二维GaAs 基光子晶体微腔的制作与光谱特性分析

研究了以InAs量子点为有源区的二维GaAs基光子晶体微腔的设计与制作,测试并分析了室温下微腔的光谱特性.观察到了波长约为1137 nm,谱线半高宽度约为1 nm的尖锐低阶谐振模式发光峰.我们比较了不同刻蚀条件下光子晶体微腔的发光谱线,结果表明空气孔洞截面的垂直度是影响光子晶体微腔发光特性的重要因素之一.通过调节干法刻蚀工艺,改变空气孔半径与晶格常数的比率,可以在较大范围内调节谐振模式发光峰位置,达到谐振模式与量子点发光峰调谐的目的.     

Single photon sources with single semiconductor quantum dots

In t.his contribution, we briefly recall the basic concepts of quantum optics and properties of semicon- ductor quantum clot. （QD） which a.re necessary to the nnderstanding of the physics of single-photon generation with single QDs. Firstly, we address the theory of quantmn emitter-cavity system, the fluorescence and optical properties of semiconductor QDs, and the photon statistics as well as opti- cal properties of the QDs. We then review the localizatioll of single semiconductor QDs in quantum confined optical microcavity systems to achieve their overall optical properties and perfornances in terms of strong coupling regime, elfieiency, directionality, and polarization control. Furthermore, we will discuss the recenl, progress on the fabrication of single photon sources, and various a.pproaehes for embedding single QDs into mieroca,vities or photonic crystal nanoeavities and show how to ex- tend the wavelength range. We focus in part;icular on new generations of electrically driven QD single photon source leading to high repetition rates, efficiencies at elevated temperature operation. Besides strong eoupling regime, and high collection new development;s of room temperature sin- gle photon emission in the strong coupling regime are reviewed. The generation of indistinguishable photons and remaining challenges for pract ical single-photon sources are also discussed.     

InAs/GaAs量子点1.3 μm单光子发射特性

采用双层耦合量子点的分子束外延生长技术生长了InAs/GaAs量子点样品,把量子点的发光波长成功地拓展到1.3 μm.采用光刻的工艺制备了直径为3 μm的柱状微腔,提高了量子点荧光的提取效率.在低温5 K下,测量得到量子点激子的荧光寿命约为1 ns;单量子点荧光二阶关联函数为0.015,显示单量子点荧光具有非常好的单光子特性;利用迈克耳孙干涉装置测量得到单光子的相干时间为22 ps,对应的谱线半高全宽度为30 μeV,且荧光谱线的线型为非均匀展宽的高斯线型.     

Positioning photonic crystal cavities to single InAs quantum dots

We have investigated the optical properties of planar photonic crystal cavities formed by removing a single hole from a two-dimensional square lattice of air holes etched through a thin GaAs slab. We have demonstrated cavity resonances with quality factors (Q’s) as high as 8500, using an internal light source provided by an ensemble of InAs quantum dots (QDs) grown by molecular beam epitaxy (MBE). The high-Q modes are confined to a very small mode volume, V = 0.7(λ/n)³, making them attractive to study in the context of cavity quantum electrodynamics with single QDs, where a high is needed to observe the strong coupling between an electronic state of the dot and the optical cavity mode. To this end, we have developed an accurate and robust alignment technique that positions a photonic crystal cavity to a single QD with 25 nm resolution. We present the details of this new technology and demonstrate its effectiveness by strategically positioning a number of QDs within photonic crystal cavities at points where the electric field intensity is high.     

偶极子位置及偏振对激发光子晶体H1微腔的影响

光子晶体微腔和量子点的集成是实现量子信息处理非常具有潜力的平台之一,利用微腔和量子点的耦合可以制备纠缠光子对,实现对量子态的操控.因为光子晶体微腔具有品质因子高、模场体积小等优点,可以极大地增强光与物质之间的相互作用,从而易于实现量子态在不同物理体系之间的转换.通过单量子点和光子晶体H1微腔的耦合可以产生纠缠光子对,因为H1微腔具有简并的、模式偏振正交的基态模式.通常微腔模式的激发随着量子点在微腔中的位置变化而改变,本文用时域有限差分方法研究了偶极子光源的位置及偏振对激发光子晶体H1微腔模式的影响.结果表明:通过改变偶极子光源位置可以选择性地激发H1微腔简并模式中的一个;具有某一偏振的偶极子光源只能激发相应偏振的微腔模式;模式激发强度的大小也是由偶极子光源在微腔中的位置决定的.鉴于目前量子点在微腔中的位置尚不能精确控制,所以微腔模式受激发光源位置的影响的研究具有重要意义.     

