Coherent Array of White-Light Continuum Generated by Microlens Array

We generated a white-light continuum array by directing femtosecond laser pulses into a liquid with a microlens array. Experimental evidence demonstrates that the spatial coherence is high within a single light source in the array. We also confirmed that all the light sources in the white-light continuum array are mutually coherent. We found that the simple self-phase modulation model cannot explain this high coherence between the white continuum sources.     

Self-transformation of a powerful femtosecond laser pulse into a white-light laser pulse in bulk optical media (or supercontinuum generation)

We present experimental and theoretical results on white-light generation in the filamentation of a high-power femtosecond laser pulse in water and atmospheric air. We have shown that the high spatio-temporal localization of the light field in the filament, which enables the supercontinuum generation, is sustained due to the dynamic transformation of the light field on the whole transverse scale of the beam, including its edges. We found that the sources of the supercontinuum blue wing are in the rings, surrounding the filament, as well as at the back of the pulse, where shock-wave formation enhanced by self-steepening takes place. We report on the first observation and demonstration of the interference of the supercontinuum spectral components arising in the course of multiple filamentation in a terawatt laser pulse. We demonstrate that the conversion efficiency of an initially narrow laser pulse spectrum into the supercontinuum depends on the length of the filament with high intensity gradients and can be increased by introducing an initial chirp. PACS 42.65.Jx; 42.65.Re; 42.25.Bs; 42.50.Hz     

Generation of sub-4-fs pulses via compression of a white-light continuum using only chirped mirrors

Using noble gases as a nonlinear medium, it has become possible to compress energetic laser pulses into the sub-10-fs regime. Hollow fiber capillaries can serve to increase the effective interaction length of the pulses, and impressive white-light continua have been reported as a result. With demonstrated bandwidths exceeding the optical octave, this method holds the potential for generating single-cycle optical pulses. On the practical side, however, it becomes very difficult to compensate for dispersive effects and to fully exploit the enormous bandwidth. We will discuss chirped mirrors as one means for pulse compression. A further challenge lies on the characterization side. Utilizing advanced characterization schemes, we were able to demonstrate compression of a white-light continuum down to a pulse duration of 3.8 fs, which corresponds to only about 1.6 cycles at the carrier wavelength. These are the shortest pulses in the visible/near-infrared wavelength range that have ever been produced with a non-adaptive approach to dispersion compensation. Moreover, these are the shortest pulses generated using chirped mirrors, which compares favorably to previous results that were achieved with much more elaborate and lossier adaptive compression schemes. PACS 42.65.Re; 42.65.Wi     

Calorimetric detection of THz radiation from femtosecond filaments in air

Calorimetric measurements of the THz radiation from plasma filaments created in air by intense IR fs laser pulses were performed. The decay kinetics of the THz radiation from this extended plasma source is shown to be different from that of a localized air plasma source produced by the same laser. PACS 42.65.Wi; 42.65.Re; 52.40.Db     

All-optical control of the carrier-envelope phase with multi-stage optical parametric amplifiers verified with spectral interference

Intense ultrashort laser pulses with stabilized carrier-envelope phase (CEP) are generated at 800 nm by using multi-stage collinear and non-collinear optical parametric amplifiers (OPAs). The first-stage collinear OPA is directly pumped by the fundamental-wave pulses and tuned to generate idler pulses at 1600 nm, which are further amplified by a second-stage collinear OPA, and then frequency-doubled to generate CEP-stabilized pulses at 800 nm. A non-collinear OPA is used to amplify the CEP-stabilized pulses at 800 nm. The combination of different OPAs can generate and amplify CEP-stabilized pulses at 800 nm without any detrimental influence from the fundamental-wave pulses. The CEP stabilization is verified with a simple and robust spectral interference setup. The stable interference pattern is measured for every single pulse and compared with the unstable pattern from pulses of random CEP. PACS 42.65.Re; 42.65.Yj; 42.25.Kb     

Phase-locked white-light continuum pulses: toward a universal optical frequency-comb synthesizer

We demonstrate that two white-light continuum pulses that are independently generated by phase-locked ultrashort laser pulses are locked in phase and show surprisingly clear and stable Young interference fringes. The experiment shows that the two generated continua emit essentially in phase and that random phase jitter can remain negligible. This result is not only of interest for studies of nonlinear field-matter interactions but also suggests that such white-light continuum pulses can be used to realize a broad frequency comb for absolute frequency measurements from the IR to the UV.     

