Isotopic production cross sections of residues in reactions induced by relativistic heavy ions with protons and deuterons

The isotopic production cross sections of heavy residues in relativistic heavy-ion collisions have been investigated in inverse kinematics. The primary reaction products were fully identified in mass and atomic number prior to beta decay using the fragment separator FRS. The huge collection of data obtained helps in the understanding of the two main reaction mechanisms involved: fragmentation and fission. These data provide basic information for future radioactive ion beam facilities and for technical applications like intense neutron sources by means of spallation targets.     

An improved path flux analysis with multi generations method for mechanism reduction

An improved path flux analysis with a multi generations (IMPFA) method is proposed to eliminate unimportant species and reactions, and to generate skeletal mechanisms. The production and consumption path fluxes of each species at multiple reaction paths are calculated and analysed to identify the importance of the species and of the elementary reactions. On the basis of the indexes of each reaction path of the first, second, and third generations, the improved path flux analysis with two generations (IMPFA2) and improved path flux analysis with three generations (IMPFA3) are used to generate skeletal mechanisms that contain different numbers of species. The skeletal mechanisms are validated in the case of homogeneous autoignition and perfectly stirred reactor of methane and n-decane/air mixtures. Simulation results of the skeletal mechanisms generated by IMPFA2 and IMPFA3 are compared with those obtained by path flux analysis (PFA) with two and three generations, respectively. The comparisons of ignition delay times, final temperatures, and temperature dependence on flow residence time show that the skeletal mechanisms generated by the present IMPFA method are more accurate than those obtained by the PFA method, with almost the same number of species under a range of initial conditions. By considering the accuracy and computational efficiency, when using the IMPFA (or PFA) method, three generations may be the best choice for the reduction of large-scale detailed chemistry.     

Extension of the Monte-Carlo code MOCADI to fusion-evaporation reactions

The Monte-Carlo code MOCADI has been extended, besides to fission and fragmentation reactions, also to fusion-evaporation reactions. The updated version includes the cross sections and the reaction kinematics for the production of evaporation residues calculated according to the statistical model code PACE2, while the atomic interaction with matter can be treated either with the code ATIMA or with the code TRIM. The present version of MOCADI can now be employed world-wide for design studies of new low-energy nuclear physics facilities and for the optimization of experiments involving fusion-evaporation reactions, e.g. mass measurements, laser spectroscopy, super-heavy synthesis.     

Two mechanisms of multiplicity production and clan structure

Some characteristics of clan structure have been analysed by the phenomenological model which is based on an assumption that there are two mechanisms of secondary particle production where the first of which causes secondary particle generation by decays of primary generated resonances (clans) and the second of which calls forth secondary particle production by inverse processes of merging of couple of particles into one particle.     

Resonances and final-state interactions in the reaction pp → pK+Λ

A study of the strangeness production reaction pp → pK⁺Λ for excess energies of ε≤150MeV, accessible at high-luminosity accelerator facilities like COSY, is presented. Methods to analyze the Dalitz plot distribution and angular spectra in the Jackson and helicity frames are worked out and suitable observables for extracting information on low-lying resonances that couple to the KΛ system and for determining the Λp effective-range parameters from the final-state interaction are identified and discussed. Furthermore, the chances for identifying the reaction mechanism of strangeness production are investigated.     

Intense radioactive-ion beams produced with the ISOL method

For fifty years the isotope separation on-line (ISOL) technique has been used for the production of radioactive-ion beams (RIBs). Thick-target ISOL facilities can provide very intense RIBs for a wide range of applications. The important design parameters for an ISOL facility are efficiency, rapidity and selectivity of all steps of the separation process. To achieve the anticipated beam intensities with the next-generation RIB facilities, the production rate in the ISOL target has to be increased by orders of magnitude. This is only possible by adapting the projectile beam for optimum production cross-sections and simultaneously minimizing the target heating due to the electronic stopping power of charged-particle projectiles. ISOL beams of 75 different elements have been produced up to now and further beam development is under way to produce a still greater variety of isotopes and to improve existing beams in intensity and purity. Received: 21 March 2002 / Accepted: 16 May 2002 / Published online: 31 October 2002 RID="a" ID="a"e-mail: Ulli.Koster@cern.ch     

Atomic layer deposition of iridium(III) acetylacetonate on alumina, silica-alumina, and silica supports

The deposition of noble metal particles and films by atomic layer deposition (ALD) has recently gained interest in the fields of catalysis and microelectronics. However, there is little information on the mechanisms governing the reactions of noble metals with high surface area supports. In this work, iridium(III) acetylacetonate was deposited from gas phase onto alumina, silica-alumina, and silica supports to gain insight into the reaction mechanisms. According to elemental analysis and infrared spectroscopy, ligand exchange reaction between iridium acetylacetonate and surface OH groups took place on all substrate surfaces, but the iridium deposition on alumina and silica-alumina appeared to be hindered by sterical effects of the acetylacetonate ligands. Part of the iridium on silica was in metallic form. To reduce the content of iridium, reactive sites of the support surfaces were blocked with H-acetylacetonate (2,4-pentanedione). The blocking reduced the iridium content by more than 90% on alumina but by only 30-50% on silica-alumina. The attempted blocking had almost no effect on silica as expected. According to the results of this work, ALD can provide a feasible method for preparing iridium catalyst with reasonable iridium loadings.     

