured and analyzed under different laser output powers. It is found that all laser pulses appear at the falling edge of the current pulse and shift forward to the current pulse with increasing laser output power.     

Theoretical and experimental study of single mode-locking pulse generation with low repetition rate in a dual-loss-modulated QML YVO4/Nd:YVO4 laser with EO and GaAs

Using electro-optic (EO) modulator and GaAs saturable absorber, a diode-pumped doubly Q-switched and mode-locked (QML) YVO₄/Nd:YVO₄ laser at 1.06 μm is realized. The experimental results show that the number of the mode-locking pulses underneath the Q-switched envelope decreased with increasing pump power. With an output coupling of 6.5 %, the single mode-locking pulse underneath the Q-switched envelope with 1 kHz repetition rate was obtained when the pump power exceeded 4.65 W. At a pump power of 8.25 W for an output coupling of 10 %, a stable mode-locking pulse train at a repetition rate of 1 kHz was achieved with pulse energy as high as 582 μJ and pulse duration of about 580 ps, corresponding to a peak power of 1 MW. Using a hyperbolic secant square function and considering the Gaussian distribution of the intracavity photon density, the coupled rate equations for diode-pumped doubly QML YVO₄/Nd:YVO₄ laser are given and the numerical solutions of the equations are basically in accordance with the experimental results.