基于闪锌矿晶体中受激电磁耦子散射产生可调谐太赫兹波的理论研究

基于受激电磁耦子散射原理,采用已报道的利用非线性光学参量振荡方法产生可调谐太赫兹波的实验条件作为理论分析的实验模型,以GaAs,GaP, InP,ZnTe晶体为代表,计算分析了在闪锌矿晶体中参量振荡产生太赫兹波的吸收、增益特性,对输出THz波的调谐特性给出了详尽分析.分析太赫兹波高效耦合输出的腔型结构,并与掺氧化镁铌酸锂晶体组成的太赫兹波参量振荡器做对比. 关键词： 太赫兹波 太赫兹波参量振荡 电磁耦子 闪锌矿晶体     

Second-order nonlinear optical materials for efficient generation and amplification of temporally-coherent and narrow-linewidth terahertz waves

We have considered forward and backward optical parametric oscillation and amplification, and difference-frequency generation for efficiently generating and amplifying terahertz waves in several second-order nonlinear optical materials. We have used a single crystal of CdSe as an example. We have also investigated GaSe, periodically-poled LiNbO₃ and LiTaO₃, and diffusion-bonded-stacked GaAs and GaP plates. The advantage of using birefringence in CdSe and GaSe is tunability of the output terahertz frequency. Furthermore, both CdSe and GaSe can be used to achieve the backward parametric oscillation without any cavity. On the other hand, in periodically-poled LiNbO₃ and LiTaO₃, one can take advantage of large diagonal elements of second-order nonlinear susceptibility tensor. In the diffusion-bonded-stacked GaAs and GaP plates, quasi-phase matching can be achieved by alternatively rotating the plates. We have shown that it is feasible to achieve forward optical parametric oscillation in the THz domain using these plates. The advantage of using coherent parametric processes is possibility of efficiently generating and amplifying temporally-coherent and narrow-linewidth terahertz waves. Compared with a noncollinear configuration, by using the parallel wave propagation configurations, the conversion efficiency can be higher because of longer effective interaction length among all the waves.     

cw dual-wavelength operation of a diode-end-pumped Nd:YVO4 laser

A dual-wavelength continuous wave (cw) diode-end-pumped Nd:YVO₄ laser that generates simultaneous laser action at the wavelengths 1064 nm and 1342 nm is demonstrated. The optimum oscillation condition for the simultaneous dual-wavelength operation in a diode-end-pumped solid-state laser has been derived. The relationship between the laser cavity and the output stability is also studied. Experimental results show that the stability of the output power at the two wavelengths could be enhanced by use of a three-mirror cavity. Received: 26 August 1999 / Revised version: 11 October 1999 / Published online: 23 February 2000     

Optical parametric oscillation in a vertical triple microcavity

We report the realization of a monolithic vertical-cavity, surface emitting micro-optical parametric conversion nanostructure, triply resonant with the parametric frequencies, allowing parametric oscillation with ultra-low pump power threshold. The photonic phase-space naturally provides triple resonance for the parametric frequencies, together with built-in cavity phase matching for the pump wave at normal incidence. Parametric oscillation is observed in both the strong and weak exciton–photon coupling regime, allowing high operating temperature. Signal and idler beams can be collected at 0 or at finite angles. The OPO threshold is low enough to envisage the realization of an all-semiconductor electrically-pumped micro-parametric oscillator.     

Multiline coherent oscillation in photorefractive crystals with two species of movable carriers

The coherent oscillation, because of nearly degenerate four-wave mixing in photorefractive crystals with two types of movable charge carriers, occurs at two spectral lines symmetrically shifted with respect to the pump frequency. Consequently the output oscillation exhibits the high contrast intensity modulation. The frequency separation of two oscillation modes (and modulation frequency of the output intensity) depend on the incident light intensity and spatial frequency of the developing grating. A model is presented explaining this type of oscillation by the two-maxima shape of the gain spectrum in crystals with sufficiently different relaxation times of two space-charge gratings, one formed by movable electrons and the other one by movable holes. The experimental data for coherent oscillator with tin hypothiodiphosphate (Sn₂P₂S₆) are in reasonable quantitative agreement with the calculations. Received: 12 November 1998 / Revised version: 11 January 1999 / Published online: 7 April 1999     

Synchronously pumped femtosecond optical parametric oscillator based on AgGaSe2 tunable from 2 μm to 8 μm

