Kondo-peak splitting and coherent transport in a single-electron transistor

The peculiar behavior of Kondo-peak splitting under a magnetic field and bias can be explained by calculating the nonequilibrium retarded Green's function via the nonperturbative dynamical theory (NDT). In the NDT, the application of a lead-dot-lead system reveals that new resonant tunneling levels are activated near the Fermi level and the conventional Kondo peak at the Fermi level diminishes when a bias is applied. Magnetic field causes asymmetry in the spectral density and transforms the new resonant peak into a major peak whose behavior explains all the features of the nonequilibrium Kondo phenomenon. We also show the mechanism of coherent transport through the new resonant tunneling level.     

Kondo effect in a deformed molecule coupled asymmetrically to ferromagnetic electrodes

The nonequilibrium Kondo effect is studied in a molecule quantum dot coupled asymmetrically to two ferromagnetic electrodes by employing the nonequilibrium Green function technique. The current-induced deformation of the molecule is taken into account, modeled as interactions with a phonon system, and phonon-assisted Kondo satellites arise on both sides of the usual main Kondo peak. In the antiparallel electrode configuration, the Kondo satellites can be split only for the asymmetric dot-lead couplings, distinguished from the parallel configuration where splitting also exists, even though it is for symmetric case. We also analyze how to compensate the splitting and restore the suppressed zero-bias Kondo resonance. It is shown that one can change the TMR ratio significantly from a negative dip to a positive peak only by slightly modulating a local external magnetic field, whose value is greatly dependent on the electron--phonon coupling strength.     

Density of states of a strongly correlated quantum dot coupled to Luttinger liquid leads

We theoretically investigate the density of states (DOS) of a quantum dot weakly coupled to Luttinger liquid (LL) leads in the Kondo regime by use of the equation-of-motion technique of the nonequilibrium Green functions. At zero temperature, the Kondo peak in DOS is suppressed by the intralead interaction. When the LL interaction parameter K   is about 0.77, a moderately strong interaction, the Kondo peak disappears and then a dip develops, a signature of the intermediate two-channel Kondo (2CK) physics. This shows that the condition for the 2CK to occur ever addressed is not necessary. Applying a finite voltage bias splits the dip in the DOS. Each split dip is located at the chemical potential of a LL lead. This again appears the stabilized 2CK physics for moderately strong interaction K<1$K<1$.     

Universal scaling in nonequilibrium transport through a single channel Kondo dot

Scaling laws and universality play an important role in our understanding of critical phenomena and the Kondo effect. We present measurements of nonequilibrium transport through a single-channel Kondo quantum dot at low temperature and bias. We find that the low-energy Kondo conductance is consistent with universality between temperature and bias and is characterized by a quadratic scaling exponent, as expected for the spin-1/2 Kondo effect. We show that the nonequilibrium Kondo transport measurements are well described by a universal scaling function with two scaling parameters.     

Splitting and Restoration of Kondo Peak in a Deformed Molecule Quantum Dot Coupled to Ferromagnetic Electrodes

We adopt the nonequilibrium Green＇s function method to theoretically study the Kondo effect in a deformed molecule, which is treated as an electron-phonon interaction （EPI） system. The self-energy for phonon part is calculated in the standard many-body diagrammatic expansion up to the second order in EPI strength. We find that the multiple phonon-assisted Kondo satellites arise besides the usual Kondo resonance. In the antiparallel magnetic configuration the splitting of main Kondo peak and phonon-assisted satellites only happen for asymmetrical dot-lead couplings, but it is free from the symmetry for the parallel magnetic configuration. The EPI strength and vibrational frequency can enhance the spin splitting of both main Kondo and satellites. It is shown that the suppressed zero-bias Kondo resonance can be restored by applying an external magnetic field, whose magnitude is dependent on the phononic effect remarkably. Although the asymmetry in tunnel coupling has no contribution to the restoration of spin splitting of Kondo peak, it can shrink the external field needed to switch tunneling magnetoresistance ratio between large negative dip and large positive peak.     

Thermoelectric Phenomena in a Quantum Dot Attached to Ferromagnetic Leads in Kondo Regime

We have studied the thermoelectric properties through ferromagnetic leads-QD coupled system (F-QD-F) in the Kondo regime by nonequilibrium Green's functions method. The spin-flip effect induced by ferromagnetic leads and Kondo effect influence the thermoelectric properties significantly. The peak-valley structure emerges at the low temperature due to Kondo resonance, and the peak-valley structure also relies on the polarization angle θ, the spin-dependent linewidth function Γ_γσ and the energy level of QD ε_d. Novel resonant peak also emerges in the curve of ZT_c versus polarization angle θ. The Kondo effect suppresses the figure of merit ZT_c and the spin-dependent figure of merit ZT_s. In addition, the spin-dependent figure of merit ZT_s is relate with the gap between Γ_γ↑ and Γ_γ↓.     

