Research on glass cells for He neutron spin filters

Glass cells play an important role in polarized ³He neutron spin filters. To evaluate the scattering and absorption contribution from glass cells during neutron scattering experiments, we measured small-angle scattering and neutron transmission in GE180 and other glasses. The small-angle neutron scattering measurements revealed that the glasses used for ³He spin filters have acceptably lower scattering: dΣ(Q)/dΩ=4-7×10⁻⁴ cm⁻¹ at Q=0.03-0.12 Å⁻¹. The transmission measurement was performed at J-PARC. Neutron transmission of about 92% through empty GE180 cells was observed over a wide wavelength range 0.014-7.0 Å. To pursue the possibility of being a structural influence on ³He spin relaxation in GE180 glass cells, we performed precise X-ray diffraction measurement using synchrotron radiation at SPring-8. From these measurements, a structural difference was observed among GE180 glasses with different thermal treatments.     

Optimal x-ray beam formation using a focusing mirror at the Langmuir synchrotron station

A beam focusing method is proposed for the Langmuir station of the Kurchatov synchrotron radiation source. This method can be implemented during experiments on recording the fluorescence yield intensity as a function of the angle between an incident beam and a sample surface. The x-ray beam is focused by a cylindrical mirror in such a way that the dimensions of the spot illuminated by the beam on a Langmuir film remain within the input angular aperture of an energy dispersive detector during scanning in the angle of incidence. The relationships for calculating the dimension of the illuminated spot in the scattering plane and the angular divergence of the focused x-ray beam are derived taking into account the dimension of the synchrotron radiation source and spherical aberration. Recommendations for optimizing station parameters and experimental conditions are presented.     

High-Pressure Studies of Magnetism and Lattice Dynamics by Nuclear Resonant Scattering of Synchrotron Radiation

A review is given on recent high-pressure experiments using nuclear resonant scattering of synchrotron radiation. We shortly introduce the methodological aspects connected with high-pressure experiments applying nuclear forward scattering and nuclear inelastic scattering of synchrotron radiation. Selected examples for the study of magnetism are given for the Laves phases LuFe₂ and ScFe₂, where we studied the variation of the magnetic ordering temperature and of the Fe band moment as a function of pressure. An actual example for the study of lattice dynamics is a recent investigation of the phonon density-of-states in metallic iron with special emphasis on hcp ε-Fe, where the pressure-induced texture is used, in conjunction with theoretical calculations, to extract density of phonon states as seen parallel and perpendicular to the hexagonal c-axis. This revised version was published online in August 2006 with corrections to the Cover Date.     

Dielectric loss measurements on silver halide sheet crystals

Abstract

A series of studies on the partial X-ray diffuse scattering intensities from ternary alloys analysed through synchrotron radiation experiments has been reviewed. An intensity expression for the short-range order diffuse scattering has been developed, which is necessary in understanding the separation method of an observed X-ray diffuse intensity into partial intensities contributed from different origins. Techniques have been described in detail mainly concerning the Cu₂NiZn alloy, which have shown the benefits of the anomalous scattering effect of synchrotron radiation. The negative partial intensity maximum for the Cu-Ni pair found in the Cu-Ni-Zn alloy has been discussed from the viewpoints of crystallography and thermodynamics. In addition, at the end of the paper, local atomic arrangements causing the diffuse scatterings have been discussed.     

Suppression of synchrotron radiation due to beam crystallization

With respect to a “hot”, non-crystallized beam the synchrotron radiation of a cold crystallized beam is considerably modified. We predict suppression of synchrotron radiation emitted by a crystallized beam in a storage ring. We also propose experiments to detect this effect. Received: 19 June 1998 / Revised version: 10 August 1998     

Synchrotron radiation photoelectron spectroscopy and near-edge X-ray absorption fine structure study on oxidative etching of diamond-like carbon films by hyperthermal atomic oxygen

Surface structural changes of a hydrogenated diamond-like carbon (DLC) film exposed to a hyperthermal atomic oxygen beam were investigated by Rutherford backscattering spectroscopy (RBS), synchrotron radiation photoelectron spectroscopy (SR-PES), and near-edge X-ray absorption fine structure (NEXAFS). It was confirmed that the DLC surface was oxidized and etched by high-energy collisions of atomic oxygen. RBS and real-time mass-loss data showed a linear relationship between etching and atomic oxygen fluence. SR-PES data suggested that the oxide layer was restricted to the topmost surface of the DLC film. NEXAFS data were interpreted to mean that the sp² structure at the DLC surface was selectively etched by collisions with hyperthermal atomic oxygen, and an sp³-rich region remained at the topmost DLC surface. The formation of an sp³-rich layer at the DLC surface led to surface roughening and a reduced erosion yield relative to the pristine DLC surface.     

Taking into account channels of focused intensity losses for refractive optics elements

Methods are proposed for taking into account intensity losses due to random deviations of composition profiles and due to small-angle scattering effects in amorphous materials and wide-angle scattering effects in polycrystalline materials. Experimental data are presented on the study of polycrystalline-diamond lenses using a synchrotron radiation beam.     

