Demagnetization in photomagnetic films

We present a model for demagnetization in photomagnetic films, and investigate different regimes for the magnetizing process using finite element analysis. It is found that the demagnetizing factor may depend strongly upon the high-spin fraction of the film, and the specifics of the dependence are dictated by the microscopic morphology of the photomagnetic domains. This picture allows for facile interpretation of existing data on photomagnetic films, and can even explain an observed photoinduced decrease in low-field magnetization concurrent with increase in high-spin fraction. As a whole, these results reiterate the need to consider demagnetizing effects in photomagnetic films.     

Photomagnetic effect in molecular magnets based on nitrosyl complexes of ruthenium and rare-earth ions

The magnetic properties of new bifunctional molecular magnets based on nitrosyl complexes of ruthenium and thiacalix[4]arenes of rare-earth ions (Gd³⁺, Dy³⁺) have been investigated. A photoinduced decrease in the magnetization of the molecular magnet with rare-earth ions Gd³⁺ and the absence of a photomagnetic effect in crystals with rare-earth ions Dy³⁺ have been revealed at a temperature of 2 K. It has been found that, in the sample containing Dy³⁺ ions, the magnetization deviates by 6% from the calculated value for noninteracting ions. A comparison of the results obtained for two groups of isostructural samples, which differ only in the type of rare-earth ions, has demonstrated that the observed deviation of the magnetization is caused by the interaction of the orbital moment of the Dy³⁺ ions with the crystal field.     

Magnetic and photomagnetic studies in Nd0.7Sr0.3CoO3

We report magnetic and photomagnetic studies on polycrystalline Nd_0.7Sr_0.3CoO₃. Strong irreversibility in field cooled and zero field cooled data is observed. The hysteresis plot exhibits a very high coercivity at low temperatures. On photon irradiation, a decrease in the coercivity and an irreversible magnetization enhancement are observed. The analysis of all these data suggest that microscopic phase separation of competing ferromagnetism and antiferromagnetism and/or light-induced spin conversion processes among low, intermediate and high spin states of cobalt ions are responsible for all the properties.     

Magnetization and photomagnetic effects in diluted magnetic microcrystalline Cd1-xMnxTe

We have investigated the magnetic and photomagnetic properties of microcrystalline Cd_1-xMn_xTe prepared by rf sputtering. Magnetization measurements were carried out using an rf SQUID magnetometer in the temperature range of 1.8 to 300 K at various magnetic fields up to 5.5 T. For temperatures above 40 K, the sample showed Curie-Weiss behaviour with a Curie temperature indicating predominantly antiferromagnetic interactions. A spin-glass phase transition was also observed. Photomagnetization measurements were performed using a fibre-optic system. The light was shone onto the sample utilizing an optical fibre and the subsequent change in the magnetization was sensed by the SQUID. Photo-induced magnetization was observed when the sample was illuminated by unpolarized light. Our results enable qualitative and quantitative conclusions to be drawn on the magnetic behaviour and the interplay between optical and magnetic properties of the diluted magnetic microcrystalline semiconductors.PACS: 68.55.Gi; 75.50.Pp.     

The photomagnetic effect in Mn delta-doped heteronanostructures with an InGaAs/GaAs quantum well

The influence of embedding a Mn delta layer into heteronunostructures with an InGaAs/GaAs quantum well on the photomagnetic spectra was investigated. The recombination parameters of a number of model structures were determined by the photomagnetic effect and planar photoconduction at high illumination.     

光磁效应研究的新进展

光磁效应研究始于六十年代末，它是磁光效应的一种逆效应。近年来光磁效应研究取得了相当明显的进展，本文分（1）光磁各向异性和光磁效应的可逆特性，（2）光磁电流和光磁电阻，（3）分子基磁体中的光磁效应及其形成机制等三个方面对光磁效应最近几年来的发展进行较为系统的论述。     

Partial magnetization reversal using laser annealing in patterned NiFe/FeMn film

We have studied local magnetization reversal by laser annealing in exchange biased NiFe/FeMn bilayer. Local magnetization reversal was performed by using the Nd:YAG laser under external magnetic field. When the laser illuminated the patterned film with the power of above 300 mW during 15 min, a magnetoresistance (MR) curve with symmetric peaks at the opposite field was obtained due to the local reversal of exchange biasing. A similar result was observed in NiFe/FeMn/NiFe trilayer. As the exposed area expanded, the intensity of opposite MR peak increased. The direction of exchange anisotropy in the partially reversed region can be restored by local laser annealing under alternating magnetic field, even if its MR peak was reduced by the damage and interdiffusion. The magnetic new domain structures of the partially reversed region was generated by laser annealing near the exposed area.     

