Verzweigungsverhältnisse und Konversionskoeffizienten von angeregten Zuständen des208Tl

The branching ratios of theγ rays of the second and fourth excited states of²⁰⁸Tl have been investigated by coincidence measurements between the α rays of²¹²Bi and subsequent 40keVγ ray. The detectors employed were a silicon surface barrier counter for α particles, and a 1.5 in ×2 mm NaJ (Tl) crystal forγ rays. It has been found that (75.6±3.7)% of all transitions of the 328 keV state and (94±7)% of all transitions of the (492 keV+473 keV) states populate the first excited state of²⁰⁸Tl. The 40 keV state is excited to (3.4±0.3)% by transitions of higher excited states relative to the direct excitation by α particles. The number of α particles with energyE _α = 6.047 MeV and the number of subsequent 40keVγ rays resulted in a conversion coefficient α(40keV)=22.55± 0.46. Similarly coincidence measurements between Tl-x rays and α particles have been used to determine theK- conversion coefficients α_K(328 keV)=0.31±0.03 and α_K(492 keV+ 473keV)=0.100±0.015. The experimental results are in good agreement with the theoretical values ofSliv.     

Study of Er171 decay by means of an electron-gamma coincidence technique

The decay scheme of Er¹⁷¹ (7.8 h) has been reinvestigated by means of an electron-gamma coincidence spectrometer and a scintillation spectrometer with a transistorized RIDL-400 channel analyser. A careful unfolding of the high energy region of the gamma-ray spectrum revealed the presence of photopeaks at energies of approximately 371, 404, 543, 572, 618, 675, 738, 796, 869, 910 and 962 keV. The existence of 32 transitions in Tm¹⁷¹ was confirmed. Also, it is proved that the 277, 362 keV transitions are in coincidence with the 210 keV and that the 175 keV transition is in coincidence with the 86 keV transition. We revealed the doubt for the existence of the 166, 210, 236, 277 and 419 keV transitions. From coincidence and single counting rates the followingK-conversion coefficients of the 111, 116, 124, 296 and 308 keV transitions were determined to be: α _K (111)=1.561±0.062, α _K (116)=0.699±0.035, α _K (124)=0.608±0.024, α _K (296)=0.0197±0.0010, α _K (308)=0.0183±0.0009, which give the 116, 124 keV transitions an electric quadrupole character; the 111 keV transition a magnetic dipole character withE2/M1 equal 0.4528; and the 296, 308 keV transitions an electric dipole character withM2/E1 equal 0.0058 and 0.0071 respectively.     

Winkelkorrelationsmessungen an >30y Holmium 166 und Bestimmung desg R -Faktors des 4+-Rotationsniveaus von Erbium 166

The spins of several excited states of Er¹⁶⁶ have been investigated byγγ-angular correlation measurements. The spin sequence 0+, 2+, 4+, 6+ for the ground state rotational band was presumed to be correct. Unique assignments were derived for the states of 1076 keV, 1377 keV and 1785 keV asI=5, 7 and 6 respectively. These results are in agreement with the spins proposed byGallagher jr. andSoloviev. The multipolarities of theγ-transitions of 408 keV, 709 keV, 811 keV and 831 keV were derived as 95%E1+(5±1)%M2, 99·6%E1+(0·4±0·5)%M2, 99·1%E2+(0·9±0·3)%M1, and 96·1%E2+(3·9±1)%M1 respectively. The unusual mixing ratios of the transitions of 811 keV and 831 keV can be understood as a consequence of theK-selection rule. Eachγ-transition from the 1785 keV state should be stronglyK-forbidden and one expects a half-life ofT _1/2≈3·10^?9s. A measurement of the time spectrum of the coincidences between theβ-radiation and the high energyγ-lines gave however:T _1/2(1785 keV state)≦3·10^?10s. The rotation of the angular correlation between the 184 keV line and theγ-group at 820 keV has been measured in an external magnetic field of 53000 gauss as:ω·τ(4+)=0·083±0·006. This value contains small corrections for an additional rotation of the angular correlation of the 831 keV–184 keV triple cascade in the 6+state and for a small attenuation by internal fields. WithT _1/2(4+state)=1·23·10^?10s, andβ=7·08 one gets for theg-factorg _R=+0·266±0·024 in good agreement with recent results for the 2+ state.     

