A pulsed optical parametric oscillator, based on periodically poled lithium niobate (PPLN), for high-resolution spectroscopy

-1 ), approaching the limit imposed by the Fourier transform of the pulse duration. Received: 31 August 1998     

Angle-tuned signal-resonated optical parametric oscillator based on periodically poled lithium niobate

We demonstrate an angle-tuned signal-resonated optical parametric oscillator (OPO) with periodically poled lithium niobate (PPLN) pumped by a diode-pumped Nd:YVO4 laser. 1499.8 - 1506.6 nm of signal wavelength is achieved at 140℃ by rotating a 29-μm period PPLN from 0° - 10.22° in the x-y plane while keeping the pump wave vertical to the resonator mirrors. Two pairs of the signal and idler waves of the same wavelengths can be achieved symmetrically for each pair of angles of rotation with same absolute value and opposite sign. Theoretical analyses on angle-tuned PPLN-OPO with pump wave vertical to the resonator mirrors are presented and in good agreement with our experimental results. It is also found that all interacting waves in the cavity (not inside the crystal) are always collineax for PPLN-OPO with the pump wave vertical to the resonator mirrors while phase-matching is noncollinear within the crystal.     

High-power picosecond optical parametric oscillator based on periodically poled lithium niobate

A high-power picosecond optical parametric oscillator (OPO) based on a 47-mm periodically poled lithium niobate crystal is described. More than 12 W of total average power-almost 8 W of signal power at 1.85 microm and more than 4 W of idler radiation at 2.5 microm -is simultaneously extracted from less than 18 W of average pump power. The OPO is synchronously pumped by 80-ps (FWHM) cw mode-locked pulses at 1.064 microm , and its output is tunable from 1.7 to 2.84microm . Nearly transform-limited signal pulses are obtained following the introduction of two intracavity etalons.     

Frequency-agile kilohertz repetition-rate optical parametric oscillator based on periodically poled lithium niobate

We report kilohertz repetition-rate pulse-to-pulse wavelength tuning from 3.22 to 3.7 mum in a periodically poled lithium niobate (PPLN) optical parametric oscillator (OPO). Rapid tuning over 400 cm(-1) with random wavelength accessibility is achieved by rotation of the pump beam angle by no more than 24 mrad in the PPLN crystal by use of an acousto-optic beam deflector. Over the entire tuning range, a near-transform-limited OPO bandwidth can be obtained by means of injection seeding with a single-frequency 1.5-mum laser diode. The frequency agility, high repetition rate, and narrow bandwidth of this mid-IR PPLN OPO make it well suited as a lidar transmitter source.     

Continuous-wave 532-nm-pumped singly resonant optical parametric oscillator based on periodically poled lithium niobate

We report a continuous-wave (cw) 532-nm-pumped singly resonant optical parametric oscillator (SRO) based on periodically poled lithium niobate. The pump source is a commercial 5-W cw diode-pumped, multilongitudinal-mode, intracavity-doubled Nd:YVO(4) laser. Using a four-mirror ring SRO cavity and single-pass pumping, we achieved subwatt internal oscillation threshold, 56% quantum efficiency, and output tuning from 917 to 1266 nm.     

Low-threshold singly-resonant continuous-wave optical parametric oscillator based on MgO-doped PPLN

We present a 532 nm-pumped singly-resonant cw optical parametric oscillator based on MgO-doped PPLN with a minimum threshold pump power of 0.3 W. The OPO with a two-mirror standing-wave cavity is optimized by using a tunable diode laser on the path of the resonant signal beam. The maximum output power is 200 mW at an idler wavelength near 1330 nm at a pump power of 2 W. We report the degradation of the output power and beam characteristics at high pump power indicating a strong thermal lensing in the crystal. The continuous tuning range of the OPO is measured to be 800 MHz which is close to 90% of the free spectral range of the OPO cavity.     

High-efficiency,high-repetition-rate,temperature-tuning optical parametric oscillator based on periodically poled MgO-doped lithium niobate

We report a compact and viable source of high-efficiency, high-repetition-rate, temperature-tuning, mid-IR optical parametric oscillator (OPO) based on periodically poled MgO-doped lithium niobate (PPMgOLN) pumped by a homemade high power AOM Q-switched Nd:YVO₄ laser centered at 1.064 μm. With an optimal plane-concave resonator configuration, average output power of 5.7 W at 2.73 μm was obtained when the pump power was 25 W at the repetition rate of 80 kHz. The conversion efficiency from the 1.064 μm laser to the 2.73 μm laser was 22.8%. Temperature tuning of the OPO yielded a signal wavelength range from 1.67 to 1.75 μm and an idler wavelength in the range of 2.72 to 2.92 μm.     