光磁效应研究的新进展

光磁效应研究始于六十年代末 ,它是磁光效应的一种逆效应。近年来光磁效应研究取得了相当明显的进展 ,本文分 ( 1 )光磁各向异性和光磁效应的可逆特性 ,( 2 )光磁电流和光磁电阻 ,( 3)分子基磁体中的光磁效应及其形成机制等三个方面对光磁效应最近几年来的发展进行较为系统的论述     

Modeling magnetization oscillations in ferromagnetic cobalt disks exposed to picosecond laser pulses

Magnetic reversal of a ferromagnetic single-domain nanoparticle in the form of a disk contained in a multilayer nanostructure irradiated by linearly and circularly polarized picosecond laser pulses is modeled. It is shown that heating of the disk by the laser light causes a change in its direction of magnetization. This is accompanied by oscillations in the magnetization that decay over 1–16 ns. The frequencies of these oscillations lie in the range of 0.5–26 GHz. The main reason for the magnetic reversal of the disk is a change in the magnetic anisotropy energy during heating. The laser pulses also create a spin-polarized current and an inverse Faraday magneto-optical field in the structure, which influence the duration, amplitude, and frequency of the magnetization oscillations.     

Photomagnetic effect in n-type InSb at 77 °K

The steady-state odd photomagnetic effect was studied at liquid-nitrogen temperatures (77 °K) in n-type InSb having a carrier density of 4.2 · 10¹⁶ cm^-3. When the rate of surface recombination on the illuminated surface is higher than on the dark surface, the photomagnetic effect becomes negative in suitable magnetic fields.Translated from Izvestiya VUZ. Fizika, No. 7, pp. 28–31, June, 1970.The authors thank V. A. Gridin for useful discussions.     

铁磁薄膜中圆偏振光感应的瞬态磁光Kerr峰的物理起源

使用飞秒时间分辨抽运-探测磁光Kerr光谱技术,实验研究了圆偏振光抽运面内磁化FePt和垂直磁化GdFeCo薄膜的磁化演化动力学,发现在时间延迟零点处均出现瞬态Kerr峰.分析了此Kerr峰的起源,指出此瞬态Kerr峰与铁磁性无关,可能起源于自由电子的顺磁磁化,而顺磁磁化的外磁场来自圆偏振抽运光的逆Faraday效应.基于顺磁磁化模型的计算结果支持此观点.基于此观点,逆Faraday效应感应的磁场脉冲宽度应该与激光脉冲宽度一致.     

Spatially nonuniform distribution of magnetization in laser-irradiated ferromagentic materials

Ferromagnetic austenite–martensite steels are laser-irradiated to obtain spatially nonuniform distribution of magnetization. An original setup that employs the Faraday effect in epitaxial ferrite-garnet films is used to visualize and measure the spatial distribution of magnetization in steels that are processed with the aid of a fiber laser at different scanning rates. It is demonstrated that rapid laser heating of samples causes modification of the microstructure from the martensite state to the austenite state that provides paramagnetic properties.     

Replica behavior in direct overwritable exchange-coupled magneto-optical multilayer system

The process of direct overwriting by light intensity modulation has been simulated for an exchange-coupled multilayer film without an initializing magnetization. Using the mean-field theory, the temperature dependence of the interlayer wall energy has been calculated for a magnetic triple layer, and the effect of interlayer exchange coupling on magnetization reversals has been investigated. The simulation has shown that replica can be easily realized by the arrangement of the Curie and compensation temperatures of the magnetic layers. A new mechanism of achieving replication from the initializing to the writing layers in the writing process is described in terms of subnetwork moments with high laser power.     

聚焦光在单轴晶体中的感应磁化

运用矢量衍射理论,分析了高度聚焦的圆偏振激光脉冲在具有逆法拉第效应的单轴晶体中产生的感应磁化分布.详细研究了界面位置不同对磁化分布的影响,比较了小双折射效应的单轴晶体中的磁化分布与均匀介质中的磁化分布.计算结果发现:随着界面向透镜移动,磁化强度的最大值和磁化斑的最小值位置沿着光轴方向移动.在单轴晶体中的磁化强度大于在均匀介质中的磁化强度.但是,在单轴晶体中的磁化斑的大小比在均匀介质中的小.描述单轴晶体各向异性的光磁常量与各向同性的光磁常量的比值愈大,磁化强度愈大,磁化斑愈小.     

