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1.
The expressions for the energy spectra of monolayer, bilayer, and multilayer graphene, as well as epitaxial graphene, are derived using the quantum Green’s functions method. Analytic expressions are obtained for the densities of states of these systems. It is shown that a bandgap can appear the spectrum of an epitaxial graphene bilayer. A number of problems in the thermodynamics of electrons in free and epitaxial graphene layers are considered as applications. Analytic expressions are obtained for the chemical potential and heat capacity in the limiting cases of low and high temperatures. Quantum oscillations of heat capacity in graphene are analyzed taking into account the Coulomb interaction. The Berry phase of epitaxial graphene is investigated.  相似文献   

2.
Quantum magnetic oscillations of the density of states of a weakly doped graphene bilayer in the presence of a voltage on the gate have been studied. It has been shown that there are additional peaks in the spectrum of oscillations, when the chemical potential is located in the region of the inverted (owing to the voltage on the gate) part of the energy spectrum. Owing to the inverted band structure, quantum oscillations also exist in undoped graphene, when the chemical potential is inside the band gap. A clear physical interpretation of the results is given.  相似文献   

3.
The phenomenon of Rabi oscillations far from resonance is described in bilayer and few-layer graphene. These oscillations in the population and polarization at the Dirac point in n-layer graphene are seen in the nth harmonic term in the external driving frequency. The underlying reason behind these oscillations is attributable to the pseudospin degree of freedom possessed by all these systems. Conventional Rabi oscillations, which occur only near resonance, are seen in multiple harmonics in multilayer graphene. However, the experimentally measurable current density exhibits anomalous behaviour only in the first harmonic in all the graphene systems. A fully numerical solution of the optical Bloch equations is in complete agreement with the analytical results, thereby justifying the approximation schemes used in the latter. The same phenomena are also described in twisted bilayer graphene with and without an electric potential difference between the layers. It is found that the anomalous Rabi frequency is strongly dependent on twist angle for weak applied fields – a feature absent in single-layer graphene, whereas the conventional Rabi frequency is relatively independent of the twist angle.  相似文献   

4.
We study dynamical thermal conductivity of doped biased bilayer graphene for both AA and AB-stacking in the context of tight binding model Hamiltonian. The effects of bias voltage and chemical potential on the behavior of dynamical thermal conductivity are discussed for different stacking of bilayer graphene. Green's function approach has been implemented to find the behavior of thermal conductivity of bilayer graphene within linear response theory. We have found that thermal conductivity decreases with chemical potential for different values of temperature and frequency. Also thermal conductivity of AB stacked bilayer graphene versus bias voltage includes a peak for each value of chemical potential. Furthermore we study the frequency dependence of thermal conductivity of AA stacked bilayer graphene for different values of temperature and bias voltage.  相似文献   

5.
储开龙  王孜博  周娇娇  江华 《中国物理 B》2017,26(6):67202-067202
The transport study of graphene based junctions has become one of the focuses in graphene research. There are two stacking configurations for monolayer–bilayer–monolayer graphene planar junctions. One is the two monolayer graphene contacting the same side of the bilayer graphene, and the other is the two-monolayer graphene contacting the different layers of the bilayer graphene. In this paper, according to the Landauer–Büttiker formula, we study the transport properties of these two configurations. The influences of the local gate potential in each part, the bias potential in bilayer graphene,the disorder and external magnetic field on conductance are obtained. We find the conductances of the two configurations can be manipulated by all of these effects. Especially, one can distinguish the two stacking configurations by introducing the bias potential into the bilayer graphene. The strong disorder and the external magnetic field will make the two stacking configurations indistinguishable in the transport experiment.  相似文献   

6.
We use the T-matrix approximation to analyze the effect of a localized impurity on the local density of states in monolayer and bilayer graphene. For monolayer graphene the Friedel oscillations generated by intranodal scattering obey an inverse-square law, while the internodal ones obey an inverse law. In the Fourier transform this translates into a filled circle of high intensity in the center of the Brillouin zone, and empty circular contours around its corners. For bilayer graphene both types of oscillations obey an inverse law.  相似文献   