Continuous wave monolithic quasi-phase-matched optical parametric oscillator in periodically poled lithium niobate

We demonstrate a monolithic and quasi-phasematched singly resonant cw optical parametric oscillator in periodically poled lithium niobate. The threshold is 1.0 W and the OPO delivers up to 0.98 W signal power tunable between 1750 and 1950 nm (2710 and 2340 nm idler, respectively). We identify cascaded parasitic oscillation effects and analyze their behavior theoretically, showing good agreement with our experiment. The analysis of parasitic effects points the way to improved device designs that should enable stable, compact, and frequency-tunable sources.     

Five-optical-cycle pulse generation in the mid infrared from an optical parametric oscillator based on aperiodically poled lithium niobate

We describe an optical parametric oscillator based on aperiodically poled lithium niobate that generates nearly transform-limited 53-fs duration pulses at a center wavelength of 3mum, corresponding to only 5 optical cycles. Results are presented illustrating the effect of pump- and grating-period chirp on the idler pulses, and a configuration capable of producing idler bandwidths in excess of 700 nm is discussed.     

Broadly tunable mid-infrared femtosecond optical parametric oscillator using all-solid-state-pumped periodically poled lithium niobate

We describe a high-repetition-rate femtosecond optical parametric oscillator (OPO) that was broadly tunable in the mid infrared. The all-solid-state-pumped OPO was based on quasi-phase matching in periodically poled lithium niobate. The idler was tunable from approximately 1.7 mum to beyond 5.4 mum, with maximum average power levels greater than 200 mW and more than 20 mW of average power at 5.4 mum. We used interferometric autocorrelation to characterize the mid-infrared idler pulses, which typically had durations of 125 fs. This OPO had a pumping threshold as low as 65 mW of average pump power, a maximum conversion efficiency of >35% into the near-infrared signal, a slope efficiency for the signal of approximately 60%, and a maximum pump depletion of more than 85%.     

Self-guided operation of singly resonant continuous-wave optical parametric oscillator based on bulk MgO-doped PPLN

We report on a self-guided operation of a green-pumped singly resonant continuous-wave optical parametric oscillator with a bulk MgO-doped PPLN crystal. It is achieved by increasing the OPO cavity length beyond the stability boundary so that the OPO can only oscillate with formation of a thermally induced waveguide inside the crystal. The effects of the thermal waveguide on the OPO performance are studied by measuring output power characteristics at different cavity lengths. Improvement of spatial mode quality and stability of output power by self-guiding is demonstrated. Measurement of temporal characteristics proves that formation of the waveguide originates from the photo-thermal effect in the nonlinear crystal by absorption of pump power.     

Aging effect in proton-exchanged optical waveguides based on lithium niobate crystals

The optical characteristics of planar waveguides produced by proton exchange in lithium niobate crystals in different acids (with and without additives) are unstable with time (“aging” effect). The aging effects in LiNbO₃ optical waveguides are investigated at room and elevated (50, 60, or 70°C) temperatures. In all cases, variations in the refractive index of the waveguide layer with time, i.e., for two or three years at room temperature and for several weeks at elevated temperatures, are determined for waveguides prepared in different media. The dependences of the optical characteristics of waveguides on the nature of proton sources and the aging conditions are obtained experimentally.     

Tunable mid-infrared optical parametric oscillator with intracavity parametric amplification based on a dual-grating PPLN crystal

Intracavity amplification of the idler radiation of a nanosecond optical parametric oscillator (OPO) is achieved within a single dual-grating PPLN crystal composed of a uniform-grating section followed by a fan-out grating section. While all the OPO wavelength-tuning capabilities are preserved, this configuration leads to a 60?% increase of the 4-??m idler power and a significant beam quality improvement when compared to a conventional singly resonant OPO.     

Nonlinear multiwavelength conversion based on an aperiodic optical superlattice in lithium niobate

We have demonstrated what is to our knowledge the first successful achievement of multiwavelength conversion in an aperiodic optical superlattice (AOS) lithium niobate crystal with equalized gain. The two AOS devices in our experiment, numerically synthesized from 2857 crystal blocks with a unit block thickness of 3.5 microm, have fundamental wavelengths of 1540 and 1545 nm for double-wavelength second-harmonic generation (SHG) and of 1540, 1545, and 1553 nm for triple-wavelength SHG at 50 degrees C. Our experiment and simulation show that the output spectrum of an AOS wavelength converter is fairly insensitive to typical fabrication errors.     