Laser induced ultrafast demagnetization in diluted magnetic semiconductor nanostructures

We present a dynamical model that reproduces the observed time evolution of the magnetization in diluted magnetic semiconductor films after weak laser excitation. Based on a many-particle expansion of the exact p–d exchange interaction, our approach goes beyond the usual mean-field approximation. Numerical results demonstrate that the hole spin relaxation plays a crucial role for explaining the ultrafast demagnetization processes observed experimentally. The influence of the laser power on the magnetization dynamics is also investigated.     

All-optical magnetic recording with circularly polarized light

We experimentally demonstrate that the magnetization can be reversed in a reproducible manner by a single 40 femtosecond circularly polarized laser pulse, without any applied magnetic field. This optically induced ultrafast magnetization reversal previously believed impossible is the combined result of femtosecond laser heating of the magnetic system to just below the Curie point and circularly polarized light simultaneously acting as a magnetic field. The direction of this opto-magnetic switching is determined only by the helicity of light. This finding reveals an ultrafast and efficient pathway for writing magnetic bits at record-breaking speeds.     

Optical detection in a ferromagnet

The detection of plane-polarized amplitude-modulated infrared laser radiation in a transparent yttrium-iron garnet ferromagnet at room temperature is performed experimentally. The nonlinear interaction mechanism is suggested. It is found that the magnitude and sign of the detected signal depend significantly on the magnetizing external magnetic field. The signal is observed when the magnetization of the ferromagnet approaches the saturated value. The measured dependence of the amplitude of the detected signal on the angle of polarization of the laser radiation with respect to the magnetization of the ferromagnetic sample supports the suggested nonlinearity mechanism. The largest nonlinearity appears when the magnetic field of the plane-polarized laser radiation is parallel to the magnetic moment of the magnetized ferromagnet.     

The role of magnetization compensation point for efficient ultrafast control of magnetization in Gd<Subscript>24</Subscript>Fe<Subscript>66.5</Subscript>Co<Subscript>9.5</Subscript> alloy

The ability of a femtosecond laser pulse to manipulate and reverse the magnetization in a ferrimagnetic Gd₂₄Fe_66.5Co_9.5 thin film was studied experimentally as a function of temperature. For a fixed energy of the laser pulse, the dynamics of magnetization showed different behavior depending on whether the sample temperature was below or above the magnetization compensation point (T _M ). The conditions for full ultrafast demagnetization and magnetization reversal were easily achieved below T _M , while the same laser excitation caused just 50% demagnetization above T _M . This interesting change in magnetization dynamics is qualitatively explained in terms of effective changes in the magnitudes of magnetizations of atomic sublattices.     

High-density all-optical magnetic recording using a high-NA lens illuminated by circularly polarized pulse lights

We propose a method for high-density all-optical magnetic recording. Our analyses, based on the vector diffraction theory, show that owing to the inverse Faraday effect, circularly polarized laser pulses focused by a high numerical aperture (NA) lens can induce a small magnetization domain. For an example, the FWHM of the effective magnetization domain is 0.4646λ when NA=0.85. The magnetization direction is basically perpendicular to the surface of the optic-magneto film within the effective magnetization domain and the switching direction of magnetization can be controlled by the helicity of the incident circularly polarized light. These characteristics are useful to next-generation high-density all-optical magnetic storage.     

The study of ultrafast magnetization dynamics induced by femtosecond laser pulses in GdFeCo amorphous film

The time-resolved magneto-optical Kerr spectroscopy technique is used to study the ultrafast magnetization dynamics induced by femtosecond laser pulses in GdFeCo amorphous film. We study concretely the influence of the different pump fluence and the different external magnetic field on magnetization dynamics of ultrafast demagnetization, magnetization reversal and magnetization recovery. The pump fluence dependence magnetization dynamics shows that the degree of demagnetization, the degree of magnetization reversal and the time of magnetization recovery increase with pump fluence, which can be interpreted by the “three-temperature” model. The external magnetic field dependence magnetization dynamics shows that the rate of magnetization reversal increases with the external field, which accord with the magnetization reversal mechanism based on the reversed magnetic domain nucleation and domain-wall motion.