7.
赵小明  吴亚杰  陈婵  梁颖  寇谡鹏 《中国物理 B》2016,25(11):117303-117303
In this paper,we study the quantum properties of a bilayer graphene with(asymmetry) line defects.The localized states are found around the line defects.Thus,the line defects on one certain layer of the bilayer graphene can lead to an electric transport channel.By adding a bias potential along the direction of the line defects,we calculate the electric conductivity of bilayer graphene with line defects using the Landauer-Biittiker theory,and show that the channel affects the electric conductivity remarkably by comparing the results with those in a perfect bilayer graphene.This one-dimensional line electric channel has the potential to be applied in nanotechnology engineering.  相似文献   

8.
We studied and compared the transport properties of charge carriers in bilayer graphene, monolayer graphene, and the conventional semiconductors (the two-dimensional electron gas (2DEG)). It is elucidated that the normal incidence transmission in the bilayer graphene is identical to that in the 2DEG but totally different from that in the monolayer graphene. However, resonant peaks appear in the non-normal incidence transmission profile for a high barrier in the bilayer graphene, which do not occur in the 2DEG. Furthermore, there are tunneling and forbidden regions in the transmission spectrum for each material, and the division of the two regions has been given in the work. The tunneling region covers a wide range of the incident energy for the two graphene systems, but only exists under specific conditions for the 2DEG. The counterparts of the transmission in the conductance profile are also given for the three materials, which may be used as high-performance devices based on the bilayer graphene.  相似文献   

9.
Monolayer and bilayer graphenes have generated tremendous excitement as the potentially useful electronic materials due to their unique features.We report on monolayer and bilayer epitaxial graphene field-effect transistors(GFETs)fabricated on SiC substrates.Compared with monolayer GFETs,the bilayer GFETs exhibit a significant improvement in dc characteristics,including increasing current density Ids,improved transconductance g_m,reduced sheet resistance R_(on),and current saturation.The improved electrical properties and tunable bandgap in the bilayer graphene lead to the excellent dc performance of the bilayer GFETs.Furthermore,the improved dc characteristics enhance a better rf performance for bilayer graphene devices,demonstrating that the quasifree-standing bilayer graphene on SiC substrates has a great application potential for the future graphene-based electronics.  相似文献   

10.
Various physical properties of epitaxial graphene grown on SiC(0001) are studied. First, the electronic transport in epitaxial bilayer graphene on SiC(0001) and quasi-free-standing bilayer graphene on SiC(0001) is investigated. The dependences of the resistance and the polarity of the Hall resistance at zero gate voltage on the top-gate voltage show that the carrier types are electron and hole, respectively. The mobility evaluated at various carrier densities indicates that the quasi-free-standing bilayer graphene shows higher mobility than the epitaxial bilayer graphene when they are compared at the same carrier density. The difference in mobility is thought to come from the domain size of the graphene sheet formed. To clarify a guiding principle for controlling graphene quality, the mechanism of epitaxial graphene growth is also studied theoretically. It is found that a new graphene sheet grows from the interface between the old graphene sheets and the SiC substrate. Further studies on the energetics reveal the importance of the role of the step on the SiC surface. A first-principles calculation unequivocally shows that the C prefers to release from the step edge and to aggregate as graphene nuclei along the step edge rather than be left on the terrace. It is also shown that the edges of the existing graphene more preferentially absorb the isolated C atoms. For some annealing conditions, experiments can also provide graphene islands on SiC(0001) surfaces. The atomic structures are studied theoretically together with their growth mechanism. The proposed embedded island structures actually act as a graphene island electronically, and those with zigzag edges have a magnetoelectric effect. Finally, the thermoelectric properties of graphene are theoretically examined. The results indicate that reducing the carrier scattering suppresses the thermoelectric power and enhances the thermoelectric figure of merit. The fine control of the Fermi energy position is thought to be key for the practical use of graphene as a thermoelectric material, which could be achieved with epitaxial graphene. All of these results reveal that epitaxial graphene is physically interesting.  相似文献   

11.
LING-FENG MAO 《Pramana》2013,81(2):309-317
The quantum capacitance, an important parameter in the design of nanoscale devices, is derived for armchair-edge single-layer graphene nanoribbon with semiconducting property. The quantum capacitance oscillations are found and these capacitance oscillations originate from the lateral quantum confinement in graphene nanoribbon. Detailed studies of the capacitance oscillations demonstrate that the local channel electrostatic potential at the capacitance peak, the height and the number of the capacitance peak strongly depend on the width, especially a few nanometres, of the armchair-edge graphene nanoribbon. It implies that the capacitance oscillations observed in the experiments can be utilized to measure the width of graphene nanoribbon. The results also show that the capacitance oscillations are not seen when the width is larger than 30 nm.  相似文献   