Nonequilibrium Shot Noise Spectrum Through a Quantum Dot in the Kondo Regime:A Master Equation Approach under Self-Consistent Born Approximation

We construct a number(n)-resolved master equation(ME)approach under self-consistent Born approximation(SCBA)for noise spectrum calculation.The formulation is essentially non-Markovian and incorporates properly the interlay of the multi-tunneling processes and many-body correlations.We apply this approach to the challenging nonequilibrium Kondo system and predict a profound nonequilibrium Kondo signature in the shot noise spectrum.The proposed n-SCBA-ME scheme goes completely beyond the scope of the Born-Markovian master equation approach,in the sense of being applicable to the shot noise of transport under small bias voltage,in non-Markovian regime,and with strong Coulomb correlations as favorably demonstrated in the nonequilibrium Kondo system.     

Giant charge relaxation resistance in the Anderson model

We investigate the dynamical charge response of the Anderson model viewed as a quantum RC circuit. Applying a low-energy effective Fermi liquid theory, a generalized Korringa-Shiba formula is derived at zero temperature, and the charge relaxation resistance is expressed solely in terms of static susceptibilities which are accessible by Bethe ansatz. We identify a giant charge relaxation resistance at intermediate magnetic fields related to the destruction of the Kondo singlet. The scaling properties of this peak are computed analytically in the Kondo regime. We also show that the resistance peak fades away at the particle-hole symmetric point.     

Mediation of long range charge transfer by Kondo bound States

We present a theory of nonequilibrium long range charge transfer between donor and acceptor centers in a model polymer mediated by magnetic exciton (Kondo) bound states. Our model produces electron tunneling lengths easily exceeding 10 A, as observed recently in DNA and organic charge transfer systems. This long ranged tunneling is effective for weak to intermediate donor-bridge coupling, and is enhanced both by weak to intermediate strength Coulomb hole-electron attraction (through the orthogonality catastrophe) and by coupling to local vibrational modes.     

Out-of-equilibrium Kondo effect in a mesoscopic device

We study the nonequilibrium regime of the Kondo effect in a quantum dot laterally coupled to a narrow wire. We observe a split Kondo resonance when a finite bias voltage is imposed across the wire. The splitting is attributed to the creation of a double-step Fermi distribution function in the wire. Kondo correlations are strongly suppressed when the voltage across the wire exceeds the Kondo temperature. A perpendicular magnetic field enables us to selectively control the coupling between the dot and the two Fermi seas in the wire. Already at fields of order 0.1 T only the Kondo resonance associated with the strongly coupled reservoir survives.     

Nonequilibrium Kondo effect and Andreev reflection through double quantum dots with spin-flip scattering

The Kondo effect and the Andreev reflection tunneling through a normal (ferromagnet)-double quantum dots-superconductor hybrid system is examined in the low temperature by using the nonequilibrium Green's function technique in combination with the slave-boson mean-field theory. The interplay of the Kondo physics and the Andreev bound state physics can be controlled by varying the interdot hopping strength. The Andreev differential conductance is mainly determined by the competition between Kondo states and Andreev states. The spin-polarization of the ferromagnetic electrode increases the zero-bias Kondo peak. The spin-flip scattering influences the Kondo effect and the Andreev reflection in a nontrivial way. For the ferromagnetic electrode with sufficiently large spin polarization, the negative Andreev differential conductance is found when the spin flip strength in the double quantum dots is sufficiently strong.     

Evolution of the Kondo effect in a quantum dot probed by shot noise

We measure the current and shot noise in a quantum dot in the Kondo regime to address the nonequilibrium properties of the Kondo effect. By systematically tuning the temperature and gate voltages to define the level positions in the quantum dot, we observe an enhancement of the shot noise as temperature decreases below the Kondo temperature, which indicates that the two-particle scattering process grows as the Kondo state evolves. Below the Kondo temperature, the Fano factor defined at finite temperature is found to exceed the expected value of unity from the noninteracting model, reaching 1.8±0.2.     

