Frequency modulation spectroscopy by means of quantum-cascade lasers

In this paper we investigate the performance of quantum cascade (QC) lasers for high frequency modulation spectroscopy, particularly using frequency modulation (FM) and two-tone (2T) techniques. The coupling of the rf signal to the QC laser through the cryostat is studied in detail as well as the noise contributions of both the detector and the laser source to the final spectra. The experimental traces are obtained by spectroscopy on low-pressure N₂O and CH₄ gases at 8.0 μm and 7.3 μm wavelength, respectively, and reproduce the line profiles predicted by theory. As a preliminary result, an enhancement of a factor six is measured with respect to direct absorption line recording. PACS 42.62.Fi; 42.72.A1; 07.88.+y     

Frequency stabilization of blue extended cavity diode lasers by external cavity optical feedback

Optical feedback from a high-finesse V-resonator, developed for this study, results in efficient coupling with an extended cavity diode laser, stabilizing its emission frequency and strongly decreasing the laser linewidth. This in turn enhances resonator output power, thus increasing the signal-to-noise ratio when used for the detection of gas phase species by absorption spectroscopy. This effect was directly measured by heterodyning two extended cavity diode lasers at a wavelength of 409 nm with and without the influence of optical feedback from a high-finesse V-resonator. The heterodyne signal of freely running lasers is composed of a set of sharp peaks whose envelope shows a width on the order of 4.5 MHz at a sweep rate of 80 MHz/0.8 s, leading to a laser linewidth of 3 MHz. Optical feedback from the high-finesse V-resonator reduces the heterodyne signal to a single peak with a mean width of 10 kHz, leading to a laser linewidth of 7 kHz. This is the lowest value of linewidth, reported thus far, for diode lasers operating in this wavelength region.     

Frequency stabilization in semiconductor lasers

Three promising methods of improving temporal coherence in semiconductor lasers are reviewed. They are the development of novel laser devices, a technique of optical feedback and a technique of electrical feedback. The main discussion in this paper is focused on the technique of electrical feedback. The theoretical limit of frequency stability and recent experimental results are presented with respect to the following five subjects which are indispensable in the realization of highly coherent lasers: (a) frequency stabilization; (b) improvements in frequency reproducibility; (c) linewidth reduction; (d) frequency tracking; and (e) stable, accurate and wideband frequency sweep.     

Design of nonlinearity-enhanced quantum-cascade lasers

We present simulations of mid-infrared quantum-cascade lasers (QCL) with optimized second-harmonic generation (SHG). The optimized design was obtained utilizing techniques from supersymmetric quantum mechanics with both material-dependent effective mass and band nonparabolicity. Two-photon processes are analyzed for resonant cascading triple levels designed for enhancing SHG. Nonunity pumping efficiency from one period of the QCL to the next is taken into account by including all relevant carrier scattering mechanisms between the injector/collector and active regions. Carrier transport and power output of the structure are analyzed by self-consistently solving rate equations for the carriers and photons. Current-dependent linear optical output power is derived based on the steady-state photon population in the active region. The SH power is derived from the Maxwell equations with the phase mismatch and modes overlapping included. Due to stronger coupling between lasing levels, the optimized structure has both higher linear and SH output powers. The optimized structure can be fabricated through digitally grading the submonolayer alloys by molecular beam epitaxy (MBE) technique.     

Photoacoustic spectroscopy using quantum-cascade lasers

Photoacoustic spectra of ammonia and water vapor were recorded by use of a continuous-wave quantum-cascade distributed-feedback (QC-DFB) laser at 8.5 mum with a 16-mW power output. The gases were flowed through a cell that was resonant at 1.6 kHz, and the QC-DFB source was temperature tuned over 35 nm for generation of spectra or was temperature stabilized on an absorption feature peak to permit real-time concentration measurements. A detection limit of 100 parts in 10(9) by volume ammonia at standard temperature and pressure was obtained for a 1-Hz bandwidth in a measurement time of 10 min.     

Terahertz tomography using quantum-cascade lasers

The interfaces of a dielectric sample are resolved in reflection geometry using light from a frequency agile array of terahertz quantum-cascade lasers. The terahertz source is a 10-element linear array of third-order distributed-feedback QCLs emitting at discrete frequencies from 2.08 to 2.4 THz. Emission from the array is collimated and sent through a Michelson interferometer, with the sample placed in one of the arms. Interference signals collected at each frequency are used to reconstruct an interferogram and detect the interfaces in the sample. Because of the long coherence length of the source, the interferometer arms need not be adjusted to the zero-path delay. A depth resolution of 360 μm in the dielectric is achieved with further potential improvement through improved frequency coverage of the array. The entire experiment footprint is <1 m×1 m with the source operated in a compact, closed-cycle cryocooler.     