The operation of a continuous-wave mode-locked silver gallium selenide (AgGaSe₂) optical parametric oscillator (OPO) is reported. The OPO was synchronously excited by 120-fs-long pulses of 1.55-μm radiation at a repetition rate of 82 MHz. The 1.55-μm radiation is generated by a noncritically phasematched cesium-titanyl-arsenate (CTA)-OPO pumped by a mode-locked Ti:sapphire laser. The AgGaSe₂-OPO generates signal and idler radiation in the range from 1.93 μm to 2.49 μm and from 4.1 μm to 7.9 μm, respectively. Up to 67 mW of signal wave output power has been obtained. The experimentally determined pulse duration and chirp parameters are in reasonable agreement with results from a numerical model taking into account group velocity mismatch, group velocity dispersion, self phase modulation, and chirp enhancement. Received: 6 August 1999 / Revised version: 4 October 1999 / Published online: 3 November 1999     

Parametric generation of twin photons in vertical triple microcavities

We report the realization of a monolithic vertical-cavity, surface emitting micro-optical parametric conversion nanostructure, triply resonant with the parametric frequencies, allowing parametric oscillation with ultra-low pump power threshold. The photonic phase-space naturally provides triple resonance for the parametric frequencies, together with built-in cavity phase-matching for the pump wave at normal incidence. Parametric oscillation is observed in both the strong and weak exciton–photon coupling regime, allowing a high operating temperature. Signal and idler beams can be collected at 0° or at finite angles. The OPO threshold is low enough to envisage the realization of an all-semiconductor electrically-pumped micro-parametric oscillator. To cite this article: C. Diederichs et al., C. R. Physique 8 (2007).     

级联参量振荡产生太赫兹辐射的理论研究

针对光学参量振荡产生太赫兹波转换效率低的缺点, 提出了级联参量振荡产生太赫兹波的新机理以提高转换效率. 以周期极化铌酸锂晶体为例, 对级联参量振荡产生太赫兹波的原理和过程进行了理论研究. 分析了抽运光波长、周期极化铌酸锂晶体极化周期和工作温度对产生一阶、二阶闲频光频率的影响. 推导了三波共线相互作用条件下太赫兹波的增益特性和吸收特性. 计算结果表明, 通过级联参量振荡可以有效提高太赫兹波的转换效率, 并可以得到宽调谐的太赫兹波输出. 基于分析结果, 设计了周期极化铌酸锂晶体级联参量振荡产生高效率、宽调谐、窄线宽、连续太赫兹波的实验. 关键词： 太赫兹波 太赫兹波参量振荡 级联参量振荡     

Experimental Evidence of Parametric Instabilities in an Unmagnetized Plasma Subjected to a Strong H.F. Electric Field

Experimental evidence of parametric excitation, by an intense external H.F. field, of an electron surface mode and an ion wave is presented. The pumping electromagnetic energy density is equal to or slightly larger than the thermal energy density of the electrons. The value of f_pc/f₀ (electron plasma frequency/external field frequency) is that for an electron surface wave. Depending on the pressure and field intensity, this decay instability can lead to three types of low frequency oscillations, with frequencies close to the ion plasma frequency. Two of these are described by Aliev and Silin's intense field theory: one is the volume ion plasma oscillation and the other a surface ion plasma oscillation. The third corresponds to no known ion eigenmode. Several other features of the theory by Aliev and co-workers are also confirmed experimentally, such as the harmonic excitation of the instability (nf₀ ≈ f_pe/√2, where n is an integer), the instability amplitude as a function of f_pe/f₀ (above threshold conditions), the value of the mismatch parameter as a function of field strength and ion mass, and the existence of a fine structure corresponding to the symmetric and antisymmetric electron surface oscillations. Even at high pump field strengths, the decay products are nearly monochromatic i.e. the plasma does not become turbulent.     