TheK-conversion coefficient of the 321 keVE1 transition in Hf177

TheK-conversion coefficient of the 321 keVE1 transition in Hf¹⁷⁷ has been measured by means of an iron free double focusing beta-ray spectrometer, using the internalexternal conversion method. The result obtained for α _K (321)=0.162±0.016 is in disagreement with the theoretical values for pureE1 transition (α _K =0.0154) calculated bySliv andBand. The large anomaly observed in theK-conversion process of the inhibitedE1 transition is compatible with a largeM2 admixture or, more probable with the presence of penetration matrix elements.     

Concerning internal conversion coefficients in Hf180

The gamma-ray relative intensities from transitions in Hf¹⁸⁰ following the 5.5 hour Hf^180m decay have been measured using a bent-crystal gamma-ray diffraction monochromator and a least-squares fitting technique. From these measurements it was possible to deduce a value for the internal conversion coefficient for the 93.3-keV transition of α _T ⁹³ =4.91±0.23. From previous measurements of conversion electron intensities byEdwards andBoehm and our gamma-ray relative intensities, internal conversion coefficients for all transitions except the 57.5-keV transition were obtained. These coefficients agree well with the previous determinations byEdwards andBoehm, however, our measurements have improved precision, particularly in the case of 501.3-keV transition. The present measurements of α _K for the 215.3-, 332.5-and 443.8-keVE2 transitions are 11% lower than theoretical values while α_K for 93.3 keV E2 transition agrees closely with the theoretical value. These results are in close agreement with the previous measurements ofEdwards andBoehm. The present experimental α_K for the 501-keV transition agrees closely with the theoretical α_K for an E3 multipolarity.     

Dasβ-Spektrum des Cs137

Theβ-ray spectrum of Cs¹³⁷ has been measured with an iron-free spectrometer. The energy of the soft component was found to beE ₀=514±2 keV. The parameterk of the hard-component shape factorC _2VA ⁽²⁾ (W)=q ²+kp ² was determined to bek=0.015±0.004. Theβ intensities amount to 6.5% (hard component) and 93.5% (soft component). TheK conversion coefficient of the isomeric transition was measured to beα _K=0.093±0.003, in excellent agreement withSliv's theoretical value.     

Die Faktoren der inneren Umwandlung beim35Br80m (4,4 Std)

The intensities of the 37keV- and 49keV-γ-rays of Br^80m have been measured with the aid of Na J-scintillation spectrometers and compared with the intensity of the conversion electrons registered by an anthracene split crystal spectrometer. It was possible to separate the 49 keV-γ-radiation from the intense 37 keV-line by selctive absorption with balanced Sm- and Gd-filters. The internal conversion coefficientsα(49 keV)=298±30 andα (37 keV)=1,59±0,10 are in good agreement with the calculated values for M₃- and E₁-transitions. The half life was measured yielding a value ofT _1/2=(4,40±0,05) h.     

Messung der 2P-1S-Übergangsenergie im Myon-Barium-Atom

As a means of studying the nuclear charge radius, the 2P-1S-transition energy of the muon-barium-atom (μ-mesonicK _α -line) was measured. A 3″×3″ NaJ-spectrometer was used at the muon channel of the CERN-synchrocyclotron. Since the muon intensity was high, measurements could be repeated under various conditions. Experiment, checks, and results are described. The 2P-1S-energy obtained, (3981±30) keV, agrees with the value calculated byFord andWills (3974 keV) for a “family II”-charge distribution fitted to the Stanford electron scattering data.     

Niederenergetische Gammalinien vom Neutroneneinfang in Lu 175 und Lu 176

The low energy gamma-rays from neutron-capture in Lu 175 and Lu 176 have been investigated by means of the bent crystal-spectrometer at the DR-3-reactor at Risø. From the transitions in Lu 177 3 rotational bands have been determined. The levels of the (404)K=7/2⁺ groundstate rotational band are: 121,62 keV (I=9/2), 268,79keV (I=11/2), 440,66 keV (I=13/2), 636,22 keV (I=15/2), 854,34 keV (I=17/2). The level-sequence of the (514)K=9/2^?-band is: 150,39 keV (I=9/2), 288,99 keV (I=11/2), 451,49 keV (I=13/2), 637,05 keV (I=15/2) and 844,88 keV (I=17/2). At 457,92 keV is the basis for the (402)K=5/2⁺-band the higher levels of which are 552,05 keV (I=7/2), 671,89 keV (I=9/2), 816,63 keV (I=11/2), 985,23 keV (I=13/2), 1176,73keV (I=15/2) and probably 1389,5 keV (I=17/2). The energies of the levels apart from the 1389 keV-level have an accuracy of 7×10^?5. The energy differences between the 3 bands agree very well with the values expected from the Bohr-Mottelson-formulaE=A·I(I+1)+B·I ²(I+1)². The calculated branching-ratios within the 3 bands are in fairly good agreement with the experimental values. Theg _K -factors have been determined for 2 bands: It was found that for the (514)-bandg _K =1,16±0,04 and for the (402)-bandg _K =1,33±0,07.     