12.
The hybrid graphene-quantum dot devices can potentially be used to tailor the electronic, optical, and chemical properties of graphene. Here, the low temperature electronic transport properties of bilayer graphene decorated with PbS colloid quantum dots(CQDs) have been investigated in the weak or strong magnetic fields. The presence of the CQDs introduces additional scattering potentials that alter the magnetotransport properties of the graphene layers, leading to the observation of a new set of magnetoconductance oscillations near zero magnetic field as well as the high-field quantum Hall regime.The results bring about a new strategy for exploring the quantum interference effects in two-dimensional materials which are sensitive to the surrounding electrostatic environment, and open up a new gateway for exploring the graphene sensing with quantum interference effects.  相似文献   

13.
Multi-band pairing of effectively ultrarelativistic electrons and holes in asymmetrically biased graphene bilayer in strong coupling regime is considered. In this regime, the pairing affects both conduction and valence bands of the both graphene layers, and the order parameter is a matrix, which indices correspond to the bands. For band-diagonal s-wave pairing, we derive the system of multi-band gap equations for the gaps in the valence and conduction bands and solve it in the approximation of constant gaps and in the approximation of separable pairing potential. For a characteristic width of the pairing region of order of magnitude of the chemical potential, the gap values are not much different from single-band BCS estimations. However, if the pairing region is wider, then the gaps can be much larger and depend exponentially on its energy width. We also predict gapped and soliton-like oscillations of a relative phase of the gaps and unpairing of quarter-vortices at Kosterlitz-Thouless transition.  相似文献   

14.
In-plane elastic instability of bilayer graphene sheets is investigated using atomistic finite element approaches. The equivalent homogenised properties of graphene sheet are expressed in terms of the thickness, equilibrium lengths and force-field models used to represent the C–C bonds of the graphene lattice. The covalent bonds are represented as structural beams with stretching, bending, torsional and shear deformation, and the strain energies associated to affine deformation mechanisms. The overall mechanical properties and geometric configurations of the nano-structures represented as truss assemblies are then calculated minimising the total potential energy associated to the loading, thickness and average equilibrium lengths of the bonds. Different boundary conditions and aspect ratios are considered for both bilayer and single-layer graphene sheets. The bilayer graphene sheets are found to be offering remarkably higher buckling strengths as compared to single-layer sheets.  相似文献   

15.
We calculate the plasmon frequency and damping rate in a 3-layer graphene system made of parallel monolayer and bilayer graphene sheets using the random-phase-approximation dielectric function and taking into account the inhomogeneity of the dielectric background of the system. Numerical results show that two out-of-phase acoustic and one in-phase optical plasmon modes can be found from the zeroes of dynamical dielectric function of the structure. Plasmon frequencies and damping rate of plasma oscillations depend significantly on the inhomogeneity of environment, so plasmon curves become more distinctive from each other in single-particle excitation region, compared to the case of homogeneous medium. Finally, Plasmon dispersion patterns depend remarkably on the number (but not order) of bilayer graphene sheet constructing to the system.  相似文献   

16.
This study reports the Raman analysis of bilayer graphene films prepared on commercial dilute Cu(0.5 at% Ni) foils using atmospheric pressure chemical vapor deposition. A bilayer graphene film obtained on Cu foil is known to have small areas of bilayer (islands) with a significant fraction of non‐Bernal stacking, while that obtained on Cu/Ni is known to grow over a large area with Bernal stacking. In the Raman optical microscope images, a wafer‐scale monolayer and large‐area bilayer graphene films were distinguished and confirmed with Raman spectra intensities ratios of 2D to G peaks. The large‐area part of bilayer graphene film obtained was assisted by Ni surface segregation because Ni has higher methane decomposition rate and carbon solubility compared with Cu. The Raman data suggest a Bernal stacking order in the prepared bilayer graphene film. A four‐point probe sheet resistance of graphene films confirmed a bilayer graphene film sheet resistance distinguished from that of monolayer graphene. A relatively higher Ni surface concentration in Cu(0.5 at% Ni) foil was confirmed with time‐of‐flight secondary ion mass spectrometry. The inhomogeneous distribution of Ni in a foil and the diverse crystallographic surface of a foil (confirmed with proton‐induced X‐ray emission and electron backscatter diffraction, respectively) could be a reason for incomplete wafer‐scale bilayer graphene film. The Ni surface segregation in dilute Cu(0.5 at% Ni) foil has a potential to impact on atmospheric pressure chemical vapor deposition growth of large‐area bilayer graphene film. Copyright © 2015 John Wiley & Sons, Ltd.  相似文献   