Polarization properties of coherent VUV light at 125 nm generated by sum-frequency four-wave mixing in mercury

The polarization of the VUV light generated by four-wave sum-frequency mixing process ω₄=2ω₁+ω₂ in mercury vapor at room temperature is analyzed in detail. Due to the specific two-photon transition used to enhance the nonlinear process, the polarization of the VUV wave is shown to be identical to the polarization of the wave at the frequency ω₂. In particular, circularly polarized VUV is observed with degree of circular polarization exceeding 0.99. Received: 11 July 1999 / Revised version: 8 October 1999 / Published online: 8 March 2000     

Submillimeter wave induced resistance oscillations in ultra-high mobility two-dimensional electron systems

Submillimeter wave induced resistance oscillations in two ultra-high mobility GaAs/Al_0.24Ga_0.76As quantum well samples have been investigated by means of a backward wave oscillator and far-infrared laser at ³He temperatures. Subnikov–de Haas oscillation, submillimeter wave induced resistance oscillation, and magnetoplasmon resonance occur simultaneously in this frequency regime. The primary radiation induced resistance minimum shifts toward cyclotron resonance with increasing radiation frequency. The positions of these minima agree well with those of the magnetoplasmon resonance. The higher-order harmonics of the resistance oscillation remain around the multiples of the cyclotron resonance frequency. An in situ transmission measurement exhibits an asymmetric broadening of the cyclotron resonance, appearing as a combination of the cyclotron resonance and the magnetoplasmon resonance, but no features directly linked to the microwave induced resistance oscillation can be seen.     

Noncascading THz-wave parametric oscillator synchronously pumped by mode-locked picosecond Ti:sapphire laser in doubly-resonant external cavity

A noncascading terahertz (THz) wave parametric oscillator synchronously pumped by a mode-locked picosecond Ti:sapphire laser whose average power was less than 1 W was demonstrated with a noncollinear phase-matching MgO:LiNbO₃ crystal in an external enhancement cavity doubly resonant for both pump (780 nm) and signal (781-784 nm) waves. In the external cavity, in which the pump wave enhanced so as to reduce the pumping threshold of parametric processes, the signal wave could also resonate and thus be enhanced simultaneously, resulting in a THz wave output at approximately 0.9 THz as the idler wave. The novel dual enhancement of pump and signal waves reduced the threshold pumping intensity to approximately 50 MW/cm², which was much lower than that of a conventional externally pumped THz wave parametric oscillator with a crystal.     

Simultaneous intracavity optical parametric oscillation and stimulated Raman scattering pumped by a doubly passively Q-switched Nd:GGG laser

By using a doubly passively Q-switched Nd:Gd₃Ga₅O₁₂(Nd:GGG) laser with Cr⁴⁺:YAG and GaAs as saturable absorbers as pump laser, simultaneous intracavity optical parametric oscillation and stimulated Raman scattering based on a single X-cut KTiOPO₄ (KTP) crystal have been realized. Under an incident diode pump power of 10.5 W, the output powers at the signal wave near 1,569 nm and the first Stokes emission near 1,094 nm were 218 and 72 mW, corresponding to the optical-to-optical conversion efficiencies of 2.08 and 0.69 %, respectively. The measured shortest pulse duration at the signal wave near 1,569 nm was 580 ps, generating a pulse peak power of 43.7 kW, while the minimum pulse duration at the first Stokes emission near 1,094 nm was 1.61 ns. By adjusting the tilt angle of the KTP crystal, up to the third Stokes scattering was also obtained.     

Laser oscillation by the F3− and F2− color centers in LiF crystal at room temperature

A stable, free-running LiF:F₃ ⁻ and LiF:F₂ ⁻ color center laser oscillation is achieved at room temperature by pumping with the 930-nm laser radiation. The LiF:F₃ ⁻ laser radiation has a peak at 1100 nm and shifts from the peak wavelength of the F₃ ⁻ luminescence band because of the absorption of the F₃ ⁻ luminescence by the F₂ ⁻ center, which co-exists with the F₃ ⁻ center. Received: 2 March 1999 / Revised version: 16 March 1999 / Published online: 12 May 1999     

Near-infrared properties of periodically poled KTiOPO<Subscript>4</Subscript> and stoichiometric MgO-doped LiTaO<Subscript>3</Subscript> crystals for high power optical parametric oscillation with femtosecond pulses

A thorough theoretical analysis of the near-infrared properties of periodically poled KTiOPO₄ (PPKTP) and stoichiometric MgO-doped LiTaO₃ (MgO:PPSLT) crystals for optical parametric oscillation with excitation at 1 μm is presented. To the best of our knowledge, the optical, phasematching, wavelength tuning, and dispersive properties of these crystals for parametric interactions are discussed in detail for the first time. In addition, a new design for high power parametric devices based on PPKTP or MgO:PPSLT crystals with ultrafast Yb-ion laser pump is proposed. The results form a useful reference for the selection of materials and operating conditions for the practical design of high power femtosecond optical parametric oscillators with excitation at 1 μm.     