Surface chemistry and optimization of focused ion beam iodine-enhanced etching of indium phosphide

Focused ion beam physical sputtering and iodine-enhanced etching of indium phosphide (InP) were performed. Up to 15× enhanced etching rates over sputtering were measured at room temperature, due to the addition of iodine to the sputter-process. Reaction mechanisms and products are discussed and characterized. The reaction is limited by the desorption of indium triiodide (InI₃) at room temperature. InI₃ has to be removed by sputtering, which simultaneously amorphizes the underlying substrate. Surface roughness and stoichiometry of InP are compared for sputtering and etching. Gallium-contamination and the damaged zone in InP are significantly reduced by iodine-enhanced etching. Based on the reaction mechanisms, an optimum beam scanning strategy is proposed which allows precise microfabrication in reduced time and minimizes damage to the substrate. The method is also applicable for other halide gas etching processes of III-V semiconductors.     

Some physical insights for active acoustic structure

Active acoustic structure (AAS) proposed in recent years has been viewed as an encouraging approach to actively control sound radiation from vibrating structures. Much work of AAS has been done on theoretical model, arrangement of the secondary panel and error sensing, and experimental investigation of AAS system, but physical mechanisms is little understanding. In this study, under minimization of the total sound power output, the physical mechanism of noise reduction is investigated by analyzing the sound power output change of primary and secondary structures and the distribution of sound intensity. The results show that there are two kinds of energetic behaviors, which includes the suppression of the sound power radiated by the primary panel and absorption of sound power by the primary and secondary panels.     

High-energy probes

We review some results on energetic particle production in heavy-ion collisions below roughly 100A·MeV, both theoretically and experimentally. We discuss the possible mechanisms of particle production, as well as the possibility to gather information on the nuclear equation of state (EOS) from data. Results on subthreshold pions, energetic photons, nucleons and light charged particles (Z ⩽ 2) are discussed and contrasted to microscopic models. Important information about the first stages of the reaction are obtained by such probes. At present, we can conclude that we have at least a qualitative understanding of the processes involved when such particles are produced. However, a quantitative determination of relevant EOS parameters is still missing. The production mechanism close to the kinematical threshold (incoherent, cooperative or statistical) is not completely elucidated either. This calls for new data using more modern detector systems and comparison to more refined microscopic models.     

Angular Distribution of the 12C(6He, 7Li)11B Reaction

Angular distribution of the ¹²C(⁶He,⁷Li)¹¹B transfer reaction is measured with a secondary ⁶He beam of 36.4MeV for the first time. The experimental angular distribution is well reproduced by the distorted-wave Born approximation (DWBA) calculation. The success of the present experiment shows that it is feasible to measure one-nucleon transfer reaction on a light nucleus target with the secondary beam facility of the HI-13 tandem accelerator at China Institute of Atomic Energy (CIAE), Beijing.     

Production of fragments with Z≥ 8 in interaction of 12.7 GeV 4He+U, Pb, Au and Ag: track detector study

The processes of production of fragments with Z≥ 8 in the interaction of 12.7 GeV ⁴He with U, Pb, Au and Ag have been analyzed using the polycarbonate track detector Makrofol. The sandwich technique was used which enables direct observation of multiply charged fragment emission by a single nucleus. The decay channels ending with one, two, or more (three, four) fragments were detected. A classification scheme based on the multiplicity of heavy fragments with Z > 20 was used in order to identify the events belonging to the different reaction channels. The cross sections, excitation energies and multiplicities of intermediate-mass fragments 8 ≤Z≤ 20 have been determined for the various reaction mechanisms, and their variation as a function of the target mass has been investigated. Received: 28 November 1997 / Revised version: 24 April 1998     

Co-Adsorption of CO in NO-CO Reaction on a Metal Catalytic Surface Studied by Computer Simulation

The effect of co-adsorption of CO molecules in the NO-CO reaction on a metal catalytic surface like Pt（001） is studied by applying the Langmuir-Hinshelwood mechanism using the Monte Carlo simulations. The system is investigated by two approaches of NO adsorption; dissociatively at two empty surface sites and molecularly at a single vacant site. The elementary steps are the same as those in the conventional Ziff-Gulari-Barshad model. With the additional reaction step of co-adsorption, the sustained production of CO2 is obtained, which has never been seen on a square lattice without introducing additional parameters. The most interesting result is the elimination of continuous second order phase transition, i.e. the production of CO2 starts as soon as the partial pressure of CO departs from zero, which is in accordance with the experimental observations. The effect of co-adsorption probability on the phase diagrams has also been studied.     

