A study of high spin states in the transitional nucleus90Mo

The reaction⁵⁸Ni(³⁶Ar, 4p)⁹⁰Mo has been studied at a beam energy of 149 MeV. A detector array consisting of the OSIRIS spectrometer (12 Compton-suppressed Ge detectors), four charged-particleδE detectors and seven NE-213 neutron detectors at the VICKSI accelerator in Berlin has been used to measure the gamma radiation inγγ- and particle-γγ-coincidence mode. An additional Ge detector was placed at 162? to the beam direction to provide information on DCO ratios. The level scheme of⁹⁰Mo has been extended up to an excitation energy of about 12 MeV and probable spin 23?. Some 70 transitions and 40 levels have been newly identified. Spin assignments have been proposed on the basis of measured DCO ratios. Shell model calculations in a model space consisting of the proton 1f _5/2, 2p _3/2, 2p _1/2, and 1g _9/2 orbits and the neutron 2p _1/2, 1g _9/2, 1g _7/2, 2d _5/2, 2d _3/2, and 3s _1/2 orbits with some truncation were made for states above 9? and the predicted structure of these states is discussed.     

Identification and structure of high spin particle-hole states in89Mo

Particle-γ andγ-coincidences of the reaction⁵⁸Ni(³⁶Ar, 4pn)⁸⁹Mo have been used to gain more information about high spin states in⁸⁹Mo and to establish the yrast sequence up to 7.6 MeV excitation energy and probable spin 37/2 ?. Spins and parities were assigned on the basis of DCO-ratios measured with the OSIRIS spectrometer and a large volume Ge detector placed at 162° to the beam. Furthermore, aγ-ray angular distribution experiment was carried out using the reaction⁵⁸Ni(³⁵Cl, 3pn)⁸⁹Mo. As in the neighboring isotopes⁸⁸Mo and⁹⁰Mo, the positive-parity high-spin states can be grouped into shell model multiplets characterized by increasing seniorities of proton particles and neutron holes in the 1g_9/2 shell. The negative-parity states can be explained with one nucleon moving in thep _1/2 orbit. The energies and wave functions of these states have been deduced by means of the shell model code RITSSCHIL. The 2584 keV (21/2⁺) is an isomeric state the mean life of which has been estimated from delayedγγ-coincidences.     

The gamma-decay of34Ar

States in³⁴Ar up to 5.5 MeV excitation energy, populated by the³²S(³He,nγ) reaction at 8–12 MeV bombarding energy, have been investigated with the Doppler shift attenuation method,nγ angular correlation andnγγ triple coincidence measurements. For the states at 2.09, 3.29 and 4.52 MeV the lifetimes 200±60 fs, 130±60 fs and 260±80 fs have been found, respectively. Thenγ correlations yielded the spin assignmentsJ ^μ=(2⁺) for the level at 4.13 MeV andJ ^μ=3^? for the 4.52 MeV state, and the mixing ratiosδ(3.29→2.09)=?0.12±0.05 andδ(4.13→3.29)=?0.52±0.15. The results are compared with shell model calculations and predictions from the weak coupling unified model.     

Single-neutron transfer reactions 76, 78, 80, 82Se(p,d)75, 77, 79, 81Se at EP = 33MeV

Single-neutron transfer reactions on even-even Se nuclei have been studied using 33 MeV incident proton energy from the ANU cyclograaff facility. A total of 120 levels have been seen below 4 MeV excitation energy in ^{75, 77, 79, 81}Se isotopes. Angular distributions for 88 states were extracted and analysed with DWBA theory yielding a number of new l_n assignments. Coriolis coupling calculations have been carried out for low-level spin states in all four isotopes.     

Excited states of100Tc from100Mo(p,nγ)100Tc reaction and the parabolic rule

γ-spectra and excitation functions of the¹⁰⁰Mo(p, nγ)¹⁰⁰Tc reaction were measured in the 1.2–3.6 MeV proton energy range by using thick, enriched targets, Ge(Li) and low energy photon (hyperpure Ge) spectrometers. These detectors were used inγγ-coincidence experiments, too. Conversion electron spectrum measurements were performed by means of a superconducting magnet transporter Si(Li) spectrometer (SMS) atE _p =4 MeV and multipolarities of some transitions have been determined. Based on the experimental results a level scheme of¹⁰⁰Tc has been constructed. Level energies of¹⁰⁰Tc were calculated on the basis of the parabolic rule, derived from the cluster-vibration model.     

