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Velocity of a Molecule Evaporated from a Water Nanodroplet: Maxwell–Boltzmann Statistics versus Non‐Ergodic Events 下载免费PDF全文
Assist. Prof. Dr. Hassan Abdoul‐Carime Francis Berthias Dr. Linda Feketeová Dr. Mathieu Marciante Dr. Florent Calvo Dr. Valérian Forquet Prof. Dr. Henry Chermette Dr. Bernadette Farizon Prof. Dr. Michel Farizon Prof. Dr. Tilmann D. Märk 《Angewandte Chemie (International ed. in English)》2015,54(49):14685-14689
The velocity of a molecule evaporated from a mass‐selected protonated water nanodroplet is measured by velocity map imaging in combination with a recently developed mass spectrometry technique. The measured velocity distributions allow probing statistical energy redistribution in ultimately small water nanodroplets after ultrafast electronic excitation. As the droplet size increases, the velocity distribution rapidly approaches the behavior expected for macroscopic droplets. However, a distinct high‐velocity contribution provides evidence of molecular evaporation before complete energy redistribution, corresponding to non‐ergodic events. 相似文献
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Cover Picture: Velocity of a Molecule Evaporated from a Water Nanodroplet: Maxwell–Boltzmann Statistics versus Non‐Ergodic Events (Angew. Chem. Int. Ed. 49/2015) 下载免费PDF全文
Assist. Prof. Dr. Hassan Abdoul‐Carime Francis Berthias Dr. Linda Feketeová Dr. Mathieu Marciante Dr. Florent Calvo Dr. Valérian Forquet Prof. Dr. Henry Chermette Dr. Bernadette Farizon Prof. Dr. Michel Farizon Prof. Dr. Tilmann D. Märk 《Angewandte Chemie (International ed. in English)》2015,54(49):14587-14587
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Norberto Garcia‐Cairasco Miguel Moyses‐Neto Flavio DelVecchio Jos A. C. Oliveira Francisco L. dosSantos Olagide W. Castro Gabriel M. Arisi Mrcio Dantas Ruither O. G. Carolino Joaquim Coutinho‐Netto Andre L. A. Dagostin Marcelo C. A. Rodrigues Ricardo M. Leo Samir A. P. Quintiliano Luiz F. Silva Leonardo Gobbo‐Neto Norberto P. Lopes 《Angewandte Chemie (Weinheim an der Bergstrasse, Germany)》2013,125(49):12981-12981
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