Calorimetric evidence for a Fulde-Ferrell-Larkin-Ovchinnikov superconducting state in the layered organic superconductor kappa-(BEDT-TTF)2Cu(NCS)2

The specific heat of the layered organic superconductor kappa-(BEDT-TTF)(2)Cu(NCS)(2), where BEDT-TTF is bisethylenedithio-tetrathiafulvalene, has been studied in magnetic fields up to 28 T applied perpendicular and parallel to the superconducting layers. In parallel fields above 21 T, the superconducting transition becomes first order, which signals that the Pauli-limiting field is reached. Instead of saturating at this field value, the upper-critical-field increases sharply and a second first-order transition line appears within the superconducting phase. Our results give strong evidence that the phase, which separates the homogeneous superconducting state from the normal state is a realization of a Fulde-Ferrell-Larkin-Ovchinnikov state.     

Topological structure of a vortex in the Fulde-Ferrell-Larkin-Ovchinnikov state

We find theoretically that the vortex core in the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state is quite different from the ordinary core for a simple topological reason. The intersection point of a vortex and nodal plane of the FFLO state empties the excess spins. This leads to observable consequences in the spatial structure of the spontaneous magnetization. We analyze this topological structure based on the low lying excitation spectrum by solving a microscopic Bogoliubov-de Gennes equation to clarify its physical origin.     

Fulde-Ferrell-Larkin-Ovchinnikov state in layered superconductors

The phase diagram of a layered superconductor in a large parallel magnetic field is calculated. This includes a calculation of the lower critical field beyond which the superconductor is in the FFLO-state and possesses a spatially modulated order parameter and spin polarization. The order parameter, spin polarization, free-energy density, and phase boundaries of this unconventional superconducting phase are evaluated numerically in the complete B–T plane. The analysis suggests that the transition at the lower critical field is of second order, and not of first order, as previously assumed. The order parameter of the FFLO-state merges continuously into the uniform superconducting state.     

Vortex dynamics in Pb-doped Hg-1234 superconductor by AC susceptibility response

The general equation that describes the AC magnetic susceptibility response of the superconducting system due to the change of varying AC field has been reviewed. By using the AC susceptibility measurements, the temperature, magnetic field and current density dependence of the effective pinning potential U(T, H, J) for our Pb-doped Hg-1234 superconductor has been determined. It is found that the fast drop of the effective pinning potential with current density is due to the large value of the characteristic exponent μ which depends on the existing types of non-superconducting phases that form the intergrowth structures with the dominant matrix. The characteristic curve of electric field E(J) against the current density J has been obtained from the AC susceptibility technique. For consideration of current relaxation due to the presence of giant flux creep, we have studied and determined the temperature dependence of the critical current density J_c for our specimen.     

Vortex lines in a ferromagnetic spin-triplet superconductor

Based on Duan's topological current theory, we show that in a ferromagnetic spin-triplet superconductor there is a topological defect of string structures which can be interpreted as vortex lines. Such defects are different from the Abrikosov vortices in one-component condensate systems. We investigate the inner topological structure of the vortex lines. The topological charge density, velocity, and topological current of the vortex lines can all be expressed in terms of δ function, which indicates that the vortices can only arise from the zero points of an order parameter field. The topological charges of vortex lines are quantized in terms of the Hopf indices and Brouwer degrees of φ-mapping. The divergence of the self-induced magnetic field can be rigorously determined by the corresponding order parameter fields and its expression also takes the form of a δ-like function. Finally, based on the implicit function theorem and the Taylor expansion, we conduct detailed studies on the bifurcation of vortex topological current and find different directions of the bifurcation.     

Vortex sublattice melting in a two-component superconductor

We consider the vortices in a superconductor with two individually conserved condensates in a finite magnetic field. The ground state is a lattice of cocentered vortices in both order parameters. We find two phase transitions: (i) a "vortex sublattice melting" transition where vortices in the field with lowest phase stiffness ("light vortices") lose cocentricity with the vortices with large phase stiffness ("heavy vortices"), entering a liquid state (the structure factor of the light vortices vanishes continuously; this transition is in the 3Dxy universality class); (ii) a first-order melting transition of the lattice of heavy vortices, in a liquid of light vortices.     

Possible Fulde-Ferrell-Larkin-Ovchinnikov superconducting state in CeCoIn5

We report specific heat measurements of the heavy fermion superconductor CeCoIn5 in the vicinity of the superconducting critical field H(c2), with magnetic fields in the [110], [100], and [001] directions, and at temperatures down to 50 mK. The superconducting phase transition changes from second to first order for fields above 10 T for H parallel [110] and H parallel [100]. In the same range of magnetic fields, we observe a second specific heat anomaly within the superconducting state. We interpret this anomaly as a signature of a Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) inhomogeneous superconducting state. We obtain similar results for H parallel [001], with the FFLO state occupying a smaller part of the phase diagram.     

Generalized Fulde-Ferrell-Larkin-Ovchinnikov state in heavy-fermion and intermediate-valence systems

Anomalous properties of the magnetization, the crystal dilatation, and other physical quantities observed in the mixed state of compounds such as UPd₂Al₃ and CeRu₂ suggest the occurrence of a new state near H _c2. In such compounds with large spin susceptibility and high H _c2, a new inhomogeneous superconducting state is theoretically predicted to occur in high magnetic fields. In this inhomogeneous state which is shown to be a generalized Fulde-Ferrell-Larkin-Ovchinnikov state, the order parameter is spatially modulated, and planar nodes of the order parameter are periodically aligned perpendicular to the vortices. Various theoretical predictions are compared with experimental results on UPd₂Al₃ and CeRu₂ related to this new superconducting high-field state.     