Thermal-noise limit in the frequency stabilization of lasers with rigid cavities

We evaluate thermal noise (Brownian motion) in a rigid reference cavity used for frequency stabilization of lasers, based on the mechanical loss of cavity materials and the numerical analysis of the mirror-spacer mechanics with the direct application of the fluctuation dissipation theorem. This noise sets a fundamental limit for the frequency stability achieved with a rigid frequency-reference cavity of order 1 Hz/ square root Hz (0.01 Hz/ square root Hz) at 10 mHz (100 Hz) at room temperature. This level coincides with the world-highest level stabilization results.     

Second-harmonic generation in GaAs-based quantum-cascade lasers

We report second-harmonic (SH) and sum-frequency generation in GaAs-based quantum-cascade lasers. A doping dependence study of the second-order susceptibility in one of the investigated structure is shown. We also demonstrate that grating-coupled surface emission is a highly efficient way to couple out the SH radiation.     

Second-harmonic generation in GaAs-based quantum-cascade lasers

We report second-harmonic (SH) and sum-frequency generation in GaAs-based quantum-cascade lasers. A doping dependence study of the second-order susceptibility in one of the investigated structure is shown. We also demonstrate that grating-coupled surface emission is a highly efficient way to couple out the SH radiation.     

Frequency stabilization of multiple lasers and Rydberg atom spectroscopy

In this paper we report details of the apparatus and experimental techniques used to excite Rydberg states of ⁷Li using multiple diode lasers. Special attention is paid to frequency stabilization of the lasers and we show how three lasers can be stabilized using the fluorescence from a single atomic state. Laser spectroscopy of the 8p,9p, and 11p–15p states is then performed to determine the quantum defects of these states. Our measurement precision exceeds that of previous measurements of these defects by as much as a factor of 25. This work substantially extends our previous measurement of the 10p quantum defect, and we compare our measured defects with recent theoretical calculations for the np states across the range 8≤n≤15. The agreement with theory is excellent.     

Frequency stabilization and measurements of 543 nm HeNe lasers

In this paper we report our investigations on the frequency stabilization and frequency measurements of 543 nm HeNe laser. It contains following four different works. (1) Using a metal laser tube we have built an iodine-stabilized 543 nm HeNe laser by the Frequency-Modulation (FM) spectroscopy. The signal-to-noise ratio of the hyperfine spectrum reached 2 × 10^–12 at 1 s sampling time. (2) We have built a compact iodine-stabilized 543 nm HeNe laser system using the third-harmonic locking technique. Stability better than 1 × 10^–12 for sampling time >1 s is obtained. We also suggest the b₁₀ line for the future recommendation. (3) We constructed the Lamb-dip stabilized He-²⁰Ne and He-²²Ne lasers and measured their frequency stability, reproducibility, and absolute frequencies. The results suggest that the Lamb-dip stabilized lasers are appropriate for secondary wavelength standards. We have also deduced the isotope shift of Ne atom at 543 nm. (4) We have developed two two-mode stabilized 543 nm HeNe lasers using the bang-bang control method. The Allan variance is 1 × 10^–11 at 1 s sampling time.     

Nature of charge transport in quantum-cascade lasers

The first global quantum simulation of semiconductor-based quantum-cascade lasers is presented. Our three-dimensional approach allows us to study in a purely microscopic way the current-voltage characteristics of state-of-the-art unipolar nanostructures, and therefore to answer the long-standing controversial question: Is charge transport in quantum-cascade lasers mainly coherent or incoherent? Our analysis shows that (i) quantum corrections to the semiclassical scenario are minor and (ii) inclusion of carrier-phonon and carrier-carrier scattering gives excellent agreement with experimental results.     

Cavity ringdown spectroscopy using mid-infrared quantum-cascade lasers

Cavity ringdown spectra of ammonia at 10 parts in 10(9) by volume (ppbv) and higher concentrations were recorded by use of a 16-mW continuous-wave quantum-casacde distributed-feedback laser at 8.5 mum whose wavelength was continuously temperature tuned over 15 nm. A sensitivity (noise-equivalent absorbance) of 3.4x10(-9) cm(-1) Hz(-1/2) was achieved for ammonia in nitrogen at standard temperature and pressure, which corresponds to a detection limit of 0.25 ppbv.     