光子晶体在半导体激光器中的应用

激光的发明，将人类带入光通信、光存储、光显示的高科技文明中，随着高科技的不断发展、进步和应用范围的不断扩大，对激光的要求更高，例如低阈值、高效率、高亮度、高速、小体积、好的模式特性等，这些要求在现有的传统激光器理论及技术中是难以达到的。但是当人们将光子晶体的理论与现有激光物理和技术相结合时，则有望突破传统激光器的性能瓶颈。例如，提高自发辐射速率，同时获得更高的自发辐射向受激辐射的耦合效率，实现激光器的无阈值工作；利用光子晶体对光子态的调制作用，可以获得比传统激光器大几个数量级的光学腔品质因子，大幅度提高激光的亮度、单色性；结合光子晶体微腔及其显著增加的光学腔品质因子，可以提高激光器的调制速率等，因此，人们预期光子晶体科学与技术将成为未来光电子领域发展的核心之一。文章介绍了光子晶体在半导体激光器中的应用，指出光子晶体科学技术引入发展了几十年的半导体激光器中，使半导体激光器展现出更加优异的性能。最后文章作者展望了光子晶体激光器的未来发展和应用的方向。     

Modified spontaneous emission of CdTe quantum dots inside a photonic crystal

The angular dependence of the spontaneous emission of CdTe quantum dots (QDs) inside a photonic crystal with a pseudogap is reported. The sensitive dependences of the radiative lifetime and the photoluminescence spectrum of CdTe QDs on the observation angle demonstrate the effect of the photonic bandgap on the spontaneous emission of the QDs.     

非线性光子晶体中原子辐射光场的非经典性质

讨论了非线性光子晶体微腔中二能级原子在相干场驱动下腔场的频谱特性及光子的统计性质.研究结果表明,当光子晶体的态密度很大时,如果腔场模与原子共振荧光Mollow峰的中心峰共振,则腔场的涨落压缩到量子散弹噪声之下,且与线性光子晶体微腔的情况相比其谱线峰值变大.当驱动场频率较大时光子服从亚Poisson分布,且非常接近Poisson分布. 关键词： 光子晶体 参量振荡 非弹性谱 二阶相关函数     

非线性光子晶体中原子辐射光场的非经典性质

讨论了非线性光子晶体微腔中二能级原子在相干场驱动下腔场的频谱特性及光子的统计性质.研究结果表明,当光子晶体的态密度很大时,如果腔场模与原子共振荧光Mollow峰的中心峰共振,则腔场的涨落压缩到量子散弹噪声之下,且与线性光子晶体微腔的情况相比其谱线峰值变大.当驱动场频率较大时光子服从亚Poisson分布,且非常接近Poisson分布.     

Advances in quantum dots for classical and non-classical light sources Invited Paper

Recent advances in quantum dots (QDs) for classical and non-classical light sources are presented. We have established metal organic chemical vapor deposition (MOCVD) technology for InAs-based QD lasers at 1.3 μm and achieved ultralow threshold in QD lasers with photonic crystal (PhC) nanocavity. In addition, single photon emitters at 1.55/μm, GaN-based single photon sources operating at 200 K, and high-Q PhC nanocavity have been demonstrated.     

