Generation of terahertz radiation by the axicon focusing of ionizing laser pulses

Experimental results on the generation of terahertz radiation in the gas breakdown by high-power quasi-monochromatic laser pulses focused by an axicon lens are presented. A theoretical model developed for the terahertzradiation generation includes the nonlinear interaction of a femtosecond pulse with an ionized gas and the excitation of transverse oscillations of the plasma column. The results of the theoretical analysis are compared with the experimental data.     

Generation of long plasma channels in air by focusing ultrashort laser pulses with an axicon

We show that by focusing ultrashort-pulsed laser beams in air with an axicon, relatively long plasma channels can be generated. The axicon generates Bessel-like beams, where the on-axis intensity stays high over distances much longer compared to focusing with conventional lenses. We developed a scheme to detect the presence of the plasma, based on its screening property. Using this scheme, we detected plasma channels longer than 1 m and 3.5 m generated by 8 mJ and 90 mJ input pulse energies, respectively. Our simulations show that axicon focusing can yield self-guided propagation with or without contribution of plasma, depending on the input pulse power.     

On focusing of terahertz radiation beams and pulses

We show that, for terahertz (THz) radiation, the effective focal length of a lens differs significantly from its geometrical-optics (nominal) focal length. As a pulse of THz radiation with a bell-shaped (Gaussian) transverse profile is incident on a lens, the field-amplitude distribution in the nominally focal plane of the lens may radically change, up to the formation of dips in the paraxial region. These changes in the spatiotemporal shape of the beam (pulse) may considerably distort the results of pulsed THz spectroscopy. These distortions can be minimized by using media with anomalous dispersion, including metamaterials.     

Generation of widely tunable Fourier-transform-limited terahertz pulses using narrowband near-infrared laser radiation

Widely tunable, Fourier-transform-limited pulses of terahertz (THz) radiation have been generated using (i) crystals of the highly nonlinear organic salt 4-N,N-dimethylamino-4′-N′-methyl stilbazolium tosylate (DAST), (ii) zinc telluride (ZnTe) crystals, (iii) gallium phosphide (GaP) crystals, and (iv) low-temperature-grown gallium arsenide (LTG-GaAs) photomixers with THz spiral antennas. Outputs from two narrowband (Δν < 1 MHz, λ ∼ 800 nm) cw titanium-doped sapphire (Ti:Sa) ring lasers with a well-controlled frequency difference were shaped into pulses using acousto-optic modulators (AOM), coupled into an optical fiber, pulse amplified in Nd:YAG-pumped Ti:Sa crystals and used as optical sources to pump the THz emitters. The THz radiation was detected over a broad frequency range and its bandwidth was determined to be ∼10 MHz. The spectroscopic potential of the THz source is illustrated by the absorption spectrum of a pure rotational transition of OCS.     

Enhancement and modulation of terahertz radiation by multi-color laser pulses

We study theoretically intense terahertz radiation from multi-color laser pulse with uncommon frequency ratios. Comparing the two-color laser scheme, of which the uncommon frequency ratio should be set to be a specific value, we show that by using multi-color harmonic laser pulses as the first pump component, the lasers as the second pump component can be adjusted in a continuous frequency range. Moreover, these multi-color laser pulses can effectively modulate and enhance the terahertz radiation, and the terahertz yield increases with the increase of the wavelength of the uncommon pump component and is stable to the laser relative phase. Finally, we utilize the electron densities and velocities of ionization events to illustrate the physical mechanism of the intense terahertz generation.     

Generation of terahertz radiation during reflection of femtosecond laser pulses from a metal surface

The features of terahertz radiation generated upon oblique incidence of a femtosecond laser pulse on a metal surface are investigated theoretically. We propose a Cherenkov-type generation mechanism associated with excitation of low-frequency surface currents by a p-polarized optical field. The nonlinear surface currents and corresponding electrodynamic characteristics of low-frequency radiation are calculated analytically and by numerical simulation using the hydrodynamic model. The features of Cherenkov generation of terahertz radiation are analyzed, and techniques are proposed for increasing efficiency.     

Shock-wave generation upon axicon focusing of femtosecond laser radiation in transparent dielectrics

It is shown experimentally that the axicon focusing of intense femtosecond laser pulses in transparent dielectrics leads to efficient excitation of shock waves. A method is developed for measuring the dynamics of shock waves, which uses a frequency-chirped probe pulse and has high spatial (～1 μm) and time (～10 ps) resolutions. The initial stage of the evolution of an intense (up to 10 GPa) shock wave is studied by this method.     

Multiple filamentation generated by focusing femtosecond laser with axicon

Multiple filamentation has been observed when focusing a femtosecond laser pulse into a methanol solution with an axicon. It is found that multiple long filaments are located on the central spot and ring structures of the quasi-Bessel beam created by the axicon. Since the quasi-Bessel profile is determined by the axicon properties, the axicon has been suggested as a simple optics to control multiple filaments.     

Theoretical model of terahertz radiation generation by laser pulses with tilted wave fronts

A theoretical model is proposed for terahertz radiation generation by femtosecond laser pulses with tilted wave fronts. Self-consistent evolution of the optical and terahertz pulses is investigated. The red shift of the pumping pulse spectrum and the formation of short-long-wave quasi-solitons are examined.     

