Double-peak Splitting in High-order Harmonics Generation

When the intensity of the driving pulse is much higher than the saturation intensity of the media involved, the double-peak splitting in frequency domain emerges in the generated high-order harmonic spectra. The possible origins of this splitting are carefully investigated. The ionization of the gas media and the propagation effect of harmonic field are the main reason for the double-peak splitting observed.     

飞秒激光参数对三态阶跃型分子Autler-Townes分裂的影响

利用三态模型和含时波包法, 研究了K₂分子在强飞秒泵浦-探测激光场中泵浦/探测场强、波长对光电子能谱Autler-Townes(AT)分裂的影响．通过分别改变两激光场的场强或者波长预测AT峰移和间距,并且首次量化了AT分裂的峰移和间距．光电子能谱在共振时显示为对称双峰,失谐时为非对称双峰。AT分裂间距随泵浦场强增大而增大,但不因探测场强改变而改变．     

An Intense Wave in Defective Media Containing Both Quadratic and Modular Nonlinearities: Shock Waves,Harmonics, and Nondestructive Testing

The observed nonclassical power-law dependence of the amplitude of the second harmonic wave on the amplitude of a harmonic pump wave is explained as a phenomenon associated with two types of nonlinearity in a structurally inhomogeneous medium. An approach to solving the inverse problem of determining the nonlinearity parameters and the exponent in the above-mentioned dependence is demonstrated. To describe the effects of strongly pronounced nonlinearity, equations containing a double nonlinearity and generalizing the Hopf and Burgers equations are proposed. The possibility of their exact linearization is demonstrated. The profiles, spectral composition, and average wave intensity in such doubly nonlinear media are calculated. The shape of the shock front is found, and its width is estimated. The wave energy losses that depend on both nonlinearity parameters—quadratic and modular—are calculated.     

空气中激光等离子体通道的三次谐波光谱特性研究

对不同条件下强激光在空气中形成等离子体通道的三次谐波光谱特性进行了研究。单脉冲能量12 mJ,脉宽30 fs,重复频率10 Hz,中心波长795 nm的飞秒激光脉冲经0.5 m焦距的凹面镜聚焦,在空气中形成了等离子体通道, 并在前 向观测到谱线半峰全宽（FWHM）为15 nm的三次谐波。随着脉冲啁啾的变化,三次谐波的光谱出现红移或兰移,当激光脉冲附带+1.3×105fs2的二阶色散时,三次谐波谱线红移且谱峰强度增长了两倍。同时 ,通过改变可编程声光色散滤波器（AOPDF）光谱调制的位置（Hole position）,三次谐波的光谱也发生频移。     

铜掺杂氧化锌纳米棒的非线性光学响应竞争特性

利用飞秒脉冲激光激发Cu掺杂ZnO纳米棒,研究其特有的非线性光学性质和激发机制。在激发波长为750 nm的荧光光谱中,二次谐波峰非常弱,几乎可以忽略,存在非常强的激子发光峰和Cu掺杂导致缺陷发光峰。激发强度的增大会导致这两个发光峰强度呈非线性增大,激子发光峰位产生明显红移,而缺陷发光峰位没有变化。进一步增大激发强度,缺陷发光峰强度会出现饱和甚至有所下降,而激子发光峰强度持续增大。当激发波长增加到760 nm时,从样品的荧光光谱可以清楚地识别到二次谐波峰和激子发光峰以及缺陷发光峰并存。随着激发波长的进一步增加,二次谐波强度不断增大,而激子发光峰和缺陷发光峰的强度却随之下降。当激发波长为790 nm和800 nm时,未发现激子发光峰和缺陷发光峰,非线性光谱以二次谐波为主导。研究结果表明,通过选择合适的激发波长和激发强度,可以实现发光颜色的转变,使得Cu掺杂ZnO纳米棒在全光显示方面具有潜在的发展前景。     

Oscillator Laser Model

A laser model is formulated in terms of quantum harmonic oscillators. Emitters in the low lasing states are usual harmonic oscillators, and emitters in the upper states are inverted harmonic oscillators. Diffusion coefficients, consistent with the model and necessary for solving quantum nonlinear laser equations analytically, are found. Photon number fluctuations of the lasing mode and fluctuations of the population of the lasing states are calculated. Collective Rabi splitting peaks are predicted in the intensity fluctuation spectra of the superradiant lasers. Population fluctuation mechanisms in superradiant lasers and lasers without superradiance are discussed and compared with each other.     