Zur Isomerie des Tl197

Tl^197m was produced by the (α, 4n) reaction on Au¹⁹⁷ using 49 MeVα particles. The following results were obtained: Half-lifeT _1/2=(0.55±0.02) sec; energy of the isomeric level (607±4) keV, determined directly by summing up the cascade transitions in a well-type scintillator; energy of the isomeric transition (222±2) keV; conversion coefficients of this transitionα _K222=0.41±0.05 andα _tot222=2.1±0.2, indicating anE3 multipolarity; energy of the second transition (385±3)keV; conversion coefficientsα _K385=0.09±0.03 andα _tot385<0.1. This transition was identified asE2 with aM1 admixture of 20 to 30%. Spins and parities are 1/2⁺, 3/2⁺ and 9/2^? for the ground state, the 385 keV state and the 607 keV isomeric state, respectively, in disagreement with the extreme single-particle model. If this model were correct, anotherM1 transition should appear. No furtherM1 transition having an energy greater than theL-shell binding energy of T1 was observed.     

Nuclearg-factors of the first excited states in Ir191 and Ir193

Mössbauer experiments were performed to determine the nuclearg-factor of the 82 keV 1/2⁺ state in Ir¹⁹¹ (g=+1.083±0.009) and the 73 keV 1/2⁺ state in Ir¹⁹³ (g=+0.9400±0.0019). TheE2/M1 mixing parameters of the corresponding (1/2⁺) (E2/M1) (3/2⁺) transitions were found to be ¦δ¦ (Ir¹⁹¹, 82 keV)=0.80±0.06 andδ(Ir¹⁹³, 73 keV)=?0.558±0.005.     

Measurement of the Lamb shift 42S1/2-42P1/2 of the helium ion

Helium ions were produced in then=4 states by electron collisions with ground state atoms, resulting in simultaneous ionization and excitation. Dipole transitions between the Zeeman levels of the states 4² S _1/2 and 4² P _1/2 were induced by a microwave electric field. The intensity of the emitted Fowlerα line 4686 Å, corresponding to transitions from then=4 to then=3 states was then reduced by about 3%. From the measurements, a value of the Lamb shiftδ=1751±25 MHz was obtained, compared with the theoretical valueδ=1768.23±0.55 MHz, and the results ofLea, Leventhal andLamb ofδ=1765±20 MHz.     

Der Zerfall Co58m →Co58g

Co^58m , Co^58g and Co⁵⁵ were obtained by radiating nickel-foiles with deuterons of energies 11,5 MeV and 2,07 MeV. The γ-radiation was measured with NaJ scintillation spectrometers. For the isomeric transition of Co^58m was determinedT _1/2=(9.15±0.1)h,T _γ=(25±1)keV,α _K=2200±300 and α_L+M=1100±300. From these values it follows, that the radiation is ofM3-type. Twoγ-energies of 95 keV and 1322 keV were found belonging to Co⁵⁵.     

Die Konversion des79m Br

⁷⁹ mBr was produced by irradiation of natural Br with fast neutrons. The half-lifeT _1/2=(4.87±0.15) sec and the energyE _γ=(208±1) keV were remeasured. For the first time the conversion coefficients were determined to beα _K=0.25±0.02 and α_total=0.28±0.05, yielding the multipolarityE3 for the isomeric transition.     

Study of penetration effects in the <Emphasis Type="Italic">E</Emphasis>1 and <Emphasis Type="Italic">M</Emphasis>1 transitions in <Superscript>44</Superscript>Sc

Conversion coefficients for the E1 and M1 transitions in the ⁴⁴Ti decay have been measured with high accuracy using the sum peak and multidimensional coincidence methods. The following values have been obtained: α_K(E1) = 0.077 ± 0.003 and α_K(M1) = 0.014 ± 0.001. A significant contribution of the penetration effects for the M1 transition has been shown. The penetration parameter λ is determined to be ?260 ± 30 has been determined.     