Generation of sub-mJ terahertz pulses by optical rectification

Recent theoretical calculations predicted an order-of-magnitude increase in the efficiency of terahertz pulse generation by optical rectification in lithium niobate when 500 fs long pump pulses are used, rather than the commonly used ~100 fs pulses. Even by using longer than optimal pump pulses of 1.3 ps duration, 2.5× higher THz pulse energy (125 μJ) was measured with 2.5× higher pump-to-THz energy conversion efficiency (0.25%) than reported previously with shorter pulses. These results verify the advantage of longer pump pulses and support the expectation that mJ-level THz pulses will be available by cooling the crystal and using large pumped area.     

Efficient generation of terahertz radiation by the method of optical rectification of terawatt laser pulses

Factors that lead to a decrease in the width and the mean frequency of the spectrum of terahertz (THz) radiation that were observed in recent experiments on optical rectification of powerful (∼0.5 TW) femtosecond laser pulses with a tilted amplitude front in a lithium niobate crystal are considered. A simple method is proposed that allows one to avoid the above transformation of the spectrum and to ensure a high efficiency of generation of THz radiation when laser pulses with a power of several TW are used.     

Generation of terahertz radiation by the optical breakdown induced by a bichromatic laser pulse

Experimental results are presented on generation of terahertz radiation by the air breakdown induced by a high-intensity laser pulse having not only a fundamental component, but also a second-harmonic one. A theoretical explanation of the experimental data is proposed, based on a model of field ionization of a gas by a bichromatic laser.     

Generation of nanosecond terahertz pulses by the optical rectification method

The possibility of the generation of quasi-cw terahertz radiation by the optical rectification method for broad-band Fourier unlimited nanosecond laser pulses has been experimentally demonstrated. The broadband radiation of a LiF dye-center laser is used as a pump source of a nonlinear optical oscillator. The energy efficiency of terahertz optical frequency conversion in a periodically polarized lithium niobate crystal is 4 × 10⁻⁹ at a pump power density of 7 MW/cm².     

Generation and focusing of submilliwatt-average-power 50-nm pulses by the fifth harmonic of a KrF laser

We demonstrate generation and focusing of 49.7-nm pulses with an average power of 0.1 mW at 200 Hz and with a pulse energy of >1 microJ at 10 Hz by the fifth harmonic of a femtosecond KrF laser. The fifth harmonic is selected and focused with a concave Sc/Si multilayer mirror to a diameter of 2microm, resulting in a peak intensity of 0.5 TW/cm(2), which will make extreme-ultraviolet nonlinear optics feasible. A novel single-shot linear in situ method of spot-size measurement by use of self-trapped exciton luminescence is also demonstrated.     

Generation of short-lived large-amplitude magnetohydrodynamic pulses by dispersive focusing

Large-amplitude MHD waves are routinely observed in space plasmas. We suggest that dispersive focusing, previously proposed for the excitation of freak waves in the ocean, can be also responsible for the excitation of short-lived large-amplitude MHD waves in space plasmas. The DNLS equation describes MHD waves propagating in plasmas at moderate angles with respect to the equilibrium magnetic field. We obtained an analytical solution of the linearised DNLS equation governing the generation of large-amplitude MHD waves from small-amplitude wave trains due to the dispersive focusing. Our numerical solutions of the full DNLS equation confirm this result.     

Optimal control of quantum rings by terahertz laser pulses

Complete control of single-electron states in a two-dimensional semiconductor quantum-ring model is established, opening a path into coherent laser-driven single-gate qubits. The control scheme is developed in the framework of optimal-control theory for laser pulses of two-component polarization. In terms of pulse lengths and target-state occupations, the scheme is shown to be superior to conventional control methods that exploit Rabi oscillations generated by uniform circularly polarized pulses. Current-carrying states in a quantum ring can be used to manipulate a two-level subsystem at the ring center. Combining our results, we propose a realistic approach to construct a laser-driven single-gate qubit that has switching times in the terahertz regime.     

Generation of ultrabroadband terahertz radiation under optical breakdown of air by two femtosecond pulses of different frequencies

Experimental results on the generation of terahertz (THz) electromagnetic radiation under ionization of air by femtosecond pulses at fundamental and second-harmonic frequencies of a Ti-sapphire laser are presented. The mean power of the generated THz radiation as a function of the time delay between two pulses of different frequencies is found to be quasi-periodical. Theoretically, we show that efficient generation of THz radiation is governed by the inertial part of the nonlinear response of the medium, which is determined by the dynamics of population of highly excited states with subsequent emission of electrons.     

Generation of XUV attosecond pulses in the process of atomic ionization by few-cycle laser radiation

Ionization of a model two-electron atom in the presence of a strong field of ultrashort laser pulses is investigated using the numerical integration of the nonstationary Schrödinger equation, which describes the dynamics of a quantum system in the presence of an electromagnetic wave. The features of two-electron ionization in the presence of one-and two-cycle pulses are analyzed. The suppression of double ionization in the presence of ultrashort laser pulses related to a finite-time interelectron energy exchange upon the laser action is demonstrated. The features of the generation of high-order harmonics and single XUV attosecond pulses are studied for the atomic ionization by few-cycle laser pulses. The parameters of the laser pulse are optimized for the effective generation of a single XUV attosecond pulse.     

Generation of high-power terahertz pulses in a prism

A compact, high-power emitter of half-cycle terahertz (THz) radiation is demonstrated. The device consists of an epitaxial InAs emitter upon a GaAs prism and produces THz pulses that are 20 times more powerful than those from conventional planar InAs emitters. This improvement is a direct result of reorienting the transient THz dipole such that its axis is not perpendicular to the emitting surface.