Synchronously pumped femtosecond optical parametric oscillator of congruent and stoichiometric MgO-doped periodically poled lithium niobate

A synchronously pumped femtosecond optical parametric oscillator based on congruent MgO-doped periodically poled lithium niobate (c-MgO:PPLN) is reported. The system, operating at room temperature, was pumped by a mode-locked Ti:sapphire laser. The wavelengths of the signal and idler waves were tuned from 870 nm to 1.54 μm and 1.58 to 5.67 μm, respectively, by changing the pump wavelength, the grating period or the cavity length. Pumped by 1.1 W of 755 nm laser radiation, the OPO generated 310 mW of 1080 nm radiation. This signal output corresponds to a total conversion efficiency of 50%. Without dispersion compensation the OPO generated phase-modulated signal pulses of 200 fs duration. Besides the OPO of c-MgO:PPLN, an OPO of stoichiometric (s) MgO:PPLN was investigated. Because of the reduced sensitivity to photorefractive damage, both crystals allowed efficient OPO operation at room temperature. Received: 19 August 2002 / Revised version: 11 December 2002 / Published online: 19 March 2003 RID="*" ID="*"Corresponding author. Fax: +49-631/205-3906, E-mail: andres@physik.uni-kl.de     

Generation of femtosecond pulses from order-of-magnitude pulse compression in a synchronously pumped optical parametric oscillator based on periodically poled lithium niobate

We demonstrate the generation of compressed, transform-limited 250-fs pulses, tunable in the near infrared, by means of synchronously pumped optical parametric oscillation in periodically poled lithium niobate. The almost 20-fold compression from the 4-ps pulse duration of the cw mode-locked Nd:YLF pump results in signal peak powers well in excess of the pump power.     

Integrated optical electric field sensor based on a Bragg grating in lithium niobate

We demonstrate a new sensor concept for the measurement of oscillating electric fields that is based on Bragg gratings in LiNbO₃:Ti channel waveguides. This miniaturized sensor that works in a retroreflective scheme does not require metallic electrodes and can be directly immersed in an oscillating electric field. The electric field induces a shift of the Bragg wavelength of the reflection grating that is due to the electro-optic effect. The operating point of the sensor is chosen by adjusting the laser wavelength to the slope of the spectral reflectivity function of the grating. In this way the magnitude of an external electric field is measured precisely as the amplitude of modulated reflected light intensity by using a lock-in amplifier. The sensor principle is demonstrated by detecting low-frequency electric fields ranging from 50 V/cm to 5 kV/cm without any conducting parts of the sensor head. Furthermore, the ability of the sensor to determine the three-dimensional orientation of an external electric field by a single rotation along the waveguide direction is demonstrated. PACS 42.40.Eq; 42.82.-m; 42.82.Et     

Periodic poling of magnesium-oxide-doped stoichiometric lithium niobate grown by the top-seeded solution method

Magnesium-oxide-doped stoichiometric lithium niobate has been produced using the technique of top-seeded solution growth from a lithium-rich melt. Optical tests, performed with a combination of argon-ion laser lines, have confirmed a previously published result (at 532 nm) that this material has superior resistance to photorefractive damage. This material has been shown, for the first time, to be amenable to periodic poling. Optical parametric oscillator tests have shown that this material maintains the advantages of periodically poled, congruent, un-doped lithium niobate while showing no evidence of photorefractive damage under typical operating conditions. Operating wavelengths as a function of quasi-phase-matching period and temperature have been measured for the optical parametric oscillator, providing useful new information about refractive-index dispersion in this material. This work establishes periodically poled, magnesium-oxide-doped stoichiometric lithium niobate as a viable material for nonlinear optics. Received: 28 June 2000 / Revised version: 12 September 2000 / Published online: 7 February 2001     

Ordered nano-scale domains in lithium niobate single crystals via phase-mask assisted all-optical poling

We report the formation of directionally ordered nano-scale surface domains on the +z face of undoped congruent lithium niobate single crystals by using UV illumination through a phase mask of sub-micron periodicity with an energy fluence between ∼90 mJ/cm² and 150 mJ/cm² at λ = 266 nm. We clearly show here that the UV-induced surface ferroelectric domains only nucleate at and propagate along maxima of laser intensity. Although the domain line separation varies and is greater than 2 μm for this set of experimental conditions, this enables a degree of control over the all-optical poling process.