Tentative level diagram of146Pm below 1.1 MeV

The level scheme of the doubly odd nucleus¹⁴⁶Pm was investigated by means of in-beam spectroscopy. The¹⁴⁶Nd(p, n) reaction in the 3.5–8 MeV proton energy interval on enriched targets has been used to populate the exited states of¹⁴⁶Pm. High resolutionγ-ray spectra using Ge(Li) and hyperpure Ge detectors and conversion electrons with a mini-orange spectrometer were measured. Withγ-exitation functions andnγ-coincidences usingnγ-discriminated NE231 neutron detectors transitions in¹⁴⁶Pm were identified,γγ-coincidences gave information aboutγ-cascades. With these data a level scheme of 38 levels below 1.1 MeV exitation energy has been deduced including 73 transitions. For 12 transitions experimental conversion coefficients have been evaluated, which agree with the expected values forM1/E2-transitions.     

Two-quasiparticle bands in72Br

High spin states in the doubly odd nucleus⁷²Br were investigated via the reaction⁵⁸Ni(¹⁶O,pn) at 52–65 MeV beam energy. A multi-element detector system consisting of ten Compton supressed Ge detectors (OSIRIS) and two NE213 neutron detectors was used to establish the yrast bands up to 5 MeV excitation energy and probable spins of 15⁺ resp. 14^?. The lifetimes of 12 states and lifetime limits of four states were measured with the recoil distance method, among them four 0.5–3.1 ns isomers. Doppler broadened line shapes obtained in an additionalγγ-coincidence experiment via the reaction⁴⁰Ca(³⁶Ar, 3pn) at 125 MeV revealed further lifetimes and (very short) side feeding times. Three rotational bands were established with deformation parameters ¦β ₂¦≈0.3 and moment of inertia parameters \(\tilde f\) /? ²=36 MeV^?1 (K ^ρ=1^?) resp. 23 MeV^?1; their quasi-particle configurations are being discussed.     

Spectroscopy of88Y homologous levels

The⁹¹Zr( $z\bar p$ ,α)⁸⁸Y reaction has been studied at incident energy of 22 MeV using a polarized proton source and a Q3D spectrometer. The differential cross sections and asymmetries for transitions to levels of⁸⁸Y homologous to the lowest excitation energy states of⁸⁷Y have been measured and interpreted both in terms of the experimental differential cross sections and asymmetries of the parent⁸⁷Y states and by means of the finite-range distorted wave Born approximation theory using conventional Woods-Saxonα-particle potential. The advantage of the concept of homology consists in having to deal with a uniquel-transfer, that given by the transition to the corresponding parent state. In order to validate the concept of homology as a spectroscopic tool to identify spin, parity and dominant configuration of highly excited states in ( $z\bar p$ ,α) reaction on odd mass target nuclei, shell model calculations have been performed. Several new attributions of spin and parity for⁸⁸Y residual nucleus are proposed.     

Nuclear structure of 216 Ra at high spin

High-spin states of ²¹⁶Ra ( $\emph{Z}=88$ , $\emph{N}=128$ ) have been investigated through ²⁰⁹Bi(¹⁰B, 3n) reaction at an incident beam energy of 55?MeV and ²⁰⁹Bi(¹¹B, 4n) reaction at incident beam energies ranging from 65 to 78?MeV. Based on ??? coincidence data, the level scheme for ²¹⁶Ra has been considerably extended up to ~ 33 $\hbar$ spin and 7.2 MeV excitation energy in the present experiment with placement of 28 new ??-transitions over what has been reported earlier. Tentative spin-parity assignments are done for the newly proposed levels on the basis of the DCO ratios corresponding to strong gates. Empirical shell model calculations were carried out to provide an understanding of the underlying nuclear structure.     