单轴应力对一维镜像光子晶体光子局域态透射峰的影响

利用传输矩阵法研究了镜像异质三周期一维光子晶体中的光子局域态随单轴应力发生变化的特性. 对于镜像异质三周期光子晶体, 由于其镜像结构, 破坏了光子晶体的有序性, 产生了一个缺陷态, 使其在较宽的光子禁带中心有一个光子局域态透射峰. 研究表明: 当对镜像异质三周期光子晶体施加单轴应力时, 其中的光子局域态透射峰会随着应力的改变而发生剧烈的变化. 当外部微弱的机械应力施加到光子晶体上时, 对光子晶体形成一个拉伸应变, 拉伸应变引起光子晶体结构的变化, 进而大幅度影响光子局域态透射峰的透射率.结果表明: 透射峰的透射率明显受单轴应力的影响. 这些特性可为用此结构的光子晶体设计超高灵敏度压力传感器提供理论参考. 关键词： 光子晶体 单轴应力 光子局域态 传输矩阵     

On‐chip single photon sources using planar photonic crystals and single quantum dots

We review the basic light‐matter interactions and optical properties of chip‐based single photon sources, that are enabled by integrating single quantum dots with planar photonic crystals. A theoretical framework is presented that allows one to connect to a wide range of quantum light propagation effects in a physically intuitive and straightforward way. We focus on the important mechanisms of enhanced spontaneous emission, and efficient photon extraction, using all‐integrated photonic crystal components including waveguides, cavities, quantum dots and output couplers. The limitations, challenges, and exciting prospects of developing on‐chip quantum light sources using integrated photonic crystal structures are discussed.     

Fabrication of three‐dimensional photonic crystals in quantum‐dot‐based materials

Controlling spontaneous emission (SE) is of fundamental importance to a diverse range of photonic applications including but not limited to quantum optics, low power displays, solar energy harvesting and optical communications. Characterized by photonic bandgap (PBG) property, three‐dimensional (3D) photonic crystals (PCs) have emerged as a promising synthetic material, which can manipulate photons in much the same way as a semiconductor does to electrons. Emission tunable nanocrystal quantum dots (QDs) are ideal point sources to be embedded into 3D PCs towards active devices. The challenge however lies in the combination of QDs with 3D PCs without degradation of their emission properties. Polymer materials stand out for this purpose due to their flexibility of incorporating active materials. Combining the versatile multi‐photon 3D micro‐fabrication techniques, active 3D PCs have been fabricated in polymer‐QD composites with demonstrated control of SE from QDs. With this milestone novel miniaturized photonic devices can thus be envisaged.     

驱动场作用下光子晶体中三能级原子的自发发射

讨论了在双光子驱动场作用下,三能级原子在光子晶体中的自发发射问题．由于量子干涉和光的局域化作用,两个上能级中的占据数将具有周期振荡或准周期振荡的性质,这不仅依赖于两个上能级与禁带的相对位置,同时也依赖于原子的初始状态,而且还与驱动场的强度、驱动场的入射位相有关．这些性质既与真空中带有驱动场的原子的自发发射性质不同,也有别于无驱动场作用下光子晶体中三能级原子的自发发射性质． 关键词：     

Implementing a Multi-Qubit Quantum Phase Gate Encoded by Photonic Qubit

A protocol is proposed to implement a three-qubit phase gate for photonic qubits in a three-mode cavity. The idea can be extended to directly implement a N-qubit phase gate. We also show that the interaction time remains unchanged with the increasing number of qubits. In addition, the influence of cavity decay and atomic spontaneous emission on the gate fidelity and photon loss probability is also discussed by numerical calculation.     

Electrically Driven InAs Quantum-Dot Single-Photon Sources

Electrically driven single photon source based on single InAs quantum dot （QDs） is demonstrated. The device contains InAs QDs within a planar cavity formed between a bottom AlCaAs/CaAs distributed Bragg reflector （DBR） and a surface CaAs-air interface. The device is characterized by I-V curve and electroluminescence, and a single sharp exciton emission line at 966nm is observed. Hanbury Brown and Twiss （HBT） correlation measurements demonstrate single photon emission with suppression of multiphoton emission to below 45% at 80 K     