Violation of the Fluctuation-Dissipation Theorem and Heating Effects in the Time-Dependent Kondo Model

The fluctuation-dissipation theorem (FDT) plays a fundamental role in understanding quantum many-body problems. However, its applicability is limited to equilibrium systems and it does in general not hold in nonequilibrium situations. This violation of the FDT is an important tool for studying nonequilibrium physics. In this paper we present results for the violation of the FDT in the Kondo model where the impurity spin is frozen for all negative times, and set free to relax at positive times. We derive exact analytical results at the Toulouse point, and results within a controlled approximation in the Kondo limit, which allow us to study the FDT violation on all time scales. A measure of the FDT violation is provided by the effective temperature, which shows initial heating effects after switching on the perturbation, and then exponential cooling to zero temperature as the Kondo system reaches equilibrium.     

Measurement of quantum noise in a carbon nanotube quantum dot in the Kondo regime

The current emission noise of a carbon nanotube quantum dot in the Kondo regime is measured at frequencies ν of the order or higher than the frequency associated with the Kondo effect k(B)T (K)/h, with TK the Kondo temperature. The carbon nanotube is coupled via an on-chip resonant circuit to a quantum noise detector, a superconductor-insulator-superconductor junction. We find for hν ≈ k(B)T(K) a Kondo effect related singularity at a voltage bias eV ≈ hν, and a strong reduction of this singularity for hν ≈ 3k(B)T(K), in good agreement with theory. Our experiment constitutes a new original tool for the investigation of the nonequilibrium dynamics of many-body phenomena in nanoscale devices.     

SU(4) Kondo effect in carbon nanotubes

We investigate theoretically the nonequilibrium transport properties of carbon nanotube quantum dots. Owing to the two-dimensional band structure of graphene, a double orbital degeneracy plays the role of a pseudospin, which is entangled with the spin. Quantum fluctuations between these 4 degrees of freedom result in an SU(4) Kondo effect at low temperatures. This exotic Kondo effect manifests as a four-peak splitting in the nonlinear conductance when an axial magnetic field is applied.     

Spin-flip Fano–Kondo resonant tunneling through a quantum dot interferometer responded by a rotating magnetic field

The Fano and Kondo cooperated resonant tunneling through a quantum dot interferometer under the perturbation of a rotating magnetic field is investigated theoretically. The spin-polarized current components have been derived generally by employing the Keldysh nonequilibrium Green?s function method, through which the charge and spin currents are determined directly. The numerical calculations on spin and charge currents are performed to show the compound features of mesoscopic transport associated with the Kondo, Fano, and Zeeman effects intimately. The induced spin current in the Kondo regime is much different from the one in the non-interacting regime. The spin current is tuned from resonant peak to valley by varying external parameters.     

Scaling and decoherence in the nonequilibrium Kondo model

We study the Kondo effect in quantum dots in an out-of-equilibrium state due to an applied dc-voltage bias. Using the method of infinitesimal unitary transformations ("flow equations"), we develop a perturbative scaling picture that naturally contains both equilibrium coherence and nonequilibrium decoherence effects. This framework allows one to study the competition between Kondo effect and current-induced decoherence, and it establishes a large regime dominated by single-channel Kondo physics for asymmetrically coupled quantum dots.     

Transition from the Kondo effect to a Coulomb blockade in an electron shuttle

We investigate the effect of the mechanical motion of a quantum dot on the transport properties of a quantum dot shuttle.Employing the equation of motion method for the nonequilibrium Green’s function,we show that the oscillation of the dot,i.e.,the time-dependent coupling between the dot’s electron and the reservoirs,can destroy the Kondo effect.With the increase in the oscillation frequency of the dot,the density of states of the quantum dot shuttle changes from the Kondo-like to a Coulomb-blockade pattern.Increasing the coupling between the dot and the electrodes may partly recover the Kondo peak in the spectrum of the density of states.Understanding of the effect of mechanical motion on the transport properties of an electron shuttle is important for the future application of nanoelectromechanical devices.     

Full counting statistics for the Kondo dot

The generating function for the cumulants of charge current distribution is calculated for two generalized Majorana resonant level models: the Kondo dot at the Toulouse point and the resonant level embedded in a Luttinger liquid with the interaction parameter g=1/2. We find that the low-temperature nonequilibrium transport in the Kondo case occurs via tunneling of physical electrons as well as by coherent transmission of electron pairs. We calculate the third cumulant ("skewness") explicitly and analyze it for different couplings, temperatures, and magnetic fields. For the g=1/2 setup the statistics simplifies and is given by a modified version of the Levitov-Lesovik formula.