碳碳双键法研究萝卜不同部位的β-胡萝卜素含量分布

β-胡萝卜素广泛存在于植物体中,是典型的线性多稀分子,具有重要的生物功能。由于β-胡萝卜素是碳碳单、双键(C-C,C=C)交替的短链共轭多稀分子,含有大量离域的π电子,具有重要的光电特性。根据Andreas等对拉曼散射强度的研究,当激发光波长落在分子的电子吸收带时,会产生共振拉曼效应,能使拉曼光谱强度提高106倍。利用共振拉曼光谱技术,测量了β胡萝卜素分子及胡萝卜、青萝卜、白萝卜肉质直根不同部位其拉曼光谱,发现含β-胡萝卜素较高的胡萝卜的拉曼光谱与β-胡萝卜素的吻合很好。Gellerman等研究表明,样品浓度与拉曼峰强成正比关系,从拉曼光谱中容易发现三种萝卜的光谱强度纵向根头到主根及横向表皮到根芯逐渐降低,且青萝卜和白萝卜拉曼光谱强度都很低,并在碳碳单键的振动峰处发生峰劈裂。分别计算了碳碳单键和碳碳双键与碳氢键拉曼强度比,三种萝卜的I_CC/I_C-H随着测量部位(横向和纵向)的不同变化幅度接近：胡萝卜的表皮和根芯纵向的变化率分别为A₁=0.213 3和A₂=0.215 9,青萝卜表皮外和里的变化率分别为B₁=0.219 1和B₂=0.211 4,白萝卜表皮外和里分别为D₁=0.223 9和D₂=0.224 1;而对于I_C-C/I_C-H随着测量部位不同其变化率相差很大：胡萝卜的变化率a₁=0.212 1和a₂=0.232 4,青萝卜的变化率b₁=0.263 5和b₂=0.268 7,白萝卜的变化率d₁=0.369 0和d₂=0.304 9。对比发现三种萝卜的碳碳单键与碳氢键振动强度比随着测量部位的不同变化幅度相差很大,而从碳碳双键与碳氢键振动强度比发现三种萝卜中不同部位的β胡萝卜含量有相似的分布。这是由于青萝卜和白萝卜中β-胡萝卜素的含量少, 随着测量部位的不同C-C伸缩振动峰发生峰劈裂, 即在1 130和1 156 cm-1处出现两个振动峰, 经过计算和分析这两个峰都属于碳碳单键的伸缩振动峰, 且随着β-胡萝卜素含量的减少C-C整体的强度降低, 劈裂的新峰峰强度却有增加的趋势, 这使得原峰位的峰强度大幅度降低, 这与计算I_C-C/I_C-H的结果一致,不同品种的萝卜中β-胡萝卜素含量随测量部位的不同变化幅度截然不同。因此, 当样品中β-胡萝卜含量较少时,利用C=C振动峰峰强度同时分析样品不同部位的β-胡萝卜素含量分布变化会更准确。同时,研究和了解萝卜中不同部位β-胡萝卜素的含量为日常消费和膳食营养提供了很好的理论依据。     

Splitting of vibrational mode of CO isotopic species in the unstable trapping site in argon matrix