The effect of parametrically excited spin waves on the dispersion and damping of magnetostatic surface waves in ferrite films

This paper describes an experimental study of variations of the dispersion and damping of magnetostatic surface waves in ferrite films, caused by three-and four-magnon interactions with parametric spin waves excited by an auxiliary surface magnetostatic pump wave with frequency f _p. The variations in the dispersion and damping were identified, respectively, with variations Δk″ in the real part and Δk′ in the imaginary part of the wave number of the surface magnetostatic wave. The Δk″ and Δk′ values were determined from the ratio of the changes of the phase increment Δφ and the amplitude increment ΔA of the surface magnetostatic wave to the length L of the nonequilibrium section of the film, where the parametric spin waves exist. It is found that, when three-magnon decay processes are allowed for the pump wave and the surface magnetostatic probe wave, the probe wave can substantially alter the distribution of the parametric spin waves in the film. Zh. éksp. Teor. Fiz. 115, 318–332 (January 1999)     

Intracavity Raman conversion for 16-μm Stokes pulse generation in para-hydrogen

16-μm Stokes pulses were directly generated for the first time to our knowledge by an intracavity configuration for the para-hydrogen Raman laser. We have analyzed Stokes field growth using a focused gain model and designed a pump/Stokes cavity to satisfy CO₂ pump power and pulse duration requirements for Raman oscillation. The CO₂ laser oscillation with circular polarization was realized by seeding externally circularly polarized CO₂ radiation. An output energy of 2.4 mJ was obtained with the output coupler of 0.5% transmittance, which indicated that 420 mJ of Stokes pulse energy was stored inside the cavity. This suggests that a much higher energy can be extracted by the optimization of cavity parameters. Received: 18 November 1998 / Published online: 26 May 1999     

Numerical analysis of the spatial behaviour of nanosecond optical parametric oscillators of beta-barium borate

We report on a numerical analysis of the temporal and spatial beam properties of nanosecond optical parametric oscillators (OPOs). The analysis is performed for a 355-nm-pumped critically phase-matched OPO of beta-barium borate. The calculations provide detailed information on the dependence of the OPO beam quality (measured by the quality factor M ²) on pump energy. An important result is the strong increase of the M ² value for pump energies exceeding 1–2 times the energy at threshold. Furthermore, a temporal analysis of single OPO pulses indicates that the M ² value strongly increases during the first few nanoseconds of the OPO oscillation. This increase is understood by considering the temporal dynamics of the spatial profiles of the OPO signal beam and the depleted pump radiation. Received: 1 April 1999 / Revised version: 26 July 1999 / Published online: 20 October 1999     

Critical Coupling Constants and Eigenvalue Asymptotics of Perturbed Periodic Sturm–Liouville Operators

Perturbations of asymptotic decay c/r ² arise in the partial-wave analysis of rotationally symmetric partial differential operators. We show that for each end-point λ₀ of the spectral bands of a perturbed periodic Sturm–Liouville operator, there is a critical coupling constant c _crit such that eigenvalues in the spectral gap accumulate at λ₀ if and only if c/c _crit>1. The oscillation theoretic method used in the proof also yields the asymptotic distribution of the eigenvalues near λ₀. Received: 23 September 1999 / Accepted: 21 December 1999     

Structural, electrical, and surface characteristics of La0.5Sr0.5CoO3 thin films prepared by pulsed-laser deposition

A parametric study of the growth of La_0.5Sr_0.5CoO₃ (LSCO) thin films on (100) MgO substrates by pulsed-laser deposition (PLD) is reported. Films are grown under a wide range of substrate temperature (450–800 °C), oxygen pressure (0.1–0.9 mbar), and incident laser fluence (0.8–2.6 J/cm²). The optimum ranges of temperature, oxygen pressure, and laser fluence to produce c-axis oriented films with smooth surface morphology and high metallic conductivity are identified. Films deposited at low temperature (500 °C) and post-annealed in situ at higher temperatures (600–800 °C) are also investigated with respect to their structure, surface morphology, and electrical conductivity. Received: 20 November 1998 / Accepted: 6 July 1999 / Published online: 21 October 1999