17.
林奎鑫  李多生  叶寅  江五贵  叶志国  Qinghua Qin  邹伟 《物理学报》2018,67(24):246802-246802
石墨烯是一种准二维蜂窝网状结构新型纳米材料,石墨烯的层数和构型对其性能产生重要影响.固体中准粒子的量子状态由其本身的对称性质所决定,扭转双层石墨烯打破了对称性,引起了强烈的层间耦合作用,改变了扭转双层石墨烯的电子能带、声子色散、形成能垒等物性,产生了独特的性能,如可以连续调控带隙0-250 meV,光电效应的响应度相比于单层石墨烯提高了80倍,因此对扭转双层石墨烯功能化研究有重大意义.本文同时还论述了扭转双层石墨烯向类金刚石转变的理论与实验研究进展,发现扭转双层石墨烯呈现出具有类金刚石结构与性能特征.进一步阐述调控扭转双层石墨烯的扭转角度对其内在性能的影响,揭示这种新型纳米结构在原子层次的行为特征.最后介绍了如何调控制备扭转双层石墨,分析其调控机理,讨论了各种制备工艺的不足与发展趋势.因此本文从扭转双层石墨烯的输运性质、晶体结构转变、制备三个方面展开阐述,并对其在先进电子器件领域的潜在应用进行了展望.  相似文献   

18.
Due to its many superior properties, bilayer graphene is expected to serve as a proper candidate in various applications, and further provokes intensive research on how it deforms. Based on atomistic simulations, the elastic behavior of bilayer graphenes, including fracture under tension and buckling under compression, is investigated under in-plane loadings. The elastic property, e.g. Young's modulus and fracture strain, of either armchair or zigzag graphene is sensitive to both chirality and loading direction when tension is applied. However, the armchair-zigzag bilayer graphene with mixed chirality has no dependency on loading direction and its tensile rupture process is in a step-by-step manner. Under different loading histories, the bilayer graphene also exhibits quite different mechanical response. These results are useful for both further investigation and potential application of graphene in nano-electromechanical systems.  相似文献   

19.
伞晓娇  韩柏  赵景庚 《中国物理 B》2016,25(3):37305-037305
We have studied the structural and optical properties of semi-fluorinated bilayer graphene using density functional theory. When the interlayer distance is 1.62 , the two graphene layers in AA stacking can form strong chemical bonds.Under an in-plane stress of 6.8 GPa, this semi-fluorinated bilayer graphene becomes the energy minimum. Our calculations indicate that the semi-fluorinated bilayer graphene with the AA stacking sequence and rectangular fluorinated configuration is a nonmagnetic semiconductor(direct gap of 3.46 e V). The electronic behavior at the vicinity of the Fermi level is mainly contributed by the p electrons of carbon atoms forming C=C double bonds. We compare the optical properties of the semifluorinated bilayer graphene with those of bilayer graphene stacked in the AA sequence and find that the semi-fluorinated bilayer graphene is anisotropic for the polarization vector on the basal plane of graphene and a red shift occurs in the [010]polarization, which makes the peak at the low-frequency region located within visible light. This investigation is useful to design polarization-dependence optoelectronic devices.  相似文献   

20.
惠治鑫  贺鹏飞  戴瑛  吴艾辉 《物理学报》2014,63(7):74401-074401
采用Tersoff势函数与Lennard-Jones势函数,结合速度形式的Verlet算法和Fourier定律,对单层和两层硅功能化石墨烯沿长度方向的导热性能进行了正向非平衡态分子动力学模拟.通过模拟发现,硅原子的加入改变了石墨烯声子的模式、平均自由程和移动速度,使得单层硅功能化石墨烯模型的热导率随着硅原子数目的增加而急剧地减小.在300 K至1000 K温度变化范围内,单层硅功能化石墨烯的热导率呈下降趋势,具有明显的温度效应.对双层硅功能化石墨烯而言,少量的硅原子嵌入,起到了提高热导率的作用,但当硅原子数目达到一定数量后,材料的导热性能下降.  相似文献   

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