FTIR spectra of the antisymmetric stretch and symmetric bending vibrational modes of isotopic species of CO₂ trapped in argon matrix are recorded at 5 K with a resolution of . A splitting of the mode is observed for the different species in the trapping site termed unstable. Considering this splitting and the width of the line observed for this unstable site, one expects this site to be larger than the stable one. A theoretical model is elaborated to interpret this splitting. Calculations performed at harmonic level of approximation for vibrational modes in a single substitutional site (S1) and a double substitutional one (S2) in a fcc distorted argon lattice to minimize the free energy of the molecule-matrix system, show the splitting to occur in the larger site. The latter result leads us to invert former attribution of the sites: the stable site is a single substitutional one, whereas the unstable site is a double substitutional one. Received: 27 January 1998 / Revised: 30 July 1998 / Accepted: 17 August 1998     

Generation of second optical harmonic and magnetooptical Kerr effect in ferromagnet-semiconductor heterostructures CaF2/MnAs/Si(111)

The second optical harmonic generation and magnetooptical Kerr effect are investigated for the light (λ=800 nm) reflected by ferromagnet-semiconductor heterostructures CaF₂/MnAs/Si(111). The observed change in the second-harmonic intensity is odd in magnetization. A phenomenological analysis of possible contributions to the second harmonic is carried out, and the sources of optically nonlinear signals are determined from the experimental azimuthal dependences of the light intensity at double frequency. The difference in the field dependences of the second harmonic and the magnetooptical Kerr effect is observed.     

双沃拉斯顿棱镜光强分束比精确分析

利用折射定律,介质膜两侧折射率不同时多光束干涉理论和菲涅耳公式,精确推导了双沃拉斯顿棱镜的光强分束比的具体表达式。以公式为基础,通过Matlab软件数值模拟作图分析光强分束比随入射角、入射波长和结构角的变化关系曲线。结果表明:在棱镜为介质胶合型时,光强分束比随入射角和入射波长的变化很小,光强分束比基本为1;棱镜为空气胶合型时,光强分束比随入射角,结构角和波长的变化很大。两种情况下,光强分束比随各参量的变化基本呈周期性变化。     

强激光场高次谐波的两能级原子模型

利用两能级原子模型，通过直接求解含时薛定谔方程得到了强激光场中的高次谐波谱，和实验中观察到的谐波谱相似，这种模型可用于研究激光强度，激光频率以及介质的电离能等因素对高次谐波的影响。     

Optical absorption in asymmetric double quantum wells driven by two intense terahertz fields

Optical absorption is investigated for asymmetric double quantum wells driven by a resonant terahertz field and a varied terahertz field both polarized along the growth direction. Rich nonlinear dynamics of the replica peak and the Autler-Townes splitting of various dressed states are systematically studied in undoped asymmetric double quantum wells by taking account of multiple factors, such as the frequency of the varied terahertz field and the strength of the resonant terahertz field. Each electron subband splits into two dressed states when the resonant terahertz field is applied in the absence of the varied terahertz field, the optical absorption spectrum shows the first order Autler-Townes splitting of the electron subbands. When a varied terahertz field is added into the resonant system, the replica peak and the second order Autler-Townes splitting of the dressed states near the band edge respectively emerge when the varied terahertz field is non-resonant and resonant with these dressed states. When the strength of the resonant terahertz field is increased, the first order Autler-Townes double peaks and the replica peak in the optical absorption spectrum shift with the shifts of the dressed states. The presented results have potential applications in electro-optical devices.     

Transverse and longitudinal phase-matching in third harmonic generation induced by the Bessel beams

Influence of transverse and longitudinal phase matching on the spectral and intensity properties of third harmonic generation induced by the Bessel pump beams has been investigated both theoretically and experimentally. Transverse phase matching, revealing itself as a ring pattern in the third harmonic intensity angular spectrum was demonstrated in both the normally and anomalously dispersive media. The conditions were found for the optimization of this conical third harmonic signal.     