Mössbauer optics of synchrotron radiation at an isotopic boundary

The inelastic coherent Mössbauer scattering (ICMS) of synchrotron radiation at an isotopic boundary—a flat interface between two regions of matter which have different concentrations of the Mö ssbauer isotope—is investigated theoretically. Attention is focused primarily on the ICMS component for which the absorption of a synchrotron radiation photon by a nucleus occurs with recoil, i.e., with the creation or annihilation of lattice phonons, and the subsequent process of reemission of a photon by the Mössbauer nucleus occurs without recoil, as a result of which radiation is pumped from the wide synchrotron radiation line into the narrow Mö ssbauer line. Formulas similar to the Fresnel formulas, well known in optics, for the transmission and reflection of light at a dielectric boundary are obtained for ICMS at an isotopic boundary. Specifically, it is shown that the angle of reflection for ICMS at an isotopic boundary is different from the angle of mirror reflection of a synchrotron radiation beam, and the direction of the ICMS transmitted through the isotopic boundary depends on the deviation of its frequency from the exact value of the Mössbauer resonance frequency and in general is different from the direction of propagation of the synchrotron radiation beam. The suppression of ICMS at grazing angles of incidence of the synchrotron radiation beam is analyzed. A similar problem is solved for a plate-shaped sample containing a Mössbauer isotope. It is shown that the specific nature of the ICMS at an isotopic boundary could be helpful in the problem of Mö ssbauer filtering of synchrotron radiation.     

High-pressure Mössbauer spectroscopy with nuclear forward scattering of synchrotron radiation

Abstract

Using a diamond anvil cell, high-pressure ⁵⁷Fe Mössbauer spectroscopy has been performed with the nuclear forward scattering of synchrotron radiation. A pressure-induced magnetic hyperfine interaction at ⁵⁷Fe in SrFeO_{2, 97} has been detected at 44 GPa and 300 K for a first time by a quantum-beat modulation of the decay rate after collective nuclear excitation by the synchrotron pulse. The basic concept and method used to detect nuclear forward scattering with synchrotron radiation are discussed.     

Windowless transition between atmospheric pressure and high vacuum via differential pumping for synchrotron radiation applications

A differential pump assembly is introduced which can provide a windowless transition between the full atmospheric pressure of an in‐air sample environment and the high‐vacuum region of a synchrotron radiation beamline, while providing a clear aperture of approximately 1 mm to pass through the X‐ray beam from a modern third‐generation synchrotron radiation source. This novel pump assembly is meant to be used as a substitute for an exit vacuum window on synchrotron beamlines, where the existence of such a window would negatively impact the coherent nature of the X‐ray beam or would introduce parasitic scattering, distorting weak scattering signals from samples under study. It is found that the length of beam pipe necessary to reduce atmospheric pressure to below 10 mbar is only about 130 mm, making the expected photon transmission for hard X‐rays through this pipe competitive with that of a regular Be beamline window. This result is due to turbulent flow dominating the first pumping stage, providing a mechanism of strong gas conductance limitation, which is further enhanced by introducing artificial surface roughness in the pipe. Successive reduction of pressure through the transitional flow regime into the high‐vacuum region is accomplished over a length of several meters, using beam pipes of increasing diameter. While the pump assembly has not been tested with X‐rays, possible applications are discussed in the context of coherent and small‐angle scattering.     

High pressure experiments with synchrotron radiation

Using a diamond anvil cell (DAC), high pressure ⁵⁷Fe Mössbauer spectroscopy has been performed with the nuclear forward scattering of synchrotron radiation. We used monochromatized synchrotron radiation from an in‐vacuum type undulator as a high‐density strong Mössbauer source with a quite small beam size. Pressure‐induced magnetic hyperfine interactions at ⁵⁷Fe in SrFeO_2.97 has been detected at 74 GPa by a quantum‐beat modulation of the decay rate after collective nuclear excitation with the synchrotron radiation pulse. Evidence for a transition from antiferromagnetism to ferromagnetism of Fe in SrFeO_2.97 at 74 GPa and 300 K has been obtained from the nuclear forward scattering under a transverse magnetic field.     

Introduction to nuclear resonant scattering with synchrotron radiation

The concepts leading to the application of synchrotron radiation to elastic and inelastic nuclear resonant scattering are discussed. The resulting new experimental techniques are compared to conventional Mössbauer spectroscopy. A survey of situations that favor experiments with synchrotron radiation is offered.

     

Characterization of spatial coherence of synchrotron radiation with non‐redundant arrays of apertures

A method to characterize the spatial coherence of soft X‐ray radiation from a single diffraction pattern is presented. The technique is based on scattering from non‐redundant arrays (NRAs) of slits and records the degree of spatial coherence at several relative separations from 1 to 15 µm, simultaneously. Using NRAs the spatial coherence of the X‐ray beam at the XUV X‐ray beamline P04 of the PETRA III synchrotron storage ring was measured as a function of different beam parameters. To verify the results obtained with the NRAs, additional Young's double‐pinhole experiments were conducted and showed good agreement.     