Interaction of 80 MeV12C with88Sr; Neutron transfer,inelastic scattering and spin alignment of the 2+ State of12C

Level structure of¹⁰²Cd has been studied via both¹⁰²In decay and nuclear reactions. Using⁹²Mo+¹⁴N at 86 MeV, the nucleus¹⁰²In was identified and its decay (T _1/2=24 ±4s) studied with the aid of on-line mass separation techniques. Levels of¹⁰²Cd were also populated with⁹²Mo+¹²C at 50 MeV and¹⁰²Pd+³He at 35 MeV reactions and investigated by means of standard in-beam techniques. A level scheme including states up to 4.5 MeV excitation energy is proposed and then discussed in the frame of available calculations.     

High resolution investigation of 91Mo and 92Mo via (p,d) and (p,t) reactions on 90Mo

The (p, d) and (p, t) reactions on ⁹²Mo have been studied at a proton energy of 28.0 MeV. Using an Enge split-pole spectrograph, resolutions of 11–15 keV for the detected deuterons and tritons were obtained. A total of 87 levels up to 4.9 MeV in ⁹¹Mo and 25 levels up to 4.0 MeV in ⁹⁰Mo were found, several of which were previously unknown. By comparing the measured angular distributions with DWBA calculations l-values and spectroscopic factors were determined. The results are compared with data from previous experiments on ⁹¹Mo and ⁹⁰Mo, with experiments on other N = 49 and 48 nuclei, and with theoretical calculations.     

102Ag: In-beam gamma-ray spectroscopy

Gamma-rays associated with the decay of states in the ¹⁰²Ag nucleus have been identified, sixty-four of them for the first time following the reaction ⁵⁰Cr(⁵⁶Fe, 3pn)¹⁰²Ag at a mean energy of 195 MeV. Identification was made using an array of nine escape-suppressed Ge detectors coupled to the Daresbury Recoil Separator. Excited states in ¹⁰²Ag were identified using recoil-gamma and γγ coincidences. From the intensity balance and the coincidence data, a new set of levels was identified which may be interpreted as reminiscent of “three-quasiparticle” bands in neighboring odd-mass nuclei and similar to a four-quasi-particle band observed in ¹⁰⁶Ag.     

Properties of electromagnetic transitions from high-spin states in94Mo

The multipole mixing ratios of transitions from 6⁺ and 8⁺ states in⁹⁴Mo, following the decay of⁹⁴Tc, have been measured by means ofγγ angular correlations. The spin of the 2423.4 keV state, being important for the interpretation ofγ cascades feeding this level, has been firmly established as 6⁺ by a method in which the angular correlation data are utilized in a non-conventional way. Furthermore, properties of electromagnetic transitions in⁹⁴Mo have been calculated in the shell model framework and are compared with the corresponding experimental quantities.     

Structure of 74Ge from the 72Ge(t,p) reaction

The reaction ⁷²Ge(t, p)⁷⁴Ge has been investigated with a 15 MeV triton beam. Fifty energy levels of ⁷⁴Ge were identified up to about 4.9 MeV excitation, eighteen of which were previously unreported. Angular distributions were measured and compared with DWBA calculations. Two low-lying states at 1.913 and 2.164 MeV have been assigned as J^π = 0⁺, corresponding to the 0₃⁺ and 0₄⁺ states in ⁷⁴Ge. The 4₂⁺ state has been located at 2.674 MeV, and the 2₄⁺ at 2.836 MeV. Many additional spin and parity assignments have been made. The ⁷⁴Ge nucleus shows a considerably different structure of 0⁺ states compared with the neighboring ⁷⁶Ge and ⁷⁸Ge nuclei, perhaps further evidence for the shape transition suggested recently for the Ge isotopes.     

Nuclei in the vicinity of ‘island of inversion’ through the fusion reaction

The level structures of N ～ 19 nuclei such as ^32,34P have been investigated using the ¹⁸O(¹⁸O,xnyp) and ¹⁸O(¹⁶O,xnyp) reactions at an incident beam energy of about 34 MeV. The de-exciting γ-transitions were recorded using an array of clover detectors. These detectors have the dual advantage of higher efficiency at E _γ ≥ 2 MeV, and are capable of providing information on the linear polarization of the observed γ-transitions. These polarization measurements when coupled with the angular correlations help us to assign uniquely the spin parity for the observed levels. The experimental results have been compared with the predictions of the spherical shell model. The shell-model calculations are able to reproduce the observed energy levels to a reasonable degree. However, the observed transition probabilities are not reproduced by the calculations. Hence there is a need to re-visit these calculations using more detailed and microscopic effective interactions.     