Short-term frequency stabilization of diode-laser-pumped Nd:YAG lasers using double-pendulum suspended cavities

We describe the improvement of short-term frequency stability of diode-laser-pumped Nd:YAG lasers. To improve the vibrational isolation of reference cavities, the reference cavities were suspended by a double pendulum with magnetic damping. The frequency noise was reduced to lower than 1 Hz/Hz at Fourier frequencies higher than 5 Hz and the minimum noise of 7 × 10^–3 Hz/Hz was recorded. The minimum root Allan variance was about 10^–14 for the sampling time of 0.01 s. Heating of the reference cavity by absorbed laser power caused the thermal drift of cavity resonance frequencies. It resulted in the laser linewidth in the range of 30–50 Hz.     

半绝缘等离子体波导太赫兹量子级联激光器工艺研究

采用气态源分子束外延设备生长了GaAs/AlGaAs束缚态到连续态跃迁结构的太赫兹（THz）量子级联激光器（QCL）有源区结构,研究了半绝缘等离子体波导THz QCL的器件工艺,采用远红外傅里叶变换光谱仪以及探测器测量了器件的电光特性.器件激射频率为32 THz,10 K下的阈值电流密度为275 A/cm². 关键词： 太赫兹 量子级联激光器 波导 器件工艺     

太赫兹量子级联激光器材料生长及表征

采用气态源分子束外延方法生长了束缚态到连续态跃迁太赫兹量子级联激光器（terahertz quantum-cascade laser,简称THz QCL）有源区结构,并且采用电化学CV仪、霍尔测试仪以及高分辨X射线衍射对材料的质量进行表征,得出THz QCL有源区具有很高的晶体质量.另外,采用蒙特卡罗方法模拟了共振声子THz QCL器件的I-V曲线,分析了在不同偏压下子能级的对齐状况和电子的输运特征. 关键词： 太赫兹 量子级联激光器 分子束外延 X射线衍射     

Frequency stabilization of multiple semiconductor lasers using digital feedback loop

We propose and demonstrate a simple technique to stabilize the frequencies of multiple semiconductor lasers simultaneously using a Fabry-Perot etalon filter and a digital signal processing. Unlike other stabilization techniques, the proposed technique could stabilize DFB lasers using only one digital feedback control loop. The result shows that the proposed technique could maintain the frequency stability of 16 DFB lasers within ±150 MHz.     

Perfectly phase-matched third-order distributed feedback terahertz quantum-cascade lasers

We report a novel laser cavity design in third-order distributed feedback (DFB) terahertz quantum-cascade lasers based on a perfectly phase-matching technique. This approach substantially increases the usable length of the third-order DFB laser and leads to narrow beam patterns. Single frequency emissions from 151 apertures (5.6 mm long device) are coherently added up to form a narrow beam with (FWHM≈6×11°) divergence. A similar device with 40 apertures shows more than 5 mW of optical power with slope efficiency ～140 mW/A at 10 K pulsed operation.     

Frequency stabilization of mode-locked Erbium fiber lasers using pump power control

Mode-locked erbium fiber lasers can serve as frequency comb generators in the 1.5 m telecommunication band or as frequency dividers generating low noise pulse trains at microwave repetition rates from a visible or near infrared frequency standard. Such applications require suitable stabilization methods both for the lasers carrier frequency and the pulse repetition frequency. While control of the optical resonator length with the help of a piezo actuator is an obvious method, we investigate in this paper frequency stabilization of the fiber laser via pump power control. Using this method, we stabilize the pulse repetition rate of the Er:fiber-laser with respect to a hydrogen-maser with residual averaged timing errors of a few femtoseconds (for averaging times between one and one hundred seconds), an order of magnitude below the timing noise of the maser itself. PACS 42.55Wd; 42.62.Eh     

Integrated wavelength stabilization of in-plane semiconductor lasers by use of a dual-grating reflector

We summarize a novel integrated wavelength-stabilization scheme for broad stripe surface-emitting lasers. The method is based on two gratings fabricated on opposite sides of a device in which the first grating disperses light through the substrate to the opposite side, where the second surface has a feedback grating that operates under total internal reflection and in the Littrow condition to provide feedback into the gain medium. Experimental results have been obtained for both high power and a narrow linewidth, showing a CW slope of 0.85 W/A.