The external magnetic field dependence of RF splitting of57Fe hyperfine lines. NMR + Mössbauer double resonance experiment

We present the results of an experimental investigation of a RF splitting of⁵⁷Fe hyperfine lines in the regime of NMR and Mössbauer double resonance. The experiments have been performed as a function of RF field intensity and static magnetic field magnitude. The intensity of the RF components and the separation between them are extremely sensitive to the frequency and amplitude of the RF magnetic field. The RF splitting of hyperfine lines is inversely proportional to the strength of the static magnetic field.     

Dynamics of non-linear optical processes

We study the statistical properties of parametric processes (parametric amplification, frequency conversion, splitting of frequency, etc.) described by the trilinear Hamiltonian and of the second harmonic generation including the lossy mechanism and rotating terms. In a short-time approximation some conservation laws are derived and the existence of the Glauber-Sudarshan weighting function is discussed. It is shown in the second harmonic generation case that good coherence of the incident radiation is lost proportionally to the intensity in interaction while the second harmonic radiation has tendency to be coherent. The effects of the spontaneous emission of the medium and of the physical vacuum are also discussed. In this approximation the statistics is generally described by the superposition of coherent and chaotic fields with correlated components.     

Strong bonding magnetic plasmon hybridizations in double split-ring resonators

The complex magnetic dipole plasmon couplings in double split-ring resonators are investigated. Two split peaks in the absorption spectrum of these coupled systems are observed, but even the shorter-wavelength resonance peak can be redshifted compared to the peaks of individual rings. The magnetic plasmon fields outside rings are found to play an important role in these strong couplings. Because of them, both bonding and antibonding plasmon hybridizations occur at each split peak. When bonding coupling effects are stronger than those of antibonding ones, this abnormal splitting behavior appears. When the coupling between rings becomes weaker, the splitting phenomenon tends to be normal.     

Vortex splitting in the interference effect for a quantized vortex released from an optical lattice

For a quantized vortex in a harmonic trap and an optical lattice, we study the interference effect after the combined potentials are switched off. Both numerical and analytical calculations show that there is a vortex splitting in the interference effect of this freely expanding quantum gas, i.e. every interference peak is also a quantized vortex. The experimental scheme to verify this interference effect is discussed.     

Second harmonic generation in scattering of intense beam of radiation by bound electrons near-resonance

Second harmonic generation in near-resonance scattering of intense beams of radiation by bound electrons is investigated by solving the equations of motion exactly to all orders in the intensity of the incident radiation. A two-level model for the atom and a one-mode classical field for the incident radiation is assumed and the rotating wave approximation is taken. It is shown that (i) the second harmonic radiation is an equally spaced triplet, (ii) the middle frequency in these is exactly two times the incident frequency and (iii) the splitting depends on the difference of incident frequency and resonance frequency and on the incident intensity. The counting rates for the three frequencies have been studied in the weak and the high intensity limits.     

一维介观结链中的双电荷孤子

采用半经典模型研究了一维介观结链中两个岛上各存在一个剩余电子时的电势分布,发现在一维介观链中存在双电荷孤子.双电荷孤子的主要特征是它的电势峰发生了劈裂,形成双峰,两峰在通常情况下不等高.研究了双电荷孤子电势峰和阈电压对一维介观结链结构参数的依赖关系.提出了研究双电荷孤子的等效单电荷孤子方法,表明在等效电荷区域,双电荷孤子的电势分布与等效单电荷孤子在同一区域的电势分布相同. 关键词： 双电荷孤子 介观结 单电子效应     

Enhanced vacuum Rabi splitting and double dark states in a composite atom-cavity system

The transmission spectrum of four-level atoms in a cavity is calculated. It is shown that the four separate peaks associated with normal mode splitting and intra-cavity double dark states can be observed simultaneously. The position and intensity of the four peaks can be controlled by the intensity of the third interacting light. Therefore, the enhancement of normal mode splitting by a third coupling light of the intra-cavity four-level atoms is developed.