Shape evolution in odd-A 137 Pm

The odd mass nucleus ¹³⁷Pm has been studied to high spins through the ¹⁰⁹Ag(³²S, 2p2n)¹³⁷Pm reaction at an incident beam energy of 150 MeV. The de-exciting ??-rays were detected using an array of 18 Compton suppressed clover detectors. The level scheme of ¹³⁷Pm has been extended up to $J^\pi = \tfrac{{43}} {2}^ -$ and excitation energy of E _x ? 6 MeV with the observation of 42 new gamma transitions. The linear polarization (IPDCO) measurements for the ??-ray transitions have been done for the first time. The spin and parity assignments for most of the reported levels have been made using these results and the coincidence angular anisotropy (R_DCO) measurements. The nuclear shape evolution is discussed in the light of Total Routhian Surface (TRS) and Cranked Shell Model (CSM) calculations.     

Spins and parities of low-lying states in 81Kr from the 80kr(d̄, p)81kr reaction and implications for a 81Br solar neutrino detector

The structure of ⁸¹Kr has been investigated via the ⁸⁰Kr(d?, p)⁸¹Kr reaction using an 11.0 MeV vector-polarized deuteron beam. Differential cross sections σ and vector analyzing powers A_y have been measured from 20° to 90° for 17 excited states below 3.0 MeV excitation energy. Comparisons of these distributions to DWBA calculations and empirical shapes were made to extract spectroscopic factors and values of spin and parity for these states. The significance of these measurements to the design of a bromine solar neutrino detector is discussed.     

Two proton high-spin excitations and dipole bands in192Hg

The¹⁹²Hg nucleus was populated in the¹⁶⁰Gd(³⁶S, 4n) reaction at a beam energy of E=159 MeV. Emittedγ-rays were detected with the EUROGAM array comprising 43 Compton-suppressed large volume Ge detectors. The level scheme of¹⁹²Hg has been extended up to an excitation energy of E=10.4 MeV and spin I=34 ?. Two new structures, made of competing ΔI=1 and ΔI=2 transitions have been observed and their connexions with the low-lying levels established. Their lowest levels are located at 6.304 MeV and 6.879 MeV excitation energy. The experimental results are compared with mean-field HF+BCS calculations. It is proposed that the new structures originate from deformation-aligned quasi-proton excitations π(i_13/2 * h_9/2)_K=11 andπ (h_9/2) _K=8 ² , coupled to rotation-aligned quasi-neutron ν(i_13/2)ⁿ and quasi-proton π(h_11/2)² excitations.     

Levels excited in73Ge by (d,p) and (p,p′) reactions

Angular distributions from the reactions⁷²Ge(d, p)⁷³Ge and⁷³Ge(p, p′)⁷³Ge have been studied with 8.0 MeV deuterons and 12.0 MeV protons, respectively, using the Aldermaston Tandem Van de Graaff generator and multi-angle magnetic spectrograph. The ground stateQ-value of the (d, p) reaction was measured to be 4.571±0.004 MeV. The energies, values of the transferred orbital angular momenta, parities and transition strengths in both reactions were determined by use of distorted-wave Bornapproximation calculations, for levels up to 3 MeV excitation energy. The sums of the transition strengths are compared with shell model calculations as well as with values obtained in neighbouring nuclei. Discrepancies between parity and possible spin assignments of states observed in the two reactions are discussed.     

Shape coexistence and strong shape changes in very neutron deficient platinum isotopes

High spin states of^{175, 176}Pt have been populated in¹⁴⁴Sm(³⁵Cl,pxn) reactions at beam energies of 175–185 MeV. In-beamγ-ray spectroscopic techniques using the ESSA30 spectrometer array were adopted. Levels up to spin 26 in¹⁷⁶Pt and tentatively up to spin 45/2 in¹⁷⁵Pt have been identified. The data are interpreted within the framework of Cranked Shell Model calculations using the deformed Woods-Saxon potential and including monopole pairing.