Precompound charged particle emission (PCE) — a mechanism beyond element production by complete fusion

Complete fusion reactions (xn-channels) using actinide targets are observed for values of the effective fissilities x _eff ∼ 0.80 in the sub-pb range of production cross sections. The elements produced at this limit are Z = 108–112. Beyond complete fusion, heavier elements might still be produced by reaction mechanisms releasing part of the nuclear charge before an equilibrated compound system might have been reached. Precompound Charged particle Emission (PCE) is proposed as a possible mechanism following complete fusion. A scheme delivering isotopes of elements Z = 110–115 is discussed, and experimental evidence for such a process is presented. Compound systems, the atomic numbers of which are smaller than in complete fusion reactions, might be produced in ⁴⁸Ca induced reactions on actinides with larger cross sections than those at the limits of complete fusion. Besides complete fusion, the PCE-mechanism should be considered as an alternative to interpret the ⁴⁸Ca-induced reactions on actinides.     

新型羟基和醌碳自由基产生的分子机理

羟基自由基（·OH）被公认是生物系统中最具活性的活性氧物种,能导致生物体内DNA等生物大分子氧化损伤. 目前,最被广泛接受的·OH的产生机理是过渡金属离子催化的Fenton反应. 五氯酚(PCP)是一种重要的生物杀灭剂,主要用作木材保护. 采用电子自旋共振二级自旋捕获等分析手段,发现H₂O₂和五氯酚的代谢产物之一四氯苯醌（TCBQ）能通过不依赖于金属离子的途径产生·OH;进一步的研究发现是TCBQ,而非其相应的半醌自由基对·OH的产生极其重要. 基于这些数据和分析,提出以下新型·OH产生分子机理：H₂O₂对TCBQ进行亲核攻击形成不稳定的三氯氢过氧基苯醌中间产物,其可均裂产生·OH. 综合采用电子自旋共振自旋捕获和其他分析方法,第1次检测到一种新型的以碳为中心的醌自由基.     

Towards optical spectroscopy of the element nobelium ({\sf Z }= \mathsf{102}) in a buffer gas cell

For the investigation of the atomic level structure of heavy elements which can only be produced at on-line facilities such as GSI, a novel experimental procedure has been developed. It is based on Radiation Detected Resonance Ionization Spectroscopy (RADRIS) and can be applied to elements like nobelium produced at rates of a few ions per second. Fusion reaction products are separated from the primary beam by the velocity filter SHIP at GSI, stopped in a buffer gas cell, collected on a tantalum filament and then re-evaporated as atoms. The ions produced by resonance ionization with tunable laser beams are detected via their characteristic α decay. First on-line experiments on α-active ¹⁵⁵Yb, which is supposed to have an atomic level structure similar to nobelium, were performed. These test experiments focused on the optimization of the collection and re-evaporation process of the radioactive ions, the laser ionization efficiency and the detection via α decay. An overall efficiency for RADRIS of 0.8% with respect to the target production rate was measured. While further improvements of this efficiency are in progress it should already be sufficient for the search for atomic levels in nobelium.     

Study of temperature effects on the conduction and trapping of charges in the alkali-silicate glass under electron beam irradiation

A scanning electron microscope (SEM) is employed to investigate the temperature effect on the charging behaviour of alkali-silicate glasses under electron beam irradiation using electrostatic influence method (EIM). A modified special arrangement adapted to the SEM allows to study charging mechanisms and charge transport characteristics of these glasses using the simultaneous measurement of displacement and leakage currents. The trapping process during continuous electron irradiation can be directly determined by the EIM. The experimental results reveal that the charging ability of glasses decreases with increasing temperature. The variation of charge process has been confirmed by measuring the surface potential in response to the sample temperature. In this report, we introduce also the secondary electron emission (SEE) yield. It was found the strong dependence of the SEE yield on the temperature variation. The higher is the temperature and the lower is the SEE yield. The trapping ability is analyzed taking into account the regulation mechanisms involved under electron irradiation.     

高自旋同质异能态束流及其在核谱学中的应用

介绍了在日本理化学研究所利用高自旋同质异能态束流装置上取得的核谱学研究结果。强调了可利用重离子核反应中逆运动学产生高自旋同质界能态束流,并用其进行二次核反应,描述了首次利用高自旋同质异能态束流完成的物理实验． The study of nuclear spectroscopy by using the High spin isomer Beam(HSIB)facility in RIKEN was introduced.The production of HSIB based on the inverse kinematics in heavy ion nuclear reaction,and its application for secondary nuclear reaction were stressed The first experimental result by using HSIB was also briefly discribed.     

Prospects for strangeness measurement in ALICE

The study of strangeness production at LHC will bring significant information on the bulk chemical properties, its dynamics, and the hadronization mechanisms involved at these energies. The ALICE experiment will measure strange particles from topology (secondary vertices) and from resonance decays over a wide range in transverse momentum and shed light on this new QCD regime. These motivations will be presented as well as the identification performance of ALICE for strange hadrons. (for the ALICE Collaboration) The text was submitted by the author in English.