光子晶体对nc-Ge/Si岛发光增强的模拟

在Si基集成光电子学的发展中,高效的Si基光源是人们不懈追求的目标。但是Si材料的间接带隙特性导致其发光效率低,更谈不上受激发射。于是人们探索了多种Si基材料体系来提高Si材料的发光效率,并在不同程度上取得了重要的进展。在众多的Si基发光材料体系中,Ge/Si量子点材料,不仅生长工艺与标准的CMOS工艺有很好的兼容性,而且发光波长能够覆盖重要的光通信波段即1.3~1.55μm,因此成为实现Si基发光器件的重要途径之一。但是目前这种材料的发光效率仍很低,所以提高其发光效率自然成为人们关注的焦点。如果将光子晶体引入到nc-Ge/Si材料中,它不仅可以改变材料本身的自发发射特性,而且可以改变发射的光子的提取效率,从而使材料的发光效率得到增强。提出了在Ge/Si量子点材料中引入光子晶体结构来提高其发光效率,包括光子晶体点缺陷腔结构和带边模式工作的完整光子晶体结构,并从理论上分析了发光效率提高的原理。针对发光波长在1.5μm附近的材料结构,模拟出了相应的光子晶体的结构参数。从模拟结果可以看出,对于缺陷腔的光子晶体结构,采用单点缺陷微腔很好地实现了单模运作,但是微腔内有源材料的体积很小,因此得到的发光效率很低。而采用耦合缺陷腔的结构和H₂腔都增加了腔内有源区的体积。但是耦合腔与H₂腔相比,谐振腔模减少,主谐振模式的峰值强度增加,更容易实现单模发光。因而更适用于提高nc-Ge/Si的发光效率。而带边模式工作的光子晶体结构,尺寸较大,不需引入缺陷,工艺上更容易实现。     

Far field emission of micropillar and planar microcavities lattice-matched to ZnTe

We investigate light emission from ZnTe-based microcavities containing CdTe quantum dots (QDs), with 2D (planar cavity) and 0D (pillar cavities) photonic confinement. The angular distribution from the planar cavity is presented as well as 2D cross-sections of the far field distribution of radiation from the micropillars. The efficient and desirable modification of the isotropic radiation of the QDs is shown for such structures. The diffraction observed is found to be inherent for such experiments with large numerical aperture of the lens and small diameters of the investigated pillars. This diffraction is successfully modeled.     

Quantum dots in photonic crystals: From quantum information processing to single photon nonlinear optics

Quantum dots in photonic crystals are interesting both as a testbed for fundamental cavity quantum electrodynamics (QED) experiments and as a platform for quantum and classical information processing. We describe a technique to coherently access the QD-cavity system by resonant light scattering. Among other things, the coherent access enables a giant optical nonlinearity associated with the saturation of a single quantum dot strongly coupled to a photonic crystal cavity. We explore this nonlinearity to implement controlled phase and amplitude modulation between two modes of light at the single photon level—a nonlinearity observed so far only in atomic physics systems. We also measured the photon statistics of the reflected beam at various detunings with the QD/cavity system. These measurements reveal effects such as photon blockade and photon-induced tunneling, for the first time in solid state. These demonstrations lie at the core of a number of proposals for quantum information processing, and could also be employed to build novel devices, such as optical switches controlled at the single photon level.     

量子点操控的光子探测和圆偏振光子发射

半导体量子点是研究光子与电子态相互作用的优选固态体系,并在光子探测和发射两个方向上展现出独特的技术机遇.其中基于量子点的共振隧穿结构被认为在单光子探测方面综合性能最佳,但受到光子数识别、工作温度两个关键性能的制约.利用腔模激子态外场耦合效应,有望获得圆偏振态可控的高频单光子发射.本文介绍作者提出的量子点耦合共振隧穿（QD-cRTD）的光子探测机理,利用量子点量子阱复合电子态的隧穿放大,将QD-cRTD光子探测的工作温度由液氦提高至液氮条件,光电响应的增益达到10⁷以上,并具备双光子识别能力;同时,由量子点能级的直接吸收,原型器件获得了近红外的光子响应.在量子点光子发射机理的研究方面,作者实现了量子点激子跃迁和微腔腔模共振耦合的磁场调控,在Purcell效应的作用下增强激子自旋态的自发辐射速率,从而增强量子点中左旋或右旋圆偏振光的发射强度,圆偏度达到90%以上,形成一种光子自旋可控发射的新途径.