Towards a control of multiple filamentation by spatial regularization of a high-power femtosecond laser pulse

We propose a new method for controlling randomly generated multiple filaments during the propagation of femtosecond laser pulses in optical media. The method is based on introducing a periodic amplitude modulation of the transverse beam profile. It is shown both experimentally and numerically that the introduction of a periodic mesh into a propagation path of a femtosecond near-infrared laser pulse leads to a deterministic spatial distribution of multiple filaments in the presence of initial random fluctuations. As a result, the number of filaments is increased as compared to the random case. PACS 42.65.Jx; 42.25.Bs; 42.60.Jf     

Plasma effects and the modulation of white light spectra in the propagation of ultrashort, high-power laser pulses in barium fluoride

We report the results of a study of white light generation in a 7.5 cm long crystal of a high band-gap material, barium fluoride, using ultrashort (<42 fs) laser pulses over a range of values of incident laser power that extend up to more than three orders of magnitude larger than the critical power for self-focusing (P_cr). We explore white light generation and the intensity and spectral distributions within filaments that are formed as a result of the interplay of self-focusing and plasma-induced defocusing. The onset of plasma effects occurs at power levels in excess of 7 GW for ultrashort pulses in BaF₂. For incident power levels that are three orders of magnitude larger than the critical power, blue-shifting of the incident laser wavelength is observed in addition to asymmetric continuum generation. The blue shift enables us to estimate the temporal variation of the electron density in the plasma that is generated within the BaF₂ crystal. PACS 52.38.Hb; 42.65.Jx; 42.65.Tg; 33.80.Wz; 52.35.Mw     

Single-shot dynamics of pulses from a gas-filled hollow fiber

We present measurements of the performance characteristics of few-cycle laser pulses generated by propagation through a gas-filled hollow fiber. The pulses going into the fiber and the compressed pulses after the fiber were simultaneously fully characterized shot-by-shot by using two kHz SPIDER setups and kHz pulse energy measurements. Output-pulse properties were found to be exceptionally stable and pulse characteristics relevant for non-linear applications like high-harmonic generation are discussed. PACS 42.65.Re; 42.65.Ky; 42.65.Sf; 42.65.Jx     

UV–Supercontinuum generated by femtosecond pulse filamentation in air: Meter-range experiments versus numerical simulations

We report new experimental and numerical results on supercontinuum generation at ultraviolet/visible wavelengths produced by the propagation of infrared femtosecond laser pulses in air. Spectral broadening is shown to similarly affect single filaments over laboratory distance scales, as well as broad beams over long-range propagation distances. Numerical simulations display evidence of the crucial role of third harmonic generation in the build-up of UV–visible wavelengths, by comparison with current single-envelope models including chromatic dispersion and self-steepening. PACS 52.38.Hb; 42.65.Tg; 42.65.Jx; 42.68.Ay     

Optical parametric amplifier pumped by two mutually incoherent laser beams

We report on the experimental proof-of-principle demonstration of the ultrashort pulse single-pass beta-barium borate, BBO optical parametric amplifier pumped by two mutually incoherent laser sources. We show that the amplified signal at 1054 nm gains energy from both pump pulses with wavelengths of 680 and 527 nm, respectively, with overall energy conversion of 36%, and exhibits low wavefront distortions and improved energy stability in the gain saturation regime. PACS 42.65.Yj; 42.65.Re     

Standing electron plasma wave mechanism of void array formation inside glass by femtosecond laser irradiation

We investigate the mechanism of formation of periodic void arrays inside fused silica and BK7 glass irradiated by a tightly focused femtosecond (fs) laser beam. Our results show that the period of each void array is not uniform along the laser propagation direction, and the average period of the void array decreases with increasing pulse number and pulse energy. We propose a mechanism in which a standing electron plasma wave created by the interference of a fs-laser-driven electron wave and its reflected wave is responsible for the formation of the periodic void arrays. PACS 61.80.Ba; 42.65.Re; 42.70.Ce; 61.72.Qq; 52.35.Mw     

Rectangular pulse formation in a laser harmonic generation

In a harmonic generation process the temporal profile of the up-converted pulse undergoes significative changes depending on the input profile and crystal length. A simple theoretical treatment and the corresponding physical view are presented. The matter and the properties of two shaping systems are investigated in view of producing rectangular up-converted pulses, as required by laser driven radio-frequency electron sources. PACS 42.65.Re; 42.65.k; 42.79.Hp     

Generation of accurately synchronized pump source for optical parametric chirped pulse amplification