A possibility of a new type of the Fulde-Ferrell-Larkin-Ovchinnikov state

We propose a new type of the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state with a cylindrical symmetric order-parameter. We study the Ginzburg-Landau (GL) theory of the strongly Pauli limited type II superconductor with a spherical symmetric fermi surface, near the critical magnetic field of the FFLO state in the ground state. We find that the cylindrical state has a lower energy than the stripe state, which has the lowest energy in the states examined so far.     

Fulde-Ferrell-Larkin-Ovchinnikov state in a perpendicular field of quasi-two-dimensional CeCoIn5

A Fulde-Ferrell-Larkin-Ovchinnkov (FFLO) state was previously reported in the quasi-2D heavy fermion CeCoIn5 when a magnetic field was applied parallel to the ab plane. Here, we conduct 115In NMR studies of this material in a perpendicular field, and provide strong evidence for FFLO in this case as well. Although the topology of the phase transition lines in the H-T phase diagram is identical for both configurations, there are several remarkable differences between them. Compared to H parallelab, the FFLO phase for H perpendicularab is confined in a much narrower region at the low-T-high-H corner in the H-T plane, and the critical field separating the FFLO and non-FFLO superconducting states almost ceases to have a temperature dependence. Moreover, directing H perpendicularab results in a notable change in the quasiparticle excitation spectrum within the planar node associated with the FFLO transition.     

Theory of a magnetic-field-induced superconductive state in heavy fermion systems

We propose a possible theoretical explanation of recently observed magnetic-field-induced superconductivity in heavy fermion CePb₃ crystals based on the Ginzburgh-Landau phenomenological theory.     

Possible Fulde-Ferrell-Larkin-Ovchinnikov inhomogeneous superconducting state in CeCoIn5

We present specific heat and thermal conductivity of the heavy fermion superconductor CeCoIn5 in the vicinity of the superconducting critical fieldH _c2, measured with magnetic field in the plane of this quasi-2D compound and at temperatures down to 50 mK. The superconducting phase diagram and the first order nature of the superconducting phase transition at high fields close to a critical fieldH _c2 indicate the importance of the Pauli limiting effect in CeCoIn₅. In the same range of magnetic field we observe a second specific heat anomaly within the superconducting state, and interpret it as a signature of a Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) inhomogeneous superconducting state. In addition, the thermal conductivity data as a function of field display a kink at a fieldH _k below the superconducting critical field, which closely coincides with the low temperature anomaly in specific heat tentatively identified with the appearance of the FFLO superconducting state. The enhancement of thermal conductivity within the FFLO state calls for further theoretical investigations of the real space structure of the order parameter (and in particular, the structure of vortices) and of the thermal transport within the inhomogeneous FFLO state.     

Pressure dependence of the Fulde-Ferrell-Larkin-Ovchinnikov state in CeCoIn5

Pressure studies of the thermodynamics of CeCoIn5 under magnetic fields H parallel to c and H parallel to ab have been made up to P = 1.34 GPa. We recorded the signature of the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state for all pressures when H parallel to ab. Also remarkably, the FFLO regime suddenly expands for P = 1.34 GPa. With the help of a microscopic theory for d-wave superconductivity, we have extracted the gyromagnetic ratio g and the Fermi velocities nu(a) and nu(c). Our study is the first evidence for the existence of the FFLO state away from the influence of the antiferromagnetic fluctuations. We find a close parallel between the T-P phase diagram of CeCoIn5 and the T-x phase diagram of the high-Tc cuprates, where x is the hole concentration.     

Commensurate spin dynamics in the superconducting state of an electron-doped cuprate superconductor

We report neutron scattering studies on two single crystal samples of the electron-doped (n-type) superconducting (SC) cuprate Nd2-xCexCuO4 (x=0.15) with T(c)=18 and 25 K. Unlike the hole-doped (p-type) SC cuprates, where incommensurate magnetic fluctuations commonly exist, the n-type cuprate shows commensurate magnetic fluctuations at the tetragonal (1/2 1/2 0) reciprocal points both in the SC and in the normal state. A spin gap opens up when the n-type cuprate becomes SC, as in the optimally doped p-type La2-xSrxCuO4. The gap energy, however, increases gradually up to about 4 meV as T decreases from T(c) to 2 K, which contrasts with the spin pseudogap behavior with a T-independent gap energy in the SC state of p-type cuprates.     

Local tunneling spectroscopy as a signature of the Fulde-Ferrell-Larkin-Ovchinnikov state in s- and d-wave superconductors

The Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) states for two-dimensional s- and d-wave superconductors (s- and d-SCs) are self-consistently studied under an in-plane magnetic field. While the stripe solution of the order parameter is found to have lower free energy in s-SCs, a square lattice solution appears to be energetically more favorable in the case of d-SCs. At certain symmetric sites, we find that the features in the local density of states (LDOS) can be ascribed to two types of bound states. We also show that the LDOS maps for d-SCs exhibit bias-energy-dependent checkerboard patterns. These characteristics can serve as signatures of the FFLO states.     

Resistivity of a superconductor in the intermediate state

The resistivity of a superconductor in the intermediate state is known for some limiting cases such as low temperatures, small mean free path, etc. In this paper, the resistivity is derived in the general case; it is a function of the temperature, the mean free path, the thickness of the normal and superconducting layers. The existence of a discontinuity of the electric potential at the interface between a normal and a superconducting layer is shown.