Crystallography Based on Synchrotron Radiation: Experiments of Russian Users of the ESRF BM01 Diffraction Beam Line

The review deals with studies carried out at the BM01 diffraction beam line of the European Synchrotron Radiation Facility. X-ray diffraction analysis of single-crystal proton conductors demonstrates the possibilities of a precise diffraction experiment in which phase transitions associated with the release of crystallization water and transformation of the network of hydrogen contacts are investigated. Scanning of reciprocal space with the help of a 2D detector enables us to determine the new phase symmetry in a thin-film multiferroic sample based on bismuth ferrite (the given phase is stable only under thin-film conditions). A combination of Bragg and diffusion scattering processes is employed to investigate the interdependence between the structure and dynamics of a crystal lattice and the physical properties of a relaxor material with a perovskite-like structure. The complementarity and synergy of neutron and synchrotron experiments are demonstrated using the combined study of materials from the manganese-silicide group, which has revealed a nontrivial relationship between magnetic and crystallographic chiralities in noncollinear magnets. Although the given review is limited to only a few experiments carried out by Russian scientists at the BM01 beam line, they still illustrate a variety of problems that can be solved using a modern diffraction station where the bending magnet of a third-generation synchrotron is employed as the synchrotron radiation source.     

Analytical estimation of ATF beam halo distribution

In order to study the backgrounds in the ATF2 beam line and the interaction point (IP), this paper has developed an analytical method to give an estimation of the ATF beam halo distribution based on K. Hirata and K. Yokoya''s theory. The equilibrium particle distribution of the beam tail in the ATF damping ring is presented, with each electron affected by several stochastic processes such as beam-gas scattering, beam-gas bremsstrahlung and intra-beam scattering, in addition to the synchrotron radiation damping effects. This is a general method which can also be applied to other electron rings.     

Enhancement and speedup in nuclear resonant diffraction

The interaction of Mössbauer radiation with the nuclei in a single crystal provides the unique possibility to enhance the coherent channel in nuclear resonance scattering by means of a properly phased excitation of the scattering centers. When a primary beam is incident in the exact Bragg direction, all nuclei are excited in phase. The resonance parameters of such a collective nuclear excitation of a perfect single crystal (γ-exciton) are entirely different from those of an individual nuclear excitation. In Bragg geometry diffraction, the resonance lines are shifted and broadened (enhancement effect), the lifetime of the collective excited state is shortened (speedup effect) and the reflectivity becomes total (suppression effect). Recent experiments arc reviewed, where these effects were studied in the resonant diffraction of Mössbauer and of synchrotron radiation.

     

X-ray transition radiation of electrons with energy of 300 to 900 MeV in periodic multifoil radiators

Results of experiments conducted at the Tomsk synchrotron to study resonant X-ray transition radiation generated by relativistic electrons in periodic multifoil radiators are reviewed. Both the internal synchrotron beam and the external secondary electron beam from the pair magnetic γ-spectrometer with energies ranging from 300 to 900 MeV were used in the experiments. The radiators consisted of many thin amorphous foils of various materials. The generation of X-ray radiation in a compound radiator consisting of a multifoil radiator and a crystal is also studied. In this case, the resonant X-ray transition radiation generated in the multifoil radiator is diffracted in the crystal and emitted at Bragg angles, together with the parametric X-ray radiation generated in the crystal. Spectral and angular properties of the resonant X-ray transition radiation and diffracted resonant X-ray transition radiation are investigated. The ratio between the contributions from the diffracted resonant X-ray transition radiation and other types of radiation to the total coherent X-ray radiation flux generated by electrons in periodic structures and crystals is estimated.     

Quasi-stellar objects as Čerenkov sources

If a beam of ultrarelativistic charges enters a gas cloud ?erenkov radiation may be produced. The condition for such radiation is given, and the ?erenkov power radiated per charge is compared to the synchrotron power. Intense ?erenkov pulses will excite emission lines via stimulated Raman scattering. Due to anomalous dispersion in the presence of ac Stark effect the ?erenkov field will be most intense at frequencies well red-shifted from atomic resonances, and this red-shift will be a feature of the stimulated Raman line emissions. The intensity ratios and anomalous red-shifts of the broad emission lines of QSOs can be explained. ?erenkov emission froma collimated beam will be highly directional. The emission evidently does not occur in BL Lacs, which are pure synchrotron emitters.     

Transverse coherence in nuclear resonant scattering of synchrotron radiation

Hyperfine Interactions - We discuss the effects of transverse coherence in time domain nuclear resonant scattering experiments using synchrotron radiation. The importance of source and detector...     

VEPP-2000 collider commissioning

Construction of the VEPP-2000 construction was completed at the end of 2006. The first beam was captured in a special regime without final focus solenoids. In this regime, all systems of power supplies and machine control were calibrated and tuned. In the same mode vacuum chamber treatment by synchrotron radiation was performed with an electron beam current of up to 150 mA. The first test of the round beam option was performed at an energy of 508 MeV with a solenoidal field of 10 T in two straight sections of interaction. The text was submitted by the author in English.