We demonstrate the generation of ultra-short pulses at 1064 nm by continuous-wave seeded non-collinear optical parametric amplification in a -barium borate crystal pumped by the second harmonics of a femtosecond Ti:sapphire laser. After two stages of seeded parametric amplifiers, the generated pulses at 1064 nm were accurately synchronized with the fundamental pump pulses, which could be used as seeding pulses for further amplification and then frequency doubling to produce an accurately synchronized pump source for optical parametric amplification of chirped pulses from the same Ti:sapphire laser. PACS 42.65.Re; 42.65.-k; 52.35.Mw     

Microstructure fibers as frequency-tunable sources of ultrashort chirped pulses for coherent nonlinear spectroscopy

Microstructure fibers are shown to allow the creation of new tunable sources for femtosecond nonlinear spectroscopy. These fibers provide a high efficiency of frequency upconversion of regeneratively amplified femtosecond pulses of a Cr:forsterite laser, permitting the generation of subpicosecond anti-Stokes pulses with a smooth temporal envelope and a linear positive chirp. These pulses from a microstructure fiber were used to measure the spectra of coherent anti-Stokes Raman scattering (CARS) of toluene solution by cross-correlating these pulses with the femtosecond second-harmonic output of the Cr:forsterite laser in boxcars geometry (XFROG CARS). PACS 42.65.Wi; 42.81.Qb     

All-optical stabilization of carrier-envelope phase by use of difference frequency generation with seeded amplification of colored conical emission

We stabilized the carrier-envelope phase of pulses emitted by a femtosecond regenerative amplifier through difference frequency generation between pump and seeded amplification of colored conical emission. Seeded amplification of colored conical emission was induced by modulational instability in the second harmonic generation with a supercontinuum injected and amplified. As a consequence, it inherited the origin phase of the pump pulse. After difference frequency with the pump pulses, the generated tunable idler pulses were carrier-envelope phase stabilized, which was verified with a simple and robust spectral interference setup. PACS 42.65.Re; 42.65.Yj; 42.25.Kb     

Near-infrared continuum generation of femtosecond and picosecond pulses in doped optical fibers

We report broad continuum generation in GeO₂-doped silica fibers induced by femtosecond and picosecond pulses generated by novel high-power laser sources. Over 0.5 W of average power in a broad-band picosecond continuum is generated in the near-infrared part of the spectrum from 800 to 1500 nm. PACS 42.60.By; 42.55.Xi; 42.65.Wi; 42.81.Qb     

Control of lasing filament arrays in nonlinear liquid media

Multiple filamentation in a high concentration solution of coumarin 153 in ethanol is studied. It is shown that the output filament pattern may be controlled by placing diffractive elements (circular aperture, edge) in the input beam path. These filaments are formed in highly reproducible arrays along diffraction maxima corresponding to the element used. Experimental results are supported by numerical simulations. They confirm that diffraction-induced intensity gradients swamp modulational instability on the wavefront, forcing filaments to form along diffraction maxima. The effect of two-photon absorption by coumarin molecules on filament patterns is also investigated over a range of dye concentrations. Control results are finally exploited in the production of arrays of localized lasing filaments, which should open novel applications. The resultant lasing sources are mutually coherent and highly repeatable from shot-to-shot, as is shown by their far-field interference patterns. PACS 42.65.Tg; 52.38.Hb; 42.68.Ay     

Effective length of filaments measurement using backscattered fluorescence from nitrogen molecules

The effective length of self-induced long (100 meters) plasma filaments, generated by intense femtosecond near IR laser pulses in air, was measured remotely using a lidar technique. This technique is based on detecting the backscattered fluorescence signal from nitrogen molecules excited along the intense laser pulse propagation path. This opens up the possibility of measuring remotely long filaments extending over hundreds of meters in the atmosphere. PACS 42.65.Jx; 42.68.Ay; 42.68.Wt     

Continuum generation of the third-harmonic pulse generated by an intense femtosecond IR laser pulse in air

The continuum generation by intense femtosecond IR laser pulses focused in air including the effect of third-harmonic generation is investigated. We have used a theoretical model that includes the full spatio-temporal dynamics of both the fundamental and the third-harmonic pulses. Results of our numerical calculations show that a two-color filamentation effect occurs, in which the third-harmonic conversion efficiency remains almost constant over the whole filament length. It is found that this effect is rather independent of the wavelength of the input beam and the focal geometry. During the filamentation process the third-harmonic pulse itself generates a broad continuum, which can even overlap with the continuum of the fundamental pulse for the longer pump wavelengths. In consequence, the continuum generation generated by intense IR laser pulses is further extended into the UV. PACS 42.65.Jx; 42.65.Ky; 52.35.Mw