Radioactive decay of Os191 and Os191m

Beta and gamma spectra of Os¹⁹¹ were studied using a magnetic double-focusing beta-spectrometer and a scintillation spectrometer. The isomeric state Os^191m decays through the 74·4 ± 0·1 keV (E3/M4=50) transition with a half-lifeT _1/2=13·0 ± 0·5 hours. A continuous beta spectrum withE _max=147 ± 3 keV and the gamma transitions 41·83 ± 0·05 keV (E3), 82·5 ± 0·3 keV and 129·4 ± 0·1 keV (70%M1 + 30%E2) were observed in the decay of the ground state of Os¹⁹¹. The conversion coefficient of the last transition was determined as 1·94 ±± — 0·10. Gamma transitions with energies of 47 keV and 185·8 keV were not observed.     

Der Zerfall des Tb158m

Tb^158m was produced from Tb¹⁵⁹ by (n, 2n) reaction and investigated using scintillation spectrometers. The following results were obtained: half-life\(T_{\tfrac{1}{2}} = (10.5 \pm 0.2)\) sec; energy of the isomeric transitionE _γ =(109.9±1.4) keV; conversion coefficients α _K =56±3; α _L +α _M +?=50±8; α_total=106±10;K/L-ratioK/L=1.3±0.3, yielding the multipole order of the isomeric transition to beM3. Upper limits for the direct beta transitions from the isomeric state to the ground states of the neighbouring even-even nuclei Gd¹⁵⁸ and Dy¹⁵⁸ are 10^?4 and 6·10^?3, respectively.     

Derg R -Faktor des 2+-Rotationsniveaus von Er168

The rotation of the angular correlation between theγ-group at about 820 keV and the 80 keV radiation in the decay of Tm¹⁶⁸ has been observed in an external magnetic field of 20300 gauss. The result:ω _R·τ=0,485±0,051 yields for theg _R -factor of the 80 keV state of Er¹⁶⁸:g _R =+0,25±0,03. The evaluation includes a paramagnetic correction factor of:β=7,26, (B _eff=β·B _ext). The angular correlation is slightly attenuated by internal fields. For a liquid source of Tm (NO₃)₃ solved in 3 n HNO₃, a measurement of the differential angular correlation as a function of the delay time gave:λ ₂=(5,8±2,9)·10⁷sec^?1, assumingA ₂(t)=A ₂(0)·e ^?λ ₂·t. The half life of the 80 keV state was found to be:T _1/2=(1,92±0,04)·10^?9sec in agreement with earlier measurements.     

Die Intensität der Bremsstrahlung und der charakteristischenK-Röntgenstrahlung dünner Anoden

The intensities of bremsstrahlung and characteristicK X-rays of thin Al, Mn, Cu, Se, Ag and Sn targets were measured with a scintillation counter. The angle between the 50 keV electrons and the direction of emission was 90°. — The spectral intensity of bremsstrahlung for 20 keV quantum energy was determined in agreement with the theory ofKirkpatrick andWiedmann. The result obtained isi _v=(2.7) · 10^?53.Z ^{2, 0} ergs per steradian, unit frequency interval, bombarding electron and atomper-cm². The cross section ofK-ionisation by electron impact has been found out by measuring the characteristicKX-ray intensity in agreement with known theoretical and experimental values. The result of this work isσ _K=(7.0) · 10^?16 ·Z ^?4,3 cm².     

Das K-Auger-Spektrum von Neon

TheKLL-Auger spectrum of neon was investigated with an electrostatic spectrometer with an energy resolution of 0.12%. The ionization in theK-shell was caused by electron impact. The use of a gaseous target made it possible to measure the Auger electrons without any energy loss. The relative intensities of the KLL-lines were determined to be:KL ₁ L ₁(¹ S ₀)=1.0;KL ₁ L _2,3(¹ P ₁)=3.06±0.07;KL ₁ L _2,3(³ P _0,1,2)=0.98±0.05;KL _2,3 L _2,3(¹ S ₀)=1.67±0.08;KL _2,3 L _2,3(¹ D ₂)=13.1±0.6;KL _2,3 L _2,3(² P _0,2)=0. This is in agreement with an earlier measurement byKörber andMehlhorn but disagrees with all theoretical values calculated nonrelativistically for low Z. It is shown that agreement may be achieved by applying quantitatively the configuration interaction, introduced very recently byAsaad, and using improved wave functions for the calculation of the transition amplitudes. As a consequence of the ionization by electron impact also theKL-LLL Auger spectrum was caused. 10 lines of this spectrum were measured and identified. Moreover, from the Auger energies measured, the binding energyE(K) of neon was calculated to be E(K)=(870.0±0.4) eV.